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Igal Brener

Publications and source records attributed to Igal Brener.

At least 19 recordsLinked to original sources

Quantum-Well-Metasurface to Maximize Nonlinear Polarization

Nonlinear frequency conversion unlocks technologies ranging from telecommunications to quantum computation; however, weak nonlinearities and architectures that resist miniaturization currently limit devices. Here, we combine a bandstructure-engineered GaAs/AlGaAs heterostructure with a high quality factor dielectric metasurface to simultaneously tailor the intrinsic nonlinear susceptibility and optimize the electromagnetic field within the heterostructure. By engineering a resonant interband transition, we realize a large second-order nonlinear tensor element, 1.6 nm/V at 1.57 um wavelength. We then make it free-space-accessible and boost the effective nonlinearity to ~ 14 nm/V using a metasurface patterned on the material. Our proof-of-concept experiment establishes that interband transition engineering and metasurfaces accessing otherwise unusable nonlinear tensor elements enable giant effective nonlinearities in the near-infrared to visible spectrum. This addresses material and device-level constraints in nonlinear photonics, providing a scalable route to compact, efficient devices.

physics.optics

Efficient generation of entangled photons in the telecommunications range using nonlinear metasurfaces integrated with ScAlN/GaN heterostructures

Entangled photons provide non-classical correlations that enable measurement sensitivities beyond classical limits, scalable fault-tolerant quantum computation, and fundamentally secure quantum communication, making them a foundational necessity for next-generation quantum technologies. Here we propose and analyze a novel source of entangled photons based on ScAlN/GaN quantum wells integrated with dielectric metasurfaces. Giant second-order intersubband nonlinearity of the GaN quantum wells with strain-compensated delta-doped ScAlN barriers caused by strong built-in electric fields combined with superior mode-coupling performance of metasurfaces optimized by inverse design give rise to efficient parametric down-conversion and generation of entangled photons in the telecom range. We develop a rigorous Heisenberg-Langevin formalism which includes field quantization, dissipation and fluctuations for all fields, parametric amplification of thermal noise and zero-point fluctuations, and other relevant effects. Our proposed approach of employing the emergent photonic material ScAlN promises high biphoton generation rate over $10^{10}$ s$^{-1}$ from a compact integrated structure that is only 0.5 $\mu$m thick while mitigating strain-related issues that have so far impeded progress of nitride-based heterostructures for quantum photonic applications into the infrared and visible wavelengths. Our result therefore is relevant for numerous applications ranging from quantum sensing, quantum information, and computing.

physics.optics

Simultaneous anti-bunched and super-bunched photons from a GaAs Quantum dot in a dielectric metasurface

Semiconductor quantum dots host a rich manifold of excitonic complexes, including neutral excitons that emit anti-bunched single photons and charged exciton complexes capable of producing super-bunched photons via cascade emission. Accessing both emission regimes from a single emitter would open routes to novel quantum protocols, including advanced quantum imaging. In practice, however, emission from charged exciton complexes is intrinsically weak, often orders of magnitude dimmer than neutral excitons, placing simultaneous dual-mode operation out of reach. Here, we overcome this limitation by embedding the quantum dot in a dielectric Mie-resonant metasurface that provides order-of-magnitude photoluminescence enhancement across both neutral and charged exciton transitions of a single GaAs quantum dot. Under identical non-resonant pumping conditions, the emission from the neutral exciton yields anti-bunched emission ($g^{(2)}(0) < 0.5$) and the emission from positively charged exciton complexes shows super-bunched emission ($g^{(2)}(0) > 3.5$) with comparable count rates (~12 kHz). Crucially, super-bunching emerges only when charged exciton emission spectrally overlaps with the Mie resonances and vanishes in un-patterned slabs, demonstrating that photonic engineering, is essential for accessing these weak quantum light states. These results demonstrate a scalable, position-tolerant platform for harnessing the full excitonic structure of solid-state emitters.

cond-mat.mes-hall

Enhanced Interband Optical Nonlinearities from Coupled Quantum Wells

The recent, rapid advances in nonlinear chipscale nanophotonics in the visible and near-infrared have been largely driven by manipulating the local dielectric environment proximate to decades-old workhorse bulk nonlinear optical materials, rather than increasing the inherent strength of their nonlinear response. While proposed decades ago, we demonstrate the first experimental realization of a new class of designer nonlinear materials that leverage the interband optical transition in asymmetric structures to provide strong second order susceptibility, $\chi^{(2)}$. Using simple AlGaAs/GaAs coupled quantum wells operating in the near-infrared as a prototype, we observed strong second harmonic generation enhancement of 1550 nm to 775 nm over bulk controls. Extracted $\chi^{(2)}$ values were as high as 2750 pm/V, which is $>$7x that of bulk GaAs. Furthermore, measured susceptibilities agreed well with quantum mechanical calculations of $\chi^{(2)}$ using layer profiles extracted from electron microscopy. Growth interruptions were employed to improve interfacial abruptness in response to electron microscopy characterization, resulting in increased $\chi^{(2)}$ toward the simulation predictions for ideal heterointerfaces. More complex layer designs showed predicted $\chi^{(2)}$ up to 7 nm/V. Such materials are anticipated to find myriad applications, including entangled photon generation at telecommunications wavelengths for chipscale quantum information processing.

physics.optics

Two-photon Interference of Biphotons Emitted by Overlapping Resonances in Metasurfaces

Two-photon interference, a quantum phenomenon arising from the principle of indistinguishability, is a powerful tool for quantum state engineering and plays a fundamental role in various quantum technologies. These technologies demand robust and efficient sources of quantum light, as well as scalable, integrable and multifunctional platforms. In this regard, quantum optical metasurfaces (QOMs) are emerging as promising platforms for quantum light generation, namely biphotons via spontaneous parametric down-conversion (SPDC), and its engineering. Due to the relaxation of phase matching, SPDC in QOMs allows different channels of biphoton generation, such as those supported by overlapping resonances, to occur simultaneously. In previously reported QOMs, however, SPDC was too weak to observe such effects. Here we develop QOMs based on [110]-oriented GaAs that provide more than an order of magnitude enhancement in SPDC rate, after accounting for the spectral bandwidth, compared to any other QOMs studied to date. This boosted efficiency allows the QOMs support the simultaneous generation of SPDC from several spectrally overlapping optical modes. Using polarization components in the interferometer analyzer, we intentionally erase the distinguishability between the biphotons from a high-$Q$ quasi-bound-state-in-the-continuum resonance and a low-$Q$ Mie resonance, which results in the first-time observation of two-photon interference in the spectral domain in these types of devices. This quantum interference can considerably enrich the generation of entangled photons in metasurfaces. Their advanced multifunctionality, improved nonlinear response, ease of fabrication and compact footprint of [110]-GaAs QOMs position them as promising platforms to fulfill the requirements for photonic quantum technologies.

quant-ph

AutoSciLab: A Self-Driving Laboratory For Interpretable Scientific Discovery

Advances in robotic control and sensing have propelled the rise of automated scientific laboratories capable of high-throughput experiments. However, automated scientific laboratories are currently limited by human intuition in their ability to efficiently design and interpret experiments in high-dimensional spaces, throttling scientific discovery. We present AutoSciLab, a machine learning framework for driving autonomous scientific experiments, forming a surrogate researcher purposed for scientific discovery in high-dimensional spaces. AutoSciLab autonomously follows the scientific method in four steps: (i) generating high-dimensional experiments (x \in R^D) using a variational autoencoder (ii) selecting optimal experiments by forming hypotheses using active learning (iii) distilling the experimental results to discover relevant low-dimensional latent variables (z \in R^d, with d << D) with a 'directional autoencoder' and (iv) learning a human interpretable equation connecting the discovered latent variables with a quantity of interest (y = f(z)), using a neural network equation learner. We validate the generalizability of AutoSciLab by rediscovering a) the principles of projectile motion and b) the phase transitions within the spin-states of the Ising model (NP-hard problem). Applying our framework to an open-ended nanophotonics challenge, AutoSciLab uncovers a fundamentally novel method for directing incoherent light emission that surpasses the current state-of-the-art (Iyer et al. 2023b, 2020).

cs.LG

Inverse Design of an All-Dielectric Nonlinear Polaritonic Metasurface

Nonlinear metasurfaces offer a new paradigm to realize optical nonlinear devices with new and unparalleled behavior compared to nonlinear crystals, due to the interplay between photonic resonances and materials properties. The complicated interdependency between efficiency and emission directionality of the nonlinear optical signal on the existence, localization, and lifetimes of photonic resonances, as well as on the nonlinear susceptibility, makes it extremely difficult to design optimal metasurfaces using conventional materials and geometries. Inverse design using topology optimization is a powerful design tool for photonic structures, but traditional approaches developed for linear photonics are not suitable for such high dimensional nonlinear problems. Here, we use a topology optimization approach to inverse-design a fabrication-robust nonlinear metasurface that includes quantum-engineered resonant nonlinearities in semiconductor heterostructures for efficient and directional second harmonic generation. Furthermore, we also demonstrate that under practical constraints, among all the parameters, the nonlinear modal overlap emerges as the dominant parameter that enhances conversion efficiency, a finding that contrasts with intuition-driven studies that often emphasize Purcell enhancement. Our results open new opportunities for optimizing nonlinear processes in nanophotonic structures for novel light sources, quantum information applications, and communication.

physics.optics

Nonlinear Analog Processing with Anisotropic Nonlinear Films

Digital signal processing is the cornerstone of several modern-day technologies, yet in multiple applications it faces critical bottlenecks related to memory and speed constraints. Thanks to recent advances in metasurface design and fabrication, light-based analog computing has emerged as a viable option to partially replace or augment digital approaches. Several light-based analog computing functionalities have been demonstrated using patterned flat optical elements, with great opportunities for integration in compact nanophotonic systems. So far, however, the available operations have been restricted to the linear regime, limiting the impact of this technology to a compactification of Fourier optics systems. In this paper, we introduce nonlinear operations to the field of metasurface-based analog optical processing, demonstrating that nonlinear optical phenomena, combined with nonlocality in flat optics, can be leveraged to synthesize kernels beyond linear Fourier optics, paving the way to a broad range of new opportunities. As a practical demonstration, we report the experimental synthesis of a class of nonlinear operations that can be used to realize broadband, polarization-selective analog-domain edge detection.

physics.optics

Quantum Pair Generation in Nonlinear Metasurfaces with Mixed and Pure Photon Polarizations

Metasurfaces are highly effective at manipulating classical light in the linear regime; however, effectively controlling the polarization of non-classical light generated from nonlinear resonant metasurfaces remains a challenge. Here, we present a solution by achieving polarization engineering of frequency-nondegenerate biphotons emitted via spontaneous parametric down-conversion (SPDC) in GaAs metasurfaces, where quasi-bound states in the continuum (qBIC) resonances were utilized for boosting the biphoton generation. By performing a comprehensive polarization tomography, we demonstrate that the polarization of the emitted photons directly reflects the qBIC mode's far-field properties. Furthermore, we show that both the type of qBIC mode and the symmetry of the meta-atoms can be tailored to control each single-photon polarization state, and that the subsequent two-photon polarization states are nearly separable, offering potential applications in the heralded generation of single photons with adjustable polarization. This work provides a significant step towards utilizing metasurfaces to not only generate quantum light but also engineer their polarization, a critical aspect for future quantum technologies.

quant-ph

Self-driving lab discovers principles for steering spontaneous emission

We developed an autonomous experimentation platform to accelerate interpretable scientific discovery in ultrafast nanophotonics, targeting a novel method to steer spontaneous emission from reconfigurable semiconductor metasurfaces. Controlling spontaneous emission is crucial for clean-energy solutions in illumination, thermal radiation engineering, and remote sensing. Despite the potential of reconfigurable semiconductor metasurfaces with embedded sources for spatiotemporal control, achieving arbitrary far-field control remains challenging. Here, we present a self-driving lab (SDL) platform that addresses this challenge by discovering the governing equations for predicting the far-field emission profile from light-emitting metasurfaces. We discover that both the spatial gradient (grating-like) and the curvature (lens-like) of the local refractive index are key factors in steering spontaneous emission. The SDL employs a machine-learning framework comprising: (1) a variational autoencoder for generating complex spatial refractive index profiles, (2) an active learning agent for guiding experiments with real-time closed-loop feedback, and (3) a neural network-based equation learner to uncover structure-property relationships. The SDL demonstrated a four-fold enhancement in peak emission directivity (up to 77%) over a 72° field of view within ~300 experiments. Our findings reveal that combinations of positive gratings and lenses are as effective as negative lenses and gratings for all emission angles, offering a novel strategy for controlling spontaneous emission beyond conventional Fourier optics.

physics.optics

Near-field Imaging of Optical Resonances in Silicon Metasurfaces Using Photoelectron Microscopy

Precise control of light-matter interactions at the nanoscale lies at the heart of nanophotonics. Experimental examination at this length scale is challenging, however, since the corresponding electromagnetic near-field is often confined within volumes below the resolution of conventional optical microscopy. In semiconductor nanophotonics electromagnetic fields are further restricted within the confines of individual subwavelength resonators, limiting access to critical light-matter interactions in these structures. In this work, we demonstrate that photoelectron emission microscopy (PEEM) can be used for polarization resolved near-field spectroscopy and imaging of electromagnetic resonances supported by broken-symmetry silicon metasurfaces. We find that the photoemission results, enabled through an in-situ potassium surface layer, are consistent with full-wave simulations and far-field reflectance measurements across visible and near-infrared wavelengths. In addition, we uncover a polarization dependent evolution of collective resonances near the metasurface array edge taking advantage of the far-field excitation and full-field imaging of PEEM. Here, we deduce that coupling between eight resonators or more establishes the collective excitations of this metasurface. All told, we demonstrate that the high-spatial resolution hyperspectral imaging and far-field illumination of PEEM can be leveraged for the metrology of collective, non-local, optical resonances in semiconductor nanophotonic structures.

physics.optics

Terahertz pulse generation with binary phase control in non-linear InAs metasurface

The effect of terahertz (THz) pulse generation has revolutionized broadband coherent spectroscopy and imaging at THz frequencies. However, THz pulses typically lack spatial structure, whereas structured beams are becoming essential for advanced spectroscopy applications. Non-linear optical metasurfaces with nanoscale THz emitters can provide a solution by defining the beam structure at the generation stage. We develop a non-linear InAs metasurface consisting of nanoscale optical resonators for simultaneous generation and structuring of THz beams. We find that THz pulse generation in the resonators is governed by optical rectification. It is more efficient than in ZnTe crystals, and it allows us to control the pulse polarity and amplitude, offering a platform for realizing binary-phase THz metasurfaces. To illustrate this capability, we demonstrate an InAs metalens, which simultaneously generates and focuses THz pulses. The control of spatiotemporal structure using nanoscale emitters opens doors for THz beam engineering and advanced spectroscopy and imaging applications.

physics.optics

Sub picosecond steering of ultrafast incoherent emission from semiconductor metasurfaces

The ability to dynamically steer fs pulses from a monolithically integrated source is a critical milestone for the fields of nanophotonics and ultrafast optics. The nascent field of reconfigurable metasurfaces -- made of optically resonant meta-atoms -- has shown great promise in manipulating light-matter interactions through subwavelength control of the phase, amplitude, and polarization of light. These active metasurfaces arbitrarily transform an incident wavefront using a reconfigurable spatial phase profile and thus have been limited to manipulating coherent external sources. Light emitting metasurfaces obtained through integration of incoherent emitters with meta-atoms, have been used to statically increase the quantum efficiency of the emission through Purcell factor enhancement and control the far-field emission properties of the light to collimate and focus spontaneous emission. Active manipulation of such incoherent light sources, however, remains a challenge as current phase-sensitive approaches used for coherent sources cannot be directly applied. Spatiotemporal control at ultrafast timescales of incoherent light emission could lead to a transformative technological leap allowing low-power light emitting diodes (LEDs) to replace high-power coherent laser sources, enabling holographic LED displays and other key optical transceiver applications including remote-sensing, perception, and high-speed optical communication systems. In this work, we theoretically predict and experimentally demonstrate for the first time, sub-picosecond steering over a 70° range of ultrafast incoherent emission from a light emitting metasurface.

physics.optics

Nonlinear and Ultrafast All-Dielectric Metasurfaces at the Center for Integrated Nanotechnologies

Metasurfaces control optical wavefronts via arrays of nanoscale resonators laid out across a surface. When combined with III-V semiconductors with strong optical nonlinearities, a variety of nonlinear effects such as harmonic generation and all optical modulation can be enabled and enhanced at the nanoscale. This review presents our research on engineering and boosting nonlinear effects in ultrafast and nonlinear semiconductor metasurfaces fabricated at the Center for Integrated Nanotechnologies (CINT). We cover our recent works on parametric generation of harmonic light via direct and cascaded processes in GaAs-metasurfaces using Mie-like optical resonances or symmetric-protected Bound State in the Continuum, and then describe the recent advances on harmonic generation in all-dielectric metasurfaces coupled to intersubband transitions in III-V semiconductor heterostructures. The review concludes on the potential of metasurfaces to serve as the next platform for on-chip quantum light generation.

physics.optics

Resonant Semiconductor Metasurfaces for Generating Complex Quantum States

Quantum state engineering, the cornerstone of quantum photonic technologies, mainly relies on spontaneous parametric down-conversion and four-wave mixing, where one or two pump photons decay into a photon pair. Both these nonlinear effects require momentum conservation (i.e., phase-matching) for the participating photons, which strongly limits the versatility of the resulting quantum states. Nonlinear metasurfaces, due to their subwavelength thickness, relax this constraint and extend the boundaries of quantum state engineering. Here, we generate entangled photons via spontaneous parametric down-conversion in semiconductor metasurfaces with high-quality resonances. By enhancing the quantum vacuum field, our metasurfaces boost the emission of photon pairs within narrow resonance bands at multiple selected wavelengths. Due to the relaxed momentum conservation, the same resonances support photon pair generation from pump photons of practically any energy. This enables the generation of complex frequency-multiplexed quantum states, in particular cluster states. Our results demonstrate the multifunctional use of metasurfaces for quantum state engineering.

quant-ph

Cascaded optical nonlinearities in dielectric metasurfaces

Since the discovery of the laser, optical parametric nonlinearities have been at the core of efficient light conversion sources. Typically, thick transparent crystals or quasi-phase matched waveguides, are utilized in conjunction with phase-matching techniques to select a single parametric process. In recent years, due to the rapid developments in artificially structured materials, optical frequency mixing has been achieved at the nanoscale in subwavelength resonators arrayed as metasurfaces. Phase matching becomes relaxed for these wavelength-scale structures, and all allowed nonlinear processes can, in principle, occur on an equal footing. This could promote harmonic generation via a cascaded (consisting of several frequency mixing steps) process. However, so far, all reported work on dielectric metasurfaces have assumed frequency mixing from a direct (single step) nonlinear process. In this work, we prove the existence of cascaded second-order optical nonlinearities by analyzing the second and third wave mixing from a highly nonlinear metasurface in conjunction with polarization selection rules and crystal symmetries. We find that the third wave mixing signal from a cascaded process can be of comparable strength to that from conventional third harmonic generation, and that surface nonlinearities are the dominant mechanism that contributes to cascaded second order nonlinearities

physics.optics

Manipulation of Exciton Dynamics in Single-Layer WSe2 Using a Toroidal Dielectric Metasurface

Recent advances in emerging atomically thin transition metal dichalcogenide semiconductors with strong light-matter interactions and tunable optical properties provide novel approaches for realizing new material functionalities. Coupling two-dimensional semiconductors with all-dielectric resonant nanostructures represents an especially attractive opportunity for manipulating optical properties in both the near-field and far-field regimes. Here, by integrating single-layer WSe2 and titanium oxide (TiO2) dielectric metasurfaces with toroidal resonances, we realized robust exciton emission enhancement over one order of magnitude at both room and low temperatures. Furthermore, we could control exciton dynamics and annihilation by using temperature to tailor the spectral overlap of excitonic and toroidal resonances, allowing us to selectively enhance the Purcell effect. Our results provide rich physical insight into the strong light-matter interactions in single-layer TMDs coupled with toroidal dielectric metasurfaces, with important implications for optoelectronics and photonics applications.

cond-mat.mes-hall

Structurally Tunable Nonlinear Terahertz Metamaterials using Broadside Coupled Split Ring Resonators

We present an experimental and numerical study of a terahertz metamaterial with a nonlinear response that is controllable via the relative structural positioning of two stacked split ring resonator arrays. The first array is fabricated on an n-doped GaAs substrate and the second array is fabricated vertically above the first using a polyimide spacer layer. Due to GaAs carrier dynamics, the on-resonance terahertz transmission at 0.4 THz varies in a nonlinear manner with incident terahertz power. The second resonator layer dampens this nonlinear response. In samples where the two layers are aligned, the resonance disappears and total nonlinear modulation of the on-resonance transmission decreases. The nonlinear modulation is restored in samples where an alignment offset is imposed between the two resonator arrays. Structurally tunable metamaterials can therefore act as a design template for tunable nonlinear THz devices by controlling the coupling of confined electric fields to nonlinear phenomena in a complex material substrate or inclusion.

physics.optics