arXiv subjects

I. G. Hughes

Publications and source records attributed to I. G. Hughes.

17 recordsLinked to original sources

arXiv2020

Nano-structured alkali-metal vapor cells

Atom-light interactions in nano-scale systems hold great promise for novel technologies based on integrated emitters and optical modes. We present the design architecture, construction method, and characterization of an all-glass alkali-metal vapor cell with nanometer-scale internal structure. Our cell has a glue-free design which allows versatile optical access, in particular with high numerical aperture optics, and incorporates a compact integrated heating system in the form of an external deposited ITO layer. By performing spectroscopy in different illumination and detection schemes, we investigate atomic densities and velocity distributions in various nanoscopic landscapes. We apply a two-photon excitation scheme to atoms confined in one dimension within our cells, achieving resonance line-widths more than an order of magnitude smaller than the Doppler width. We also demonstrate sub-Doppler line-widths for atoms confined in two dimensions to micron-sized channels. Furthermore, we illustrate control over vapor density within our cells through nano-scale confinement alone, which could offer a scalable route towards room-temperature devices with single atoms within an interaction volume. Our design offers a robust platform for miniaturized devices that could easily be combined with integrated photonic circuits.

physics.atom-ph↗

arXiv2019

Measurement of the atom-surface van der Waals interaction by transmission spectroscopy in a wedged nano-cell

We demonstrate a method for measuring atom-surface interactions using transmission spectroscopy of thermal vapors confined in a wedged nano-cell. The wedged shape of the cell allows complementary measurements of both the bulk atomic vapor and atoms close to surfaces experiencing strong van der Waals atom-surface interaction. These are used to tightly constrain the dipole-dipole collisional parameters of a theoretical model for transmission spectra that accounts for atom-surface interactions, cavity effects, collisions with the surface of the cell and atomic motion. We illustrate this method on a cesium vapor in a sapphire cell, find $C_3=1.3\pm0.1$\,kHz.$μ$m$^3$ and demonstrate that even the weakest of the van der Waals atom-surface interaction coefficients - for ground-state alkali atom transitions - can be determined with a very good precision. This result paves the way towards a precise quantitative characterization of atom-surface interactions in a wide range of atom-based nano-devices.

physics.atom-ph↗

arXiv2019

Quantitative optical spectroscopy of $^{87}$Rb vapour in the Voigt geometry in DC magnetic fields up to 0.4T

We present a detailed spectroscopic investigation of a thermal $^{87}$Rb atomic vapour in magnetic fields up to 0.4T in the Voigt geometry. We fit experimental spectra with our theoretical model \textit{ElecSus} and find excellent quantitative agreement, with RMS errors of $\sim 0.3$%. We extract the magnetic field strength and the angle between the polarisation of the light and the magnetic field from the atomic signal and find excellent agreement to within $\sim 1$% with a commercial Hall probe. Finally, we present an investigation of the relative sensitivity of this technique to variations in the field strength and angle with a view to enabling atom-based high-field vector magnetometry.

physics.atom-ph↗

arXiv2019

Optical transmission of an atomic vapor in the mesoscopic regime

By measuring the transmission of near-resonant light through an atomic vapor confined in a nano-cell we demonstrate a mesoscopic optical response arising from the non-locality induced by the motion of atoms with a phase coherence length larger than the cell thickness. Whereas conventional dispersion theory -- where the local atomic response is simply convolved by the Maxwell-Boltzmann velocity distribution -- is unable to reproduce the measured spectra, a model including a non-local, size-dependent susceptibility is found to be in excellent agreement with the measurements. This result improves our understanding of light-matter interaction in the mesoscopic regime and has implications for applications where mesoscopic effects may degrade or enhance the performance of miniaturized atomic sensors.

physics.atom-ph↗

arXiv2018

An intuitive approach to structuring the three polarization components of light

This paper presents intuitive interpretations of tightly focused beams of light by drawing analogies to two-dimensional electrostatics, magnetostatics and fluid dynamics. We use a Helmholtz decomposition of the transverse polarization components in the transverse plane to introduce generalized radial and azimuthal polarization states. This reveals the interplay between transverse and longitudinal polarization components in a transparent fashion. Our approach yields a comprehensive understanding of tightly focused laser beams, which we illustrate through several insightful examples.

physics.optics↗

arXiv2018

The Collective Lamb Shift of a Nanoscale Atomic Vapour Layer within a Sapphire Cavity

We measure the near-resonant transmission of light through a dense medium of potassium vapor confined in a cell with nanometer thickness in order to investigate the origin and validity of the collective Lamb-shift. A complete model including the multiple reflections in the nano-cell accurately reproduces the observed strong asymmetry of the line shape and allows extraction of a density dependent shift of the atomic resonance. We observe an additional, unexpected dependence of this shift with the thickness of the medium. This extra dependence demands further experimental and theoretical investigations.

physics.atom-ph↗

arXiv2018

Creating Complex Optical Longitudinal Polarization Structures

In this paper we show that it is possible to structure the longitudinal polarization component of light. We illustrate our approach by demonstrating linked and knotted longitudinal vortex lines acquired upon non-paraxially propagating a tightly focused sub-wavelength beam. Remaining degrees of freedom in the transverse polarization components can be exploited to generate customized topological vector beams.

physics.optics↗

arXiv2016

Excitation of knotted vortex lines in matter waves

We study the creation of knotted ultracold matter waves in Bose-Einstein condensates via coherent two-photon Raman transitions with a $Λ$ level configuration. The Raman transition allows an indirect transfer of atoms from the internal state $\left| a \right\rangle$ to the target state $\left| b \right\rangle$ via an excited state $\left| e \right\rangle$, that would be otherwise dipole-forbidden. This setup enables us to imprint three-dimensional knotted vortex lines embedded in the the probe field to the density in the target state. We elaborate on experimental feasibility as well as on subsequent dynamics of the matter wave.

cond-mat.quant-gas↗

arXiv2015

Spectroscopic detection of atom-surface interactions in an atomic vapour layer with nanoscale thickness

We measure the resonance line shape of atomic vapor layers with nanoscale thickness confined between two sapphire windows. The measurement is performed by scanning a probe laser through resonance and collecting the scattered light. The line shape is dominated by the effects of Dicke narrowing, self-broadening, and atom-surface interactions. By fitting the measured line shape to a simple model we discuss the possibility to extract information about the atom-surface interaction.

physics.atom-ph↗

arXiv2015

The Hilbert transform: Applications to atomic spectra

In many areas of physics, the Kramers-Kronig (KK) relations are used to extract information about the real part of the optical response of a medium from its imaginary counterpart. In this paper we discuss an alternative but mathematically equivalent approach based on the Hilbert transform. We apply the Hilbert transform to transmission spectra to find the group and refractive indices of a Cs vapor, and thereby demonstrate how the Hilbert transform allows indirect measurement of the refractive index, group index and group delay whilst avoiding the use of complicated experimental set ups.

physics.atom-ph↗

arXiv2014

Optical response of gas-phase atoms at less than $λ/80$ from a dielectric surface

We present experimental observations of atom-light interactions within tens of nanometers (down to 11~nm) of a sapphire surface. Using photon counting we detect the fluorescence from of order one thousand Rb or Cs atoms, confined in a vapor with thickness much less than the optical excitation wavelength. The asymmetry in the spectral lineshape provides a direct read-out of the atom-surface potential. A numerical fit indicates a power-law $-C_α/r^α$ with $α=3.02\pm0.06$ confirming that the van der Waals interaction dominates over other effects. The extreme sensitivity of our photon-counting technique may allow the search for atom-surface bound states.

physics.atom-ph↗

arXiv2013

Cooperative Enhancement of Energy Transfer in a High-Density Thermal Vapor

We present an experimental study of energy transfer in a thermal vapor of atomic rubidium. We measure the fluorescence spectrum in the visible and near infra-red as a function of atomic density using confocal microscopy. At low density we observe energy transfer consistent with the well-known energy pooling process. In contrast, above a critical density we observe a dramatic enhancement of the fluorescence from high-lying states that is not to be expected from kinetic theory. We show that the density threshold for excitation on the D1 and D2 resonance line corresponds to the value at which the dipole-dipole interactions begins to dominate, thereby indicate the key role of these interactions in the enhanced emission.

physics.atom-ph↗

arXiv2012

Maximal refraction and superluminal propagation in a gaseous nanolayer

We present an experimental measurement of the refractive index of high density Rb vapor in a gaseous atomic nanolayer. We use heterodyne interferometry to measure the relative phase shift between two copropagating laser beams as a function of the laser detuning and infer a peak index n = 1.26 \pm 0.02, close to the theoretical maximum of 1.31. The large index has a concomitant large index gradient creating a region with steep anomalous dispersion where a sub-nanosecond optical pulse is advanced by >100 ps over a propagation distance of 390 nm, corresponding to a group index of -1x10^5, the largest negative group index measured to date.

physics.atom-ph↗

arXiv2012

An optical isolator using an atomic vapor in the hyperfine Paschen-Back regime

A light, compact optical isolator using an atomic vapor in the hyperfine Paschen-Back regime is presented. Absolute transmission spectra for experiment and theory through an isotopically pure 87Rb vapor cell show excellent agreement for fields of 0.6 T. We show π/4 rotation for a linearly polarized beam in the vicinity of the D2 line and achieve an isolation of 30 dB with a transmission > 95 %.

physics.atom-ph↗

arXiv2010

Design and Characterization of a Field-Switchable Nanomagnetic Atom Mirror

We present a design for a switchable nanomagnetic atom mirror formed by an array of 180° domain walls confined within Ni80Fe20 planar nanowires. A simple analytical model is developed which allows the magnetic field produced by the domain wall array to be calculated. This model is then used to optimize the geometry of the nanowires so as to maximize the reflectivity of the atom mirror. We then describe the fabrication of a nanowire array and characterize its magnetic behavior using magneto-optic Kerr effect magnetometry, scanning Hall probe microscopy and micromagnetic simulations, demonstrating how the mobility of the domain walls allow the atom mirror to be switched "on" and "off" in a manner which would be impossible for conventional designs. Finally, we model the reflection of 87Rb atoms from the atom mirror's surface, showing that our design is well suited for investigating interactions between domain walls and cold atoms.

cond-mat.mes-hall↗

arXiv2009

Modulation-free pump-probe spectroscopy of strontium atoms

We have performed polarization spectroscopy and sub-Doppler DAVLL on the (5s5s) 1^S_0 -> (5s5p) 1^P_1 transition of atomic strontium. Both techniques generated a dispersion-type lineshape suitable for laser stabilization, without the need for frequency modulation. In both cases the signal is generated primarily by saturation effects, rather than optical pumping. The dependence of the amplitude and gradient on intensity and magnetic field were also investigated.

physics.atom-ph↗

arXiv2006

Polarization spectroscopy in rubidium and cesium

We develop a theoretical treatment of polarization spectroscopy and use it to make predictions about the general form of polarization spectra in the alkali atoms. Using our model, we generate theoretical spectra for the D2 transitions in 87Rb, 85Rb, and 133Cs. Experiments demonstrate that the model accurately reproduces spectra of transitions from the upper hyperfine level of the ground state only. Among these, the closed transition F -> F' = F + 1 dominates, with a steep gradient through line center ideally suited for use as a reference in laser locking.

physics.atom-ph↗