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Isabelle Sagnes

Publications and source records attributed to Isabelle Sagnes.

At least 37 records · Page 2Linked to original sources
arXiv2024

Indistinguishability of remote quantum dot-cavity single-photon sources

Generating identical photons from remote emitter-based bright single-photon sources is an important step for scaling up optical quantum technologies. Here, we study the Hong-Ou-Mandel interference of photons emitted from remote sources based on semiconductor quantum dots. We make use of a deterministic fabrication technique to position the quantum dots in a spectrally resonant micropillar cavity and fine tune their operation wavelength electrically. Doing so, we can match four pairs of sources between five distinct sources, study them under various excitation schemes and measure their degree of indistinguishability. We demonstrate remote indistinguishabiltiy between 44$\pm$1% and 69$\pm$1% depending on the pair of sources and excitation conditions, record values for quantum dots in cavities. The relative contribution of pure dephasing and spectral diffusion is then analysed, revealing that the remaining distinguishability is mostly due to low frequency noise

quant-ph↗
arXiv2024

Regenerative vectorial breathers in a delay-coupled neuromorphic microlaser with integrated saturable absorber

We report on the polarization dynamics of regenerative light pulses in a micropillar laser with integrated saturable absorber coupled to an external feedback mirror. The delayed self-coupled microlaser is operated in the excitable regime, where it regenerates incident pulses with a supra-threshold intensity -- resulting in a pulse train with inter-pulse period approximately given by the feedback delay time, in analogy with a self-coupled biological neuron. We report the experimental observation of vectorial breathers in polarization angle, manifesting themselves as a modulation of the linear polarized intensity components without significant modulation of the total intensity. Numerical analysis of a suitable model reveals that the observed polarization mode competition is a consequence of symmetry-breaking bifurcations induced by polarization anisotropy. Our model reproduces well the observed experimental results and predicts different regimes as a function of the polarization anisotropy parameters and the pump parameter. We believe that these findings are relevant for the fabrication of flexible sources of polarized pulses with controlled properties, as well as for neuroinspired on-chip computing applications, where the polarization may be used to encode or process information in novel ways.

physics.optics↗
arXiv2024

Harnessing coupled nanolasers near exceptional points for directional emission

Tailoring the losses of optical systems within the frame of non-Hermitian physics has appeared very fruitful in the last few years. In particular, the description of exceptional points (EPs) with coupled resonators have become widespread. The on-chip realization of these functionalities is highly significant for integrated nanophotonics, but requires fine control techniques of the nanodevice properties. Here, we demonstrate pump-controlled directional emission of two coupled nanolasers that distantly interact via an integrated waveguide. This coupling scheme unusually enables both frequency- and loss-couplings between two cavities, which can be advantageously exploited to reach EPs by either detuning the cavities or controlling the gain of nanolasers. The system can be readily reconfigured from bidirectional to unidirectional emission by adjusting the pump power.

physics.optics↗
arXiv2024

Certified randomness in tight space

Reliable randomness is a core ingredient in algorithms and applications ranging from numerical simulations to statistical sampling and cryptography. The outcomes of measurements on entangled quantum states can violate Bell inequalities, thus guaranteeing their intrinsic randomness. This constitutes the basis for certified randomness generation. However, this certification requires spacelike separated devices, making it unfit for a compact apparatus. Here we provide a general method for certified randomness generation on a small-scale application-ready device and perform an integrated photonic demonstration combining a solid-state emitter and a glass chip. In contrast to most existing certification protocols, which in the absence of spacelike separation are vulnerable to loopholes inherent to realistic devices, the protocol we implement accounts for information leakage and is thus compatible with emerging compact scalable devices. We demonstrate a 2-qubit photonic device that achieves the highest standard in randomness yet is cut out for real-world applications. The full 94.5-hour-long stabilized process harnesses a bright and stable single-photon quantum-dot based source, feeding into a reconfigurable photonic chip, with stability in the milliradian range on the implemented phases and consistent indistinguishability of the entangled photons above 93%. Using the contextuality framework, we certify private randomness generation and achieve a rate compatible with randomness expansion secure against quantum adversaries.

quant-ph↗
arXiv2024

Origin of optical nonlinearity in plasmonic semiconductor nanostructures

The development of nanoscale nonlinear elements in photonic integrated circuits is hindered by the physical limits to the nonlinear optical response of dielectrics, which requires that the interacting waves propagate in transparent volumes for distances much longer than their wavelength. Here we present experimental evidence that optical nonlinearities in doped semiconductors are due to free-electron and their efficiency could exceed by several orders of magnitude that of conventional dielectric nonlinearities. Our experimental findings are supported by comprehensive computational results based on the hydrodynamic modeling, which naturally includes nonlocal effects, of the free-electron dynamics in heavily doped semiconductors. By studying third-harmonic generation from plasmonic nanoantenna arrays made out of heavily n-doped InGaAs with increasing levels of free-carrier density, we discriminate between hydrodynamic and dielectric nonlinearities. As a result, the value of maximum nonlinear efficiency as well as its spectral location can now be controlled by tuning the doping level. Having employed the common material platform InGaAs/InP that supports integrated waveguides, our findings pave the way for future exploitation of plasmonic nonlinearities in all-semiconductor photonic integrated circuits.

physics.optics↗
arXiv2024

Spin Noise Spectroscopy of a Single Spin using Single Detected Photons

Spin noise spectroscopy has become a widespread technique to extract information on spin dynamics in atomic and solid-state systems, in a potentially non-invasive way, through the optical probing of spin fluctuations. Here we experimentally demonstrate a new approach in spin noise spectroscopy, based on the detection of single photons. Due to the large spin-dependent polarization rotations provided by a deterministically-coupled quantum dot-micropillar device, giant spin noise signals induced by a single-hole spin are extracted in the form of photon-photon cross-correlations. Ultimately, such a technique can be extended to an ultrafast regime probing mechanisms down to few tens of picoseconds.

quant-ph↗
arXiv2023

Elliptical micropillars for efficient generation and detection of coherent acoustic phonons

Coherent acoustic phonon generation and detection assisted by optical resonances are at the core of efficient optophononic transduction processes. However, when dealing with a single optical resonance, the optimum generation and detection conditions take place at different laser wavelengths, i.e. different detunings from the cavity mode. In this work, we theoretically propose and experimentally demonstrate the use of elliptical micropillars to reach these conditions simultaneously at a single wavelength. Elliptical micropillar optophononic resonators present two optical modes with orthogonal polarizations at different wavelengths. By employing a cross-polarized scheme pump-probe experiment, we exploit the mode splitting and couple the pump beam to one mode while the probe is detuned from the other one. In this way, at a particular micropillar ellipticity, both phonon generation and detection processes are enhanced. We report an enhancement of a factor of ~3.1 when comparing the signals from elliptical and circular micropillars. Our findings constitute a step forward in tailoring the light-matter interaction for more efficient ultrahigh-frequency optophononic devices.

physics.optics↗
arXiv2022

Tracking exceptional points above laser threshold

Recent studies on non-Hermitian optical systems having exceptional points (EPs) have revealed a host of unique characteristics associated with these singularities, including unidirectional invisibility, chiral mode switching and laser self-termination, to mention just a few examples. The vast majority of these works focused either on passive systems or active structures where the EPs were accessed below the lasing threshold, i.e. when the system description is inherently linear. In this work, we experimentally demonstrate that EP singularities in coupled semiconductor nanolasers can be accessed and tracked above the lasing threshold, where they become branch points of a nonlinear dynamical system. Contrary to the common belief that unavoidable cavity detuning will impede the formation of an EP, here we demonstrate that this same detuning is necessary for compensating the carrier-induced frequency shift, hence restoring the nonlinear EP in the lasing regime. Furthermore, unlike linear non-Hermitian systems, we find that the spectral location of EPs above laser threshold varies as a function of total pump power and can therefore be continuously tracked. Our work is a first step towards the realization of lasing EPs in more complex laser geometries, and enabling the enhancement of photonic local density of states through non-Hermitian symmetries combined with nonlinear interactions in coupled laser arrays.

physics.optics↗
arXiv2022

Controlling photon polarisation with a single quantum dot spin

In the framework of optical quantum computing and communications, a major objective consists in building receiving nodes that implement conditional operations on incoming photons, using the interaction with a single stationary qubit. In particular, the quest for scalable nodes motivated the development of cavity-enhanced spin-photon interfaces with solid-state emitters. An important challenge remains, however, to produce a stable, controllable, spin-dependant photon state, in a deterministic way. Here we use a pillar-based high-Q cavity, embedding a singly-charged semiconductor quantum dot, to demonstrate the control of giant polarisation rotations induced by a single electron spin. A complete tomography approach is used to deduce the output polarisation Stokes vector, conditioned by a single spin state. We experimentally demonstrate rotation amplitudes such as $\pm \fracπ{2}$ and $π$ in the Poincaré sphere, as required for applications based on spin-polarisation mapping and spin-mediated photon-photon gates. In agreement with our modeling, we observe that the environmental noise does not limit the amplitude of the spin-induced rotation, yet slightly degrades the polarisation purity of the output states. We find that the polarisation state of the reflected photons can be manipulated in most of the Poincaré sphere, through controlled spin-induced rotations, thanks to moderate cavity birefringence and limited noise. This control allows the operation of spin-photon interfaces in various configurations, including at zero or low magnetic fields, which ensures compatibility with key protocols for photonic cluster state generation.

quant-ph↗
arXiv2022

High-fidelity generation of four-photon GHZ states on-chip

Mutually entangled multi-photon states are at the heart of all-optical quantum technologies. While impressive progresses have been reported in the generation of such quantum light states using free space apparatus, high-fidelity high-rate on-chip entanglement generation is crucial for future scalability. In this work, we use a bright quantum-dot based single-photon source to demonstrate the high fidelity generation of 4-photon Greenberg-Horne-Zeilinger (GHZ) states with a low-loss reconfigurable glass photonic circuit. We reconstruct the density matrix of the generated states using full quantum-state tomography reaching an experimental fidelity to the target $|{\text{GHZ}_4}\rangle$ of $\mathcal{F}_{\text{GHZ}_4} (86.0\pm0.4)\,\%$, and a purity of $\mathcal{P}_{\text{GHZ}_4}=(76.3\pm0.6)\,\%$. The entanglement of the generated states is certified with a semi device-independent approach through the violation of a Bell-like inequality by more than 39 standard deviations. Finally, we carry out a four-partite quantum secret sharing protocol on-chip where a regulator shares with three interlocutors a sifted key with up to 1978 bits, achieving a qubit-error rate of $10.87\,\%$. These results establish that the quantum-dot technology combined with glass photonic circuitry for entanglement generation on chip offers a viable path for intermediate scale quantum computation and communication.

quant-ph↗
arXiv2022

Ultra-low-noise Microwave to Optics Conversion in Gallium Phosphide

Mechanical resonators can act as excellent intermediaries to interface single photons in the microwave and optical domains due to their high quality factors. Nevertheless, the optical pump required to overcome the large energy difference between the frequencies can add significant noise to the transduced signal. Here we exploit the remarkable properties of thin-film gallium phosphide to demonstrate bi-directional on-chip conversion between microwave and optical frequencies, realized by piezoelectric actuation of a Gigahertz-frequency optomechanical resonator. The large optomechanical coupling and the suppression of two-photon absorption in the material allows us to operate the device at optomechanical cooperativities greatly exceeding one. Alternatively, when using a pulsed upconversion pump, we demonstrate that we induce less than one thermal noise phonon. We include a high-impedance on-chip matching resonator to mediate the mechanical load with the 50-Ohm source. Our results establish gallium phosphide as a versatile platform for ultra-low-noise conversion of photons between microwave and optical frequencies.

quant-ph↗
arXiv2022

Brillouin Scattering Selection Rules in Polarization-Sensitive Photonic Resonators

The selection rules governing spontaneous Brillouin scattering in crystalline solids are usually taken as intrinsic material properties, locking the relative polarization of excitation and signal in bulk. In this work, we independently manipulate these polarization states by means of optical resonances in elliptical micropillars and demonstrate a polarization-based filtering scheme for Brillouin spectroscopy in the 20-100 GHz range, important for telecom applications. This strong modification of selection rules using elliptical micropillars can be extended to any optical system with localized, polarization-sensitive modes, such as plasmonic resonators, photonic crystals, birefringent micro-, and nanostructures. Our polarization control protocol will thus find applications in the engineering of light-matter interactions in optomechanical, optoelectronic and quantum optics devices.

physics.optics↗
arXiv2022

Merging and disconnecting resonance tongues in a pulsing excitable microlaser with delayed optical feedback

Excitability, encountered in numerous fields from biology to neurosciences and optics, is a general phenomenon characterized by an all-or-none response of a system to an external perturbation. When subject to delayed feedback, excitable systems can sustain multistable pulsing regimes, which are either regular or irregular time sequences of pulses reappearing every delay time. Here, we investigate an excitable microlaser subject to delayed optical feedback and study the emergence of complex pulsing dynamics, including periodic, quasiperiodic and irregular pulsing regimes. This work is motivated by experimental observations showing these different types of pulsing dynamics. A suitable mathematical model, written as a system of delay differential equations, is investigated through an in-depth bifurcation analysis. We demonstrate that resonance tongues play a key role in the emergence of complex dynamics, including non-equidistant periodic pulsing solutions and chaotic pulsing. The structure of resonance tongues is shown to depend very sensitively on the pump parameter. Successive saddle transitions of bounding saddle-node bifurcations constitute a merging process that results in unexpectedly large locking regions, which subsequently disconnect from the relevant torus bifurcation curve; the existence of such unconnected regions of periodic pulsing is in excellent agreement with experimental observations. As we show, the transition to unconnected resonance regions is due to a general mechanism: the interaction of resonance tongues locally at an extremum of the rotation number on a torus bifurcation curve. We present and illustrate the two generic cases of disconnecting and of disappearing resonance tongues. Moreover, we show how a maximum and a minimum of the rotation number appears naturally when two torus bifurcation curves undergo a saddle transition (where they connect differently).

math.DS↗
arXiv2022

Observation of KPZ universal scaling in a one-dimensional polariton condensate

Revealing universal behaviors is a hallmark of statistical physics. Phenomena such as the stochastic growth of crystalline surfaces, of interfaces in bacterial colonies, and spin transport in quantum magnets all belong to the same universality class, despite the great plurality of physical mechanisms they involve at the microscopic level. This universality stems from a common underlying effective dynamics governed by the non-linear stochastic Kardar-Parisi-Zhang (KPZ) equation. Recent theoretical works suggest that this dynamics also emerges in the phase of out-of-equilibrium systems displaying macroscopic spontaneous coherence. Here, we experimentally demonstrate that the evolution of the phase in a driven-dissipative one-dimensional polariton condensate falls in the KPZ universality class. Our demonstration relies on a direct measurement of KPZ space-time scaling laws, combined with a theoretical microscopic analysis that consistently reveals the other key signatures of this universality class, together with the possible resilience of KPZ dynamics to the presence of space-time vortices. Our results highlight fundamental physical differences between out-of-equilibrium condensates and their equilibrium counterparts, and open a new paradigm for exploring universal behaviors in open systems.

cond-mat.mes-hall↗
arXiv2022

Continuous-Wave Second-Harmonic Generation in Orientation-Patterned GaP Waveguides at Telecom Wavelengths

A new process to produce Orientation-Patterned Gallium Phosphide (OP-GaP) on GaAs with almost perfectly parallel domain boundaries is presented. Taking advantage of the chemical selectivity between phosphides and arsenides, OP-GaP is processed into suspended shallow-ridge waveguides. Efficient Second-Harmonic Generation from Telecom wavelengths is achieved in both Type-I and Type-II polarisation configurations. The highest observed conversion efficiency is \SI{200}{\percent\per\watt\per\centi\meter\squared}, with a bandwidth of \SI{2.67}{\nano\meter} in a \SI{1}{\milli\meter}-long waveguide. The variation of the conversion efficiency with wavelength closely follows a squared cardinal sine function, in excellent agreement with theory, confirming the good uniformity of the poling period over the entire length of the waveguide.

physics.optics↗
arXiv2022

Quantifying n-photon indistinguishability with a cyclic integrated interferometer

We report on a universal method to measure the genuine indistinguishability of n-photons - a crucial parameter that determines the accuracy of optical quantum computing. Our approach relies on a low-depth cyclic multiport interferometer with N = 2n modes, leading to a quantum interference fringe whose visibility is a direct measurement of the genuine n-photon indistinguishability. We experimentally demonstrate this technique for a 8-mode integrated interferometer fabricated using femtosecond laser micromachining and four photons from a quantum dot single-photon source. We measure a four-photon indistinguishability up to 0.81$\pm$0.03. This value decreases as we intentionally alter the photon pairwise indistinguishability. The low-depth and low-loss multiport interferometer design provides an efficient and scalable path to evaluate the genuine indistinguishability of resource states of increasing photon number.

quant-ph↗
arXiv2021

Few-photon all-optical phase rotation in a quantum-well micropillar cavity

Photonic platforms are an excellent setting for quantum technologies because weak photon-environment coupling ensures long coherence times. The second key ingredient for quantum photonics is interactions between photons, which can be provided by optical nonlinearities in the form of cross-phase-modulation (XPM). This approach underpins many proposed applications in quantum optics and information processing, but achieving its potential requires strong single-photon-level nonlinear phase shifts and also scalable nonlinear elements. In this work we show that the required nonlinearity can be provided by exciton-polaritons in micropillars with embedded quantum wells. These combine the strong interactions of excitons with the scalability of micrometer-sized emitters. We observe XPM up to $3 \pm 1$ mrad per particle using laser beams attenuated to below single photon average intensity. With our work serving as a first stepping stone, we lay down a route for quantum information processing in polaritonic lattices.

physics.optics↗