arXiv subjects

Itamar Kimchi

Publications and source records attributed to Itamar Kimchi.

At least 37 records · Page 2Linked to original sources

arXiv2019

Nonequilibrium Orbital Transitions via Applied Electrical Current in Calcium Ruthenate

Simultaneous control of structural and physical properties via applied electrical current poses a key, new research topic and technological significance. Studying the spin-orbit-coupled antiferromagnet Ca2RuO4, with 3% Mn doping to weaken the violent first-order transition at 357 K for more robust measurements, we find that a small applied electrical current couples to the lattice by significantly reducing its orthorhombicity and octahedral rotations, concurrently diminishing the 125 K- antiferromagnetic transition and inducing a new, orbital order below 80 K. Our effort to establish a phase diagram reveals a critical regime near a current density of 0.15 A/cm2 that separates the vanishing antiferromagnetic order and the new orbital order. Further increasing current density (> 1 A/cm2) enhances competitions between relevant interactions in a metastable manner, leading to a peculiar glassy behavior above 80 K. The coupling between the lattice and nonequilibrium driven current is interpreted theoretically in terms of t2g orbital occupancies. The current-controlled lattice is the driving force of the observed novel phenomena.

cond-mat.str-el↗

arXiv2019

Hidden spin-orbital order in the Kitaev hyperhoneycomb $β$-Li$_2$IrO$_3$

We report the existence of a phase transition at high temperature in the 3D Kitaev candidate material, $β$-Li$_2$IrO$_3$. We show that the transition is bulk, intrinsic and orders a tiny magnetic moment with a spatially anisotropic saturation moment. We show that even though this transition is global, it does not freeze the local Ir moments, which order at much lower temperatures into an incommensurate state. Rather, the ordered moment has an orbital origin that is coupled to spin correlations, likely of a Kitaev origin. The separate ordering of spin-correlated orbital moments and of local Ir moments reveals a novel way in which magnetic frustration in Kitaev systems can lead to coexisting magnetic states.

cond-mat.str-el↗

arXiv2019

Anomalous localization at the boundary of an interacting topological insulator

The boundary of a topological insulator (TI) hosts an anomaly restricting its possible phases: e.g. 3D strong and weak TIs maintain surface conductivity at any disorder if symmetry is preserved on-average, at least when electron interactions on the surface are weak. However the interplay of strong interactions and disorder with the boundary anomaly has not yet been theoretically addressed. Here we study this combination for the edge of a 2D TI and the surface of a 3D weak TI, showing how it can lead to an "Anomalous Many Body Localized" (AMBL) phase that preserves the anomaly. We discuss how the anomalous Kramers parity switching with pi flux arises in the bosonized theory of the localized helical state. The anomaly can be probed in localized boundaries by electrostatically sensing nonlinear hopping transport with e/2 shot noise. Our AMBL construction in 3D weak TIs fails for 3D strong TIs, suggesting that their anomaly restrictions are distinguished by strong interactions.

cond-mat.str-el↗

arXiv2019

Magnetic field-dependent low-energy magnon dynamics in $α$-RuCl3

Revealing the spin excitations of complex quantum magnets is key to developing a minimal model that explains the underlying magnetic correlations in the ground state. We investigate the low-energy magnons in $α$-RuCl$_3$ by combining time-domain terahertz spectroscopy under an external magnetic field and model Hamiltonian calculations. We observe two absorption peaks around 2.0 and 2.4 meV, which we attribute to zone-center spin waves. Using linear spin-wave theory with only nearest-neighbor terms of the exchange couplings, we calculate the antiferromagnetic resonance frequencies and reveal their dependence on an external field applied parallel to the nearest-neighbor Ru-Ru bonds. We find that the magnon behavior in an applied magnetic field can be understood only by including an off-diagonal $Γ$ exchange term to the minimal Heisenberg-Kitaev model. Such an anisotropic exchange interaction that manifests itself as a result of strong spin-orbit coupling can naturally account for the observed mixing of the modes at higher fields strengths.

cond-mat.str-el↗

arXiv2019

Quantum entropic self-localization with ultracold fermions

We study a driven, spin-orbit coupled fermionic system in a lattice at the resonant regime where the drive frequency equals the Hubbard repulsion, for which non-trivial constrained dynamics emerge at fast timescales. An effective density-dependent tunneling model is derived, and examined in the sparse filling regime in 1D. The system exhibits entropic self-localization, where while even numbers of atoms propagate ballistically, odd numbers form localized bound states induced by an effective attraction from a higher configurational entropy. These phenomena occur in the strong coupling limit where interactions only impose a constraint with no explicit Hamiltonian term. We show how the constrained dynamics lead to quantum few-body scars and map to an Anderson impurity model with an additional intriguing feature of non-reciprocal scattering. Connections to many-body scars and localization are also discussed.

quant-ph↗

arXiv2019

A Novel ground state in a new dimer iridate Ba13Ir6O30 with Ir6+(5d3) Ions

We have synthesized and studied a new iridate, Ba13Ir6O30, with unusual Ir oxidation states: 2/3 Ir6+(5d3) ions and 1/3 Ir5+(5d4) ions. Its crystal structure features dimers of face-sharing IrO6 octahedra, and IrO6 monomers, that are linked via long, zigzag Ir-O-Ba-O-Ir pathways. Nevertheless, Ba13Ir6O30 exhibits two transitions at TN1 = 4.7 K and TN2 = 1.6 K. This magnetic order is accompanied by a huge Sommerfeld coefficient 200 mJ/mole K below TN2, signaling a coexisting frustrated/disordered state persisting down to at least 0.05 K. This iridate hosts unusually large Jeff=3/2 degrees of freedom, which is enabled by strong spin-orbit interactions (SOI) in the monomers with Ir6+ ions and a joint effect of molecular orbitals and SOI in the dimers occupied by Ir5+ and Ir6+ ions. Features displayed by the magnetization and heat capacity suggest that the combination of covalency, SOI and large effective spins leads to highly frustrated ferrimagnetic ordering, possibly into a skyrmion crystal, a novelty of this new high-spin iridate.

cond-mat.str-el↗

arXiv2018

Scaling and data collapse from local moments in frustrated disordered quantum spin systems

Recently measurements on various spin-1/2 quantum magnets such as H$_3$LiIr$_2$O$_6$, LiZn$_2$Mo$_3$O$_8$, ZnCu$_3$(OH)$_6$Cl$_2$ and 1T-TaS$_2$ -- all described by magnetic frustration and quenched disorder but with no other common relation -- nevertheless showed apparently universal scaling features at low temperature. In particular the heat capacity C[H,T] in temperature T and magnetic field H exhibits T/H data collapse reminiscent of scaling near a critical point. Here we propose a theory for this scaling collapse based on an emergent random-singlet regime extended to include spin-orbit coupling and antisymmetric Dzyaloshinskii-Moriya (DM) interactions. We derive the scaling $C[H,T]/T \sim H^{-γ} F_q[T/H]$ with $F_q[x] = x^{q}$ at small $x$, with $q \in$ (0,1,2) an integer exponent whose value depends on spatial symmetries. The agreement with experiments indicates that a fraction of spins form random valence bonds and that these are surrounded by a quantum paramagnetic phase. We also discuss distinct scaling for magnetization with a $q$-dependent subdominant term enforced by Maxwell's relations.

cond-mat.str-el↗

arXiv2018

Paired exciton condensate and topological charge-$4e$ composite fermion pairing in half-filled quantum Hall bilayers

Half-filled Landau levels admit the theoretically powerful fermion-vortex duality but longstanding puzzles remain in their experimental realization as $ν_T=1$ quantum Hall bilayers, further complicated by Zheng et al's recent numerical discovery of an unknown phase at intermediate layer spacing. Here we propose that half-filled quantum Hall bilayers ($ν_T=1$) at intermediate values of the interlayer distance $d/\ell_B$ enter a phase with \textit{paired exciton condensation}. This phase shows signatures analogous to the condensate of interlayer excitons (electrons bound to opposite-layer holes) well-known for small $d$ but importantly condenses only exciton pairs. To study it theoretically we derive an effective Hamiltonian for bosonic excitons $b_k$ and show that the single-boson condensate suddenly vanishes for $d$ above a critical $d_{c1} \approx 0.95 l_B$. The nonzero condensation fraction $n_0=\langle b(0) \rangle ^2$ at $d_{c1}$ suggests that the phase stiffness remains nonzero for a range of $d>d_{c1}$ via an intermediate phase of paired-exciton condensation, exhibiting $\langle bb \rangle \neq 0$ while $\langle b \rangle =0$. Motivated by these results we derive a $K$-matrix description of the paired exciton condensate's topological properties from composite boson theory. The elementary charged excitation is a half meron with $\frac{1}{4}$ charge and fractional self-statistics $θ_s=\fracπ{16}$. Finally we argue for an equivalent description via the $d=\infty$ limit through topological charge-$4e$ pairing of composite fermions. We suggest graphene double layers should access this phase and propose various experimental signatures, including an Ising transition $T_{Ising}$ below the Berezinskii-Kosterlitz-Thouless transition $T_{BKT}$ at $d \sim d_{c1}$.

cond-mat.str-el↗

arXiv2018

Robust non-Abelian spin liquid and possible intermediate phase in antiferromagnetic Kitaev model with magnetic field

We investigate the non-Abelian topological chiral spin liquid phase in the two-dimensional (2D) Kitaev honeycomb model subject to a magnetic field. By combining density matrix renormalization group (DMRG) and exact diagonalization (ED) we study the energy spectra, entanglement, topological degeneracy, and expectation values of Wilson loop operators, allowing for robust characterization. While the ferromagnetic (FM) Kitaev spin liquid is already destroyed by a weak magnetic field with Zeeman energy $H_*^\text{FM} \approx 0.02$, the antiferromagnetic (AFM) spin liquid remains robust up to a magnetic field that is an order of magnitude larger, $H_*^\text{AFM} \approx 0.2$. Interestingly, for larger fields $H_*^\text{AFM} < H < H_{**}^\text{AFM}$, an intermediate gapless phase is observed, before a second transition to the high-field partially-polarized paramagnet. We attribute this rich phase diagram, and the remarkable stability of the chiral topological phase in the AFM Kitaev model, to the interplay of strong spin-orbit coupling and frustration enhanced by the magnetic field. Our findings suggest relevance to recent experiments on RuCl$_3$ under magnetic fields.

cond-mat.str-el↗

arXiv2018

Valence Bonds in Random Quantum Magnets: Theory and Application to YbMgGaO4

We analyze the effect of quenched disorder on spin-1/2 quantum magnets in which magnetic frustration promotes the formation of local singlets. Our results include a theory for 2d valence-bond solids subject to weak bond randomness, as well as extensions to stronger disorder regimes where we make connections with quantum spin liquids. We find, on various lattices, that the destruction of a valence-bond solid phase by weak quenched disorder leads inevitably to the nucleation of topological defects carrying spin-1/2 moments. This renormalizes the lattice into a strongly random spin network with interesting low-energy excitations. Similarly when short-ranged valence bonds would be pinned by stronger disorder, we find that this putative glass is unstable to defects that carry spin-1/2 magnetic moments, and whose residual interactions decide the ultimate low energy fate. Motivated by these results we conjecture Lieb-Schultz-Mattis-like restrictions on ground states for disordered magnets with spin-1/2 per statistical unit cell. These conjectures are supported by an argument for 1d spin chains. We apply insights from this study to the phenomenology of YbMgGaO$_4$, a recently discovered triangular lattice spin-1/2 insulator which was proposed to be a quantum spin liquid. We instead explore a description based on the present theory. Experimental signatures, including unusual specific heat, thermal conductivity, and dynamical structure factor, and their behavior in a magnetic field, are predicted from the theory, and compare favorably with existing measurements on YbMgGaO$_4$ and related materials.

cond-mat.str-el↗

arXiv2017

Mean-field scaling of the superfluid to Mott insulator transition in a 2D optical superlattice

The mean-field treatment of the Bose-Hubbard model predicts properties of lattice-trapped gases to be insensitive to the specific lattice geometry once system energies are scaled by the lattice coordination number $z$. We test this scaling directly by comparing coherence properties of $^{87}$Rb gases that are driven across the superfluid to Mott insulator transition within optical lattices of either the kagome ($z=4$) or the triangular ($z=6$) geometries. The coherent fraction measured for atoms in the kagome lattice is lower than for those in a triangular lattice with the same interaction and tunneling energies. A comparison of measurements from both lattices agrees quantitatively with the scaling prediction. We also study the response of the gas to a change in lattice geometry, and observe the dynamics as a strongly interacting kagome-lattice gas is suddenly "hole-doped" by introducing the additional sites of the triangular lattice.

cond-mat.quant-gas↗

arXiv2017

Physics of the Kitaev model: fractionalization, dynamical correlations, and material connections

Quantum spin liquids have fascinated condensed matter physicists for decades because of their unusual properties such as spin fractionalization and long-range entanglement. Unlike conventional symmetry breaking the topological order underlying quantum spin liquids is hard to detect experimentally. Even theoretical models are scarce for which the ground state is established to be a quantum spin liquid. The Kitaev honeycomb model and its generalizations to other tri-coordinated lattices are chief counterexamples --- they are exactly solvable, harbor a variety of quantum spin liquid phases, and are also relevant for certain transition metal compounds including the polymorphs of (Na,Li)$_2$IrO$_3$ Iridates and RuCl$_3$. In this review, we give an overview of the rich physics of the Kitaev model, including 2D and 3D fractionalization as well as dynamical correlations and behavior at finite temperatures. We discuss the different materials, and argue how the Kitaev model physics can be relevant even though most materials show magnetic ordering at low temperatures.

cond-mat.str-el↗

arXiv2017

Field-induced intertwined orders in 3D Mott-Kitaev honeycomb $β$-Li2IrO3

Honeycomb iridates are thought to have strongly spin-anisotropic exchange interactions that could lead to an extraordinary state of matter known as the Kitaev quantum spin liquid. The realization of this state requires almost perfectly frustrated interactions between the magnetic Ir$^{4+}$ ions, but small imbalances in energy make other ordered states more favorable. Indeed, the closeness in energy of these ordered states is itself a signature of the intrinsic frustration in the system. In this work, we illustrate that small magnetic fields can be employed to drive the frustrated quantum magnet $β-$Li$_2$IrO$_3$,between different broken symmetry states, but without causing a true thermodynamic phase transition. This field-induced broken symmetry phase has all the signatures of a thermodynamic order parameter, but it is never truly formed in zero field. Rather, it is summoned when the scales of frustration are appropriately tipped, intertwined with other nearby quantum states.

cond-mat.str-el↗

arXiv2016

Spin dynamics of counterrotating Kitaev spirals via duality

Incommensurate spiral order is a common occurrence in frustrated magnetic insulators. Typically, all magnetic moments rotate uniformly, through the same wavevector. However the honeycomb iridates family Li2IrO3 shows an incommensurate order where spirals on neighboring sublattices are counter-rotating, giving each moment a different local environment. Theoretically describing its spin dynamics has remained a challenge: the Kitaev interactions proposed to stabilize this state, which arise from strong spin-orbit effects, induce magnon umklapp scattering processes in spin-wave theory. Here we propose an approach via a (Klein) duality transformation into a conventional spiral of a frustrated Heisenberg model, allowing a direct derivation of the dynamical structure factor. We analyze both Kitaev and Dzyaloshinskii-Moriya based models, both of which can stabilize counterrotating spirals, but with different spin dynamics, and we propose experimental tests to identify the origin of counterrotation.

cond-mat.str-el↗

arXiv2016

Composite fermion duality for half-filled multicomponent Landau Levels

We study the interplay of particle-hole symmetry and fermion-vortex duality in multicomponent half-filled Landau levels, such as quantum Hall gallium arsenide bilayers and graphene. For the $ν{=}1/2{+}1/2$ bilayer, we show that particle-hole-symmetric interlayer Cooper pairing of composite fermions leads to precisely the same phase as the electron exciton condensate realized in experiments. This equivalence is easily understood by applying the recent Dirac fermion formulation of $ν{=}1/2$ to two components. It can also be described by Halperin-Lee-Read composite fermions undergoing interlayer $p_x{+}ip_y$ pairing. An RG analysis showing strong instability to interlayer pairing at large separation $d\rightarrow \infty$ demonstrates that two initially-decoupled composite Fermi liquids can be smoothly tuned into the conventional bilayer exciton condensate without encountering a phase transition. We also discuss multicomponent systems relevant to graphene, derive related phases including a $Z_2$ gauge theory with spin-half visons, and argue for symmetry-enforced gaplessness under full SU$(N_f)$ flavor symmetry when the number of components $N_f$ is even.

cond-mat.str-el↗

arXiv2016

Transport evidence for Fermi-arc mediated chirality transfer in the Dirac semimetal Cd$_3$As$_2$

Dirac semi-metals show a linear electronic dispersion in three dimension described by two copies of the Weyl equation, a theoretical description of massless relativistic fermions. At the surface of a crystal, the breakdown of fermion chirality is expected to produce topological surface states without any counterparts in high-energy physics nor conventional condensed matter systems, the so-called "Fermi Arcs". Here we present Shubnikov-de Haas oscillations involving the Fermi Arc states in Focused Ion Beam prepared microstructures of Cd$_3$As$_2$. Their unusual magnetic field periodicity and dependence on sample thickness can be well explained by recent theoretical work predicting novel quantum paths weaving the Fermi Arcs together with chiral bulk states, forming "Weyl orbits". In contrast to conventional cyclotron orbits, these are governed by the chiral bulk dynamics rather than the common momentum transfer due to the Lorentz force. Our observations provide evidence for direct access to the topological properties of charge in a transport experiment, a first step towards their potential application.

cond-mat.mes-hall↗

arXiv2016

Minimal models for topological Weyl semimetals

Topological Weyl semimetals (TWS) can be classified as type-I TWS, in which the density of states vanishes at the Weyl nodes, and type-II TWS where an electron and a hole pocket meet with finite density of states at the nodal energy. The dispersions of type-II Weyl nodes are tilted and break Lorentz invariance, allowing for physical properties distinct from those in a type-I TWS. We present minimal lattice models for both time-reversal-breaking and inversion-breaking type-II Weyl semimetals, and investigate their bulk properties and topological surface states. These lattice models capture the extended Fermi pockets and the connectivities of Fermi arcs. In addition to the Fermi arcs, which are topologically protected, we identify surface "track states" that arise out of the topological Fermi arc states at the transition from type-I to type-II with multiple Weyl nodes, and persist in the type-II TWS.

cond-mat.mes-hall↗

arXiv2015

Topological Crystalline Bose Insulator in Two Dimensions via Entanglement Spectrum

Strongly correlated analogues of topological insulators have been explored in systems with purely on-site symmetries, such as time-reversal or charge conservation. Here, we use recently developed tensor network tools to study a quantum state of interacting bosons which is featureless in the bulk, but distinguished from an atomic insulator in that it exhibits entanglement which is protected by its spatial symmetries. These properties are encoded in a model many-body wavefunction that describes a fully symmetric insulator of bosons on the honeycomb lattice at half filling per site. While the resulting integer unit cell filling allows the state to bypass `no-go' theorems that trigger fractionalization at fractional filling, it nevertheless has nontrivial entanglement, protected by symmetry. We demonstrate this by computing the boundary entanglement spectra, finding a gapless entanglement edge described by a conformal field theory as well as degeneracies protected by the non-trivial action of combined charge-conservation and spatial symmetries on the edge. Here, the tight-binding representation of the space group symmetries plays a particular role in allowing certain entanglement cuts that are not allowed on other lattices of the same symmetry, suggesting that the lattice representation can serve as an additional symmetry ingredient in protecting an interacting topological phase. Our results extend to a related insulating state of electrons, with short-ranged entanglement and no band insulator analogue.

cond-mat.str-el↗