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Itamar Kimchi

Publications and source records attributed to Itamar Kimchi.

At least 19 recordsLinked to original sources

Topological Impurity Bands

The effects of disorder on topological phases of matter are typically either preservation of topology or its destruction. For example, the quantum Hall effect's quantization and chiral edge mode remain robust until a strong-disorder percolation transition exits the topological phase. Disorder can also enlarge a preexisting topological phase, yielding a topological Anderson insulator (TAI). However, the reliance of TAI and other theoretical treatments on perturbatively averaging out long-wavelength randomness suggests that additional effects might appear when the disorder involves localized defects. Here we show that a finite density of randomly distributed defects can generate various new topological phase transitions. This route to disorder-induced topology can be viewed as the formation of topological impurity bands (TIB) and is applicable even if the initial clean model is a trivial band insulator. The theory relies on an orbital-dependent vorticity of impurity bound states, which we derive analytically near a generic Dirac cone phase transition as well as using the Chern insulator lattice models of Qi-Wu-Zhang and Haldane. Their numerically computed phase diagrams at 3% defect density show robust topological transitions in distinct TIB and TAI regimes, suggesting a local route to topological phases.

cond-mat.mes-hall

Generation of chirality and orbital magnetization by Stone-Wales-type lattice defects in the Kitaev spin liquid

In this work we extend our study of the effect of certain crystallographic defects on the spin-1/2 Kitaev honeycomb spin liquid (arXiv:2511.19409), focusing on its gapless phase and contrasting with the gapped phase. We identify a Stone-Wales (SW) local defect consisting of a 90$^\circ$ bond rotation that preserves Kitaev bond labels for edge-sharing octahedra and thereby enables exact solvability. These SW-type defects involve odd-sided plaquettes with $\pm \pi/2$ fluxes, but can be created locally. An isolated defect hosts a time-reversal pair of ground-state flux configurations with large net chirality. Certain excitations are also chiral. The chirality manifests in Majorana local Chern marker and in scalar spin chirality, producing electronic orbital magnetization. T-matrix analysis and numerics at finite defect density $n_d$ show that defect chiralities generate a topological gap of $11 n_d$ protecting a Chern number $C=\pm 1$. Emergent ferromagnetic long range Ising interactions $r^{-\gamma}$ with $2<\gamma < 3$ between defect chiralities lead to a finite temperature $T_c$ phase transition into the chiral spin liquid. The $T_c$ is proportional to $n_d$ and diverges when $\gamma\rightarrow 2$. We also consider additional solvable impurity potentials and find that $\gamma$ can be reduced to below $2.3$ and correspondingly enhance $T_c$. Our results offer applications to 2D Dirac cone systems with a finite density of fluctuating Ising magnetic impurities and to identifying spin liquids with lattice defects.

cond-mat.str-el

Chiral spin liquid instability of the Kitaev honeycomb model with crystallographic defects

We study the spin-1/2 Kitaev honeycomb gapless spin liquid in the presence of Stone-Wales-type local lattice defects with odd-sided plaquettes. While the clean Kitaev model has no finite-temperature phase transitions, we find that introducing a finite defect density $n_d\approx 10^{-4}$--$10^{-2}$ produces a true phase transition with a sizeable $T_c \approx 2 n_d$ in units of the Kitaev exchange. The resulting non-Abelian chiral quantum spin liquid exhibits scalar spin chirality and electron orbital magnetization which peak near lattice defects. This disorder-driven instability relies on an emergent long range ferromagnetic interaction $r^{-\gamma}$ ($\gamma \approx 2.7$) between defect chiralities, mediated by the nearly-gapless fermions, with implications for topology generation in Dirac cones with fluctuating mass terms.

cond-mat.str-el

Chirality reversal at finite magnetic impurity strength and local signatures of a topological phase transition

We study the honeycomb lattice with a single magnetic impurity modeled by adding imaginary next-nearest-neighbor hopping ih on a single hexagon. This Haldane defect gives a topological mass term to the gapless Dirac cones and generates chirality. For a small density of defects Neehus et al [arXiv:2405.19289] found that the system's chirality reverses at a critical hc ~ 0.95 associated with an unexpected tri-critical point of Dirac fermions at zero defect density. We investigate this zero-density limit by analyzing a single defect and computing two experimentally relevant measures of chirality: (1) orbital magnetization via local Chern marker, a bulk probe of all occupied states; and (2) electronic currents of low-energy states. Both probes show a chirality reversal at a critical hc ~ 0.9--1. Motivated by this consistency we propose a defect-scale toy model whose low energy states reverse their chirality at hc' ~ 0.87. Remarkably, the same pair of zero energy bound states also generate the critical point hc in the full impurity projected T-matrix. Our results show how the chirality reversal produced by an impurity can be observed either in local probes or in the global topology and suggest a possible role of the microscopic defect structure at the critical point.

cond-mat.mes-hall

Emergent Inductance from Chiral Orbital Currents in a Bulk Ferrimagnet

We report the discovery of a new form of inductance in the bulk ferrimagnet Mn3Si2Te6, which features strong spin-orbit coupling, large magnetic anisotropy, and pronounced magnetoelastic interactions. Below its Curie temperature, Mn3Si2Te6 hosts chiral orbital currents (COC) that circulate within the crystal lattice and give rise to collective electronic behavior [1]. By applying a magnetic field along the hard c axis and driving the system with low-frequency currents, we uncover a giant inductive response up to millihenry scale, originating from first-order reconfigurations of COC domains. These domains act as coherent mesoscopic inductive elements that resist reversal upon current reduction, producing a large electromotive force and sharply increasing voltage. This emergent inductance defies classical models, occurs without superconductivity or engineered nanostructures, and opens a new frontier in orbital-based quantum functionality and device concepts.

cond-mat.str-el

Sharp spectroscopic fingerprints of disorder in an incompressible magnetic state

Disorder significantly impacts the electronic properties of conducting quantum materials by inducing electron localization and thus altering the local density of states and electric transport. In insulating quantum magnetic materials, the effects of disorder are less understood and can drastically impact fluctuating spin states like quantum spin liquids. In the absence of transport tools, disorder is typically characterized using chemical methods or by semi-classical modeling of spin dynamics. This requires high magnetic fields that may not always be accessible. Here, we show that magnetization plateaus -- incompressible states found in many quantum magnets -- provide an exquisite platform to uncover small amounts of disorder, regardless of the origin of the plateau. Using optical magneto-spectroscopy on the Ising-Heisenberg triangular-lattice antiferromagnet K$_2$Co(SeO$_3$)$_2$ exhibiting a 1/3 magnetization plateau, we identify sharp spectroscopic lines, the fine structure of which serves as a hallmark signature of disorder. Through analytical and numerical modeling, we show that these fingerprints not only enable us to quantify minute amounts of disorder but also reveal its nature -- as dilute vacancies. Remarkably, this model explains all details of the thermomagnetic response of our system, including the existence of multiple plateaus. Our findings provide a new approach to identifying disorder in quantum magnets.

cond-mat.mtrl-sci

Real-space chirality from crystalline topological defects in the Kitaev spin liquid

We show that certain crystalline topological defects in the gapless Kitaev honeycomb spin liquid model generate a chirality and Majorana fermion orbital magnetization that depends in a universal manner on their emergent flux. Focusing on 5-7 dislocations as building blocks, consisting of pentagon and heptagon disclinations, we identify the Kitaev bond label configurations that preserve solvability. By computing two formulations of local markers $M(r)$ we find that the 5 and 7 lattice defects generate a real-space contribution to Chern number and an associated Majorana fermion orbital magnetization proportional to $M(r)$. The sign of the $M(r)$ contribution from each 5/7 defect, i.e. its $q_M=\pm 1$ chirality, is determined by the defect Frank angle sign $F$ and emergent gauge field flux $W = \pm i$ through the expression $q_M = - i F W$. Remarkably, though lattice curvature and torsion can interplay with the surrounding gapless background to modify the profile of $M(r)$, its sign $q_M$ is determined locally, implying that crystalline defects in the Kitaev spin liquid can generate a robust and observable chirality.

cond-mat.str-el

Disorder-induced spin-cluster magnetism in a doped kagome spin liquid candidate

The search for new quantum spin liquid materials relies on systems with strong frustration such as spins on an ideal kagome lattice. However, lattice imperfections can have substantial effects which are as yet not well understood. In recent work, the two-dimensional kagome system YCu$_3$(OH)$_6$[(Cl$_x$Br$_{(1-x)}$)$_{3-y}$(OH)$_y$] has emerged as a leading candidate hosting a Dirac spin liquid which appears to survive at least for x<0.4, associated with alternating-bond hexagon (ABH) disorder. Here in magnetic samples with x=0.58, y=0.1 we report unusual in-plane ferromagnetic canting (FM) of the in-plane antiferromagnet (AFM), with an unusually wide regime of short-ranged order, and propose theoretical models to explain this behavior. First, we show that Kitaev type exchanges naturally arise on the kagome lattice to second order in the known Dzyaloshinskii-Moriya exchanges, and that these interactions can produce the unusual in-plane FM canting from antichiral AFM. Second, we propose a phenomenological model of weakly-FM-canted spin clusters to describe the short-ranged regime and analyze quantum fluctuations in an ABH toy model to show how ABH disorder can stabilize this regime. The combination of experimental observation and theory suggests that kagome-Kitaev interactions and ABH disorder are necessary for describing the magnetic fluctuations in this family of materials, with potential implications for the proposed proximate spin liquid phase.

cond-mat.str-el

Magneto-synthesis effect on magnetic order, phonons, and magnons in single-crystal Sr$_2$IrO$_4$

It was shown earlier that applying a magnetic field during the growth of Sr$_2$IrO$_4$, also known as "field-alteration", induces significant changes to its structural, magnetic, and transport properties. However, the microscopic nature of these changes is enigmatic. In this study, we employed resonant elastic and inelastic x-ray scattering, as well as Raman scattering, to investigate samples from two batches of Sr$_2$IrO$_4$ grown in magnetic fields of different strengths. Our findings reveal that samples grown in a weaker magnetic field have similar magnetic order to non-altered samples, whereas those grown in a stronger field show a different stacking of weak in-plane ferromagnetic moments. Additionally, we observed significant softening and broadening of select Raman-active phonons in the field altered samples, with a stronger effect in the samples grown in the stronger field. We discuss insights that our results provide into the microscopic nature of field-alteration in Sr$_2$IrO$_4$.

cond-mat.str-el

Non-Analytic Magnetic Response and Intrinsic Ferromagnetic Clusters in a Dirac Spin Liquid Candidate

Finding distinct signatures of a quantum spin liquid (QSL) is an ongoing quest in condensed matter physics, invariably complicated by the presence of disorder in real materials. In this regard the 2D Kagome system YCu$_3$(OH)$_6$[(Cl$_x$Br$_{(1-x)}$)$_{3-y}$(OH)$_y$] (YCOB-Cl), where the vast mismatch in size of Y and Cu avoids subsitutional disorder, otherwise present in kagome materials, has emerged as a favorable candidate. In crystals of this system, with $x<$ 0.4 and no long range order, we report an unusual field dependent magnetization $M(B)$, where $M/B$ changes linearly with $|B|$, the absolute value of the field, in contrast to the expected quadratic behavior. Model calculations with a distribution of ferromagnetic (FM) clusters faithfully capture observed features suggesting such clusters to be intrinsic to real QSL materials. YCOB-Cl has a field enhanced $T^2$ heat capacity as expected for a Dirac QSL but lacks a linear $T$ behavior in the spin susceptibility. By demonstrating that FM clusters dominate the contribution to the susceptibility but not the heat capacity, our work paves the way towards reconciling the apparent inconsistency with a Dirac QSL.

cond-mat.str-el

Crystalline topological defects within response theory

Crystal defects can highlight interesting quantum features by coupling to the low-energy Hamiltonian $H$. Here we show that independently of this $H$ coupling, topological crystalline defects can generate new features by directly modifying the response theory of electric field probes such as Raman scattering. To show this we consider an antiferromagnetic spin-1/2 model $H_{spin}$ on a zigzag chain. Crystalline domain walls between two zigzag domains appear as at most local defects in $H_{spin}$, but as topological (not locally creatable) defects in the Raman operator $R$ of inelastic photon scattering. Using time evolving block decimation (TEBD) numerics, mean field, and bosonization, we show that a finite density of crystalline domain walls shifts the entire Raman signal to produce an effective gap. This lattice-defect-induced Raman gap closes and reopens in applied magnetic fields. We discuss the effect in terms of photons sensing the lattice defects within $R$ as spin-dimerization domain walls, with $Z_2$ character, and a resulting shift of the probed wavevector from $q=0$ to $\pi+\delta q$, giving an $\textit{O}(1)$ change in contrast to local defects. The magneto-Raman singularity from topological lattice defects here relies on the $H_{spin}$ spinon liquid state, suggesting future applications using lattice topological defects to modify response-theory operators independently of $H$ and thereby generate new probes of quantum phases.

cond-mat.str-el

Control of chiral orbital currents in a colossal magnetoresistance material

Colossal magnetoresistance (CMR) is an extraordinary enhancement of the electric conductivity in the presence of a magnetic field. It is conventionally associated with a field-induced spin polarization, which drastically reduces spin scattering and thus electric resistance. However, ferrimagnetic Mn3Si2Te6 is an intriguing exception to this rule: it exhibits a 7-order-of-magnitude reduction in ab-plane resistivity with a 13-Tesla anisotropy field which occur only when a magnetic polarization is avoided [1]. Here we report an exotic quantum state that is driven by ab-plane chiral orbital currents (COC) flowing along edges of MnTe6 octahedra. The c-axis orbital moments of ab-plane COC couple to the ferrimagnetic Mn spins to drastically increase the ab-plane conductivity (CMR) when an external magnetic field is aligned along the magnetic hard c-axis. Both the COC state and its CMR are extraordinarily susceptible to small DC currents exceeding a critical threshold, and a hallmark of this COC state is an exotic time-dependent, bistable switching mimicking a first-order melting transition. The control of the COC-enabled CMR and bistable switching offers a fundamentally new paradigm for quantum technologies.

cond-mat.str-el

Magnetic memory and spontaneous vortices in a van der Waals superconductor

Doped Mott insulators exhibit some of the most intriguing quantum phases of matter, including quantum spin-liquids, unconventional superconductors, and non-Fermi liquid metals. Such phases often arise when itinerant electrons are close to a Mott insulating state, and thus experience strong spatial correlations. Proximity between different layers of van der Waals heterostructures naturally realizes a platform for experimentally studying the relationship between localized, correlated electrons and itinerant electrons. Here, we explore this relationship by studying the magnetic landscape of 4Hb-TaS2, which realizes an alternate stack of a candidate spin liquid and a superconductor. We report on a spontaneous vortex phase whose vortex density can be trained in the normal state. We show that time reversal symmetry is broken above Tc, indicating the presence of a magnetic phase independent of the superconductor. Strikingly, this phase does not generate detectable magnetic signals. We use scanning superconducting quantum interference device (SQUID) microscopy to show that it is incompatible with ferromagnetic ordering. The discovery of this new form of hidden magnetism illustrates how combining superconductivity with a strongly correlated system can lead to new, unexpected physics.

cond-mat.supr-con

Spinons and damped phonons in spin-1/2 quantum-liquid Ba$_{4}$Ir${}_3$O${}_{10}$ observed by Raman scattering

In spin-1/2 Mott insulators, non-magnetic quantum liquid phases are often argued to arise when the system shows no magnetic ordering, but identifying positive signatures of these phases or related spinon quasiparticles can be elusive. Here we use Raman scattering to provide three signatures for spinons in a possible spin-orbit quantum liquid material Ba${}_4$Ir${}_3$O${}_{10}$: (1) A broad hump, which we show can arise from Luttinger Liquid spinons in Raman with parallel photon polarizations normal to 1D chains; (2) Strong phonon damping from phonon-spin coupling via the spin-orbit interaction; and (3) the absence of (1) and (2) in the magnetically ordered phase that is produced when 2% of Ba is substituted by Sr ((Ba${}_{0.98}$Sr${}_{0.02}$)${}_4$Ir${}_3$O${}_{10}$). The phonon damping via itinerant spinons seen in this quantum-liquid insulator suggests a new mechanism for enhancing thermoelectricity in strongly correlated conductors, through a neutral quantum liquid that need not affect electronic transport.

cond-mat.str-el

Tunable-spin-model generation with spin-orbit-coupled fermions in optical lattices

We study the dynamical behaviour of ultracold fermionic atoms loaded into an optical lattice under the presence of an effective magnetic flux, induced by spin-orbit coupled laser driving. At half filling, the resulting system can emulate a variety of iconic spin-1/2 models such as an Ising model, an XY model, a generic XXZ model with arbitrary anisotropy, or a collective one-axis twisting model. The validity of these different spin models is examined across the parameter space of flux and driving strength. In addition, there is a parameter regime where the system exhibits chiral, persistent features in the long-time dynamics. We explore these properties and discuss the role played by the system's symmetries. We also discuss experimentally-viable implementations.

cond-mat.quant-gas

Strange electrical transport: Colossal magnetoresistance via avoiding fully polarized magnetization in ferrimagnetic insulator Mn3Si2Te6

Colossal magnetoresistance is of great fundamental and technological significance and exists mostly in the manganites and a few other materials. Here we report colossal magnetoresistance that is starkly different from that in all other materials. The stoichiometric Mn3Si2Te6 is an insulator featuring a ferrimagnetic transition at 78 K. The resistivity drops by 7 orders of magnitude with an applied magnetic field above 9 Tesla, leading to an insulator-metal transition at up to 130 K. However, the colossal magnetoresistance occurs only when the magnetic field is applied along the magnetic hard axis and is surprisingly absent when the magnetic field is applied along the magnetic easy axis where magnetization is fully saturated. The anisotropy field separating the easy and hard axes is 13 Tesla, unexpected for the Mn ions with nominally negligible orbital momentum and spin-orbit interactions. Double exchange and Jahn-Teller distortions that drive the hole-doped manganites do not exist in Mn3Si2Te6. The phenomena fit no existing models, suggesting a unique, intriguing type of electrical transport.

cond-mat.str-el

Quest for New Quantum States via Field-Editing Technology

We report new quantum states in spin-orbit-coupled single crystals that are synthesized using a game-changing technology that "field-edits" crystal structures (borrowing from the phrase "genome editing") via application of magnetic field during crystal growth. This study is intended to fundamentally address a major challenge facing the research community today: A great deal of theoretical work predicting exotic states for strongly spin-orbit-coupled, correlated materials has thus far met very limited experimental confirmation. These conspicuous discrepancies are due chiefly to the extreme sensitivity of these materials to structural distortions. The results presented here demonstrate that the "field-edited" materials not only are much less distorted but also exhibit novel phenomena absent in their "non-edited" counterparts. The field-edited materials include an array of 4d and 5d transition metal oxides, and three representative materials presented here are Ba4Ir3O10, Ca2RuO4, and Sr2IrO4. This study provides an entirely new paradigm for discovery of new quantum states and materials otherwise unavailable.

cond-mat.str-el

Quantum liquid from strange frustration in the trimer magnet Ba4Ir3O10

Quantum spin systems such as magnetic insulators usually show classical magnetic order, but such classical states can give way to quantum liquids with exotic entanglement through two known mechanisms of frustration: geometric frustration in lattices with triangle motifs, and spin-orbit-coupling frustration in the exactly solvable quantum liquid of Kitaev's honeycomb lattice. Here we present the experimental observation of a new kind of frustrated quantum liquid arising in an unlikely place: the magnetic insulator Ba4Ir3O10 where Ir3O12 trimers form an unfrustrated square lattice. Experimentally we find a quantum liquid state persisting down to 0.2 K that is stabilized by strong antiferromagnetic interaction with Curie-Weiss temperature - 766 K. The astonishing frustration parameter of 3800 is beyond any known iridate thus far. Heat capacity and thermal conductivity are both linear at low temperatures, a familiar feature in metals but here in an insulator pointing to an exotic quantum liquid state. A mere 2% Sr substitution for Ba produces long-range order at 130 K and destroys the linear-T features. Although the Ir4+(5d5) ions in Ba4Ir3O10 appear to form Ir3O12 trimers of face-sharing IrO6 octahedra, we propose that intra-trimer exchange is reduced and the lattice recombines into an array of coupled 1D chains with additional spins. An extreme limit of decoupled 1D chains can explain most but not all of the striking experimental observations, indicating that the inter-chain coupling plays an important role in the novel frustration mechanism leading to this quantum liquid.

cond-mat.str-el