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Izak Snyman

Publications and source records attributed to Izak Snyman.

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The covariance matrix spectrum of correlated charge insulators reveals hidden connections to Coupled Cluster, Matrix Product, and Rokhsar-Kivelson states

Charge ordering induced by strong short-range repulsion in itinerant fermion systems typically follows a two-sites alternation pattern. However, the covariance matrix spectrum of the one-dimensional, half-filled, spinless $t$-$V$ model reveals a post-Hartree-Fock picture at strong repulsion, with emergent four-site disruptions of the underlying staggered mean-field state. These disruptions are captured in a thermodynamically extensive manner by a compact four-fermion Coupled Cluster (doubles) state (CCS). Remarkably, all properties of this state may be computed analytically by combinatorial means, and also derived from an exactly solvable correlated hopping Hamiltonian. Furthermore, this Coupled Cluster state can be re-expressed as a low-rank Matrix Product State (MPS) with bond dimension exactly four. In addition, we unveil a hidden connection between this Coupled Cluster ansatz and a Rokhsar-Kivelson state (RKS), which is the ground state of a solvable parent quantum tetramer model. The broad picture that we uncover here thus provides deep connections between several core concepts of correlated fermions and quantum chemistry that have previously enjoyed limited synergy. In contrast to a recent perturbative treatment on top of Hartree-Fock theory, our approach asymptotically captures the correct correlations in the $t$-$V$ model at small $t/V$, and remains a qualitatively accurate approximation even outside the perturbative regime. Our results make the case for further studies of the covariance matrix for correlated electron systems in which ground states have non-trivial unit-cell structure.

cond-mat.str-el

Direct detection of down-converted photons spontaneously produced at a single Josephson junction

We study spontaneous photon decay into multiple photons triggered by strong non-linearities in a superconducting quantum simulator of the boundary sine-Gordon impurity model. Previously, spectroscopic signatures of photon-conversion were reported and evidenced as resonances in the many-body spectrum of these systems. Here, we report on the observation of multi-mode fluorescence of a small Josephson junction embedded in a high impedance superconducting transmission line. Measurement of the down-converted photons is achieved using state-of-the-art broadband parametric amplifiers. Photon triplet emission is explicitly demonstrated at a given frequency as the counterpart of inelastic photon decay at three-times the emission frequency. These results open exciting prospects for the burgeoning field of many-body quantum optics and offer a direct signature of the ultra-strong light-matter coupling.

cond-mat.mes-hall

Comment on "Absence versus Presence of Dissipative Quantum Phase Transition in Josephson Junctions''

In a recent Letter [Phys. Rev. Lett. 129, 087001, (2022)], Masuki, Sudo, Oshikawa, and Ashida studied a Josephson junction, with Josephson energy $E_{\rm J}$ and charging energy $E_{\rm C}$, shunted by an ohmic transmission line with conductance $α(2e)^2/h$. Their model includes a realistic high frequency cutoff of order $αE_c$, that is typically smaller than the plasma frequency $W$. The authors present a phase diagram showing surprising features, not anticipated in the established literature [eg. Schön and Zaikin, Phys. Reports 198, 237, (1990)]. For $E_{\rm J}/E_{\rm C}$ above a certain value, they find that the junction remains superconducting for all $α$, while below this value, they find that the insulating phase leads to re-entrant superconductivity at small $α$. In this Comment, we show that their Numerical Renormalization Group (NRG) implementation is uncontrolled, and that there is no evidence for the re-entrant superconductivity in the phase diagram presented in Fig. 1a of PRL 129, 087001.

cond-mat.supr-con

Revealing the finite-frequency response of a bosonic quantum impurity

Quantum impurities are ubiquitous in condensed matter physics and constitute the most stripped-down realization of many-body problems. While measuring their finite-frequency response could give access to key characteristics such as excitations spectra or dynamical properties, this goal has remained elusive despite over two decades of studies in nanoelectronic quantum dots. Conflicting experimental constraints of very strong coupling and large measurement bandwidths must be met simultaneously. We get around this problem using cQED tools, and build a precisely characterized quantum simulator of the boundary sine-Gordon model, a non-trivial bosonic impurity problem. We succeeded to fully map out the finite frequency linear response of this system. Its reactive part evidences a strong renormalisation of the nonlinearity at the boundary in agreement with non-perturbative calculations. Its dissipative part reveals a dramatic many-body broadening caused by multi-photon conversion. The experimental results are matched quantitatively to a resummed diagrammatic calculation based on a microscopically calibrated model. Furthermore, we push the device into a regime where diagrammatic calculations break down, which calls for more advanced theoretical tools to model many-body quantum circuits. We also critically examine the technological limitations of cQED platforms to reach universal scaling laws. This work opens exciting perspectives for the future such as quantifying quantum entanglement in the vicinity of a quantum critical point or accessing the dynamical properties of non-trivial many-body problems.

quant-ph

Simulating realistic screening clouds around quantum impurities: role of spatial anisotropy and disorder

Dynamical quantum impurities in metals induce electronic correlations in real space that are difficult to simulate due to their multi-scale nature, so that only s-wave scattering in clean metallic hosts has been investigated so far. However, screening clouds should show anisotropy due to lack of full rotational invariance in two- and three-dimensional lattices, while inherent disorder will also induce spatial inhomogeneities. To tackle these challenges, we present an efficient and robust algorithm based on the recursive generation of natural orbitals defined as eigenvectors of the truncated single-particle density matrix. This method provides well-converged many-body wave functions on lattices with up to tens of thousands of sites, bypassing some limitations of other approaches. The algorithm is put to the test by investigating the charge screening cloud around an interacting resonant level, both on clean and disordered lattices, achieving accurate spatial resolution from short to long distances. We thus demonstrate strong anisotropy of spatial correlations around an adatom in the half-filled square lattice. Taking advantage of the efficiency of the algorithm, we further compute the disorder-induced distribution of Kondo temperatures over several thousands of random realizations, at the same time gaining access to the full spatial profile of the screening cloud in each sample. While the charge screening cloud is typically shortened due to the polarization of the impurity by the disorder potential, we surprisingly find that rare disorder configurations preserve the long range nature of Kondo correlations in the electronic bath.

cond-mat.str-el

Spin-boson quantum phase transition in multilevel superconducting qubits

Superconducting circuits are currently developed as a versatile platform for the exploration of many-body physics, by building on non-linear elements that are often idealized as two-level qubits. A classic example is given by a charge qubit that is capacitively coupled to a transmission line, which leads to the celebrated spin-boson description of quantum dissipation. We show that the intrinsic multilevel structure of superconducting qubits drastically restricts the validity of the spin-boson paradigm due to phase localization, which spreads the wavefunction over many charge states. Numerical Renormalization Group simulations also show that the quantum critical point moves out of the physically accessible range in the multilevel regime. Imposing charge discreteness in a simple variational state accounts for these multilevel effects, that are relevant for a large class of devices.

cond-mat.mes-hall

Efficient impurity-bath trial states from superposed Slater determinants

The representation of ground states of fermionic quantum impurity problems as superpositions of Gaussian states has recently been given a rigorous mathematical foundation. [S. Bravyi and D. Gosset, Comm. Math. Phys. 356, 451 (2017)]. It is natural to ask how many parameters are required for an efficient variational scheme based on this representation. An upper bound is $\mathcal O(N^2)$, where $N$ is the system size, which corresponds to the number parameters needed to specify an arbitrary Gaussian state. We provide an alternative representation, with more favorable scaling, only requiring $\mathcal O(N)$ parameters, that we illustrate for the interacting resonant level model. We achieve the reduction by associating mean-field-like parent Hamiltonians with the individual terms in the superposition, using physical insight to retain only the most relevant channels in each parent Hamiltonian. We benchmark our variational ansatz against the Numerical Renormalization Group, and compare our results to existing variational schemes of a similar nature to ours. Apart from the ground state energy, we also study the spectrum of the correlation matrix -- a very stringent measure of accuracy. Our approach outperforms some existing schemes and remains quantitatively accurate in the numerically challenging near-critical regime.

cond-mat.str-el

Few-body nature of Kondo correlated ground states

The quenching of degenerate impurity states in metals generally induces a long-range correlated quantum state known as the Kondo screening cloud. While a macroscopic number of particles clearly take part in forming this extended structure, assessing the number of truly entangled degrees of freedom requires a careful analysis of the relevant many-body wavefunction. For this purpose, we examine the natural single-particle orbitals that are eigenstates of the single-particle density (correlation) matrix for the ground state of two quantum impurity problems: the interacting resonant level model (IRLM) and the single impurity Anderson model (SIAM). As a simple and general probe for few-body versus many-body character we consider the rate of exponential decay of the correlation matrix eigenvalues towards inactive (fully empty or filled) orbitals. We find that this rate remains large in the physically most relevant region of parameter space, implying a few-body character. Genuine many-body correlations emerge only when the Kondo temperature becomes exponentially small, for instance near a quantum critical point. In addition, we demonstrate that a simple numerical diagonalization of the few-body problem restricted to the Fock space of the most correlated orbitals converges exponentially fast with respect to the number of orbitals, to the true ground state of the IRLM. We also show that finite size effects drastically affect the correlation spectrum, shedding light on an apparent paradox arising from previous studies on short chains.

cond-mat.str-el

Zero-energy quasiparticles in an interacting nanowire containing a topological Josephson junction

We study a Josephson junction in a Kitaev chain with particle-hole symmetric nearest neighbor interactions. When the phase difference across the junction is $π$, we show analytically that the full spectrum is fourfold degenerate up to corrections that vanish exponentially in the system size. The Majorana bound states at the ends of the chain are known to survive interactions. Our result proves that the same is true for the zero-energy quasiparticle localized at the junction. We further study finite size corrections numerically, and show how repulsive interactions lead to stronger end-to-end correlations than in a noninteracting system with the same bulk gap.

cond-mat.mes-hall

Observation of quantum many-body effects due to zero point fluctuations in superconducting circuits

Electromagnetic fields possess zero point fluctuations (ZPF) which lead to observable effects such as the Lamb shift and the Casimir effect. In the traditional quantum optics domain, these corrections remain perturbative due to the smallness of the fine structure constant. To provide a direct observation of non-perturbative effects driven by ZPF in an open quantum system we wire a highly non-linear Josephson junction to a high impedance transmission line, allowing large phase fluctuations across the junction. Consequently, the resonance of the former acquires a relative frequency shift that is orders of magnitude larger than for natural atoms. Detailed modelling confirms that this renormalization is non-linear and quantum. Remarkably, the junction transfers its non-linearity to about 30 environmental modes, a striking back-action effect that transcends the standard Caldeira-Leggett paradigm. This work opens many exciting prospects for longstanding quests such as the tailoring of many-body Hamiltonians in the strongly non-linear regime, the observation of Bloch oscillations, or the development of high-impedance qubits.

cond-mat.mes-hall

A tunable Josephson platform to explore many-body quantum optics in circuit-QED

Coupling an isolated emitter to a single mode of the electromagnetic field is now routinely achieved and well understood. Current efforts aim to explore the coherent dynamics of emitters coupled to several electromagnetic modes (EM). freedom. Recently, ultrastrong coupling to a transmission line has been achieved where the emitter resonance broadens to a significant fraction of its frequency. In this work we gain significantly improved control over this regime. We do so by combining the simplicity of a transmon qubit and a bespoke EM environment with a high density of discrete modes, hosted inside a superconducting metamaterial. This produces a unique device in which the hybridisation between the qubit and up to 10 environmental modes can be monitored directly. Moreover the frequency and broadening of the qubit resonance can be tuned independently of each other in situ. We experimentally demonstrate that our device combines this tunability with ultrastrong coupling and a qubit nonlinearity comparable to the other relevant energy scales in the system. We also develop a quantitative theoretical description that does not contain any phenomenological parameters and that accurately takes into account vacuum fluctuations of our large scale quantum circuit in the regime of ultrastrong coupling and intermediate non-linearity. The demonstration of this new platform combined with a quantitative modelling brings closer the prospect of experimentally studying many-body effects in quantum optics. A limitation of the current device is the intermediate nonlinearity of the qubit. Pushing it further will induce fully developed many-body effects, such as a giant Lamb shift or nonclassical states of multimode optical fields. Observing such effects would establish interesting links between quantum optics and the physics of quantum impurities.

cond-mat.mes-hall

Microscopic bosonization of band structures: X-ray processes beyond the Fermi edge

Bosonization provides a powerful analytical framework to deal with one-dimensional strongly interacting fermion systems, which makes it a cornerstone in quantum many-body theory. Yet, this success comes at the expense of using effective infrared parameters, and restricting the description to low energy states near the Fermi level. We propose a radical extension of the bosonization technique that overcomes both limitations, allowing computations with microscopic lattice Hamiltonians, from the Fermi level down to the bottom of the band. The formalism rests on the simple idea of representing the fermion kinetic term in the energy domain, after which it can be expressed in terms of free bosonic degrees of freedom. As a result, one- and two-body fermionic scattering processes generate anharmonic boson-boson interactions, even in the forward channel. We show that up to moderate interaction strengths, these nonlinearities can be treated analytically at all energy scales, using the x-ray emission problem as a showcase. In the strong interaction regime, we employ a systematic variational solution of the bosonic theory, and obtain results that agree quantitatively with an exact diagonalization of the original one-particle fermionic model. This provides a proof of the fully microscopic character of bosonization on all energy scales for an arbitrary band structure. Besides recovering the known x-ray edge singularity at the emission threshold, we find strong signatures of correlations even at emission frequencies beyond the band bottom.

cond-mat.str-el

Universal spatial correlations in the anisotropic Kondo screening cloud: analytical insights and numerically exact results from a coherent state expansion

We analyze the spatial correlations in the spin density of an electron gas in the vicinity of a Kondo impurity. Our analysis extends to the spin-anisotropic regime, which was not investigated in the literature. We use an original and numerically exact method, based on a systematic coherent-state expansion of the ground state of the underlying spin-boson Hamiltonian, which we apply to the computation of observables that are specific to the fermionic Kondo model. We also present an important technical improvement to the method, that obviates the need to discretize modes of the Fermi sea, and allows one to tackle the problem in the thermodynamic limit. One can thus obtain excellent spatial resolution over arbitrary length scales, for a relatively low computational cost, a feature that gives the method an advantage over popular techniques such as NRG and DMRG. We find that the anisotropic Kondo model shows rich universal scaling behavior in the spatial structure of the entanglement cloud. First, SU(2) spin-symmetry is dynamically restored in a finite domain in parameter space in vicinity of the isotropic line, as expected from poor man's scaling. We are also able to obtain in closed analytical form a set of different, yet universal, scaling curves for strong exchange asymmetry, which are parametrized by the longitudinal exchange coupling. Deep inside the cloud, i.e. for distances smaller than the Kondo length, the correlation between the electron spin density and the impurity spin oscillates between ferromagnetic and antiferromagnetic values at the scale of the Fermi wavelength, an effect that is drastically enhanced at strongly anisotropic couplings. Our results also provide further numerical checks and alternative analytical approximations for the recently computed Kondo overlaps [PRL 114, 080601 (2015)].

cond-mat.str-el

Josephson-Kondo screening cloud in circuit quantum electrodynamics

We show that the non-local polarization response in a multimode circuit-QED setup, devised from a Cooper pair box coupled to a long chain of Josephson junctions, provides an alternative route to access the elusive Kondo screening cloud. For moderate circuit impedance, we compute analytically the universal lineshape for the decay of the charge susceptibility along the circuit, that relates to spatial entanglement between the qubit and its electromagnetic environment. At large circuit impedance, we numerically find further spatial correlations that are specific to a true many-body state.

cond-mat.mes-hall