arXiv subjects

Hugues de Riedmatten

Publications and source records attributed to Hugues de Riedmatten.

At least 55 records · Page 3Linked to original sources

arXiv2018

Entanglement between a photonic time-bin qubit and a collective atomic spin excitation

Entanglement between light and matter combines the advantage of long distance transmission of photonic qubits with the storage and processing capabilities of atomic qubits. To distribute photonic states efficiently over long distances several schemes to encode qubits have been investigated -- time-bin encoding being particularly promising due to its robustness against decoherence in optical fibers. Here, we demonstrate the generation of entanglement between a photonic time-bin qubit and a single collective atomic spin excitation (spin-wave) in a cold atomic ensemble, followed by the mapping of the atomic qubit onto another photonic qubit. A magnetic field that induces a periodic dephasing and rephasing of the atomic excitation ensures the temporal distinguishability of the two time-bins and plays a central role in the entanglement generation. To analyse the generated quantum state, we use largely imbalanced Mach-Zehnder interferometers to perform projective measurements in different qubit bases and verify the entanglement by violating a CHSH Bell inequality.

quant-ph↗

arXiv2017

Solid state source of non-classical photon pairs with embedded multimode quantum memory

The generation and distribution of quantum correlations between photonic qubits is a key resource in quantum information science. For applications in quantum networks and quantum repeaters, it is required that these quantum correlations be stored in a quantum memory. In 2001, Duan, Lukin, Cirac, and Zoller (DLCZ) proposed a scheme combining a correlated photon-pair source and a quantum memory in atomic gases, which has enabled fast progress towards elementary quantum networks. In this letter, we demonstrate a solid state source of correlated photon pairs with embedded spin-wave quantum memory, using a rare-earth doped crystal. We show strong quantum orrelations between the photons, high enough for performing quantum communication. Unlike the original DLCZ proposal, our scheme is inherently multimode thanks to a built-in rephasing mechanism, allowing us to demonstrate storage of 11 temporal modes. These results represent an important step towards the realization of complex quantum networks architectures using solid-state resources.

quant-ph↗

arXiv2017

Quantum correlations between single telecom photons and a multimode on-demand solid state quantum memory

Quantum correlations between long lived quantum memories and telecom photons that can propagate with low loss in optical fibers are an essential resource for the realization of large scale quantum information networks. Significant progress has been realized in this direction with atomic and solid state systems. Here, we demonstrate quantum correlations between a telecom photon and a multimode on-demand solid state quantum memory. This is achieved by mapping a correlated single photon onto a spin collective excitation in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal for a controllable time. The stored single photons are generated by cavity enhanced spontaneous parametric down conversion (SPDC) and heralded by their partner photons at telecom wavelength. These results represent the first demonstration of a multimode on-demand solid state quantum memory for external quantum states of light. They provide an important resource for quantum repeaters and pave the way for the implementation of quantum information networks with distant solid-state quantum nodes.

quant-ph↗

arXiv2017

Optimal Photon Generation from Spontaneous Raman Processes in Cold Atoms

Spontaneous Raman processes in cold atoms have been widely used in the past decade for generating single photons. Here, we present a method to optimize their efficiencies for given atomic coherences and optical depths. We give a simple and complete recipe that can be used in present-day experiments, attaining near-optimal single photon emission while preserving the photon purity.

quant-ph↗

arXiv2017

Frequency-Bin Entanglement of Ultra-Narrow Band Non-Degenerate Photon Pairs

We demonstrate frequency-bin entanglement between ultra-narrowband photons generated by cavity enhanced spontaneous parametric down conversion. Our source generates photon pairs in widely non-degenerate discrete frequency modes, with one photon resonant with a quantum memory material based on praseodymium doped crystals and the other photon at telecom wavelengths. Correlations between the frequency modes are analyzed using phase modulators and narrowband filters before detection. We show high-visibility two photon interference between the frequency modes, allowing us to infer a coherent superposition of the modes. We develop a model describing the state that we create and use it to estimate optimal measurements to achieve a violation of the Clauser-Horne (CH) Bell inequality under realistic assumptions. With these settings we perform a Bell test and show a significant violation of the CH inequality, thus proving the entanglement of the photons. Finally we demonstrate the compatibility with a quantum memory material by using a spectral hole in the praseodymium (Pr) doped crystal as spectral filter for measuring high-visibility two-photon interference. This demonstrates the feasibility of combining frequency-bin entangled photon pairs with Pr-based solid state quantum memories.

quant-ph↗

arXiv2016

Storage enhanced nonlinearities in a cold atomic Rydberg ensemble

The combination of electromagnetically induced transparency (EIT) with the nonlinear interaction between Rydberg atoms provides an effective interaction between photons. In this paper, we investigate the storage of optical pulses as collective Rydberg atomic excitations in a cold atomic ensemble. By measuring the dynamics of the stored Rydberg polaritons, we experimentally demonstrate that storing a probe pulse as Rydberg polaritons strongly enhances the Rydberg mediated interaction compared to the slow propagation case. We show that the process is characterized by two time scales. At short storage times, we observe a strong enhancement of the interaction due to the reduction of the Rydberg polariton group velocity down to zero. For longer storage times, we observe a further, weaker enhancement dominated by Rydberg induced dephasing of the multiparticle components of the state. In this regime, we observe a non-linear dependence of the Rydberg polariton coherence time with the input photon number. Our results have direct consequences in Rydberg quantum optics and enable the test of new theories of strongly interacting Rydberg systems.

physics.atom-ph↗

arXiv2016

Cavity enhanced telecom heralded single photons for spin-wave solid state quantum memories

We report on a source of heralded narrowband (3MHz) single photons compatible with solid-state spin-wave quantum memories based on praseodymium doped crystals. Widely non-degenerate narrow-band photon pairs are generated using cavity enhanced down conversion. One photon from the pair is at telecom wavelengths and serves as heralding signal, while the heralded single photon is at 606nm, resonant with an optical transition in Pr:YSO. The source offers a heralding efficiency of 28% and a generation rate exceeding 2000 pairs/mW in a single-mode. The single photon nature of the heralded field is confirmed by a direct antibunching measurement, with a measured antibunching parameter down to 0.010(4). Moreover, we investigate in detail photon cross- and autocorrelation functions proving non-classical correlations between the two photons. The results presented in this paper represent significant improvement over the state of the art and offer prospects for the demonstration of single photon spin-wave storage in an on-demand solid state quantum memory, heralded by a telecom photon.

quant-ph↗

arXiv2016

Non-classical correlations between a C-band telecom photon and a stored spin-wave

Future ground-based quantum information networks will likely use single photons transmitted through optical fibers to entangle individual network nodes. To extend communication distances and overcome limitations due to photon absorption in fibers the concept of quantum repeaters has been proposed. For that purpose, it is required to achieve quantum correlations between the material nodes and photons at telecom wavelengths which can be sent over long distances in optical fibers. Here we demonstrate non-classical correlation between a frequency converted telecom C-band photon and a spin-wave stored in an atomic ensemble quantum memory. The photons emitted from the ensemble and heralding the spin-waves are converted from 780 nm to 1552 nm by means of an all-solid-state integrated waveguide non-linear device. We show ultra-low noise operation of the device enabling a high signal to noise ratio of the converted single photon, leading to a high spin-wave heralding efficiency. The presented work is an enabling step towards the practical entanglement of remote quantum memories and the entanglement of quantum systems operating at different wavelengths.

quant-ph↗

arXiv2016

An Integrated Optical Memory based on Laser Written Waveguides

We report on the first realization of an integrated optical memory for light based on a laser written waveguide in a doped crystal. Using femto-second laser micromachining, we fabricate waveguides in Pr$^{3+}$:Y$_2$SiO$_5$ crystal. We demonstrate that the waveguide inscription does not affect the coherence properties of the material and that the light confinement in the waveguide increases the interaction with the active ions by a factor 6. We also demonstrate that, analogously to the bulk crystals, we can operate the optical pumping protocols necessary to prepare the population in atomic frequency combs, that we use to demonstrate light storage in excited and spin states of the Praseodymium ions. Our results represent the first realization of laser written waveguides in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal and the first implementation of an integrated on-demand spin wave optical memory. They open new perspectives for integrated quantum memories.

quant-ph↗

arXiv2016

A spectral hole memory for light at the single photon level

We demonstrate a solid state spin-wave optical memory based on stopped light in a spectral hole. A long lived narrow spectral hole is created by optical pumping in the inhomogeneous absorption profile of a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. Optical pulses sent through the spectral hole experience a strong reduction of their group velocity and are spatially compressed in the crystal. A short Raman pulse transfers the optical excitation to the spin state before the light pulse exits the crystal, effectively stopping the light. After a controllable delay, a second Raman pulse is sent, which leads to the emission of the stored photons. We reach storage and retrieval efficiencies for bright pulses of up to $39\,\%$ in a $5 \,\mathrm{mm}$-long crystal. We also show that our device works at the single photon level by storing and retrieving $3\,\mathrm{μs}$-long weak coherent pulses with efficiencies up to $31\,\%$, demonstrating the most efficient spin-wave solid state optical memory at the single-photon level so far. We reach an unconditional noise level of $(9\pm1)\times 10^{-3}$ photons per pulse in a detection window of $4\,\mathrm{μs}$ leading to a signal-to-noise ratio of $33 \pm 4$ for an average input photon number of 1, making our device promising for long-lived storage of non-classical light.

quant-ph↗

arXiv2016

Generation of single photons with highly tunable wave shape from a cold atomic quantum memory

We report on a single photon source with highly tunable photon shape based on a cold ensemble of Rubidium atoms. We follow the DLCZ scheme to implement an emissive quantum memory, which can be operated as a photon pair source with controllable delay. We find that the temporal wave shape of the emitted read photon can be precisely controlled by changing the shape of the driving read pulse. We generate photons with temporal durations varying over three orders of magnitude up to 10 μs without a significant change of the read-out efficiency. We prove the non-classicality of the emitted photons by measuring their antibunching, showing near single photon behavior at low excitation probabilities. We also show that the photons are emitted in a pure state by measuring unconditional autocorrelation functions. Finally, to demonstrate the usability of the source for realistic applications, we create ultra-long single photons with a rising exponential or doubly peaked wave shape which are important for several quantum information tasks.

quant-ph↗

arXiv2015

A solid state spin-wave quantum memory for time-bin qubits

We demonstrate the first solid-state spin-wave optical quantum memory with on-demand read-out. Using the full atomic frequency comb scheme in a \PrYSO crystal, we store weak coherent pulses at the single-photon level with a signal to noise ratio $> 10$. Narrow-band spectral filtering based on spectral hole burning in a second \PrYSO crystal is used to filter out the excess noise created by control pulses to reach an unconditional noise level of $(2.0 \pm 0.3) \times10^{-3}$ photons per pulse. We also report spin-wave storage of photonic time-bin qubits with conditional fidelities higher than a measure and prepare strategy, demonstrating that the spin-wave memory operates in the quantum regime. This makes our device the first demonstration of a quantum memory for time-bin qubits, with on demand read-out of the stored quantum information. These results represent an important step for the use of solid-state quantum memories in scalable quantum networks.

quant-ph↗

arXiv2015

Quantum Light Storage in Solid State Atomic Ensembles

In this chapter, we will describe the storage and retrieval of quantum light (heralded single photons and entangled photons) in atomic ensembles in a solid state environment. We will consider ensembles of rare-earth ions embedded in dielectric crystals. We will describe the methods used to create quantum light spectrally compatible with the narrow atomic transitions, as well as possible protocols based on dipole rephasing that can be used to reversibly map the quantum light onto collective atomic excitations. We will review the experimental state of the art and describe in more detail quantum light storage experiments in neodymium and praseodymium doped crystals.

quant-ph↗

arXiv2015

Controlled rephasing of single collective spin excitations in a cold atomic quantum memory

We demonstrate active control of inhomogeneous dephasing and rephasing for single collective atomic spin excitations (spin-waves) created by spontaneous Raman scattering in a quantum memory based on cold $^{87}$Rb atoms. The control is provided by a reversible external magnetic field gradient inducing an inhomogeneous broadening of the atomic hyperfine levels. We demonstrate experimentally that active rephasing preserves the single photon nature of the retrieved photons. Finally, we show that the control of the inhomogeneous dephasing enables the creation of time-separated spin-waves in a single ensemble, followed by a selective readout in time. This is an important step towards the implementation of a functional temporally multiplexed quantum repeater node.

quant-ph↗

arXiv2014

Storage of up-converted telecom photons in a doped crystal

We report on an experiment that demonstrates the frequency up-conversion of telecommunication wavelength single-photon-level pulses to be resonant with a $\mathrm{Pr}^{3+}$:$\mathrm{Y}_2\mathrm{Si}\mathrm{O}_5$ crystal. We convert the telecom photons at $1570\,\mathrm{nm}$ to $606\,\mathrm{nm}$ using a periodically-poled potassium titanyl phosphate nonlinear waveguide. The maximum device efficiency (which includes all optical loss) is inferred to be $η_{\mathrm{dev}}^{\mathrm{max}} = 22 \pm 1\,%$ (internal efficiency $η_{\mathrm{int}} = 75\pm8\,%$) with a signal to noise ratio exceeding 1 for single-photon-level pulses with durations of up to 560$\,$ns. The converted light is then stored in the crystal using the atomic frequency comb scheme with storage and retrieval efficiencies exceeding $η_{\mathrm{AFC}} = 20\,%$ for predetermined storage times of up to $5\,μ\mathrm{s}$. The retrieved light is time delayed from the noisy conversion process allowing us to measure a signal to noise ratio exceeding 100 with telecom single-photon-level inputs. These results represent the first demonstration of single-photon-level optical storage interfaced with frequency up-conversion.

quant-ph↗

arXiv2014

Quantum Storage of Heralded Single Photons in a Praseodymium Doped Crystal

We report on experiments demonstrating the reversible mapping of heralded single photons to long lived collective optical atomic excitations stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. A cavity-enhanced spontaneous down-conversion source is employed to produce widely non-degenerate narrow-band ($\approx 2\,\mathrm{MHz}$) photon-pairs. The idler photons, whose frequency is compatible with telecommunication optical fibers, are used to herald the creation of the signal photons, compatible with the Pr$^{3+}$ transition. The signal photons are stored and retrieved using the atomic frequency comb protocol. We demonstrate storage times up to $4.5\,\mathrm{μs}$ while preserving non-classical correlations between the heralding and the retrieved photon. This is more than 20 times longer than in previous realizations in solid state devices, and implemented in a system ideally suited for the extension to spin-wave storage.

quant-ph↗

arXiv2014

A Waveguide Frequency Converter Connecting Rubidium Based Quantum Memories to the Telecom C-Band

The ability to coherently convert the frequency and temporal waveform of single and entangled photons will be crucial to interconnect the various elements of future quantum information networks. Of particular importance in this context is the quantum frequency conversion of photons emitted by material systems able to store quantum information, so called quantum memories. There have been significant efforts to implement quantum frequency conversion using non linear crystals, with non classical light from broadband photon pair sources and solid state emitters. However, so far, solid state quantum frequency conversion has not been achieved with long lived optical quantum memories. Here, we demonstrate an ultra low noise solid state photonic quantum interface suitable for connecting quantum memories based on atomic ensembles to the telecommunication fiber network. The interface is based on an integrated waveguide non linear device. As a proof of principle, we convert heralded single photons at 780nm emitted by a rubidium based quantum memory to the telecommunication wavelength of 1552nm. We demonstrate a significant amount of non classical correlations between the converted photon and the heralding signal.

quant-ph↗

arXiv2013

Quantum frequency conversion of quantum memory compatible photons to telecommunication wavelengths

We report an experiment demonstrating quantum frequency conversion of weak light pulses compatible with atomic quantum memories to telecommunication wavelengths. We use a PPLN nonlinear waveguide to convert weak coherent states at the single photon level with a duration of 30ns from a wavelength of 780nm to 1552nm. We measure a maximal waveguide internal (external) conversion efficiency eta_int = 0.41 (eta_ext = 0.25), and we show that the signal to noise ratio (SNR) is good enough to reduce the input photon number below 1. In addition, we show that the noise generated by the pump beam in the crystal is proportional to the spectral bandwidth of the device, suggesting that narrower filtering could significantly increase the SNR. Finally, we demonstrate that the quantum frequency converter can operate in the quantum regime by converting a time-bin qubit and measuring the qubit fidelity after conversion.

quant-ph↗