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Huaqing Huang

Publications and source records attributed to Huaqing Huang.

At least 19 recordsLinked to original sources

Cuprate d-wave superconductivity based on Non perturbative many body theory for spin fluctuation

We employ the nonperturbative many-body spin GW method to compute the single-particle Green's function, and the covariance method to evaluate the two-body correlation functions, for the Hubbard model of superconductors. The method, benchmarked at strong coupling and low temperatures, allows simulations on lattices up to $64\times64$, thereby enabling access to the thermodynamic limit. We find the key transition temperatures---namely the Néel temperature and the superconducting critical temperature $T_c$---to be in quantitative agreement with experimental data. Above the $d$-wave superconducting dome, there exists a broad pseudogap region in which the normal-state excitations are suppressed. These results indicate our approach may offer a new route toward investigating strongly correlated systems, especially cuprate superconductors.

cond-mat.str-el

Extrinsic nonlinear spin currents in spin-orbit coupled systems: A Boltzmann transport study

We develop a semiclassical Boltzmann framework for second-order extrinsic spin transport in the presence of skew scattering. The conventional relaxation-time approximation reduces the full collision integral to a single phenomenological timescale and thereby neglects the angular structure of impurity scattering. While the transport relaxation time primarily characterizes the leading angular harmonic of the nonequilibrium distribution, nonlinear response is sensitive to its higher angular harmonics, which are governed by distinct components of the collision operator. We therefore retain the angular and band dependence of the scattering kernel and decompose both the collision integral and the distribution function into Fourier harmonics. The resulting coupled algebraic equations allow the symmetric and skew-scattering corrections to the distribution function to be obtained recursively order by order in the electric field. We apply this formalism to the gapped surface states of a topological insulator with spin-dependent impurity scattering and evaluate the corresponding second-order extrinsic spin-current response. Our results show that higher angular harmonics of the nonequilibrium distribution and scattering between distinct constant-energy contours play an essential role in extrinsic nonlinear spin transport beyond the single-relaxation-time approximation.

cond-mat.mes-hall

Terahertz frequency upconversion by coherently driving charge dynamics in the InSb/CdTe heterostructure

We investigate terahertz (THz) harmonic generation in the InSb/CdTe heterostructure, demonstrating, for the first time, efficient in-plane magnetic field-induced second-harmonic generation (SHG). We also achieve significant third-harmonic generation (THG), rivalling Dirac materials such as graphene and Cd3As2. Our theoretical analysis identifies the primary SHG mechanism as the orbital-Zeeman correction to Drude conductivity, while the dominant THG contribution also shows Drude-like behavior. The results provide a general route to efficient THz harmonic generation in high mobility materials.

cond-mat.mtrl-sci

Thickness-Independent Quantum Geometric Responses Driven by Interlayer Antiferroic Coupling

Two-dimensional ferroic materials exhibit rich and intriguing physical phenomena, but their response properties generally depend sensitively on thickness, requiring precise layer-number control and thereby limiting practical applications. Here, we propose a general strategy for realizing thickness-independent quantum geometric responses through symmetry engineering induced by interlayer antiferroic coupling. Using spatial-dependent symmetry analysis, we show that thickness-independent behavior emerges when the symmetry breaking required for a given response is generated by interlayer antiferromagnetic (AFM) or antiferroelectric (AFE) coupling, without invoking topological mechanisms. Our first-principles calculations predict that multilayer MnS in the G-type AFM configuration exhibits a surface-dominated anomalous Hall effect, whose thickness-independent behavior can be significantly influenced by the stacking order. We further propose design principles for achieving thickness-independent anomalous and nonlinear Hall effects driven by interlayer AFE coupling, and suggest potential applications in distinguishing magnetic structures. Our findings open a new route towards robust functional devices based on antiferroic materials.

cond-mat.mtrl-sci

Orbital Altermagnetism in Two Dimensions

We introduce the concept of \emph{orbital altermagnetism}, a symmetry-protected magnetic order of pure orbital degrees of freedom. It is characterized with ordered anti-parallel orbital magnetic moments in real space but momentum-dependent orbital band splittings, analogous to spin altermagnetism. Using a minimal tight-binding model with complex hoppings in a square-kagome lattice, we show that such order inherently arises from staggered loop currents, producing a $d$-wave-like orbital-momentum locking. First-principles calculations show that orbital altermagnetism emerges independent of spin ordering in in-plane ferromagnets of CuBr$_2$ and VS$_2$, so that it can be unambiguously identified experimentally. On the other hand, it may also coexist with spin altermagnetism, such as in monolayer MoO and CrO. The orbital altermagnetism offers an alternative platform for symmetry-driven magnetotransport and orbital-based spintronics, as exemplified by large nonlinear current-induced orbital magnetization.

cond-mat.mtrl-sci

Hierarchical Structures of Quantum Geometric Spectrum in Quasicrystals: A Renormalization-Group Study

Quantum geometry, characterized by the quantum metric and Berry curvature, is a powerful framework for understanding diverse physical phenomena in quantum materials, but its behavior in non-periodic systems remains largely uncharted. Here, we uncover a universal mechanism for the divergent enhancement of the quantum metric in one-dimensional quasiperiodic systems, governed by the interplay of wavefunction criticality and spectral fractality. Using the paradigmatic Fibonacci chain, we demonstrate that the quantum metric displays a hierarchical scaling structure that mirrors the fractal organization of the energy spectrum. A real-space renormalization-group analysis yields an analytic power-law scaling, $\mathcal{G} \propto (ΔE)^{-k}$, between the quantum metric $\mathcal{G}$ and spectral gap $ΔE$, with the exponent $k$ dictated by the system's self-similarity. This scaling persists in the critical Aubry-André-Harper model but disappears in both its localized and extended phases, confirming its universality across different quasiperiodic paradigms and its unique link to criticality. Our results show that the quantum metric provides a sensitive geometric indicator of quasiperiodic criticality, and highlight quasicrystals as promising platforms for realizing unconventional giant quantum geometric effects beyond the limits of periodic crystals.

cond-mat.mes-hall

Quantum geometry induced anomalous chiral transport and hidden symmetry breaking in centrosymmetric 2M-WS2

Chirality, a widely existing material property in nature involving the breaking of the left-right symmetry, has profound influences in various fields of natural sciences. Nonlinear response, such as electronic magnetochiral anisotropy (eMChA), has been recognized as a sensitive probe for the effects of symmetry breaking and nontrivial quantum geometries in solids. So far, observations of eMChA have primarily been limited to inversion-symmetry broken materials. Here, we report a remarkable chiral transport in centrosymmetric candidate topological superconductor 2M-WS2 flakes observed via second-harmonic generation under an out-of-plane magnetic field. More importantly, the eMChA becomes significant around the crossover temperature TFL ~ 25 K from the Fermi liquid (FL) to strange metal (SM) in the normal state, which interestingly echoes with the anomalously large Nernst response at the same temperature in bulk 2M-WS2. These observations reveal a direct correspondence between the nonlinear response, Nernst response, and FL-SM transition in 2M-WS2. Theoretical analysis indicates that nontrivial quantum geometry is behind the simultaneous response of eMChA and Nernst effects in 2M-WS2 and the contribution from the orbital magnetic moment at the Fermi surface becomes significant during the FL-SM transition. Based on first-principles calculations, a thick-layer-sliding mechanism with minimal energy gain in 2M-WS2 provides one possibility for the generation of such nontrivial quantum geometry. The intertwined physics of remarkable eMChA, Nernst response, and FL-SM transition make 2M-WS2 a rare quantum platform to study the chiral transport and unexplored phenomena in strange metals, which may shed light on the trans-century, unresolved scientific issue in unconventional high-temperature superconductivity.

cond-mat.str-el

Sub-50 Picosecond exceptionally Bright Perovskite Scintillation by Unlocking Giant Oscillator Strength

Ultrafast scintillators are indispensable for precise timing in high-energy physics and medical diagnostics. Fundamentally constrained by the trade-off between emission rate and light yield, conventional scintillators remain kinetically trapped in the sub-nanosecond regime, failing to break 50-picosecond limit. Here, we demonstrate a strategy to bypass this limitation by harnessing the coherent radiative acceleration in weakly confined CsPbCl3 perovskite nanocrystals to generate an ultrafast photon burst. This effect originates from the giant oscillator strength, which we unlock by suppressing exciton-phonon scattering at mild cryogenic temperatures. Consequently, our scintillator achieves an unprecedented dominant lifetime of 13.11 ps alongside a high light yield of 21,851 ph/MeV. The resulting prompt photon emission rate more than 100 times higher than that of state-of-the-art ultrafast scintillators. We validate this breakthrough in realistic detection scenarios, achieving a coincidence time resolution of 30.8 ps and accurately resolving 13.5 ps electron bunches and 16.6 ps single-shot gamma-ray pulses. Our findings establish a robust coherent framework for next-generation ultrafast scintillators, pushing extreme radiation diagnostics into the picosecond frontier.

cond-mat.mes-hall

Unconventional Altermagnetism in Quasicrystals: A Hyperspatial Projective Construction

Altermagnetism, a novel magnetic phase characterized by symmetry-protected, momentum-dependent spin splitting and collinear compensated magnetic moments, has thus far been explored primarily in periodic crystals. In this Letter, we extend the concept of altermagnetism to quasicrystals -- aperiodic systems with long-range order and noncrystallographic rotational symmetries. Using a hyperspatial projection framework, we construct decorated Ammann-Beenker and Penrose quasicrystalline lattices with inequivalent sublattices and investigate a Hubbard model with anisotropic hopping. We demonstrate that interaction-induced Néel order on such lattices gives rise to alternating spin-polarized spectral functions that reflect the underlying quasicrystalline symmetry, revealing the emergence of unconventional $g$-wave (octagonal) and $h$-wave (decagonal) altermagnetism. Our symmetry analysis and low-energy effective theory further reveal unconventional altermagnetic spin splitting, which is compatible with quasicrystalline rotational symmetry. Our work shows that quasicrystals provide a fertile ground for realizing unconventional altermagnetic phases beyond crystallographic constraints, offering a platform for novel magnetisms and transport phenomena unique to quasiperiodic systems.

cond-mat.mes-hall

Nonpertubative Many-Body Theory for the Two-Dimensional Hubbard Model at Low Temperature: From Weak to Strong Coupling Regimes

In theoretical studies of two-dimensional (2D) systems, the Mermin-Wagner theorem prevents continuous symmetry breaking at any finite temperature, thus forbidding a Landau phase transition at a critical temperature $T_c$. The difficulty arises when many-body theoretical studies predict a Landau phase transition at finite temperatures, which contradicts the Mermin-Wagner theorem and is termed a pseudo phase transition. To tackle this problem, we systematically develop a symmetrization scheme, defined as averaging physical quantities over all symmetry-breaking states, thus ensuring that it preserves the Mermin-Wagner theorem. We apply the symmetrization scheme to the GW-covariance calculation for the 2D repulsive Hubbard model at half-filling in the intermediate-to-strong coupling regime and at low temperatures, obtaining the one-body Green's function and spin-spin correlation function, and benchmark them against Determinant Quantum Monte Carlo (DQMC) with good agreement.The spin-spin correlation functions are approached within the covariance theory, a general method for calculating two-body correlation functions from a one-particle starting point, such as the GW formalism used here, which ensures the preservation of the fundamental fluctuation-dissipation relation (FDR) and Ward-Takahashi identities (WTI). With the FDR and WTI satisfied, we conjecture that the $χ$-sum rule, a fundamental relation from the Pauli exclusion principle, can be used to probe the reliability of many-body methods, and demonstrate this by comparing the GW-covariance and mean-field-covariance approaches. This work provides a novel framework to investigate the strong-coupling and doped regime of the 2D Hubbard model, which is believed to be applicable to real high-$T_c$ cuprate superconductors.

cond-mat.str-el

Magnetic-Field Tunable Möbius and Higher-Order Topological Insulators in Three-Dimensional Layered Octagonal Quasicrystals

We propose that three-dimensional layered octagonal quasicrystals can host magnetic-field-tunable Möbius insulators and various higher-order topological insulators (HOTIs), enabled by the interplay of quasicrystalline symmetry and magnetic order. By constructing a minimal model based on stacked Ammann-Beenker tilings with magnetic exchange coupling and octagonal warping, we demonstrate that an A-type antiferromagnetic (AFM) configuration yields a topological phase protected by an effective time-reversal symmetry $\mathcal{S}=\mathcal{T}τ_{1/2}$. Breaking $\mathcal{S}$ via an in-plane magnetic field induced canting of the AFM order while preserving a nonsymmorphic glide symmetry $\mathcal{G}_n=τ_{1/2}\mathcal{M}_n$ leads to Möbius-twisted surface states, realizing a Möbius insulator in an aperiodic 3D system. Furthermore, we show that the quasicrystal with a general magnetic configuration supports multiple HOTI phases characterized by distinct hinge mode configurations that can be switched by rotating the magnetic field. A low-energy effective theory reveals that these transitions are driven by mass kinks between adjacent surfaces. Our work establishes a platform for realizing symmetry-protected topological phases unique to quasicrystals and highlights the tunability of hinge and surface states via magnetic control.

cond-mat.mes-hall

Two-Terminal Electrical Detection of the Néel Vector via Longitudinal Antiferromagnetic Nonreciprocal Transport

We propose a robust two-terminal electrical readout scheme for detecting the Néel vector orientation in antiferromagnetic (AFM) materials by leveraging longitudinal nonreciprocal transport driven by quantum metric dipoles. Unlike conventional readout mechanisms, our approach does not require spin-polarized electrodes, tunneling junctions, or multi-terminal geometries, offering a universal and scalable solution for AFM spintronics. As examples, we demonstrate pronounced second-order longitudinal nonlinear conductivity (LNC) in two-dimensional (2D) MnS and 3D CuMnAs, both of which exhibit clear sign reversal of LNC under 180$^\circ$ Néel vector reorientation. We show that this LNC is predominantly governed by the intrinsic, relaxation-time-independent quantum metric mechanism rather than the extrinsic nonlinear Drude effect. Our findings provide a practical and material-general pathway for electrically reading AFM memory states, with promising implications for next-generation AFM spintronic technologies.

cond-mat.mtrl-sci

Quantum Metric-induced Oscillations in Flat Bands

The transport of Bloch electrons under strong fields is traditionally understood through two mechanisms: intraband Bloch oscillations and interband Zener tunneling. Here, we propose an oscillation mechanism induced by the interband quantum metric, which would significantly affect the electron dynamics under strong fields. By considering the multiband dynamics to the second order of the density matrix, we reveal that quantum metric induced oscillations (QMOs) persist regardless of band dispersion, even in exactly dispersionless flat bands. The resultant drift current can reach a magnitude comparable to the Bloch oscillation induced drift current in systems where interband tunneling is negligible. Notably, the QMO induced drift current increases linearly with electric field strength under the constraints of time-reversal or spatial-inversion symmetry, emerging as the primary delocalized current. We further show that both one-dimensional and two-dimensional superlattices are potential platforms for investigating QMO.

cond-mat.mes-hall

Effects of the pseudogap and the Fermi surface on the rapid Hall-coefficient changes in cuprates

High-$T_c$ cuprates are characterized by strong spin fluctuations, which give rise to antiferromagnetic and pseudogap phases and may be key to the high superconducting critical temperatures observed in these materials. Experimental studies have revealed significant changes in the Hall coefficient $R_H$ across these phases, a phenomenon closely related to both spin fluctuations and changes in the Fermi surface morphology. Using the perturbation correction to Gaussian approximation (PCGA), we investigate the two-dimensional(2D) square-lattice single-band Hubbard model and obtain the self-energy with a finite imaginary part due to scattering. We calculate the density dependence of the Hall number $n_H=1/(qR_H)$. For small hole (or electron) doping $p$ (or $x$), our numerical results show that $n_H$ transitions from $p$ to $1+p$ for hole-doped systems, and from $-x$ to $1-x$ for electron-doped systems -- both in agreement with experimental findings. Furthermore, we discuss the correlation between phase boundaries and the observed peculiar changes in the Hall number.

cond-mat.str-el

Chiral Topological Phononic Quasiparticles in Enantiomeric Crystals SrSi$_2$ and BaSi$_2$

Chiral crystals have recently garnered significant interest in condensed matter physics due to their unique electronic and optical properties. In this paper, we explore the connection between the chirality of crystal structures and the chirality of topological quasiparticles. We specifically predict and analyze several chiral enantiomeric materials, such as SrSi$_2$ and BaSi$_2$, which crystallize in the chiral space groups $P4{_3}32$ and $P4{_1}32$. Based on first-principles calculations and theoretical analysis, we reveal that the phonon spectra of these materials host various topological phononic quasiparticles, including charge-2 triple points, charge-2 Dirac points, charge-2 Weyl points, and charge-1 Weyl points. Our paper shows that in these enantiomeric materials, the opposite chirality of the crystal structure results in topological quasiparticles with opposite chiral topological charges and distinct topological surface states. Our paper elucidates the intrinsic relationship between the chirality of crystal structures and the chirality of topological quasiparticles, providing promising theoretical guidance and material platform for investigating the physical properties of chiral crystals.

cond-mat.mtrl-sci

Post-$GW$ theory and its application to pseudogap in strongly correlated system

The $GW$ approximation is a widely used framework for studying correlated materials, but it struggles with certain limitations, such as its inability to explain pseudogap phenomena. To overcome these problems, we propose a systematic theoretical framework for Green's function corrections and apply it specifically to the $GW$ approximation. In this new theory, the screened potential is reconnected to the physical response function, i.e. the covariant response function proposed in \cite{cGW_2023}, rather than using the RPA formula. We apply our scheme to calculate Green's function, the spectral function, and the charge compressibility in the two-dimensional Hubbard model. Our scheme yields significant qualitative and quantitative improvements over the standard $GW$ method and successfully captures the pseudogap behavior.

cond-mat.str-el

Intrinsic Orbital Origin for the Chirality-Dependent Nonlinear Planar Hall Effect of Topological Nodal Fermions in Chiral Crystals

Topological semimetals in chiral crystals, which possess both structural handedness and band crossings (or nodes) with topological chiral charge, exhibit many exotic physical properties. Here we demonstrate that the structural and electronic chirality of these systems can endow them with another fascinating phenomenon -- the intrinsic nonlinear planar Hall effect (INPHE), which is prominent around the nodes and reverses sign upon chirality reversal in opposite enantiomers. Taking chiral tellurium as an example, we reveal an intrinsic orbital mechanism, which manifests diverging orbital magnetic moments with hedgehog-like textures around nodes and, therefore, generates a dominant contribution to the INPHE that is proportional to the topological charge. Furthermore, we show that multifold fermions in topological chiral semimetals with B20 structures (e.g., CoSi and PtAl) induce a giant INPHE conductivity reaching the order of $1\sim 10\; \mathrm{A}\cdot\mathrm{V}^{-2}\cdot\mathrm{T}^{-1}$, which is detectable in experiments. Our study not only relates nonlinear transport to band topology and enantiomer recognition but also offers a new way to explore the exotic physical properties associated with unconventional chiral fermions.

cond-mat.mes-hall

Decomposing Electronic Structures in Twisted Multilayers: Bridging Spectra and Incommensurate Wave Functions

Twisted multilayer systems, encompassing materials like twisted bilayer graphene (TBG), twisted trilayer graphene, and twisted bilayer transition metal dichalcogenides, have garnered significant attention in condensed matter physics. Despite this interest, a comprehensive description of their electronic structure, especially in dealing with incommensurate wave functions, poses a persistent challenge. Here, we introduce a unified theoretical framework for efficiently describing the electronic structure covering both spectrum and wave functions in twisted multilayer systems, accommodating both commensurate and incommensurate scenarios. Our analysis reveals that physical observables in these systems can be systematically decomposed into contributions from individual layers and their respective ${k}$ points, even in the presence of intricate interlayer coupling. This decomposition facilitates the computation of wave function-related quantities relevant to response characteristics beyond spectra. We propose a local low-rank approximated Hamiltonian in the truncated Hilbert space that can achieve any desired accuracy, offering numerical efficiency compared to the previous large-scale calculations. The validity of our theory is confirmed through computations of spectra and optical conductivity for moiré TBG, and demonstrating its applicability in incommensurate quasicrystalline TBG. Our findings provide a generic approach to studying the electronic structure of twisted multilayer systems and pave the way for future research.

cond-mat.mtrl-sci