arXiv subjects

I. V. Iorsh

Publications and source records attributed to I. V. Iorsh.

At least 19 recordsLinked to original sources

arXiv2026

Room-temperature local strain control of moiré excitons in MoS$_2$/WSe$_2$ heterobilayers

Moiré superlattices in heterobilayers of atomically thin transition metal dichalcogenides provide a versatile platform for exploring quantum many-body physics as they can trap excitons, leading to the formation of quantized moiré exciton states. However, such moiré excitons have been predominantly studied at cryogenic temperatures, which severely limits their practical applications. Here, we demonstrate room-temperature activation and control of moiré excitons in MoS$_2$/WSe$_2$ heterobilayers using local strain engineering. Applying mechanical strain with a modified atomic force microscopy tip, we observe a series of resonances attributed to interlayer exciton states confined in the moiré potential. Power-dependent photoluminescence measurements elucidate the population dynamics of the moiré exciton states, while controlled local strain enables continuous tuning of their emission wavelength to the center of the second telecom window. We provide a theoretical model that captures all experimentally observed features, including the unconventional spectral shape of the moiré exciton emission. Our findings establish local tip-induced strain as a powerful tool for the on-demand manipulation of moiré excitons, paving the way for room-temperature quantum excitonic devices.

cond-mat.mes-hall↗

arXiv2026

Magnetic switching of self-hybridized exciton-polaritons in CrSBr photonic crystal slabs

Layered van der Waals antiferromagnet CrSBr supports strong light--matter coupling and formation of magnetically tunable exciton-polaritons, yet active magnetic control over polariton propagation direction has remained elusive. Here, we investigate self-hybridized exciton-polaritons in photonic crystal slabs fabricated from CrSBr flakes and their evolution across the antiferromagnetic-to-ferromagnetic spin-flip transition induced by moderate in-plane magnetic fields. Using angle-resolved reflectance and photoluminescence spectroscopy supported by modeling, we show that the polariton energy continuously tracks the layer-by-layer magnetization switching, revealing a gradual redistribution of oscillator strength from antiferromagnetic to ferromagnetic excitons near the critical field. Most notably, we demonstrate that the sign of the polariton group velocity can be reversed by a small change in the external magnetic field of only 40 mT, resulting in complete switching of the polariton propagation direction. Our results establish CrSBr photonic crystal slabs as a platform for magnetically controlled polariton transport, opening opportunities for active integrated photonic and polaritonic devices.

physics.optics↗

arXiv2024

Electronic states bound by repulsive potentials in graphene irradiated by a circularly polarized electromagnetic field

In the framework of the Floquet theory of periodically driven quantum systems, it is demonstrated that irradiation of graphene by a circularly polarized electromagnetic field induces an attractive area in the core of repulsive potentials. Consequently, the quasi-stationary electron states bound by the repulsive potentials appear. The difference between such field-induced states in graphene and usual systems with the parabolic dispersion of electrons is discussed and possible manifestations of these states in electronic transport and optical spectra of graphene are considered.

cond-mat.mes-hall↗

arXiv2024

Floquet engineering of the Lifshitz phase transition in the Hubbard model

Within the Floquet theory of periodically driven quantum systems, we demonstrate that an off-resonant high-frequency electromagnetic field can induce the Lifshitz phase transition in periodical structures described by the one-dimensional repulsive Hubbard model with the nearest and next-nearest-neighbor hopping. The transition changes the topology of electron energy spectrum at the Fermi level, transforming it from the two Fermi points to the four Fermi points, which facilitates the emergence of the superconducting fluctuations in the structure. Possible manifestations of the effect and conditions of its experimental observability are discussed.

cond-mat.mes-hall↗

arXiv2023

Transport regimes for exciton-polaritons in disordered microcavities

Light-matter coupling in a planar optical cavity substantially modifies the transport regimes in the system in presence of a short range excitonic disorder. Basing on Master equation for a resonantly coupled exciton-photon system, and treating disorder scattering in the Born-Markov approximation we demonstrate the onset of ballistic and diffusive transport regimes in the limits of weak and strong disorder respectively. We show that transport parameters governing the crossover between these two regimes strongly depend on the parameters characterizing light-matter coupling, in particular Rabi energy and detuning between excitonic and photonic modes. The presented theory agrees with recent experimental data on transport in disordered organic microcavities.

cond-mat.mtrl-sci↗

arXiv2023

Exciton-polaritons in GaAsbased slab waveguide photonic crystals

We report the observation of band gaps for low loss exciton-polaritons propagating outside the light cone in GaAs-based planar waveguides patterned into two-dimensional photonic crystals. By etching square lattice arrays of shallow holes into the uppermost layer of our structure, we open gaps on the order of 10 meV in the photonic mode dispersion, whose size and light-matter composition can be tuned by proximity to the strongly coupled exciton resonance. We demonstrate gaps ranging from almost fully photonic to highly excitonic. Opening a gap in the exciton-dominated part of the polariton spectrum is a promising first step towards the realization of quantum-Hall-like states arising from topologically nontrivial hybridization of excitons and photons.

physics.optics↗

arXiv2023

Polariton lasing in Mie-resonant perovskite nanocavity

Deeply subwavelength lasers (or nanolasers) are highly demanded for compact on-chip bioimaging and sensing at the nanoscale. One of the main obstacles for the development of single-particle nanolasers with all three dimensions shorter than the emitting wavelength in the visible range is the high lasing thresholds and the resulting overheating. Here we exploit exciton-polariton condensation and mirror-image Mie modes in a cuboid CsPbBr$_3$ nanoparticle to achieve coherent emission at the visible wavelength of around 0.53~$μ$m from its ultra-small ($\approx$0.007$μ$m$^3$ or $\approxλ^3$/20) semiconductor nanocavity. The polaritonic nature of the emission from the nanocavity localized in all three dimensions is proven by direct comparison with corresponding one-dimensional and two-dimensional waveguiding systems with similar material parameters. Such a deeply subwavelength nanolaser is enabled not only by the high values for exciton binding energy ($\approx$35 meV), refractive index ($>$2.5 at low temperature), and luminescence quantum yield of CsPbBr$_3$, but also by the optimization of polaritons condensation on the Mie resonances. Moreover, the key parameters for optimal lasing conditions are intermode free spectral range and phonons spectrum in CsPbBr$_3$, which govern polaritons condensation path. Such chemically synthesized colloidal CsPbBr$_3$ nanolasers can be easily deposited on arbitrary surfaces, which makes them a versatile tool for integration with various on-chip systems.

physics.optics↗

arXiv2023

All-optical magnetization control in CrI$_3$ monolayers: a microscopic theory

Bright excitons in ferromagnetic monolayers CrI$_3$ efficiently interact with lattice magnetization, which makes possible all-optical resonant magnetization control in this material. Using the combination of ab-initio simulations within Bethe-Salpeter approach, semiconductor Bloch equations and Landau-Lifshitz equations, we construct a microscopic theory of this effect. Solving numerically the resulting system of the coupled equations describing the dynamics of atomic spins and spins of the excitons, we demonstrate the possibility of a tunable control of macroscopic magnetization of a sample.

cond-mat.mes-hall↗

arXiv2023

Room-temperature exceptional-point-driven polariton lasing from perovskite metasurface

Excitons in lead bromide perovskites exhibit high binding energy and high oscillator strength, allowing for a strong light-matter coupling regime in the perovskite-based cavities localizing photons at the nanoscale. This opens up the way for the realization of exciton-polariton Bose-Einstein condensation and polariton lasing at room temperature -- the inversion-free low-threshold stimulated emission. However, polariton lasing in perovskite planar photon cavities without Bragg mirrors has not yet been observed and proved experimentally. In this work, we employ perovskite metasurface, fabricated with nanoimprint lithography, supporting so-called exceptional points to demonstrate the room-temperature polariton lasing. The exceptional points in exciton-polariton dispersion of the metasurface appear upon optically pumping in the nonlinear regime in the spectral vicinity of a symmetry-protected bound state in the continuum providing high mode confinement with the enhanced local density of states beneficial for polariton condensation. The observed lasing emission possesses high directivity with a divergence angle of around 1$^\circ$ over one axis. The employed nanoimprinting approach for solution-processable large-scale polariton lasers is compatible with various planar photonic platforms suitable for on-chip integration.

physics.optics↗

arXiv2022

Room-temperature polaron-mediated polariton nonlinearity in MAPbBr3 perovskites

Systems supporting exciton-polaritons represent solid-state optical platforms with a strong built-in optical nonlinearity provided by exciton-exciton interactions. In conventional semiconductors with hydrogen-like excitons the nonlinearity rate demonstrates the inverse scaling with the binding energy. This makes excitons stable at room temperatures weakly interacting, which obviously limits the possibilities of practical applications of the corresponding materials for nonlinear photonics. We demonstrate experimentally and theoretically, that these limitations can be substantially softened in hybrid perovskites, such as MAPbBr3 due to the crucial role of the polaron effects mediating the inter-particle interactions. The resulting exciton-polaron-polaritons remain both stable and strongly interacting at room temperature, which is confirmed by large nonlinear blueshifts of lower polariton branch energy under resonant femtosecond laser pulse excitation. Our findings open novel perspectives for the management of the exciton-polariton nonlinearities in ambient conditions.

cond-mat.mes-hall↗

arXiv2022

Dynamical stabilization by vacuum fluctuations in a cavity: Resonant electron scattering in the ultrastrong light-matter coupling regime

We developed a theory of electron scattering by a short-range repulsive potential in a cavity. In the regime of ultrastrong electron coupling to the cavity electromagnetic field, the vacuum fluctuations of the field result in the dynamical stabilization of a quasistationary polariton state confined in the core of the repulsive potential. When the energy of a free electron coincides with the energy of the confined state, the extremely efficient resonant nonelastic scattering of the electron accompanied by emission of a cavity photon appears. This effect is discussed as a basis for possible free-electron sources of nonclassical light.

cond-mat.mes-hall↗

arXiv2022

Giant and tunable excitonic optical anisotropy in single-crystal CsPbX$_3$ halide perovskites

During the last years, giant optical anisotropy demonstrated its paramount importance for light manipulation which resulted in numerous applications ranging from subdiffraction light guiding to switchable nanolasers. In spite of recent advances in the field, achieving continuous tunability of optical anisotropy remains an outstanding challenge. Here, we present a solution to the problem through chemical alteration of the ratio of halogen atoms (X = Br or Cl) in single-crystal CsPbX$_3$ halide perovskites. It turns out that the anisotropy originates from an excitonic resonance in the perovskite, which spectral position and strength are determined by the halogens composition. As a result, we manage to continually modify the optical anisotropy by 0.14. We also discover that the halide perovskite can demonstrate optical anisotropy up to 0.6 in the visible range -- the largest value among non-van der Waals materials. Moreover, our results reveal that this anisotropy could be in-plane and out-of-plane, depending on perovskite shape -- rectangular and square. Hence, it can serve as an additional degree of freedom for anisotropy manipulation. As a practical demonstration, we created perovskite anisotropic nanowaveguides and show a significant impact of anisotropy on high-order guiding modes. These findings pave the way for halide perovskites as a next-generation platform for tunable anisotropic photonics.

physics.app-ph↗

arXiv2022

Polaron-enhanced polariton nonlinearity in lead halide perovskites

Exciton-polaritons offer a versatile platform for realization of all-optical integrated logic gates due to the strong effective optical nonlinearity resulting from the exciton-exciton interactions. In most of the current excitonic materials there exists a direct connection between the exciton robustness to thermal fluctuations and the strength of exciton-exciton interaction, making materials with highest levels of exciton nonlinearity applicable at cryogenic temperatures only. Here, we show that strong polaronic effects, characteristic for perovskite materials, allow to overcome this limitation. Namely, we demonstrate the record-high value of the nonlinear optical response in nanostructured organic-inorganic halide perovskite MAPbI$_3$, experimentally detected as 19.7 meV blueshift of the polariton branch under femtosecond laser irradiation. This is substantially higher than characteristic values for the samples based on conventional semiconductors and monolayers of transition metal dichalcogenides. The observed strong polaron-enhanced nonlinearity exists for both tetragonal and orthorombic phases of MAPbI$_3$, and remains stable at elevated temperatures.

cond-mat.mes-hall↗

arXiv2022

Floquet engineering of excitons in semiconductor quantum dots

Within the Floquet theory of periodically driven quantum systems, we demonstrate that a high-frequency electromagnetic field can be used as an effective tool to control excitonic properties of semiconductor quantum dots (QDs). It is shown, particularly, that the field both decreases the exciton binding energy and dynamically stabilizes the exciton, increasing its radiative lifetime. The developed theory can serve as a basis for the ultrafast method to tune spectral characteristics of the QD-based photon emitters by a high-frequency field.

cond-mat.mes-hall↗

arXiv2021

Theory of nonlinear excitonic response of hybrid organic perovskites in the regime of strong light-matter coupling

We present a quantitative study of the nonlinear optical response of layered perovskites placed inside planar photonic microcavities in the regime of strong light matter coupling, when excitonic and photonic modes hybridize and give rise to cavity polaritons. Two sources of nonlinearity are specified, the saturation of the excitonic transition with increase of the optical pump and Coulomb interaction between the excitons. It is demonstrated, that peculiar form of the interaction potential, specific to multilayer structure of organic perovskites, is responsible for substantial increase of the exciton binding energy and Rabi splitting with respect to conventional semiconductor systems. This results in dominant contribution of the Rabi splitting quench effect in the nonlinear optical response. Moreover, due to the tightly bound character of excitons, the density of Mott transition is essentially higher, allowing to reach extremely large polariton blueshifts of about 50 meV, which is order of magnitude higher than in conventional semiconductors.

cond-mat.mes-hall↗

arXiv2021

Bound photonic pairs in 2D waveguide quantum electrodynamics

We theoretically predict the formation of two-photon bound states in a two-dimensional waveguide network hosting a lattice of two-level atoms. The properties of these bound pairs and the exclusive domains of the parameter space where they emerge due to the interplay between the on-site photon blockade and peculiar shape of polariton dispersion resulting from the long-range radiative couplings between the qubits are investigated in detail. In addition, we analyze the effect of the finite-size system on localization characteristics of these excitations.

quant-ph↗

arXiv2021

Tunable strongly interacting dipolar excitons in hybrid perovskites

We study theoretically the excitonic nonlinearity in hybrid organic-inorganic Ruddlesden-Popper perovskite thin films. The composite layered structure of these materials allows for flexible modulation of their excitonic response between the limiting cases of single atomic layer and wide quasi-two-dimensional quantum well. In particular, we demonstrate that transverse electric field leads to the spatial separation of charge carriers within the inorganic layer, giving rise to strongly interacting excitons possessing built-in dipole moment. Combined with exciton binding energy of the order of hundreds of meVs, this makes hybrid perovskites an optimal platform for tailoring of nonlinear optical response at reduced dimensionality.

cond-mat.mes-hall↗

arXiv2021

Optically induced Kondo effect in semiconductor quantum wells

It is demonstrated theoretically that the circularly polarized irradiation of two-dimensional electron systems can induce the localized electron states which antiferromagnetically interact with conduction electrons, resulting in the Kondo effect. Conditions of experimental observation of the effect are discussed for semiconductor quantum wells.

cond-mat.mes-hall↗