arXiv subjects

Hongxing Xu

Publications and source records attributed to Hongxing Xu.

At least 19 recordsLinked to original sources

arXiv2026

Polariton-mediated binding of anti-aligned dipolar excitons

Interacting bosonic quasiparticles are the cornerstone for exploring many-body physics and nonlinear quantum phenomena in correlated light-matter systems. Strongly interacting dipolar excitons in van der Waals heterostructures have attracted significant interest due to their out-of-plane electric dipole moments and high tunability via the quantum-confined Stark effect (QCSE). However, leveraging these tunable dipolar excitons in strongly coupled exciton-photon systems to explore exotic many-body physics and macroscopic quantum phenomena remains experimentally elusive. Here, we report the strong coupling of dipolar excitons in a gated bilayer MoS2 device integrated with a one-dimensional photonic crystal hosting bound-states-in-continuum (BIC). The resulting polaritons hybridize cavity photons with a coherent superposition of two electrically tunable anti-aligned dipolar excitons, effectively binding them into composite quasiparticle states. By tuning the dipolar excitons into non-degenerate states via the QCSE, we realize in situ reconfiguration of the polariton wavefunction and observe an emergent polariton branch exhibiting non-monotonic Stark shifts. Notably, these tunable polaritons allow for customized control over nonlinear interactions through distinct excitonic hybridization and dipolar configurations. This in situ tunability offers a scalable pathway toward electrically programmable quantum fluids of light and correlated polariton phases in on-chip photonic integrated circuits.

physics.optics↗

arXiv2025

Extreme polaritonic interactions in a room-temperature deterministic sub-nanocavity quantum electrodynamic platform

Pushing nanoscale optical confinement to its ultimate limits defines the regime of nano-cavity quantum electrodynamics (nano-cQED), where light--matter interactions approach the fundamental quantum limits of individual atoms, e.g., picocavities. However, realizing such extreme confinement in a stable and controllable manner remains a key challenge. Here, we introduce a van der Waals material-based nano-cQED platform by coupling monolayer MoS2 excitons to plasmonic sub-nanocavities formed via assembly of ultrasmall gold clusters (3-5 nm) in the nanogap of a nanoparticle-on-mirror nanocavity. These clusters emulate the field-confining role of atomic protrusions of the picocavities through a resonance-insensitive lightning-rod effect, achieving deep-subwavelength mode volumes. In this nano-cQED testbed, we observe pronounced multi-branch Rabi splittings and ultrastrong lower-branch polaritonic photoluminescence with up to 10^4-fold enhancement. This deterministic architecture provides a controllable pathway to access picocavity-like behavior and opens new opportunities for single-molecule spectroscopy and the exploration of nano-cQED.

physics.optics↗

arXiv2025

Spin-Based True Random Number Generation Enabled by Voltage-Amplified Quantum Fluctuations

We investigate spin quantum-fluctuation effects that originate from the Heisenberg uncertainty principle during the dynamical cycle of disentanglement, entanglement, and re-disentanglement between itinerant electrons and localized magnetic moments mediated by the s-d exchange interaction. Beyond conventional deterministic spin-transfer torque, we analyze an intrinsic mechanism that transfers spin quantum fluctuations to a nanomagnet. By extending the Landau-Lifshitz-Gilbert equation to incorporate both quantum and thermal stochastic fields, we identify a temperature regime in which quantum fluctuations dominate the magnetization dynamics. We further show that voltage-controlled magnetic anisotropy exponentially amplifies spin quantum fluctuations, enabling binary readout through magnetoresistance in magnetic tunnel junctions. These findings provide a microscopic framework for fluctuation-driven spin dynamics and outline a device-level pathway toward spin-based quantum true random number generation.

cond-mat.mes-hall↗

arXiv2025

Spatiotemporal Raman Probing of Molecular Transport in sub-2-nm Plasmonic Quasi-2D Nanochannels

Capturing molecular dynamics in nanoconfined channels with high spatiotemporal resolution is a key challenge in nanoscience, crucial for advancing catalysis, energy conversion, and molecular sensing. Bottom-up ultrathin plasmonic nanogaps, such as nanoparticle-on-mirror (NPoM) structures, are ideal for ultrasensitive probing due to their extreme light confinement, but their perceived sealed geometry has cast doubt on the existence of accessible transport pathways. Here, counterintuitively, we demonstrate that ubiquitous ligand-capped NPoM-type nanogaps can form a natural quasi-two-dimensional nanochannel, supporting molecular transport over unprecedented length scales ($\gtrsim5$ $\mu$m) with an extreme aspect ratio ($>10^3$). Using wavelength-multiplexed Raman spectroscopy, we resolve the underlying centripetal infiltration pathway with a spatial resolving power of $\sim$20 nm. This redefines the NPoM architecture as a sensitive, \textit{in-situ}, all-in-one "transport-and-probe" platform, enabling real-time, reusable monitoring of analyte with $\sim$10$^{-11}$ M. This work establishes a versatile new platform for advancing super-resolved \textit{in-situ} molecular sensing, nanoscale physicochemical studies, and on-chip nanophotofluidics.

physics.optics↗

arXiv2025

Quantitative Benchmarking of Remote Excitation in Plasmonic Sensing with Enhanced Signal-to-Noise Ratio

Remote excitation using guided optical modes -- such as waveguides, fibers, or surface waves -- offers a promising alternative to direct optical excitation for surface-enhanced Raman scattering (SERS), particularly in applications requiring reduced heating, minimal invasiveness, and on-chip integration. However, despite its widespread use, systematic comparisons between remote and direct excitation remain limited. Here, we quantitatively benchmark both schemes by measuring power-dependent SERS responses from individual plasmonic nanogaps. We statistically analyze the maximum achievable SERS intensity before structural degradation, extract local temperatures, and evaluate signal-to-noise ratios (SNR). Our findings reveal that both remote and direct SERS share a common electric-field limit, despite exhibiting different levels of heating. This suggests that spectral evolution is primarily governed by the local electric field, which drives nanoscale atomic migration rather than excessive heating. Nonetheless, the lower heating associated with remote excitation enhances the Raman SNR by approximately 30%, improving measurement quality without compromising signal strength. This study establishes a quantitative framework for evaluating excitation strategies in plasmonic sensing, and challenges common assumptions about the role of heating in nanostructural stability under strong optical excitation.

physics.optics↗

arXiv2025

Seeing Beyond RGB Capabilities: Data-Driven and Physics-Guided Broadband Spectral Extrapolation of Plasmonic Nanostructures by Deep Learning

Localized surface plasmons can confine light within a deep-subwavelength volume comparable to the scale of atoms and molecules, enabling ultrasensitive responses to near-field variations. On the other hand, this extreme localization also inevitably amplifies the unwanted noise from the response of local morphological imperfections, leading to complex spectral variations and reduced consistency across the plasmonic nanostructures. Seeking uniform optical responses has therefore long been a sought-after goal in nanoplasmonics. However, conventional probing techniques by dark-field (DF) confocal microscopy, such as image analysis or spectral measurements, can be inaccurate and time-consuming, respectively. Here, we introduce SPARX, a deep-learning-powered paradigm that surpasses conventional imaging and spectroscopic capabilities. In particular, SPARX can batch-predict broadband DF spectra (e.g., 500-1000 nm) of numerous nanoparticles simultaneously from an information-limited RGB image (i.e., below 700 nm). It achieves this extrapolative inference beyond the camera's capture capabilities by learning the underlying physical relationships among multiple orders of optical resonances. The spectral predictions only take milliseconds, achieving a speedup of three to four orders of magnitude compared to traditional spectral acquisition, which may take from hours to days. As a proof-of-principle demonstration for screening identical resonances, the selection accuracy achieved by SPARX is comparable to that of conventional spectroscopy techniques. This breakthrough paves the way for consistent plasmonic applications and next-generation microscopies.

physics.optics↗

arXiv2025

Nonlinear Chiroptical Effect in Refractory Plasmonic Molybdenum Metasurface: Chiral Saturated Absorption and Chiral Reverse Saturable Absorption

The absorptive chiral metasurface shows evidence of giant nonlinear chiroptical effects, including chiral third harmonic generation, chiral saturated absorption, and chiral reverse saturable absorption. We finally demonstrate proof of concept circular polarized light limiter based on the refractory chiral Mo metasurface and paves the way for nonlinear chiral sensing, nonlinear hot electron generation, and XOR gate of the all-optical full-adder, showcasing the potential of refractory chiral Mo metasurfaces in overcoming the limitations of traditional chiral plasmonic materials.

physics.optics↗

arXiv2023

Bose condensation of upper-branch exciton-polaritons in a transferrable microcavity

Exciton-polaritons are composite bosonic quasiparticles arising from the strong coupling of excitonic transitions and optical modes. Exciton-polaritons have triggered wide exploration in the past decades not only due to their rich quantum phenomena such as superfluidity, superconductivity and quantized vortices but also due to their potential applications for unconventional coherent light sources and all-optical control elements. Here, we report the observation of Bose-Einstein condensation of the upper polariton branch in a transferrable WS$_2$ monolayer microcavity. Near the condensation threshold, we observe a nonlinear increase in upper polariton intensity. This sharp increase in intensity is accompanied by a decrease of the linewidth and an increase of the upper polariton temporal coherence, all of which are hallmarks of Bose-Einstein condensation. By simulating the quantum Boltzmann equation, we show that the upper polariton condensation only occurs for a particular range of particle density. We can attribute the creation of Bose condensation of the upper polariton to the following requirements: 1) the upper polariton is more excitonic than the lower one; 2) there is relatively more pumping in the upper branch; and 3) the conversion time from the upper to the lower polariton branch is long compared to the lifetime of the upper polaritons.

cond-mat.quant-gas↗

arXiv2023

Transverse spin-orbit interaction of light

Light carries both longitudinal and transverse spin angular momentum. The spin can couple with its orbital counterpart via the Berry phase, known as the spin-orbit interaction (SOI) of light. The SOI of light discovered previously belongs to the longitudinal one, which relies on the Berry phase in momentum space, such as the optical Magnus effect and the spin Hall effect. Here, we show that transverse SOI, relying on the Berry phase in real space, is inherent in the Helmholtz equation when transverse spinning light propagates in curved paths. The transverse SOI lifts the degeneracy of dispersion relations of light for opposite transverse spin states, analogous to the Dresselhaus effect. Transverse SOI is ubiquitous in nanophotonic systems where transverse spin and optical path bending are inevitable. It can also explain anomalous effects like the dispersion relation of surface plasmon polariton on curved paths and the energy level of whispering gallery modes. Our results reveal the analogies of spin photonics and spintronics and offer a new degree of freedom for integrated photonics, spin photonics, and astrophysics.

physics.optics↗

arXiv2023

Ultrafast Plasmon-mediated Superradiance from Vertically Standing Molecules in Metallic Nanocavities

Plasmon-mediated superradiance for molecules around metallic nanospheres was proposed ten years ago. However, its demonstration has not been achieved yet due to the experimental difficulty of positioning molecules, and the theoretical limitation to the enhanced collective rate of low excited molecules. In this Letter, we propose that the ultrafast plasmon-mediated superradiant pulses can be observed with strongly excited methylene blue molecules standing vertically inside gold nanoparticle-on-mirror nanocavities. Our simulations indicate that in this system the molecules could interact with each other via plasmon- and free-space mediated coherent and dissipative coupling. More importantly, the coherent coupling mediated by short-ranged propagating surface plasmons cancel largely the direct dipole-dipole coupling mediated by the free-space field, and the dominated dissipative coupling mediated by relatively long-ranged gap plasmons enables the ultrafast superradiant pulses within picosecond scale. Our study opens up the possibility of studying the rich superradiant effects from the quantum emitters in a sub-wavelength volumn by engineering the plasmonic environments.

quant-ph↗

arXiv2022

Spin flips of electron beams in optical near fields

Manipulating the spin polarization of electron beams using light is highly desirable but exceedingly challenging, as the approaches proposed in previous studies using free-space light usually require enormous laser intensities. Here, we propose the use of a transverse electric optical near field, extended on nanostructures, to efficiently induce spin flips of an adjacent electron beam by exploiting the strong inelastic electron scattering in phase-matched optical near fields. Our calculations show that the use of a dramatically reduced laser intensity ($\sim 10^{12}\,$W/cm$^2$) with a short interaction length ($16\,μ$m) achieves an electron spin-flip probability of approximately $12\%$. Intriguingly, the two spin components of an unpolarized incident electron beam -- parallel and antiparallel to the electric field -- are spin-flipped and inelastically scattered to different energy states, providing an analog of the Stern--Gerlach experiment in the energy dimension. Our findings are important for optical control of free-electron spins, preparation of spin-polarized electron beams, and applications as varied as in material science and high-energy physics.

physics.optics↗

arXiv2021

Femtosecond dynamics of a polariton bosonic cascade at room temperature

Whispering gallery modes in a microwire are characterized by a nearly equidistant energy spectrum. In the strong exciton-photon coupling regime, this system represents a bosonic cascade: a ladder of discrete energy levels that sustains stimulated transitions between neighboring steps. In this work, by using femtosecond angle-resolved spectroscopic imaging technique, the ultrafast dynamics of polaritons in a bosonic cascade based on a one-dimensional ZnO whispering gallery microcavity is explicitly visualized. Clear ladder-form build-up process from higher to lower energy branches of the polariton condensates are observed, which are well reproduced by modeling using rate equations. Moreover, the polariton parametric scattering dynamics are distinguished on a timescale of hundreds of femtoseconds. Our understanding of the femtosecond condensation and scattering dynamics paves the way towards ultrafast coherent control of polaritons at room temperature, which will make it promising for high-speed all-optical integrated applications.

physics.optics↗

arXiv2020

Emergence of material momentum in optical media

Understanding the momentum of light when propagating through optical media is not only fundamental for studies as varied as classical electrodynamics and polaritonics in condensed matter physics, but also for important applications such as optical-force manipulations and photovoltaics. From a microscopic perspective, an optical medium is in fact a complex system that can split the light momentum into the electromagnetic field, as well as the material electrons and the ionic lattice. Here, we disentangle the partition of momentum associated with light propagation in optical media, and develop a quantum theory to explicitly calculate its distribution. The material momentum here revealed, which is distributed among electrons and ionic lattice, leads to the prediction of unexpected phenomena. In particular, the electron momentum manifests through an intrinsic DC current, and strikingly, we find that under certain conditions this current can be along the photonic wave vector, implying an optical pulling effect on the electrons. Likewise, an optical pulling effect on the lattice can also be observed, such as in graphene during plasmon propagation. We also predict the emergence of boundary electric dipoles associated with light transmission through finite media, offering a microscopic explanation of optical pressure on material boundaries.

physics.optics↗

arXiv2020

Anomalous thermodiffusion of electrons in graphene

We reveal a dramatic departure of electron thermodiffusion in solids relative to the commonly accepted picture of the ideal free-electron gas model. In particular, we show that the interaction with the lattice and impurities, combined with a strong material dependence of the electron dispersion relation, leads to counterintuitive diffusion behavior, which we identify by comparing a single-layer two-dimensional electron gas (2DEG) and graphene. When subject to a temperature gradient $\nabla T$, thermodiffusion of massless Dirac electrons in graphene exhibits an anomalous behavior with electrons moving along $\nabla T$ and accumulating in hot regions, in contrast to normal electron diffusion in a 2DEG with parabolic dispersion, where net motion against $\nabla T$ is observed, accompanied by electron depletion in hot regions. These findings have fundamentally importance for the understanding of the spatial electron dynamics in emerging material, establishing close relations with other branches of physics dealing with electron systems under nonuniform temperature conditions.

cond-mat.mes-hall↗

arXiv2019

Rotational Doppler cooling and heating

Doppler cooling is a widely used technique to laser cool atoms and nanoparticles exploiting the Doppler shift involved in translational transformations. The rotational Doppler effect arising from rotational coordinate transformations should similarly enable optical manipulations of the rotational degrees of freedom in rotating nanosystems. Here, we show that rotational Doppler cooling and heating (RDC and RDH) effects embody rich and unexplored physics, such as a strong dependence on particle morphology. For geometrically confined particles, such as a nanorod that can represent diatomic molecules, RDC and RDH follow similar rules as their translational Doppler counterpart, where cooling and heating are always observed at red- or blue-detuned laser frequencies, respectively. Surprisingly, nanosystems that can be modeled as a solid particle shows a strikingly different response, where RDH appears in a frequency regime close to their resonances, while a detuned frequency produces cooling of rotation. We also predict that the RDH effect can lead to unprecedented spontaneous chiral symmetry breaking, whereby an achiral particle under linearly polarized illumination starts spontaneously rotating, rendering it nontrivial compared to the translational Doppler effect. Our results open up new exciting possibilities to control the rotational motion of molecules and nanoparticles.

physics.optics↗

arXiv2019

Optical Black-hole Analog Created by Topological Phase Transition with a Long-lived Horizon

Hawking radiation, a manifestation of quantum field theory in curved spacetime, has stimulated extensive theoretical and experimental studies of various black-hole (BH) analogs. However, an undisputed confirmation of Hawking radiation remains elusive. One challenge is BH analog structures with long-lived horizons are difficult to achieve. Here, we theoretically demonstrate a new type of optical BH analog based on light cone evolution associated with topological phase transition of Dirac cones. The transition from a type-II to type-I Dirac/Weyl cone creates an analogous curved spacetime that crosses a type-III Dirac/Weyl cone, which affords a stationary configuration of long-lived event horizon. Photons tunneling through the horizon emit a spectrum of Hawking radiation. As an example, we design a laboratory version in an inhomogeneous two-dimensional graphyne-like topological photonic lattice with a Hawking temperature of 0.14 mK. Understanding Hawking-like radiation in this unique topological BH is not only of fundamental interest in its own right but may also provide new hints to gravitational physics.

cond-mat.mes-hall↗

arXiv2019

Magnetically Activated Rotational Vacuum Friction

We predict the existence of a torque acting on an isotropic neutral nanosphere activated by a static magnetic field when the particle temperature differs from the surrounding vacuum. This phenomenon originates in time-reversal symmetry breaking of the particle interaction with the vacuum electromagnetic field. We present a rigorous quantum treatment of photons and particle excitations that leads to a nonzero torque even in a motionless particle. We also find that the dynamical evolution of the particle temperature and rotation frequency follow an exotic dynamics, including spontaneous changes in the rotation direction. Magnetically activated thermal vacuum torques open a unique avenue for the investigation of the effect of time-reversal symmetry-breaking in thermal and Casimir physics.

cond-mat.mes-hall↗

arXiv2019

Collective modes in two dimensional topological superconductors

Collective modes in two dimensional topological superconductors are studied by an extended random phase approximation theory while considering the influence of vector field of light. In two situations, the s-wave superconductors without spin-orbit-coupling (SOC), and the hybrid semiconductor and s-wave superconductor layers with strong SOC, we get the analytical results for longitudinal modes which are found to be indeed gapless. Further more, the effective modes volumes can be calculated, the electric and magnetic fields can be expressed as the creation and annihilation operators of such modes. So, one can study the interaction of them with other quasi-particles through fields.

cond-mat.supr-con↗