Searcharxiv⌕ Search

arXiv subjects

Jérôme Faist

Publications and source records attributed to Jérôme Faist.

At least 19 recordsLinked to original sources

Dynamically reconfigurable THz quantum walk comb laser through subharmonic excitation

On-chip frequency combs are increasingly relevant to both laser science and applications. Broad bandwidths and flat-top spectral envelopes are especially desirable for precision spectroscopy and dense wavelength-division multiplexed communications. Toward these goals, active microwave modulation has emerged as a powerful strategy for generating, stabilizing, and reconfiguring frequency combs at the source. However, practical challenges associated with high-frequency modulation imposes an upper bound on the accessible cavity free spectral ranges. Here, we demonstrate a subharmonic locking scheme in a quantum walk comb laser, a recently introduced platform for broadband and highly controllable comb states. Using a THz ring quantum cascade laser, we realize quantum walk comb formation under strong microwave injection at successive subharmonics of the cavity round-trip frequency, tuning the comb spacing from 15.8 to 1.58 GHz. The resulting states arise from fast-gain dynamics and nonlinear microwave mixing in the laser cavity. Through two-tone injection, we exploit this mixing to dynamically control the comb bandwidth and spectral shape. These results establish subharmonic excitation as a route to broadband, reconfigurable semiconductor comb generation in high-FSR cavities.

physics.optics↗

Amplitude- and frequency-modulated combs from an actively locked metasurface external-cavity laser

Optical frequency combs are key components of several photonics applications including spectroscopy, communications, and ultrafast photonics. A central challenge in frequency-comb photonics is to develop sources whose operating state can be precisely controlled and adapted to different application needs. We introduce frequency comb functionality to a THz metasurface vertical-external-cavity-surface-emitting laser (VECSEL), combining its characteristic high output power and excellent beam quality with a reconfigurable comb output. The source exhibits reversible switching between actively mode-locked 3.5 ps-long pulses and stable frequency-modulated quantum walk comb states. The flexible control of the intermodal phase relation is achieved through careful dispersion engineering via a Gires-Tournois interferometer (GTI) output-coupler combined with resonant RF bias modulation of the metasurface. These results pave the way for on-demand comb control in the THz range and provide a versatile strategy that could be extended to other semiconductor frequency-comb platforms and wavelength ranges.

physics.optics↗

Absence of a Superradiant Phase Transition in Dirac Landau Polaritons

One of the most striking predictions in cavity quantum electrodynamics is the condensation of photons into a macroscopically populated ground state, the so-called superradiant phase transition (SRPT). SRPTs are theorized to occur in light-matter coupled systems above a critical coupling strength, yet have not been experimentally realized in equilibrium. On the contrary, the very existence of SRPTs has been largely disputed by No-Go theorems. In cavity-coupled electronic systems with Dirac dispersion, the diamagnetic $\vec{A}^2$-term crucial to No-go theorems is not present at leading order, making graphene Landau level transitions ultrastrongly coupled to terahertz cavities good candidates for SRPTs. In this work, we present the first terahertz spectroscopic measurements of an hBN-encapsulated monolayer graphene flake coupled to a highly sub-wavelength resonator mode. By tuning the graphene carrier density, we drive the resulting Landau polaritons into the ultrastrong coupling regime, with the normalized coupling reaching $\approx 40 \%$, approaching criticality. In this regime, the continuous SRPT would lead to a unique spectroscopic polariton softening, which we consistently rule out. The full polariton dispersion is instead quantitatively reproduced by a Hopfield Hamiltonian using a quasistatic near-field model that accounts for the sub-wavelength character of the cavity.

cond-mat.mes-hall↗

Free-Running Ring Quantum Cascade Laser with 50 kHz Linewidth

We report on the noise characterization of a free-running ring quantum cascade laser resonator emitting a single frequency mode around 7.7 $μ$m. Using a gas cell filled with N$_2$O as a frequency-to-voltage discriminator, we measured the frequency noise power spectral density of the laser from which we extracted its linewidth. The results show a full width at half maximum close to 50 kHz at 1 s integration time, which represents at least a sixfold improvement compared to state-of-the-art quantum cascade lasers operating in a spectral region above 7 $μ$m. We also demonstrate that such lasers can be efficiently used for frequency modulation spectroscopy, which opens up new possibilities for high resolution metrology and spectroscopic applications in the mid-infrared.

physics.optics↗

Ultrabroadband Gain-Switched and Superluminescent Terahertz Semiconductor Lasers

Terahertz quantum cascade lasers (THz QCLs) are chip-scale semiconductor lasers operating in the frequency range between 1-6 THz, useful as compact sources for spectroscopy, communications, and non-destructive imaging and testing. Here, we apply low-frequency microwave modulation on a planarized THz QCL to generate ultrabroadband emission in the THz range. For very low modulation frequencies below 1 GHz, a gain-switched octave-spanning spectrum with a smooth spectral envelope is generated between 1.9 - 4.1 THz. Increasing the modulation frequency broadens the lasing modes until a low-coherence, continuous emission spectrum is achieved in the superluminescent regime, covering the spectral region between around 3 - 4 THz, without any discrete lasing modes or spectral gaps. We complement the experimental results with extensive analytical models and numerical simulations that capture the intracavity laser dynamics and fully explain the different operation regimes. These devices could prove useful for absorption spectroscopy without any spectral gaps, and as ultrabroadband sources of THz radiation.

physics.optics↗

Spectral shaping of fast-gain frequency combs through phases in synthetic dimensions

Optical frequency comb devices have unlocked new capabilities in telecommunications, sensing, and metrology. Yet, precise in situ control of the comb spectral envelope remains extremely challenging. By introducing mode coupling with non-trivial phases, we demonstrate a spectral shaping technique that enables continuous tuning of a dominant spectral lobe across the full bandwidth of a semiconductor laser frequency comb. We achieve this jointly leveraging the engineered geometry of the synthetic lattice formed by the cavity modes of the laser and the coherent dynamics enabled by its fast-gain recovery. We use dual-tone modulation of the cavity at its repetition rate and twice this frequency with a controlled relative phase to couple the comb modes into a triangular lattice. The relative phase between the two tones defines a lattice phase that breaks time-reversal symmetry and steers the lattice dynamics through the fast gain. With this approach, we experimentally control the spectral envelope of the comb such that a targeted region contains more than twice the intensity expected from a uniform distribution, demonstrating tunable spectral selectivity. This capability, achieved directly at the light generation stage in a fast-gain device, opens routes for efficient programmable waveform engineering with potential applications in ranging, data transmission, and sensing.

physics.optics↗

Cavity modification of magnetoplasmon mode through coupling with intersubband polaritons

We investigate the coupling of a multi-mode metal-insulator-metal cavity to a two-dimensional electron gas (2DEG) in a quantum well in the presence of a strong magnetic field. The TM cavity mode is strongly hybridized with an intersubband transition of the 2DEG, forming a polaritonic mode in the ultrastrong coupling regime, while the TE mode remains an almost purely cavity mode. The magnetoplasmon excitation emerging from the presence of the magnetic field couples with both TM and TE modes, exhibiting different coupling strengths and levels of spatial field inhomogeneity. While the strong homogeneity of the bare TE mode gives rise to the standard anticrossing of strong coupling, the inhomogeneous polaritonic TM mode is shown to activate an observable Coulombic effect in the spectral response, often referred to as non-locality. This experiment demonstrates a cavity-induced modification of the 2DEG response and offers a new route to probing the effect of Coulomb interactions in ultrastrongly coupled systems via reshaping of their cavity mode profiles.

cond-mat.mes-hall↗

Quantum cascade laser roadmap

Quantum cascade lasers (QCLs) are unipolar semiconductor lasers first demonstrated in 1994. Since then, they have played a central role in advancing mid-infrared and terahertz photonics, becoming among the most reliable light sources in these regions of the electromagnetic spectrum. Their importance is further reinforced by their ability to generate self-starting optical frequency combs, whose investigation is motivated both by fundamental physics and by a wide range of applications, including molecular spectroscopy and free-space optical communications. This Roadmap provides a unified overview of current advances and emerging directions in QCL research. The chapters are organized into three main sections: device design and technology; frequency combs and pulse formation; and applications of QCLs. Each chapter reviews the relevant background, summarizes the current state of the art, and identifies key challenges and future directions within its specific research area.

physics.optics↗

Short period InGaAs/AlInAs THz quantum cascade laser in thin double metal cavities operating up to 188K

We present a two-well terahertz (THz) quantum cascade laser designed for high temperature operation based on the InGaAs/AlInAs material system. The lighter effective mass and higher energy barriers increase the gain at high temperatures (T > 150K). When processed in copper-based double metal waveguides the devices show laser action up to a maximum operating temperature of 188K with a maximum current density of 1.4kA/cm$^2$. The low Joule heating due to reduced active region thickness and low electrical bias allows operation at 10% duty cycle up to a temperature of 170K.

physics.optics↗

Infrared photonics for healthcare: A roadmap for proactive and predictive health management

The field of infrared (IR) photonics is currently undergoing remarkable progress, moving rapidly towards practical sensing applications demanded by medical therapy and diagnostics (theranostics). The Developments can be divided into three main categories: (i) novel devices and measurement concepts including advanced updates of classical approaches that push medical sensing into the spotlight; (ii) new demonstrations of photonic integrated circuit (PIC-)based IR devices enabling highly miniaturized sensors for point-of-care application as well as medical and wellness wearables; and (iii) technologically-mature IR demonstrators that enable first medical sensing and treatment applications. This roadmap paper provides a consolidated overview of this highly dynamic and interdisciplinary research field with a focus on the major roadblocks that limit the widespread adoption of IR photonics in large-scale medical diagnostics. Special attention is given to the ambivalence between the molecular-level spectroscopic interpretation and a broader health-state assessment, highlighting the need for a common framework. Additionally, the paper discusses the critical importance of unified measurement standards, calibration protocols, and medical certification processes to ensure the validity of experimental results, reproducibility, and clinical trust, particularly when novel experimental techniques and AI algorithms are involved. Perspectives from major past and current contributors to application-oriented IR photonics will be provided.

physics.app-ph↗

Bridging mid and near infrared by combining optomechanics and self mixing

This work describes a self-mixing-assisted optomechanical platform for transferring information between near- and mid-infrared radiation. In particular, the self-mixing signal of a mid-infrared quantum cascade laser is used to detect the oscillation of a membrane driven by light-induced forces exerted by a near-infrared excitation beam, which is amplitude-modulated at the membrane resonance frequency. This technique benefits from spectral broadness and, therefore, can link different spectral regions from both the excitation and probe sides. This versatility can pave the way for future applications of this self-mixing-assisted optomechanical platform in communication and advanced sensing systems.

physics.optics↗

Frequency and intensity noise of a grating-tuned external-cavity quantum cascade laser

Quantum cascade lasers (QCLs) are semiconductor-heterostructure devices known for their emission in the mid-infrared and THz spectral regions. Due to their operating regime, their intrinsic linewidth is significantly narrower compared to bipolar semiconductor lasers. Here, we demonstrate that by implementing an external-cavity (EC) configuration based on a commercial diffraction grating, we have successfully induced a Fabry-Perot QCL to emit on a single mode with a broadly-tunable wavelength in the range 4.29-4.44 μm. This very simple setup enhances the laser's performance in terms of threshold current and emitted power. We further prove that the EC configuration positively impacts the laser's noise properties. In particular, the intrinsic linewidth is substantially reduced, the full linewidth is also decreased (depending on the integration timescale), and the relative intensity noise is slightly reduced. These characteristics, which hold within the whole tuning range, make the EC-QCL a good candidate for spectroscopy applications where broad tunability and narrow linewidth are highly demanded.

physics.optics↗

Multi-mode Deep Strong Coupling in a Multi Quantum Well Fabry-Perot Cavity

We present multi-mode deep-strong coupling in a multi-quantum well (N=166) heterostructure. The heterostructure itself acts as a Fabry-Perot cavity, for which the even cavity modes strongly couple to the cyclotron resonance to form Landau polaritons. The experimentally observed vacuum Rabi splitting is larger than the mode spacing and well into the deep-strong coupling regime ($η>1$) resulting in a rich multi-mode polaritonic spectrum which is accurately reproduced by an all-to-all multi-photonic, multi-electronic Hopfield coupling model. Remarkably, light-matter decoupling is observed across the whole measurable spectrum, including in the low frequency limit ($λ>>L_{cav}$) where the normalized coupling strength reaches $η=8.1$. The system demonstrates a robust platform for exploring extreme coupling regimes and its chiral nature holds potential for chiral cavity and chiral mirror applications.

physics.optics↗

Casimir Stabilization of Fluctuating Electronic Nematic Order

Vacuum cavity control of quantum materials is the engineering of quantum materials systems through electromagnetic zero-point fluctuations. In this work we articulate a generic mechanism for vacuum optical control of correlated electronic order: Casimir control, where the zero-point energy of the electromagnetic continuum, the Casimir energy, depends on the properties of the material system. To assess the experimental viability of this mechanism we focus on the Casimir stabilization of fluctuating nematic order. In nematic Fermi liquids, different orientations of the electronic order are often energetically degenerate. Thus, while local domains of fixed orientation may form, thermal disordering inhibits long range order. By engineering the electromagnetic environment of the electronic system, however, we show that the Casimir energy can be used as a tool to preferentially stabilize particular orientations of the nematic order. As a concrete example, we examine the interplay between a birefringent crystal -- which sources an anisotropic electromagnetic environment -- and a quantum Hall stripe system, an archetypal nematic Fermi fluid. We show that for experimentally feasible setups, the anisotropy induced by the orientation dependent Casimir energy can be $10^4$ times larger than other mechanisms known to stabilize quantum Hall stripes. This finding convincingly implies that our setting may be realized with currently available experimental technology. Having demonstrated that the Casimir energy can be used to stabilize fluctuating nematic order, we close by discussing the implications for recent terahertz cavity experiments on quantum Hall stripes, as well as pave the road towards broader Casimir control of competing correlated electronic phases.

cond-mat.str-el↗

Gate-tunable single terahertz meta-atom ultrastrong light-matter coupling

We study the electrical tunability of ultrastrong light-matter interactions between a single terahertz circuit-based complementary split ring resonator (cSRR) and a two-dimensional electron gas. For this purpose, transmission spectroscopy measurements are performed under the influence of a strong magnetic field at different set points for the electric gate bias. The resulting Landau polariton dispersion depends on the applied electric bias, as the gating technique confines the electrons in-plane down to extremely sub-wavelength dimensions as small as d = 410 nm. This confinement allows for the excitation of standing plasma waves at zero magnetic field and an effective tunability of the electron number coupled to the THz resonator. This allows the normalized coupling strength to be tuned in-situ from $η$ = 0.46 down to $η$ = 0.18. This is the first demonstration of terahertz far-field spectroscopy of an electrically tunable interaction between a single terahertz resonator and electrons in a GaAs quantum well heterostructure.

cond-mat.mes-hall↗

Fast and compact time-resolved spectroscopy enabled by Quantum Walk Combs

Optical frequency combs paved the way for fast and compact multi-component optical chemical analysis due to their broadband spectra. Dual-comb spectrometers embody this technology, but their design requires a pair of matched combs, adding complexity to the system. In this study, we propose and implement a scheme for a rapid, compact spectroscopic analyser that operates without moving components, leveraging the tunability and speed of a single quantum walk comb laser. Previously, these combs have been shown to deliver stable, tunable and broadband lasing. Here, a single quantum cascade laser-based comb emitting within the significant molecular fingerprint region of the mid-infrared spectrum was employed in a non-interferometric setup for targeted and non-targeted analysis of various organic solvent vapours. With a time resolution as small as 10 microseconds and a high dynamic range reaching three orders of magnitude in concentration, this approach is suitable for the real-time analysis of chemical kinetics.

physics.optics↗

Time-resolved spectroscopy of noise-driven collective states of light

We study a collective liquid state of light in a fast-gain laser. Controlled temporal noise on the cavity modulation creates a fluctuating linear potential along the synthetic frequency lattice of the cavity modes. We identify three regimes of lattice occupation as noise increases: an extended distribution, a Gaussian envelope, and exponential localization. Time-resolved spectroscopy on single realizations of noise reveals distinct dynamics in the latter two: transport persists in the Gaussian regime, modulated by the fluctuating potential, but is fully suppressed at all times in the localized regime. Averaging over many noise realizations shows that noise reduces the transport speed and confirms ergodicity of the system.

physics.optics↗

On-chip pulse generation at 8 μm wavelength

The mid-infrared spectral region holds growing importance for applications such as gas sensing and spectroscopy. Although compact ultrashort pulse laser sources are essential to enable these applications, their realization in this spectral range remains an open challenge. We demonstrate an integrated approach to generate pulses in the mid-infrared based on chirped Bragg gratings engineered to compensate for the group delay dispersion of quantum cascade laser frequency comb sources. SiGe graded-index photonic circuits are used for operation around 8 μm wavelength. With this approach, pulses as short as 1.39 picoseconds were obtained, marking a key step towards fully integrated ultrashort pulse sources in the mid-infrared.

physics.optics↗