arXiv subjects

I. V. Iorsh

Publications and source records attributed to I. V. Iorsh.

At least 37 records · Page 2Linked to original sources

arXiv2021

Valley polarization of trions in monolayer MoSe$_2$ interfaced with bismuth iron garnet

Interfacing atomically thin van der Waals semiconductors with magnetic substrates enables additional control on their intrinsic valley degree of freedom and provides a promising platform for the development of novel valleytronic devices for information processing and storage. Here we study circularly polarized photoluminescence in heterostructures of monolayer MoSe$_2$ and thin films of ferrimagnetic bismuth iron garnet. We observe strong emission from charged excitons with negative valley polarization, which switches sign with increasing temperature, and demonstrate contrasting response to left and right circularly polarized excitation, associated with finite out-of-plane magnetization in the substrate. We propose a theoretical model accounting for magnetization-induced imbalance of charge carriers in the two valleys of MoSe$_2$, as well as for valley-switching scattering from B to A excitons and fast formation of trions with extended valley relaxation times, which shows excellent agreement with the experimental data. Our results provide new insights into valley physics in 2D semiconductors interfaced with magnetic substrates.

cond-mat.mes-hall↗

arXiv2021

All optical resonant magnetization switching in $\text{CrI}_3$ monolayers

Efficient control of a magnetization without an application of the external magnetic fields is the ultimate goal of spintronics. We demonstrate, that in monolayers of $\text{CrI}_3$, magnetization can be switched all optically, by application of the resonant pulses of circularly polarized light. This happens because of the efficient coupling of the lattice magnetization with bright excitonic transition. $\text{CrI}_3$ is thus perspective functional material with high potential for applications in the domains of spintronics and ultra-fast magnetic memory.

cond-mat.mes-hall↗

arXiv2020

Fano resonances in optical spectra of semiconductor quantum wells driven by an oscillating field

Optical spectra of semiconductor quantum wells driven by an off-resonant oscillating field are studied theoretically. Due to the dynamical stabilization effect, the field induces the quasi-stationary electron states confined at repulsive scatterers and immersed into the continuum of states of conduction electrons. As a result, the Fano resonances in the spectra of interband optical transitions appear near the energies of the quasi-stationary states.

cond-mat.mes-hall↗

arXiv2020

Two-dimensional chiral waveguide quantum electrodynamics: long range qubit correlations and flat-band dark polaritons

We consider a two-dimensional extension of the 1D waveguide quantum electrodynamics and investigate the nature of linear excitations in two-dimensional arrays of qubits coupled to networks of chiral waveguides. We show that the combined effects of chirality and long-range photon mediated qubit-qubit interactions lead to the emergence of the two-dimensional flat bands in the polaritonic spectrum, corresponding to slow strongly correlated light.

quant-ph↗

arXiv2020

Tunable optical nonlinearity for TMD polaritons dressed by a Fermi sea

We study a system of a transition metal dichalcogenide (TMD) monolayer placed in an optical resonator, where strong light-matter coupling between excitons and photons is achieved. We present quantitative theory of the nonlinear optical response for exciton-polaritons for the case of doped TMD monolayer, and analyze in detail two sources of nonlinearity. The first nonlinear response contribution stems from the Coulomb exchange interaction between excitons. The second contribution comes from the reduction of Rabi splitting that originates from phase space filling at increased exciton concentration and the composite nature of excitons. We demonstrate that both nonlinear contributions are enhanced in the presence of free electrons. As free electron concentration can be routinely controlled by an externally applied gate voltage, this opens a way of electrical tuning of the nonlinear optical response.

cond-mat.mes-hall↗

arXiv2020

Spin-valley dynamics in alloy-based transition metal dichalcogenide heterobilayers

Van der Waals heterobilayers based on 2D transition metal dichalcogenides have been recently shown to support robust and long-lived valley polarization for potential valleytronic applications. However, the role of the band structure and alignment of the constituent layers in the underlying dynamics remains largely unexplored. Here we study spin--valley relaxation dynamics in heterobilayers with different band structures engineered via the use of alloyed monolayer semiconductors. Through a combination of time-resolved Kerr rotation spectroscopic measurements and theoretical modelling for Mo$_{1-x}$W$_{x}$Se$_2$/WSe$_2$ samples with different chemical compositions and stacking angles, we uncover the roles of interlayer exciton recombination and charge carrier spin depolarization in the overall valley dynamics. Our results provide insights into the microscopic spin--valley polarization mechanisms in van der Waals heterostructures for the development of future 2D valleytronic devices.

cond-mat.mes-hall↗

arXiv2020

Spontaneous topological transitions in a honeycomb lattice of exciton-polariton condensates due to spin bifurcations

We theoretically explore nonresonantly pumped polaritonic graphene, a system consisting of a honeycomb lattice of micropillars in the regime of strong light-matter coupling. We demonstrate that, depending on the parameters of the structure, such as intensity of the pump and coupling strength between the pillars, the system shows rich variety of macroscopic ordering, including analogs of ferromagnetic, antiferromagnetic, and resonant valence bond phases. Transitions between these phases are associated with dramatic reshaping of the spectrum of the system connected with spontaneous appearance of topological order.

cond-mat.mes-hall↗

arXiv2019

Nonlinear polaritons in monolayer semiconductor coupled to optical bound states in the continuum

Optical bound states in the continuum (BICs) provide a way to engineer very narrow resonances in photonic crystals. The extended interaction time in such systems is particularly promising for enhancement of nonlinear optical processes and development of the next generation of active optical devices. However, the achievable interaction strength is limited by the purely photonic character of optical BICs. Here, we mix optical BIC in a photonic crystal slab with excitons in atomically thin semiconductor MoSe$_2$ to form nonlinear exciton-polaritons with a Rabi splitting of 27~meV, exhibiting large interaction-induced spectral blueshifts. The asymptotic BIC-like suppression of polariton radiation into far-field towards the BIC wavevector, in combination with effective reduction of excitonic disorder through motional narrowing, results in small polariton linewidths below 3~meV. Together with strongly wavevector-dependent Q-factor, this provides for enhancement and control of polariton--polariton interactions and resulting nonlinear optical effects, paving the way towards tunable BIC-based polaritonic devices for sensing, lasing, and nonlinear optics.

cond-mat.mes-hall↗

arXiv2019

Non-inverse dynamics of a quantum emitter coupled to a fully anisotropic environment

Anisotropic nanophotonic structures can couple the levels of a quantum emitter through the quantum interference effect. In this paper we study the coupling of quantum emitters excited states through the modes of a fully anisotropic structure: a structure for which all directions are physically nonequivalent. We consider an anisotropic metasurface as an illustrative example of such a structure. We point out a novel degree of freedom in controlling the temporal dynamics and spectral profiles of quantum emitters: namely, we show that a combination of the metasurface anisotropy and tilt of the emitter quantization axis with respect to the metasurface normal results in nonsymmetric dynamics between the transitions of electrons from left-circular state to the right-circular states and the inverse process. Our findings give an additional mechanism for control over the light emission by quantum systems and, vice versa, can be utilized for probing active transitions of quantum emitters.

quant-ph↗

arXiv2019

Tunable photon statistics exploiting the Fano effect in a waveguide

A strong optical nonlinearity arises when coherent light is scattered by a semiconductor quantumdot (QD) coupled to a nano-photonic waveguide. We exploit the Fano effect in such a waveguide to control the phase of the quantum interference underpinning the nonlinearity, experimentally demonstrating a tunable quantum optical filter which converts a coherent input state into either a bunched, or antibunched non-classical output state. We show theoretically that the generation of non-classical light is predicated on the formation of a two-photon bound state due to the interaction of the input coherent state with the QD. Our model demonstrates that the tunable photon statistics arise from the dependence of the sign of two-photon interference (either constructive or destructive) on the detuning of the input relative to the Fano resonance.

quant-ph↗

arXiv2018

Optically trapped polariton condensates as semiclassical time crystals

We analyse nonequilibrium phase transitions in microcavity polariton condensates trapped in optically induced annular potentials. We develop an analytic model for annular optical traps, which gives an intuitive interpretation for recent experimental observations on the polariton spatial mode switching with variation of the trap size. In the vicinity of polariton lasing threshold we then develop a nonlinear mean-field model accounting for interactions and gain saturation, and identify several bifurcation scenarios leading to formation of high angular momentum quantum vortices. For experimentally relevant parameters we predict the emergence of spatially and temporally ordered polariton condensates (time crystals), which can be witnessed by frequency combs in the polariton lasing spectrum or by direct time-resolved optical emission measurements. In contrast to previous realizations, our polaritonic time crystal is spontaneously formed from an incoherent excitonic bath and does not inherit its frequency from any periodic driving field.

cond-mat.mes-hall↗

arXiv2018

Topological Metamaterials based on polariton rings

Chern insulator phase is shown to emerge in two-dimensional arrays of polariton rings where time-reversal symmetry is broken due to the application of an out-of-plane magnetic field. The interplay of Zeeman splitting with the photonic analog of spin-orbit coupling (TE-TM splitting) inherently present in this system leads to the appearance of synthetic U(1) gauge field and the opening of topologically nontrivial spectral gaps. This results in the onset of topologically protected chiral edge states similar to those forming in quantum Hall effect. In one dimensional zigzag arrays of polariton rings edge states similar to those appearing in Su-SchriefferHeeger (SSH) model are formed.

cond-mat.mes-hall↗

arXiv2018

Quantum ring with the Rashba spin-orbit interaction in the regime of strong light-matter coupling

We developed the theory of electronic properties of semiconductor quantum rings with the Rashba spin-orbit interaction irradiated by an off-resonant high-frequency electromagnetic field (dressing field). Within the Floquet theory of periodically driven quantum systems, it is demonstrated that the dressing field drastically modifies all electronic characteristics of the rings, including spin-orbit coupling, effective electron mass and optical response. Particularly, the present effect paves the way to controlling the spin polarization of electrons with light in prospective ring-shaped spintronic devices.

cond-mat.mes-hall↗

arXiv2018

Exciton Polaritons in a Two-Dimensional Lieb Lattice with Spin-Orbit Coupling

We study exciton-polaritons in a two-dimensional Lieb lattice of micropillars. The energy spectrum of the system features two flat bands formed from $S$ and $P_{x,y}$ photonic orbitals, into which we trigger bosonic condensation under high power excitation. The symmetry of the orbital wave functions combined with photonic spin-orbit coupling gives rise to emission patterns with pseudospin texture in the flat band condensates. Our work shows the potential of polariton lattices for emulating flat band Hamiltonians with spin-orbit coupling, orbital degrees of freedom and interactions.

cond-mat.mes-hall↗

arXiv2018

Nonlinear Bound States in the Continuum in One-Dimensional Photonic Crystal Slab

Optical bound state in the continuum (BIC) is characterized by infinitely high quality factor resulting in drastic enhancement of light-matter interaction phenomena. We study the optical response of a one-dimensional photonic crystal slab with Kerr focusing nonlinearity in the vicinity of BIC analytically and numerically. We predict a strong nonlinear response including multistable behaviour, self-tuning of BIC to the frequency of incident wave, and breaking of symmetry protected BIC. We show that all of these phenomena can be observed in silicon photonic structure at the pump power of several $μ$W/cm$^2$. We also analyze the modulation instability of the obtained solutions and the effect of the finite size of the structure on the stability. Our findings have strong implications for nonlinear photonics and integrated optical circuits.

physics.optics↗

arXiv2018

Strong coupling between excitons in transition metal dichalcogenides and optical bound states in the continuum

Being motivated by recent achievements in the rapidly developing fields of optical bound states in the continuum (BICs) and excitons in monolayers of transition metal dichalcogenides, we analyze strong coupling between BICs in $\rm Ta_2O_5$ periodic photonic structures and excitons in $\rm WSe_2$ monolayers. We demonstrate that giant radiative lifetime of BICs allow to engineer the exciton-polariton lifetime enhancing it three orders of magnitude compared to a bare exciton. We show that maximal lifetime of hybrid light-matter state can be achieved at any point of $\mathbf{k}$-space by shaping the geometry of the photonic structure. Our findings open new route for the realization of the moving exciton-polariton condensates with non-resonant pump and without the Bragg mirrors which is of paramount importance for polaritonic devices.

cond-mat.mes-hall↗

arXiv2018

Periodic array of quantum rings strongly coupled to circularly polarized light as a topological insulator

We demonstrate theoretically that a strong high-frequency circularly polarized electromagnetic field can turn a two-dimensional periodic array of interconnected quantum rings into a topological insulator. The elaborated approach is applicable to calculate and analyze the electron energy spectrum of the array, the energy spectrum of the edge states and the corresponding electronic densities. As a result, the present theory paves the way to optical control of the topological phases in ring-based mesoscopic structures.

cond-mat.mes-hall↗

arXiv2017

Optically induced Lifshitz transition in bilayer graphene

It is shown theoretically that the renormalization of the electron energy spectrum of bilayer graphene with a strong high-frequency electromagnetic field (dressing field) results in the Lifshitz transition - the abrupt change in the topology of the Fermi surface near the band edge. This effect substantially depends on the polarization of the field: The linearly polarized dressing field induces the Lifshitz transition from the quadruply-connected Fermi surface to the doubly-connected one, whereas the circularly polarized field induces the multicritical point, where the four different Fermi topologies may coexist. As a consequence, the discussed phenomenon creates physical basis to control the electronic properties of bilayer graphene with light.

cond-mat.mes-hall↗