arXiv subjects

Igor Žutić

Publications and source records attributed to Igor Žutić.

At least 55 records · Page 3Linked to original sources

arXiv2017

Magnetic Proximity Effects in Transition-Metal Dichalcogenides: Converting Excitons

The two-dimensional character and reduced screening in monolayer transition-metal dichalcogenides (TMDs) lead to the ubiquitous formation of robust excitons with binding energies orders of magnitude larger than in bulk semiconductors. Focusing on neutral excitons, bound electron-hole pairs, that dominate the optical response in TMDs, it is shown that they can provide fingerprints for magnetic proximity effects in magnetic heterostructures. These proximity effects cannot be described by the widely used single-particle description, but instead reveal the possibility of a conversion between optically inactive and active excitons by rotating the magnetization of the magnetic substrate. With recent breakthroughs in fabricating Mo- and W-based magnetic TMD-heterostructures, this emergent optical response can be directly tested experimentally.

cond-mat.mtrl-sci↗

arXiv2017

Tunable Magnetic Textures: From Majorana Bound States to Braiding

A versatile control of magnetic systems, widely used to store information, can also enable manipulating Majorana bounds states (MBS) and implementing fault-tolerant quantum information processing. The proposed platform relies on the proximity-induced superconductivity in a two-dimensional electron gas placed next to an array of magnetic tunnel junctions (MTJs). A change in the magnetization configuration in the MTJ array creates tunable magnetic textures thereby removing several typical requirements for MBS: strong spin-orbit coupling, applied magnetic field, and confinement by one-dimensional structures which complicates demonstrating non-Abelian statistics through braiding. Recent advances in fabricating two-dimensional epitaxial superconductor/semiconductor heterostructures and designing tunable magnetic textures support the feasibility of this novel platform for MBS.

cond-mat.mes-hall↗

arXiv2017

Marrying excitons and plasmons in monolayer transition-metal dichalcogenides

Just as photons are the quanta of light, plasmons are the quanta of orchestrated charge-density oscillations in conducting media. Plasmon phenomena in normal metals, superconductors and doped semiconductors are often driven by long-wavelength Coulomb interactions. However, in crystals whose Fermi surface is comprised of disconnected pockets in the Brillouin zone, collective electron excitations can also attain a shortwave component when electrons transition between these pockets. Here, we show that the band structure of monolayer transition-metal dichalcogenides gives rise to an intriguing mechanism through which shortwave plasmons are paired up with excitons. The coupling elucidates the origin for the optical side band that is observed repeatedly in monolayers of WSe$_2$ and WS$_2$ but not understood. The theory makes it clear why exciton-plasmon coupling has the right conditions to manifest itself distinctly only in the optical spectra of electron-doped tungsten-based monolayers.

cond-mat.mtrl-sci↗

arXiv2017

Wurtzite spin lasers

Semiconductor lasers are strongly altered by adding spin-polarized carriers. Such spin lasers could overcome many limitations of their conventional (spin-unpolarized) counterparts. While the vast majority of experiments in spin lasers employed zinc-blende semiconductors, the room temperature electrical manipulation was first demonstrated in wurtzite GaN-based lasers. However, the underlying theoretical description of wurtzite spin lasers is still missing. To address this situation, focusing on (In,Ga)N-based wurtzite quantum wells, we develop a theoretical framework in which the calculated microscopic spin-dependent gain is combined with a simple rate equation model. A small spin-orbit coupling in these wurtzites supports simultaneous spin polarizations of electrons and holes, providing unexplored opportunities to control spin lasers. For example, the gain asymmetry, as one of the key figures of merit related to spin amplification, can change the sign by simply increasing the carrier density. The lasing threshold reduction has a nonmonotonic depenedence on electron spin polarization, even for a nonvanishing hole spin polarization.

cond-mat.mes-hall↗

arXiv2016

Excitonic Stark effect in MoS$_2$ monolayers

We theoretically investigate excitons in MoS$_2$ monolayers in an applied in-plane electric field. Tight-binding and Bethe-Salpeter equation calculations predict a quadratic Stark shift, of the order of a few meV for fields of 10 V/$μ$m, in the linear absorption spectra. The spectral weight of the main exciton peaks decreases by a few percent with an increasing electric field due to the exciton field ionization into free carriers as reflected in the exciton wave functions. Subpicosecond exciton decay lifetimes at fields of a few tens of V/$μ$m could be utilized in solar energy harvesting and photodetection. We find simple scaling relations of the exciton binding, radius, and oscillator strength with the dielectric environment and an electric field, which provides a path to engineering the MoS$_2$ electro-optical response.

cond-mat.mtrl-sci↗

arXiv2016

Tunneling Planar Hall Effect in Topological Insulators: Spin-Valves and Amplifiers

We investigate tunneling across a single ferromagnetic barrier on the surface of a three-dimensional topological insulator. In the presence of a magnetization component along the bias direction, a tunneling planar Hall conductance (TPHC), transverse to the applied bias, develops. Electrostatic control of the barrier enables a giant Hall angle, with the TPHC exceeding the longitudinal tunneling conductance. By changing the in-plane magnetization direction it is possible to change the sign of both the longitudinal and transverse differential conductance without opening a gap in the topological surface state. The transport in a topological insulator/ferromagnet junction can thus be drastically altered from a simple spin-valve to an amplifier.

cond-mat.mes-hall↗

arXiv2016

Wireless Majorana Bound States: From Magnetic Tunability to Braiding

We propose a versatile platform to investigate the existence of Majorana bound states (MBSs) and their non-Abelian statistics through braiding. This implementation combines a two-dimensional electron gas formed in a semiconductor quantum well grown on the surface of an s-wave superconductor with a nearby array of magnetic tunnel junctions (MTJs). The underlying magnetic textures produced by MTJs provide highly controllable topological phase transitions to confine and transport MBSs in two dimensions, overcoming the requirement for a network of wires. Obtained scaling relations confirm that various semiconductor quantum well materials are suitable for this proposal.

cond-mat.mes-hall↗

arXiv2016

Killing Auger recombination in nanostructures by carrier spin polarization

In semiconductor nanostructures nonradiative Auger recombination is enhanced by the presence of boundaries which relax the momentum conservation and thereby removes the threshold reduction for these processes. We propose a method to strongly reduce the Auger recombination rate by injecting spin-polarized carriers. Our method is illustrated on the example of a quantum well in which the spin-orbit coupling of conduction band is negligible as compared to valence band and thus holes can be considered as spin-unpolarized. The suppression factor of the Auger recombination is determined by the two-dimensional character of the system, given by the ratio of the Fermi energy of electrons and the separation of the electron levels quantized in the growth direction. Our predictions can be tested experimentally and we discuss their implications for semiconductor lasers relying on injection of spin-polarized electrons.

cond-mat.mes-hall↗

arXiv2015

Experimental Demonstration of XOR Operation in Graphene Magnetologic Gates at Room Temperature

We report the experimental demonstration of a magnetologic gate built on graphene at room temperature. This magnetologic gate consists of three ferromagnetic electrodes contacting a single layer graphene spin channel and relies on spin injection and spin transport in the graphene. We utilize electrical bias tuning of spin injection to balance the inputs and achieve "exclusive or" (XOR) logic operation. Furthermore, simulation of the device performance shows that substantial improvement towards spintronic applications can be achieved by optimizing device parameters such as device dimensions. This advance holds promise as a basic building block for spin-based information processing.

cond-mat.mes-hall↗

arXiv2015

Roadmap for Emerging Materials for Spintronic Device Applications

The Technical Committee of the IEEE Magnetics Society has selected 7 research topics to develop their roadmaps, where major developments should be listed alongside expected timelines; (i) hard disk drives, (ii) magnetic random access memories, (iii) domain-wall devices, (iv) permanent magnets, (v) sensors and actuators, (vi) magnetic materials and (vii) organic devices. Among them, magnetic materials for spintronic devices have been surveyed as the first exercise. In this roadmap exercise, we have targeted magnetic tunnel and spin-valve junctions as spintronic devices. These can be used for example as a cell for a magnetic random access memory and spin-torque oscillator in their vertical form as well as a spin transistor and a spin Hall device in their lateral form. In these devices, the critical role of magnetic materials is to inject spin-polarised electrons efficiently into a non-magnet. We have accordingly identified 2 key properties to be achieved by developing new magnetic materials for future spintronic devices: (1) Half-metallicity at room temperature (RT); (2) Perpendicular anisotropy in nano-scale devices at RT. For the first property, 5 major magnetic materials are selected for their evaluation for future magnetic/spintronic device applications: Heusler alloys, ferrites, rutiles, perovskites and dilute magnetic semiconductors. These alloys have been reported or predicted to be half-metallic ferromagnets at RT. They possess a bandgap at the Fermi level EF only for its minority spins, achieving 100% spin polarisation at EF. We have also evaluated L10-alloys and D022-Mn-alloys for the development of a perpendicularly anisotropic ferromagnet with large spin polarisation. We have listed several key milestones for each material on their functionality improvements, property achievements, device implementations and interdisciplinary applications within 35 years time scale.

cond-mat.mtrl-sci↗

arXiv2015

Magnetoanisotropic Andreev Reflection in Ferromagnet/Superconductor Junctions

Andreev reflection spectroscopy of ferromagnet/superconductor (FS) junctions is an important probe of spin polarization. We theoretically investigate spin-polarized transport in FS junctions in the presence of Rashba and Dresselhaus interfacial spin-orbit fields and show that Andreev reflection can be controlled by changing the magnetization orientation. We predict a giant in- and out-of-plane magnetoanisotropy of the junction conductance. If the ferromagnet is highly spin polarized---in the half-metal limit---the magnetoanisotropic Andreev reflection depends universally on the spin-orbit fields only. Our results show that Andreev reflection spectroscopy can be used for sensitive probing of interfacial spin-orbit fields in FS junction.

cond-mat.supr-con↗

arXiv2015

Magnetic ordering in quantum dots: Open vs. closed shells

In magnetically-doped quantum dots changing the carrier occupancy, from open to closed shells, leads to qualitatively different forms of carrier-mediated magnetic ordering. While it is common to study such nanoscale magnets within a mean field approximation, excluding the spin fluctuations can mask important phenomena and lead to spurious thermodynamic phase transitions in small magnetic systems. By employing coarse-grained, variational, and Monte Carlo methods on singly and doubly occupied quantum dots to include spin fluctuations, we evaluate the relevance of the mean field description and distinguish different finite-size scaling in nanoscale magnets.

cond-mat.mes-hall↗

arXiv2015

Toward high-frequency operation of spin lasers

Injecting spin-polarized carriers into semiconductor lasers provides important opportunities to extend what is known about spintronic devices, as well as to overcome many limitations of conventional (spin-unpolarized) lasers. By developing a microscopic model of spin-dependent optical gain derived from an accurate electronic structure in a quantum well-based laser, we study how its operation properties can be modified by spin-polarized carriers, carrier density, and resonant cavity design. We reveal that by applying a uniaxial strain, it is possible to attain a large birefringence. While such birefringence is viewed as detrimental in conventional lasers, it could enable fast polarization oscillations of the emitted light in spin lasers which can be exploited for optical communication and high-performance interconnects. The resulting oscillation frequency ($>200$ GHz) would significantly exceed the frequency range possible in conventional lasers.

cond-mat.mes-hall↗

arXiv2015

Probing topological transitions in HgTe/CdTe quantum wells by magneto-optical measurements

In two-dimensional topological insulators, such as inverted HgTe/CdTe quantum wells, helical quantum spin Hall (QSH) states persist even at finite magnetic fields below a critical magnetic field $B_\mathrm{c}$, above which only quantum Hall (QH) states can be found. Using linear-response theory, we theoretically investigate the magneto-optical properties of inverted HgTe/CdTe quantum wells, both for infinite two-dimensional and finite-strip geometries, and possible signatures of the transition between the QSH and QH regimes. In the absorption spectrum, several peaks arise due to non-equidistant Landau levels in both regimes. However, in the QSH regime, we find an additional absorption peak at low energies in the finite-strip geometry. This peak arises due to the presence of edge states in this geometry and persists for any Fermi level in the QSH regime, while in the QH regime the peak vanishes if the Fermi level is situated in the bulk gap. Thus, by sweeping the gate voltage, it is possible to experimentally distinguish between the QSH and QH regimes due to this signature. Moreover, we investigate the effect of spin-orbit coupling and finite temperature on this measurement scheme.

cond-mat.mes-hall↗

arXiv2015

Probing Majorana-like states in quantum dots and quantum rings

Engineering chiral $p$-wave superconductivity in semiconductor structures offers fascinating ways to obtain and study Majorana modes in a condensed matter context. Here, we theoretically investigate chiral $p$-wave superconductivity in quantum dots and quantum rings. Using both analytical as well as numerical methods, we calculate the quasiparticle excitation spectra in these structures and the corresponding excitation amplitudes and charge densities. In the topological regime, we can observe the chiral edge modes localized at the boundaries and possessing finite energy in quantum dots and quantum rings. By applying a magnetic field which is expelled from the quantum ring, but which creates a flux that is an odd integer multiple of $Φ_0/2=π\hbar/e$, Majorana modes, that is, (approximately) degenerate edge modes with zero energy and zero charge density, become possible in the topological regime. Furthermore, we investigate finite-size effects that split these degenerate edge modes as well as the effect of a magnetic field penetrating into the superconducting region that can under certain circumstances still support edge modes with approximately zero energy and charge.

cond-mat.mes-hall↗

arXiv2013

Nodal "ground states" and orbital textures in semiconductor quantum dots

Conventional understanding implies that the ground state of a nonmagnetic quantum mechanical system should be nodeless. While this notion also provides a valuable guidance in understanding the ordering of energy levels in semiconductor nanostructures, there are reports that $\textit{nodal}$ ground states for holes are possible. However, the existence of such nodal states has been debated and even viewed merely as an artifact of a $\boldsymbol{k{\cdot}p}$ model. Using complementary approaches of both $\boldsymbol{k{\cdot}p}$ and tight-binding models, further supported by an effective Hamiltonian for a continuum model, we reveal that the nodal ground states in quantum dots are not limited to a specific approach. Remarkably, the emergence of the nodal hole states at the top of the valence band can be attributed to the formation of the orbital vortex textures through competition between the hole kinetic energy and the coupling to the conduction band states. We suggest an experimental test for our predictions of the reversed energy ordering and the existence of nodal ground states. We discuss how our findings and the studies of orbital textures could be also relevant for other materials systems.

cond-mat.mes-hall↗

arXiv2013

Magneto-optical conductivity of graphene on polar substrates

We theoretically study the effect of polar substrates on the magneto-optical conductivity of doped monolayer graphene, where we particularly focus on the role played by surface polar phonons (SPPs). Our calculations suggest that polaronic shifts of the intra- and interband absorption peaks can be significantly larger for substrates with strong electron-SPP coupling than those in graphene on non-polar substrates, where only intrinsic graphene optical phonons with much higher energies contribute. Electron-phonon scattering and phonon-assisted transitions are, moreover, found to result in a loss of spectral weight at the absorption peaks. The strength of these processes is strongly temperature-dependent and with increasing temperatures the magneto-optical conductivity becomes increasingly affected by polar substrates, most noticeably in polar substrates with small SPP energies such as HfO$_2$. The inclusion of a Landau level-dependent scattering rate to account for Coulomb impurity scattering does not alter this qualitative picture, but can play an important role in determining the lineshape of the absorption peaks, especially at low temperatures, where impurity scattering dominates.

cond-mat.mes-hall↗

arXiv2012

Spin ordering in magnetic quantum dots: From core-halo to Wigner molecules

The interplay of confinement and Coulomb interactions in quantum dots can lead to strongly correlated phases differing qualitatively from the Fermi liquid behavior. We explore how the presence of magnetic impurities in quantum dots can provide additional opportunities to study correlation effects and the resulting ordering in carrier and impurity spin. By employing exact diagonalization we reveal that seemingly simple two-carrier quantum dots lead to a rich phase diagram. We propose experiments to verify our predictions, in particular we discuss interband optical transitions as a function of temperature and magnetic field.

cond-mat.mes-hall↗