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I. Tsukada

Publications and source records attributed to I. Tsukada.

40 records · Page 3Linked to original sources

Neutron Scattering Study of Temperature-Concentration Phase Diagram of (Cu1-xMgx)GeO3

In doped CuGeO3 systems, such as (Cu1-xZnx)GeO3 and Cu(Ge1-xSix)O3, the spin-Peierls (SP) ordering (T xc. They thus concluded that there is a compositional phase boundary between two distinct magnetic phases. To clarify the nature of two phases, we performed neutron-scattering measurements on (Cu1-xMgx)GeO3 single crystals with various x. Analysis of the data at fixed temperature points as a function of doping concentration has revealed sudden changes of order parameters at the critical concentration xc=0.027 +- 0.001. At finite temperatures below TN, the drastic increase of the AF moment takes place at xc. The spin-Peierls order parameter delta associated with lattice dimerization shows a precipitous decrease at all temperature below Tsp. However, it goes to zero above xc only at the low temperature limit.

cond-mat.mtrl-sci↗

BaCu_2Si_2O_7: a new quasi 1-dimensional S = 1/2 antiferromagnetic chain system

The new antiferromagnetic (AF) compound BaCu_2Si_2O_7 is studied by magnetic susceptibility and neutron scattering techniques. The observed behavior is dominated by the presence of loosely coupled S=1/2 chains with the intrachain AF exchange constant J = 24.1 meV. Long-range Neel ordering is observed below Tn = 9.2 K. The results are discussed within the framework of the Mean Field-RPA model for weakly interacting quantum spin chains.

cond-mat.str-el↗

Magnetic anisotropy and low-energy spin waves in the Dzyaloshinskii-Moriya spiral magnet Ba_2 Cu Ge_2 O_7

New neutron diffraction and inelastic scattering experiments are used to investigate in detail the field dependence of the magnetic structure and low-energy spin wave spectrum of the Dzyaloshinskii-Moriya helimagnet Ba_2 Cu Ge_2 O_7. The results suggest that the previously proposed model for the magnetism of this compound (an ideal sinusoidal spin spiral, stabilized by isotropic exchange and Dzyaloshinskii-Moriya interactions) needs to be refined. Both new and previously published data can be quantitatively explained by taking into account the Kaplan-Shekhtman-Entin-Wohlman-Aharony (KSEA) term, a special magnetic anisotropy term that was predicted to always accompany Dzyaloshinskii-Moriya interactions in insulators.

cond-mat.str-el↗

The phase transition between dimerized-antiferromagnetic and uniform-antiferromagnetic phases in impurity-doped spin-Peierls cuprate CuGeO3

We discovered a first-order phase transition between dimerized-antiferromagnetic and uniform-antiferromagnetic phases in impurity-doped spin-Peierls (SP) cuprate Cu{1-x}MgxGeO3. As impurity concentration increases, linear reduction of SP transition temperature (T{SP}) and linear increase of Neel temperature (TN) are observed up to x = 0.023. At this critical concentration (xc) SP transition suddenly disappears and TN jumps discontinuously. The peak of the susceptibility at xc around TN is not so sharp as those at other concentrations, which indicates the phase separation of low and high concentration phases. These results indicate the existence of the first-order phase transition between dimerized-antiferromagnetic and uniform-antiferromagnetic long-range orders.

cond-mat.str-el↗