arXiv subjects

Ivan V. Iorsh

Publications and source records attributed to Ivan V. Iorsh.

At least 19 recordsLinked to original sources

arXiv2026

Optical probing of Wigner crystallization in monolayer WSe$_2$ via diffraction of longitudinal excitons

Monolayer transition metal dichalcogenides (TMDs) are characterized by relatively large carrier effective masses and suppressed screening of the Coulomb interaction, which substantially enhances the correlation effects in these structures. The direct band gap allows to effectively optically probe these correlations. Here, we present an experimental observation of Wigner crystallization in monolayer $\mathrm{WSe}_2$ probed by the measurement of the exciton diffraction on the Wigner crystal (WC) periodic potential. We observe the formation of the WC phase in the absence of external magnetic fields at temperature range $T<26~\mathrm{K}$ and carrier concentrations $n$ $<2\times10^{11}~\mathrm{cm}^{-2}$. The direct observation of the exciton diffraction is enabled by the strong exciton longitudinal-transverse splitting induced by the long-range intervalley exchange interaction, leading to the large detuning between main exciton peak and first diffraction peak. Our findings highlight that the valley degree of freedom of charge carriers in TMDs facilitates optical probing of correlated electron phases in these structures.

cond-mat.mes-hall↗

arXiv2025

Nonlinear near-field spectroscopy of exciton-polaritons in a van der Waals layered waveguide

Layered van der Waals materials offer novel opportunities for on-chip waveguiding and development of integrated photonic circuits. In the strong light-matter coupling regime, their nonlinear response can be significantly enhanced, which is crucial for developing active photonic devices. However, probing the nonlinearity of waveguide modes in subwavelength-thick structures is challenging as they are not directly accessible from far-field. Here we apply a novel nonlinear near-field spectroscopic technique based on a GaP solid immersion lens and femtosecond laser excitation to study nonlinearity of guided modes in monolayer WS$_2$ encapsulated in hBN under the strong light-matter coupling regime. We reveal formation of exciton-polaritons with $\sim 50$ meV Rabi splitting and demonstrate a pump-induced transition from strong to weak coupling. Our results show that exciton resonance saturation and broadening lead to an efficient nonlinear response of guided polaritons, which can be employed for developing compact van der Waals photonic switches and modulators.

physics.optics↗

arXiv2024

Electrostatic control of nonlinear photonic-crystal polaritons in a monolayer semiconductor

Integration of 2D semiconductors with photonic crystal slabs provides an attractive approach to achieve strong light--matter coupling and exciton-polariton formation in a planar chip-compatible geometry. However, for the development of practical devices, it is crucial that the polariton excitations in the structure are easily tunable and exhibit strong nonlinear response. Here we study neutral and charged exciton-polaritons in an electrostatically gated planar photonic crystal slab with an embedded monolayer semiconductor MoSe$_2$ and experimentally demonstrate strong polariton nonlinearity, which can be tuned via gate voltage. We find that modulation of dielectric environment within the photonic crystal results in the formation of two distinct resonances with significantly different nonlinear response, which enables optical switching with ultrashort laser pulses. Our results open new avenues towards development of active polaritonic devices in a compact chip-compatible implementation.

cond-mat.mes-hall↗

arXiv2023

Probing and control of guided exciton-polaritons in a 2D semiconductor-integrated slab waveguide

Guided 2D exciton-polaritons, resulting from the strong coupling of excitons in semiconductors with non-radiating waveguide modes, provide an attractive approach towards developing novel on-chip optical devices. These quasiparticles are characterized by long propagation distances and efficient nonlinear interaction but cannot be directly accessed from the free space. Here we demonstrate a powerful approach for probing and manipulating guided polaritons in a Ta2O5 slab integrated with a WS2 monolayer using evanescent coupling through a high-index solid immersion lens. Tuning the nanoscale lens-sample gap allows for extracting all the intrinsic parameters of the system. We also demonstrate the transition from weak to strong coupling accompanied by the onset of the motional narrowing effect: with the increase of exciton-photon coupling strength, the inhomogeneous contribution to polariton linewidth, inherited from the exciton resonance, becomes fully lifted. Our results enable the development of integrated optics employing room-temperature exciton-polaritons in 2D semiconductor-based structures.

physics.optics↗

arXiv2023

Cavity-induced charge transfer in periodic systems: length-gauge formalism

We develop a length-gauge formalism for treating one-dimensional periodic lattice systems in the presence of a photon cavity inducing light-matter interaction. The purpose of the formalism is to remove mathematical ambiguities that occur when defining the position operator in the context of the Power-Zienau-Woolley Hamiltonian. We then use a diagrammatic approach to analyze perturbatively the interaction between an electronic quantum system and a photonic cavity mode of long wavelength. We illustrate the versatility of the formalism by studying the cavity-induced electric charge imbalance and polarization in the Rice-Mele model with broken inversion symmetry.

cond-mat.mes-hall↗

arXiv2023

Frequency combs with parity-protected cross-correlations from dynamically modulated qubit arrays

We develop a general theoretical framework to dynamically engineer quantum correlations in the frequency-comb emission from an array of superconducting qubits in a waveguide, rigorously accounting for the temporal modulation of the qubit resonance frequencies. We demonstrate, that when the resonance frequencies of the two qubits are periodically modulated with a $π$ phase shift, it is possible to realize simultaneous bunching and antibunching in cross-correlations of the scattered photons from different sidebands. Our approach, based on the dynamical conversion between the quantum excitations with different parity symmetry, is quite universal. It can be used to control two-particle correlations in generic dynamically modulated dissipative quantum systems.

quant-ph↗

arXiv2023

Photoluminescence imaging of single photon emitters within nanoscale strain profiles in monolayer WSe$_2$

Local deformation of atomically thin van der Waals materials provides a powerful approach to create site-controlled chip-compatible single-photon emitters (SPEs). However, the microscopic mechanisms underlying the formation of such strain-induced SPEs are still not fully clear, which hinders further efforts in their deterministic integration with nanophotonic structures for developing practical on-chip sources of quantum light. Here we investigate SPEs with single-photon purity up to 98% created in monolayer WSe$_2$ via nanoindentation. Using photoluminescence imaging in combination with atomic force microscopy, we locate single-photon emitting sites on a deep sub-wavelength spatial scale and reconstruct the details of the surrounding local strain potential. The obtained results suggest that the origin of the observed single-photon emission is likely related to strain-induced spectral shift of dark excitonic states and their hybridization with localized states of individual defects.

cond-mat.mes-hall↗

arXiv2022

Interacting exciton-polaritons in cylindric micropillars

We present a quantitative microscopic analysis of the formation of exciton-polaritons, the composite particles possessing light and material components, polariton-polariton interactions, and resonant pumping dynamics in cylindrical semiconductor micropillars. We discuss how the redistribution effect can be used in devices generating photons with non zero orbital angular momenta.

cond-mat.mes-hall↗

arXiv2022

Waveguide quantum electrodynamics: collective radiance and photon-photon correlations

This review describes the emerging field of waveguide quantum electrodynamics (WQED) concerned with the interaction of photons propagating in a waveguide with localized quantum emitters. The collective emitter-photon interactions can lead to both enhanced and suppressed coupling compared to the case of independent emitters. Here, we focus on guided photons and ordered arrays, leading to super- and sub-radiant states, bound photon states and quantum correlations with promising quantum information applications. We highlight recent groundbreaking experiments performed with different quantum platforms, including cold atoms, superconducting qubits, semiconductor quantum dots, quantum solid-state defects, and we provide a comprehensive introduction to theoretical techniques to study the interactions and dynamics of these emitters and the photons in the waveguide.

quant-ph↗

arXiv2021

Generating ${\rm N00N}$-states of surface plasmon-polariton pairs with a nanoparticle

We consider a generation of two-particle quantum states in the process of spontaneous parametric down-conversion of light by a dielectric nanoparticle with $χ^{(2)}$ response. As a particular example, we study the generation of surface plasmon-polariton pairs with a ${\rm GaAs}$ nanoparticle located at the silver-air interface. We show that for certain excitation geometries, ${\rm N00N}$-states of surface plasmon-polariton pairs could be obtained. The effect can be physically interpreted as a result of quantum interference between pairs of induced sources, each emitting either signal or idler plasmon. We then relate the resulting ${\rm N00N}$-pattern to the general symmetry properties of dyadic Green's function of a dipole emitter exciting surface waves. It renders the considered effect as a general way towards a robust generation of ${\rm N00N}$-states of surface waves using spontaneous parametric down-conversion in $χ^{(2)}$ nanoparticles.

physics.optics↗

arXiv2019

Optical valleytronics in gapped graphene

We propose a scheme to trap and filter electrons, valley dependently, on a scale beyond the diffraction limit, in a gapped Dirac system using a circularly polarized light beam and a microscale metallic resonator. The main mechanism allowing the selection is the valley dependent break of the time reversal symmetry. Indeed in one valley, the light partially closes the already existing gap while it opens it in the other one. This difference in the band structure close to the Dirac points, induces a change in the dynamics of the electrons, leading to a valley router behaviour of the system.

cond-mat.mes-hall↗

arXiv2018

Experimental observation of hybrid TE-TM polarized surface waves supported by hyperbolic metasurface

Hyperbolic metasurfaces have gained significant attention due to their extraordinary electromagnetic properties to control propagating plane waves, but the excitation and propagation of the surface plasmon-polaritons at hyperbolic metasurfaces, called hyperbolic plasmons, have been experimentally observed just recently. However, the advantages of the hyperbolic plasmons, such as hybrid TE-TM polarization discussed below, are not yet fully revealed and analyzed. In this paper we focus on the numerical and experimental characterization of surface waves in the frequency range from 2 to 8 GHz supported by a hyperbolic metasurface composed of anisotropic metallic Jerusalem crosses printed on a thin dielectric substrate. We show different shapes of equal frequency contours, which correspond to a plethora of excitation and propagation regimes of surface waves. The principal novelty of this work consists in the experimental demonstration of the surface waves with a hybrid, i.e. mixed TE-TM, polarization. Surface waves with a hybrid polarization are the promising tool in a number of applications and phenomena including polarization converters, plasmonic sensors, plasmon steering over a surface, optical forces, spin-orbit photonics, and highlight the impact for the on-chip and planar networks.

physics.app-ph↗

arXiv2017

Effective surface conductivity of plasmonic metasurfaces: from far-field characterization to surface wave analysis

Metasurfaces offer great potential to control near- and far-fields through engineering of optical properties of elementary cells or meta-atoms. Such perspective opens a route to efficient manipulation of the optical signals both at nanoscale and in photonics applications. In this paper we show that by using an effective surface conductivity tensor it is possible to unambigiously describe optical properties of an anisotropic metasurface in the far- and near-field regimes. We begin with retrieving the effective surface conductivity tensor from the comparative analysis of experimental and numerical reflectance spectra of a metasurface composed of elliptical gold nanoparticles. Afterwards restored conductivities are validated in the crosscheck versus semianalytic parameters obtained with the discrete dipole model with and without dipoles interaction contribution. The obtained effective parameters are further used for the dispersion analysis of surface plasmons localized at the metasurface. The effective medium model predicts existence of both TE- and TM-polarized plasmons in a wide range of optical frequencies and describes peculiarities of their dispersion, in particularly, topological transition from the elliptical to hyperbolic regime with eligible accuracy. The analysis in question offers a simple practical way to describe properties of metasurfaces including ones in the near-field zone by extracting effective parameters from the convenient far-field characterisation.

physics.optics↗

arXiv2017

Optical trapping of electrons in graphene

We propose an experimentally friendly scheme for trapping quasi- relativistic elec- trons in graphene by an electromagnetic beam with circular polarization and spatially inhomogeneous profile with an intensity dip. The trapping is achieved due to the ef- fect of bandgap opening outside the trapping region. The proposed mechanism allows for non- invasive electron confinement in graphene without any need of the chemical patterning of the sample or the application of metallic gates.

cond-mat.mes-hall↗

arXiv2017

Dielectric nanoantenna as an efficient and ultracompact demultiplexer for surface waves

Nanoantennas for highly efficient excitation and manipulation of surface waves at nanoscale are key elements of compact photonic circuits. However, previously implemented designs employ plasmonic nanoantennas with high Ohmic losses, relatively low spectral resolution, and complicated lithographically made architectures. Here we propose an ultracompact and simple dielectric nanoantenna (silicon nanosphere) allowing for both directional launching of surface plasmon polaritons on a thin gold film and their demultiplexing with a high spectral resolution. We show experimentally that mutual interference of magnetic and electric dipole moments supported by the dielectric nanoantenna results in opposite propagation of the excited surface waves whose wavelengths differ by less than 50 nm in the optical range. Broadband reconfigurability of the nanoantennas operational range is achieved simply by varying the diameter of the silicon sphere. Moreover, despite subwavelength size ($<λ/3$) of the proposed nanoantennas, they demonstrate highly efficient and directional launching of surface waves both in the forward and backward directions with the measured front-to-back ratio having a contrast of almost two orders of magnitude within a 50 nm spectral band. Our lithography-free design has great potential as highly efficient, low-cost, and ultracompact demultiplexer for advanced photonic circuits.

physics.optics↗

arXiv2017

Two-dimensional optical plasmons with mixed polarization on anisotropic resonant metasurface

Optical metasurfaces have great potential to form the platform for manipulation of surface waves. A plethora of advanced surface-wave phenomena utilizing negative refraction, self-collimation and channeling of 2D waves can be realized through on-demand engineering of dispersion properties of a periodic metasurface. In this letter, we report on the first-time direct experimental polarization-resolved measurement of dispersion of 2D optical plasmons supported by an anisotropic metasurface. We demonstrate that a subdiffractive array of strongly coupled resonant anisotropic plasmonic nanoparticles supports unusual optical surface waves with mixed TE- and TM-like polarizations. With the assistance of numerical simulations we identify dipole and quadrupole dispersion bands. The shape of isofrequency contours changes drastically with frequency exhibiting nontrivial transformations of their curvature and topology that is consistently confirmed by the experimental data. By revealing polarization degree of freedom for surface waves, our results open new routes for designing of planar on-chip devices for surface photonics.

physics.optics↗

arXiv2017

Exploring nonlinear topological states of matter with exciton-polaritons: Edge solitons in kagome lattice

Matter in nontrivial topological phase possesses unique properties, such as support of unidirectional edge modes on its interface. It is the existence of such modes which is responsible for the wonderful properties of a topological insulator -- material which is insulating in the bulk but conducting on its surface, along with many of its recently proposed photonic and polaritonic analogues. We show that exciton-polariton fluid in a nontrivial topological phase in kagome lattice, supports nonlinear excitations in the form of solitons built up from wavepackets of topological edge modes -- topological edge solitons. Our theoretical and numerical results indicate the appearance of bright, dark and grey solitons dwelling in the vicinity of the boundary of a lattice strip. In a parabolic region of the dispersion the solitons can be described by envelope functions satisfying the nonlinear Schrödinger equation. Upon collision, multiple topological edge solitons emerge undistorted, which proves them to be true solitons as opposed to solitary waves for which such requirement is waived. Importantly, kagome lattice supports topological edge mode with zero group velocity unlike other types of truncated lattices. This gives a finer control over soliton velocity which can take both positive and negative values depending on the choice of forming it topological edge modes.

cond-mat.mes-hall↗

arXiv2016

Spin control of light with hyperbolic metasurfaces

Transverse spin angular momentum is an inherent feature of evanescent waves which may have applications in nanoscale optomechanics, spintronics, and quantum information technology due to the robust spin-directional coupling. Here we analyze a local spin angular momentum density of hybrid surface waves propagating along anisotropic hyperbolic metasurfaces. We reveal that, in contrast to bulk plane waves and conventional surface plasmons at isotropic interfaces, the spin of the hybrid surface waves can be engineered to have an arbitrary angle with the propagation direction. This property allows to tailor directivity of surface waves via the magnetic control of the spin projection of quantum emitters, and it can be useful for optically controlled spin transfer.

physics.optics↗