arXiv subjects

Jörg Schmalian

Publications and source records attributed to Jörg Schmalian.

At least 37 records · Page 2Linked to original sources

arXiv2025

Extended strange metal regime from superconducting puddles

We study a model of mesoscale superconducting puddles in a metal, represented as dynamical impurities interacting with a finite number of electronic channels via Andreev and normal scattering. We identify conditions under which the collection of puddles make a $T$-linear contribution to the resistivity and a $T\ln(1/T)$ to the specific heat and thermopower. This behavior emerges in an intermediate temperature range that extends from an upper energy scale set by the renormalized charging energy of the puddles, and down to an exponentially small scale associated with a charge-Kondo crossover, provided that the number of electronic channels interacting with the puddle is large. The phenomenology of our model resembles the apparent extended strange metal regime observed in overdoped cuprates which exhibits $T$-linear resistivity at low $T$ over a finite range of doping. We also propose to engineer a strange metal from suitably designed superconducting grains in a metallic matrix.

cond-mat.str-el↗

arXiv2024

Binding zero modes with fluxons in Josephson junctions of time-reversal invariant topological superconductors

We study the joint dynamics of the phase bias $ϕ$ and the propagating Majorana fermions of the edge modes in Josephson junctions containing 2D time-reversal invariant topological superconductors (TRITOPS). We consider TRITOPS-TRITOPS junctions, as well as junctions between topological and non-topological superconductors (TRITOPS-S). Both types of junctions are described by effective Dirac Hamiltonians with a $ϕ$-dependent mass. We analyze the effect of the phase fluctuations in the junction, as well as solitonic solutions of $ϕ$ generated by fluxons trapped in the junction. We show that these solitons generate a spatial-dependent mass with a sign change akin to the Jackiw-Rebbi model. This enables the formation of zero-energy fermionic states localized at the fluxon. For the TRITOPS-TRITOPS junction these consist of a Kramers pair of Majorana modes, while for the TRITOPS-S one, there is a single Majorana fermion. The localized bound states hybridize in soliton-antisoliton configurations. Depending on the occupation state, these modes generate an effective attraction or repulsion in the dynamics of the soliton-antisoliton collision.

cond-mat.supr-con↗

arXiv2024

Hydride superconductivity: here to stay

The field of hydride superconductivity has recently been mired in a controversy that might divert attention from the question of central importance: do hydrides support genuine superconductivity or not? We examine some key papers from the field, and conclude that hydride superconductivity is real.

cond-mat.supr-con↗

arXiv2024

Strange metal and superconductor in the two-dimensional Yukawa-Sachdev-Ye-Kitaev model

The two-dimensional Yukawa-Sachdev-Ye-Kitaev (2d-YSYK) model provides a universal theory of quantum phase transitions in metals in the presence of quenched random spatial fluctuations in the local position of the quantum critical point. It has a Fermi surface coupled to a scalar field by spatially random Yukawa interactions. We present full numerical solutions of a self-consistent disorder averaged analysis of the 2d-YSYK model in both the normal and superconducting states, obtaining electronic spectral functions, frequency-dependent conductivity, and superfluid stiffness. Our results reproduce key aspects of observations in the cuprates as analyzed by Michon et al. (arXiv:2205.04030). We also find a regime of increasing zero temperature superfluid stiffness with decreasing superconducting critical temperature, as is observed in bulk cuprates.

cond-mat.str-el↗

arXiv2024

Unconventional superconductivity from electronic dipole fluctuations

We study electron-electron Coulomb interactions in electronic systems whose Fermi surfaces possess a finite electric dipole density. Although there is no net dipole moment, we show that electric monopole-dipole interactions can become sufficiently strong in quasi-2D Dirac metals with spin-orbit coupling to induce unconventional odd-parity superconductivity, similar to the Balian-Werthamer state of ${}^{3}$He-B. Hence materials with spin-orbit-induced band inversion, such as the doped topological insulators Bi$_2$Se$_3$, Bi$_2$Te$_3$, and SnTe, are natural candidate materials where our theory could be relevant. We discuss the conditions for an electric dipole density to appear on the Fermi surface and develop the formalism to describe its coupling to the plasmon field which mediates the Coulomb interaction. A mechanism for the enhancement of dipolar coupling is then provided for quasi-2D Dirac systems. Within a large-$N$ renormalization group treatment, we show that the out-of-plane ($z$-axis) dipole coupling is marginally relevant, in contrast to the monopole coupling which is marginally irrelevant. For physically realistic parameters, we find that dipole fluctuations can get sufficiently enhanced to result in Cooper pairing. In addition, we establish that the proposed pairing glue is directly measurable in the $z$-axis optical conductivity.

cond-mat.supr-con↗

arXiv2024

Pairing at a single Van Hove point

We show that an interacting electronic system with a single ordinary or extended Van Hove point, which crosses the Fermi energy, is unstable against triplet superconductivity. The pairing mechanism is unconventional. There is no Cooper instability. Instead, pairing is due to the divergence of the density of states at a Van Hove point, leading to a superconducting quantum critical point at a finite detuning from the Van Hove point. The transition temperature is universally determined by the exponent governing the divergence of the density of states. Enhancing this exponent drastically increases $T_c$. The Cooper pair wave function has a non-monotonic momentum dependence with a steep slope near the gap nodes. In the absence of spin-orbit coupling, pairing fluctuations suppress a $2e$ spin-triplet state, but allow pairs of triplets to condense into a charge-$4e$ singlet state at a temperature of similar order as our result.

cond-mat.supr-con↗

arXiv2024

$T_c$ and the elastocaloric effect of Sr$_2$RuO$_4$ under $\langle 110 \rangle$ uniaxial stress: no indications of transition splitting

There is considerable evidence that the superconductivity of Sr2RuO4 has two components. Among this evidence is a jump in the shear elastic modulus $c_{66}$ at the critical temperature $T_c$, observed in ultrasound measurements. Such a jump is forbidden for homogeneous single-component order parameters, and implies that $T_c$ should develop as a cusp under the application of shear strain with $\langle 110 \rangle$ principal axes. This shear strain should split the onset temperatures of the two components, if they coexist, or select one component if they do not. Here, we report measurements of $T_c$ and the elastocaloric effect of Sr2RuO4 under uniaxial stress applied along the $[110]$ lattice direction. Within experimental resolution, we resolve neither a cusp in the stress dependence of $T_c$, nor any second transition in the elastocaloric effect data. We show that reconciling these null results with the observed jumps in $c_{66}$ requires extraordinarily fine tuning to a triple point of the Ginzburg-Landau parameter space. In addition, our results are inconsistent with homogeneous time reversal symmetry breaking at a temperature $T_2 \leq T_c$ as identified in muon spin relaxation experiments.

cond-mat.supr-con↗

arXiv2024

Solvable models of two-level systems coupled to itinerant electrons: Robust non-Fermi liquid and quantum critical pairing

Strange metal behavior is traditionally associated with an underlying putative quantum critical point at zero temperature. However, in many correlated metals, e.g., high-Tc cuprate superconductors, strange metallicity persists at low temperatures over an extended range of microscopic parameters, suggesting the existence of an underlying quantum critical phase, whose possible physical origins remain poorly understood. Systematic investigations of physical scenarios giving rise to such a critical, non-Fermi liquid (NFL) phase are therefore crucial to better understand this puzzling behavior. In a previous work [Bashan et al. arXiv:2310.07768], we considered a solvable large-N model consisting of itinerant electrons coupled to local two-level systems (TLSs) via spatially random interactions, inspired by the possibility of emergent metallic glassiness due to frustrated competing orders, and found that the system hosts an NFL phase with tunable exponents at intermediate couplings. In this work, we expand our investigation to the following: (i) We study the extent to which this NFL phase is generic by considering various deformations of our theory, including coupling of electrons to multiple operators of the TLSs and arbitrarily directed TLS-fields. We find that the physical picture obtained in Bashan et al. qualitatively persist in a wide region of parameter space, showcasing the robustness of the NFL phase; (ii) We analyze the superconducting instability due to coupling of TLSs to electrons, and find a rich structure, including quantum critical pairing associated with the NFL phase and conventional BCS pairing in the weak and strong coupling limits; (iii) We elaborate on the analysis of Bashan et al., including single-particle, transport and thermodynamic properties.

cond-mat.str-el↗

arXiv2024

Mitigating crosstalk errors by randomized compiling: Simulation of the BCS model on a superconducting quantum computer

We develop and apply an extension of the randomized compiling (RC) protocol that includes a special treatment of neighboring qubits and dramatically reduces crosstalk effects caused by the application of faulty gates on superconducting qubits in IBMQ quantum computers (\texttt{ibm\_lagos} and \texttt{ibmq\_ehningen}). Crosstalk errors, stemming from CNOT two-qubit gates, are a crucial source of errors on numerous quantum computing platforms. For the IBMQ machines, their magnitude is often overlooked-9. Our RC protocol turns coherent noise due to crosstalk into a depolarising noise channel that can then be treated using established error mitigation schemes, such as noise estimation circuits. We apply our approach to the quantum simulation of the non-equilibrium dynamics of the Bardeen-Cooper-Schrieffer (BCS) Hamiltonian for superconductivity, a particularly challenging model to simulate on quantum hardware because of the long-range interaction of Cooper pairs. With 135 CNOT gates, we work in a regime where crosstalk, as opposed to either trotterization or qubit decoherence, dominates the error. Our twirling of neighboring qubits is shown to dramatically improve the noise estimation protocol without the need to add new qubits or circuits and allows for a quantitative simulation of the BCS model.

quant-ph↗

arXiv2024

Cyclotron resonance and quantum oscillations of critical Fermi surfaces

Kohn's theorem places strong constraints on the cyclotron response of Fermi liquids. Recent observations of a doping dependence in the cyclotron mass of La$_{2-x}$Sr$_x$CuO$_4$ (Legros et al., Phys. Rev. B 106, 195110 (2022)) are therefore surprising because the cyclotron mass can only be renormalized by large momentum umklapp interactions which are not expected to vary significantly with doping. We show that a version of Kohn's theorem continues to apply to disorder-free non-Fermi liquids with a critical boson near zero momentum. However, marginal Fermi liquids arising from a spatially random Yukawa coupling between the electrons and bosons do give rise to significant corrections to the cyclotron mass which we compute. This is the same theory which yields linear-in-temperature resistivity and other properties of strange metals at zero fields (Patel et al., Science 381, 790 (2023)).

cond-mat.str-el↗

arXiv2023

Superconductivity due to fluctuating loop currents

Orbital magnetism and the loop currents (LC) that accompany it have been proposed to emerge in many systems, including cuprates, iridates, and kagome superconductors. In the case of cuprates, LCs have been put forward as the driving force behind the pseudogap, strange-metal behavior, and $d_{x^2-y^2}$-wave superconductivity. Here, we investigate whether fluctuating intra-unit-cell loop currents can cause unconventional superconductivity. For odd-parity LCs, we find that they are strongly repulsive in all pairing channels near the underlying quantum-critical point (QCP). For even-parity LCs, their fluctuations do give rise to unconventional pairing. However, this pairing is not amplified in the vicinity of the QCP, in sharp contrast to other known cases of pairing mediated by intra-unit-cell order parameters, such as spin-magnetic, nematic, or ferroelectric ones. Applying our formalism to the cuprates, we conclude that pairing mediated by fluctuating intra-unit-cell LCs is unlikely to yield $d_{x^2-y^2}$-wave superconductivity. We also show that loop currents, if relevant for the cuprates, must vary between unit cells and break translation symmetry.

cond-mat.supr-con↗

arXiv2023

Tunable non-Fermi liquid phase from coupling to two-level systems

We study a controlled large-$N$ theory of electrons coupled to dynamical two-level systems (TLSs) via spatially-random interactions. Such a physical situation arises when electrons scatter off low-energy excitations in a metallic glass, such as a charge or stripe glass. Our theory is governed by a non-Gaussian saddle point, which maps to the celebrated spin-boson model. By tuning the coupling strength we find that the model crosses over from a Fermi liquid at weak coupling to an extended region of non-Fermi liquid behavior at strong coupling, and realizes a marginal Fermi liquid at the crossover. Beyond a critical coupling strength, the TLSs freeze and Fermi-liquid behavior is restored. Our results are valid for generic space dimensions $d>1$.

cond-mat.str-el↗

arXiv2023

Constraints on the superconducting state of Sr$_2$RuO$_4$ from elastocaloric measurements

Strontium ruthenate Sr$_2$RuO$_4$ is an unconventional superconductor whose pairing symmetry has not been fully clarified, despite more than two decades of intensive research. Recent NMR Knight shift experiments have rekindled the Sr$_2$RuO$_4$ pairing debate by giving strong evidence against all odd-parity pairing states, including chiral $p$-wave pairing that was for a long time the leading pairing candidate. Here, we exclude additional pairing states by analyzing recent elastocaloric measurements [YS. Li et al., Nature 607, 276--280 (2022)]. To be able to explain the elastocaloric experiment, we find that unconventional even-parity pairings must include either large $d_{x^2 - y^2}$-wave or large $\{d_{xz} \mid d_{yz}\}$-wave admixtures, where the latter possibility arises because of the body-centered point group symmetry. These $\{d_{xz} \mid d_{yz}\}$-wave admixtures take the form of distinctively body-centered-periodic harmonics that have horizontal line nodes. Hence $g_{xy(x^2-y^2)}$-wave and $d_{xy}$-wave pairings are excluded as possible dominant even pairing states.

cond-mat.supr-con↗

arXiv2023

Thermalization of non-Fermi-liquid electron-phonon systems: Hydrodynamic relaxation of the Yukawa-Sachdev-Ye-Kitaev model

We study thermalization dynamics in a fermion-phonon variant of the Sachdev-Ye-Kitaev model coupled to an external cold thermal bath of harmonic oscillators. We find that quantum critical fermions thermalize more efficiently than phonons, in sharp contrast to the behavior in the Fermi liquid regime. In addition, after a short prethermal stage, the system acquires a quasi-thermal distribution given by a time-dependent effective temperature, reminiscent of "hydrodynamic" relaxation. All physical observables relax at the same rate which scales with the final temperature through an exponent that depends universally on the low energy spectrum of the system and the bath. Such relaxation rate is derived using a hydrodynamic approximation in full agreement with the numerical solution of a set quantum kinetic equations derived from the Keldysh formalism for non-equilibrium Green's functions. Our results hint toward further research on the applicability of the hydrodynamic picture in the description of the late time dynamics of open quantum systems despite the absence of conserved quantities in regimes dominated by conserving collisions.

cond-mat.str-el↗

arXiv2023

Correlation between phase stiffness and condensation energy across the non-Fermi to Fermi-liquid crossover in the Yukawa-Sachdev-Ye-Kitaev model on a lattice

We construct and analyze a lattice generalization of the Yukawa-Sachdev-Ye-Kitaev model, where spinful fermions experience on-site, random, all-to-all interactions with an Einstein bosonic mode, and random intersite coherent hopping. We obtain the exact self-consistent numerical solution of the model at mean-field level, and analytical approximations, for all values of fermion-boson coupling and hopping, under the spin-singlet ansatz and at particle-hole symmetry, both in the normal and superconducting states, thus tracing the entire phase diagram. In the normal state, the competition between hopping and coupling leads to crossovers between Fermi-liquid and non-Fermi liquid states, as reflected by the fermionic and bosonic spectral functions and the normal-state entropy. We calculate the finite phase stiffness of the superconducting state through the equilibrium electromagnetic response. Furthermore, we study the critical temperature $T_c$, as well as the spectral functions, the quasiparticle weight, the gap, and the condensation energy in the superconducting state. At weak coupling, we retrieve a disordered generalization of Bardeen-Cooper-Schrieffer theory. At strong coupling, asymptotically $T_c$ saturates but the stiffness decreases, which suggests strong superconducting fluctuations. $T_c$ is maximum in the single-dot limit, while the stiffness peaks exactly at the crossover between non-Fermi liquid and Fermi-liquid phases. We discover that the quasiparticle weight, the stiffness, and the condensation energy, are all correlated as a function of coupling, reminiscent of the correlations observed in high-temperature cuprate superconductors.

cond-mat.supr-con↗

arXiv2023

BCS to incoherent superconductivity crossovers in the Yukawa-SYK model on a lattice

We provide a quantitative and controlled analysis of the phase diagram of the the Yukawa-SYK model on a lattice, in the normal and superconducting states. We analyze the entire crossover from BCS/weak-coupling to Eliashberg/strong coupling superconductivity, as a function of fermion-boson interaction strength and hopping parameter. Cooper pairs of sharp Fermi-liquid quasiparticles at weak coupling evolve into pairing of fully incoherent fermions in the non-Fermi liquid regime. The crossovers leave observable traces in the critical temperature, the zero-temperature and zero-energy gap, the entropy, and the phase stiffness.

cond-mat.supr-con↗

arXiv2023

Giant lattice softening at a Lifshitz transition in Sr$_{2}$RuO$_{4}$

The interplay of electronic and structural degrees of freedom in solids is a topic of intense research. Experience and intuition suggest that structural changes drive conduction electron behavior, because the large number of valence electrons dominate the structural properties. As part of a seminal paper written over sixty years ago, Lifshitz discussed an alternative possibility: lattice softening driven by conduction electrons at topological Fermi surface transitions. The effect he predicted, however, was small, and has not been convincingly observed. Using measurements of the stress-strain relationship in the ultra-clean metal Sr$_{2}$RuO$_{4}$, we reveal a huge softening of the Young's modulus at a Lifshitz transition of a two-dimensional Fermi surface, and show that it is indeed entirely driven by the conduction electrons of the relevant energy band.

cond-mat.str-el↗

arXiv2023

Bosonic excitation spectra of superconducting $\mathrm{Bi_2Sr_2CaCu_2O_{8+δ}}$ and $\mathrm{YBa_2Cu_3O_{6+x}}$ extracted from scanning tunneling spectra

A detailed interpretation of scanning tunneling spectra obtained on unconventional superconductors enables one to gain information on the pairing boson. Decisive for this approach are inelastic tunneling events. Due to the lack of momentum conservation in tunneling from or to the sharp tip, those are enhanced in the geometry of a scanning tunneling microscope compared to planar tunnel junctions. This work extends the method of obtaining the bosonic excitation spectrum by deconvolution from tunneling spectra to nodal $d$-wave superconductors. In particular, scanning tunneling spectra of slightly underdoped $\mathrm{Bi_2Sr_2CaCu_2O_{8+δ}}$ with a $T_c$ of $82\,\mathrm{K}$ and optimally doped $\mathrm{YBa_2Cu_3O_{6+x}}$ with a $T_c$ of $92\,\mathrm{K}$ reveal a resonance mode in their bosonic excitation spectrum at $Ω_\mathrm{res} \approx 63\,\mathrm{meV}$ and $Ω_\mathrm{res} \approx 61\,\mathrm{meV}$ respectively. In both cases, the overall shape of the bosonic excitation spectrum is indicative of predominant spin scattering with a resonant mode at $Ω_\mathrm{res}<2Δ$ and overdamped spin fluctuations for energies larger than $2Δ$. To perform the deconvolution of the experimental data, we implemented an efficient iterative algorithm that significantly enhances the reliability of our analysis.

cond-mat.supr-con↗