arXiv subjects

Hugues de Riedmatten

Publications and source records attributed to Hugues de Riedmatten.

At least 37 records · Page 2Linked to original sources

arXiv2022

Storage and analysis of light-matter entanglement in a fibre-integrated system

The deployment of a fully-fledged quantum internet poses the challenge of finding adequate building-blocks for entanglement distribution between remote quantum nodes. An ideal system would combine propagation in optical fibres with quantum memories for light, leveraging on the existing communication network while featuring the scalability required to extend to network sizes. Here we demonstrate a fiber-integrated quantum memory entangled with a photon at telecommunication wavelength. The storage device is based on a fiber-pigtailed laser written waveguide in a rare-earth doped solid and allows an all-fiber stable adressing of the memory. The analysis of the entanglement is performed using fibre-based interferometers. Our results feature orders of magnitude advances in terms of storage time and efficiency for integrated storage of light-matter entanglement, and constitute a significant step forward towards quantum networks using integrated devices.

quant-ph↗

arXiv2021

Ultra-low noise quantum memory for quasi-deterministic single photons generated by Rydberg collective atomic excitations

We demonstrate the storage and retrieval of an on-demand single photon generated by a collective Rydberg excitation in an ultra-low noise Raman quantum memory located in a different cold atomic ensemble. We generate single photons on demand by exciting a cold cloud of Rubidium atoms off resonantly to a Rydberg state, with a generation probability up to 15 $\%$ per trial. We then show that the single photons can be stored and retrieved with an efficiency of 21 $\%$ and a noise floor of $p_n= 2.3(3) \times 10^{-4}$ per trial in the Raman quantum memory. This leads to a signal-to-noise ratio ranging from 11 to 26 for the retrieved single photon depending on the input photon generation probability, which allows us to observe significant antibunching. We also evaluate the performances of the Raman memory as built-in unbalanced temporal beam splitter, tunable by varying the write-in control pulse intensity. In addition, we demonstrate that the Raman memory can be used to control the single-photon waveshape. These results are a step forward in the implementation of efficient quantum-repeater links using single-photon sources.

quant-ph↗

arXiv2021

Entanglement between a telecom photon and an on-demand multimode solid-state quantum memory

Entanglement between photons at telecommunication wavelengths and long-lived quantum memories is one of the fundamental requirements of long-distance quantum communication. Quantum memories featuring on-demand read-out and multimode operation are additional precious assets that will benefit the communication rate. In this work we report the first demonstration of entanglement between a telecom photon and a collective spin excitation in a multimode solid-state quantum memory. Photon pairs are generated through widely non-degenerate parametric down-conversion, featuring energy-time entanglement between the telecom-wavelength idler and a visible signal photon. The latter is stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal as a spin wave using the full Atomic Frequency Comb scheme. We then recall the stored signal photon and analyze the entanglement using the Franson scheme. We measure conditional fidelities of $92(2)\%$ for excited-state storage, enough to violate a CHSH inequality, and $77(2)\%$ for spin-wave storage. Taking advantage of the on-demand read-out from the spin state, we extend the entanglement storage in the quantum memory for up to 47.7~$μ$s, which could allow for the distribution of entanglement between quantum nodes separated by distances of up to 10 km.

quant-ph↗

arXiv2021

Topical White Paper: A Case for Quantum Memories in Space

It has recently been theoretically shown that Quantum Memories (QM) could enable truly global quantum networking when deployed in space thereby surpassing the limited range of land-based quantum repeaters. Furthermore, QM in space could enable novel protocols and long-range entanglement and teleportation applications suitable for Deep-Space links and extended scenarios for fundamental physics tests. In this white paper we will make the case for the importance of deploying QMs to space, and also discuss the major technical milestones and development stages that will need to be considered.

quant-ph↗

arXiv2021

Roadmap for Rare-earth Quantum Computing

Several platforms are being considered as hardware for quantum technologies. For quantum computing (QC), superconducting qubits and artificially trapped ions are among the leading platforms, but many others also show promise, e.g. photons, cold atoms, defect centers including Rare-Earth (RE) ions. So far, results are limited to the regime of noisy intermediate scale qubits (NISQ), with a small number of qubits and a limited connectivity, and it is likely that future QC hardware will utilize several existing platforms in different ways. Thus, it currently makes sense to invest resources broadly and explore the full range of promising routes to quantum technology. Rare-earth ions in solids constitute one of the most versatile platforms for future quantum technology. One advantage is good coherence properties even when confined in strong natural traps inside a solid-state matrix. This confinement allows very high qubit densities and correspondingly strong ion-ion couplings. In addition, although their fluorescence is generally weak, cavity integration can enhance the emission greatly and enable very good connections to photonic circuits, including at the telecom wavelengths, making them promising systems for long-term scalability. The primary aim of this roadmap is to provide a complete picture of what components a RE quantum computer would consist of, to describe the details of all parts required to achieve a scalable system, and to discuss the most promising paths to reach it. In brief, we find that clusters of 50-100 single RE ions can act as high fidelity qubits in small processors, occupying only about (10 nm)^3. Due to the high capacity for integration of the RE systems, they be optically read out and connected to other such clusters for larger scalability. We make suggestions for future improvements, which could allow the REQC platform to be a leading one.

quant-ph↗

arXiv2021

Telecom-heralded entanglement between remote multimode solid-state quantum memories

Future quantum networks will enable the distribution of entanglement between distant locations and allow applications in quantum communication, quantum sensing and distributed quantum computation. At the core of this network lies the ability of generating and storing entanglement at remote, interconnected quantum nodes. While remote physical systems of various nature have been successfully entangled, none of these realisations encompassed all of the requirements for network operation, such as telecom-compatibility and multimode operation. Here we report the demonstration of heralded entanglement between two spatially separated quantum nodes, where the entanglement is stored in multimode solid-state quantum memories. At each node a praseodymium-doped crystal stores a photon of a correlated pair, with the second photon at telecommunication wavelengths. Entanglement between quantum memories placed in different labs is heralded by the detection of a telecom photon at a rate up to 1.4 kHz and is stored in the crystals for a pre-determined storage time up to 25 microseconds. We also show that the generated entanglement is robust against loss in the heralding path, and demonstrate temporally multiplexed operation, with 62 temporal modes. Our realisation is extendable to entanglement over longer distances and provides a viable route towards field-deployed, multiplexed quantum repeaters based on solid-state resources.

quant-ph↗

arXiv2020

Transient dynamics of the quantum light retrieved from Rydberg polaritons

We study the photon statistics of weak coherent pulses propagating through a cold Rydberg atomic ensemble in the regime of Rydberg electromagnetically induced transparency. We show experimentally that the value of the second-order autocorrelation function of the transmitted light strongly depends on the position within the pulse and heavily varies during the transients of the pulse. In particular, we show that the falling edge of the transmitted pulse displays much lower values than the rest of the pulse. We derive a theoretical model that quantitatively predicts our results and explains the physical behavior involved. Finally, we use this effect to generate single photons localized within a pulse from the atomic ensemble. We show that by selecting only the last part of the transmitted pulse, the single photons show an antibunching parameter as low as 0.12 and a generation efficiency per trial larger than possible with probabilistic generation schemes with atomic ensembles.

quant-ph↗

arXiv2020

Probing the indistinguishability of single photons generated by Rydberg atomic ensembles

We investigate the indistinguishability of single photons retrieved from collective Rydberg excitations in cold atomic ensembles. The Rydberg spin waves are created either by off resonant two-photon excitation to the Rydberg state or by Rydberg electromagnetically induced transparency. To assess the indistinguishability of the generated single photons, we perform Hong-Ou-Mandel experiments between the single photons and weak coherent states of light. We analyze the indistinguishability of the single photons as a function of the detection window and for photons generated by off-resonant excitation we infer high value of indistinguishability going from 89% for the full waveform to 98% for small detection windows. In the same way, we also investigate for the first time the indistinguishability of single photons generated by Rydberg EIT, showing values lower than those corresponding to single photons generated by off-resonant excitation. These results are relevant for the use of Rydberg atoms as quantum network nodes.

quant-ph↗

arXiv2020

Fast electrical modulation of strong near-field interactions between erbium emitters and graphene

Combining the quantum optical properties of single-photon emitters with the strong near-field interactions available in nanophotonic and plasmonic systems is a powerful way of creating quantum manipulation and metrological functionalities. The ability to actively and dynamically modulate emitter-environment interactions is of particular interest in this regard. While thermal, mechanical and optical modulation have been demonstrated, electrical modulation has remained an outstanding challenge. Here we realize fast, all-electrical modulation of the near-field interactions between a nanolayer of erbium emitters and graphene, by in-situ tuning the Fermi energy of graphene. We demonstrate strong interactions with a >1,000-fold increased decay rate for 25% of the emitters, and electrically modulate these interactions with frequencies up to 300 kHz - orders of magnitude faster than the emitters radiative decay (100 Hz). This constitutes an enabling platform for integrated quantum technologies, opening routes to quantum entanglement generation by collective plasmon emission or photon emission with controlled waveform.

cond-mat.mes-hall↗

arXiv2020

A cold atom temporally multiplexed quantum memory with cavity-enhanced noise suppression

Future quantum repeater architectures, capable of efficiently distributing information encoded in quantum states of light over large distances, will benefit from multiplexed photonic quantum memories. In this work we demonstrate a temporally multiplexed quantum repeater node in a laser-cooled cloud of $^{87}$Rb atoms. We employ the DLCZ protocol where pairs of photons and single collective spin excitations (so called spin waves) are created in several temporal modes using a train of write pulses. To make the spin waves created in different temporal modes distinguishable and enable selective readout, we control the dephasing and rephasing of the spin waves by a magnetic field gradient, which induces a controlled reversible inhomogeneous broadening of the involved atomic hyperfine levels. We demonstrate that by embedding the atomic ensemble inside a low finesse optical cavity, the additional noise generated in multi-mode operation is strongly suppressed. By employing feed forward readout, we demonstrate distinguishable retrieval of up to 10 temporal modes. For each mode, we prove non-classical correlations between the first and second photon. Furthermore, an enhancement in rates of correlated photon pairs is observed as we increase the number of temporal modes stored in the memory. The reported capability is a key element of a quantum repeater architecture based on multiplexed quantum memories.

quant-ph↗

arXiv2020

Dynamic control of Purcell enhanced emission of erbium ions in nanoparticles

The interaction of single quantum emitters with an optical cavity enables the realization of efficient spin-photon interfaces, an essential resource for quantum networks. The dynamical control of the spontaneous emission rate of quantum emitters in cavities has important implications in quantum technologies, e.g. for shaping the emitted photons waveform, for generating quantum entanglement, or for driving coherently the optical transition while preventing photon emission. Here we demonstrate the dynamical control of the Purcell enhanced emission of a small ensemble of erbium ions doped into nanoparticles. By embedding the doped nanoparticles into a fully tunable high finesse fiber based optical microcavity, we show that we can tune the cavity on- and out of-resonance by controlling its length with sub-nanometer precision, on a time scale more than two orders of magnitude faster than the natural lifetime of the erbium ions. This allows us to shape in real time the Purcell enhanced emission of the ions and to achieve full control over the emitted photons' waveforms. This capability opens prospects for the realization of efficient nanoscale quantum interfaces between solid-state spins and single telecom photons with controllable waveform, and for the realization of quantum gates between rare-earth ion qubits coupled to an optical cavity.

quant-ph↗

arXiv2019

Time Entanglement between a Photon and a Spin Wave in a Multimode Solid-state Quantum Memory

The generation and distribution of entanglement are key resources in quantum repeater schemes. Temporally multiplexed systems offer time-bin encoding of quantum information which provides robustness against decoherence in fibers, crucial in long distance communication. Here we demonstrate the direct generation of entanglement in time between a photon and a collective spin excitation in a rare earth ion doped ensemble. We analyze the entanglement by mapping the atomic excitation onto a photonic qubit and by using time-bin qubits analyzers implemented with another doped crystal using the atomic frequency comb technique. Our results provide a solid-state source of entangled photons with embedded quantum memory. Moreover, the quality of the entanglement is high enough to enable a violation of a Bell inequality by more than two standard deviations.

quant-ph↗

arXiv2019

Laser-written integrated platform for quantum storage of heralded single photons

Efficient and long-lived interfaces between light and matter are crucial for the development of quantum information technologies. Integrated photonics solutions for quantum storage devices offer improved performances due to light confinement and enable more complex and scalable designs. We demonstrate a novel platform for quantum light storage based on laser written waveguides. The new writing regime adopted allows us to attain waveguides with improved confining capabilities compared to previous demonstrations. We report the first demonstration of single photon storage in laser written waveguides. While we achieve storage efficiencies comparable to those observed in massive samples, the power involved for the memory preparation is strongly reduced, by a factor 100, due to an enhancement of the light-matter interaction of almost one order of magnitude. Moreover, we demonstrate excited state storage times 100 times longer than previous realizations with single photons in integrated quantum memories. Our system promises to effectively fulfill the requirements for efficient and scalable integrated quantum storage devices.

quant-ph↗

arXiv2019

Quantum Storage of Frequency-Multiplexed Heralded Single Photons

We report on the quantum storage of a heralded frequency-multiplexed single photon in an integrated laser-written rare-earth doped waveguide. The single photon contains 15 discrete frequency modes separated by 261 MHz and spaning across 4 GHz. It is obtained from a non-degenerate photon pair created via cavity-enhanced spontaneous down conversion, where the heralding photon is at telecom wavelength and the heralded photon is at 606 nm. The frequency-multimode photon is stored in a praseodymium-doped waveguide using the atomic frequency comb (AFC) scheme, by creating multiple combs within the inhomogeneous broadening of the crystal. Thanks to the intrinsic temporal multimodality of the AFC scheme, each spectral bin includes 9 temporal modes, such that the total number of stored modes is about 130. We demonstrate that the storage preserves the non-classical properties of the single photon, and its normalized frequency spectrum.

quant-ph↗

arXiv2018

Cavity-enhanced spectroscopy of a few-ion ensemble in Eu3+:Y2O3

We report on the coupling of the emission from a single europium-doped nanocrystal to a fiber-based microcavity under cryogenic conditions. As a first step, we study the sample properties and observe a strong correlation between emission lifetime and brightness, as well as a lifetime reduction for nanocrystals embedded in a polymer film. This is explained by differences in the local density of states. We furthermore quantify the scattering loss of a nanocrystal inside the cavity and use this to deduce the crystal size. Finally, by resonantly coupling the cavity to a selected transition, we perform cavity-enhanced spectroscopy to measure the inhomogeneous linewidth, and detect the fluorescence from an ensemble of few ions in the regime of power broadening. We observe an increased fluorescence rate consistent with Purcell enhancement. The results represent an important step towards the efficient readout of single rare-earth ions with excellent optical and spin coherence properties, which is promising for applications in quantum communication and distributed quantum computation.

physics.optics↗

arXiv2018

Photonic quantum state transfer between a cold atomic gas and a crystal

Interfacing fundamentally different quantum systems is key to build future hybrid quantum networks. Such heterogeneous networks offer superior capabilities compared to their homogeneous counterparts as they merge individual advantages of disparate quantum nodes in a single network architecture. However, only very few investigations on optical hybrid-interconnections have been carried out due to the high fundamental and technological challenges, which involve e.g. wavelength and bandwidth matching of the interfacing photons. Here we report the first optical quantum interconnection between two disparate matter quantum systems with photon storage capabilities. We show that a quantum state can be faithfully transferred between a cold atomic ensemble and a rare-earth doped crystal via a single photon at telecommunication wavelength, using cascaded quantum frequency conversion. We first demonstrate that quantum correlations between a photon and a single collective spin excitation in the cold atomic ensemble can be transferred onto the solid-state system. We also show that single-photon time-bin qubits generated in the cold atomic ensemble can be converted, stored and retrieved from the crystal with a conditional qubit fidelity of more than $85\%$. Our results open prospects to optically connect quantum nodes with different capabilities and represent an important step towards the realization of large-scale hybrid quantum networks.

quant-ph↗

arXiv2018

Storing single photons emitted by a quantum memory on a highly excited Rydberg state

Strong interaction between two single photons is a long standing and important goal in quantum photonics. This would enable a new regime of nonlinear optics and unlock several applications in quantum information science, including photonic quantum gates and deterministic Bell-state measurements. In the context of quantum networks, it would be important to achieve interactions between single photons from independent photon pairs storable in quantum memories. So far, most experiments showing nonlinearities at the single-photon level have used weak classical input light. Here, we demonstrate the storage and retrieval of a paired single photon emitted by an ensemble quantum memory in a strongly nonlinear medium based on highly excited Rydberg atoms. We show that nonclassical correlations between the two photons persist after retrieval from the Rydberg ensemble. Our result is an important step towards deterministic photon-photon interactions, and may enable deterministic Bell-state measurements with multimode quantum memories.

quant-ph↗

arXiv2018

Quantum frequency conversion of memory-compatible single photons from 606 nm to the telecom C-band

We report on quantum frequency conversion of memory-compatible narrow-bandwidth photons at 606 nm to the telecom C-band at 1552$\,$nm. The 200$\,$ns long photons, compatible with Praseodymium-based solid-state quantum memories are frequency converted using a single-step difference frequency generation process in a periodically poled Lithium Niobate waveguide. We characterize the noise processes involved in the conversion and by applying strong spectral filtering of the noise, we demonstrate high signal-to-noise ratio conversion at the single photon level (SNR$\,>\,$100 for a mean input photon number per pulse of 1). We finally observe that a memory compatible heralded single photon with a bandwidth of 1.8$\,$MHz, obtained from a spontaneous parametric down conversion pair source, still shows a strong non-classical behavior after conversion. We first demonstrate that correlations between heralding and converted heralded photons stay in the non-classical regime. Moreover, we measured the heralded autocorrelation function of the heralded photon using the converter device as a frequency-domain beam splitter, yielding a value of $0.19\pm0.07$. The presented work represents a step towards the connection of several quantum memory systems emitting narrow-band visible photons to the telecommunication wavelengths.

quant-ph↗