arXiv subjects

Jörg Schmalian

Publications and source records attributed to Jörg Schmalian.

At least 55 records · Page 3Linked to original sources

arXiv2023

Magnetization Dynamics and Peierls Instability in Topological Josephson Structures

We study a long topological Josephson junction with a ferromagnetic strip between two superconductors. The low-energy theory exhibits a non-local in time and space interaction between chiral Majorana fermions, mediated by the magnonic excitations in the ferromagnet. While short ranged interactions turn out to be irrelevant by power counting, we show that sufficiently strong and long-ranged interactions may induce a $\mathbb{Z}_2$-symmetry breaking. This spontaneous breaking leads to a tilting of the magnetization perpendicular to the Majorana propagation direction and the opening of a fermionic gap (Majorana mass). It is analogous to the Peierls instability in the commensurate Fröhlich model and reflects the nontrivial interplay between Majorana modes and magnetization dynamics. Within a Gaussian fluctuation analysis, we estimate critical values for the temporal and spatial non-locality of the interaction, beyond which the symmetry breaking is stable at zero temperature -- despite the effective one-dimensionality of the model. We conclude that non-locality, i.e., the stiffness of the magnetization in space and time, stabilizes the symmetry breaking. In the stabilized regime, we expect the current-phase relation to exhibit an experimentally accessible discontinuous jump. At nonzero temperatures, as usual in the 1D Ising model, the long-range order is destroyed by solitonic excitations, which in our case carry each a Majorana zero mode. In order to estimate the correlation length, we investigate the solitons within a self-consistent mean-field approach.

cond-mat.mes-hall↗

arXiv2023

Non-local electrodynamics in ultra-pure PdCoO$_{2}$

The motion of electrons in the vast majority of conductors is diffusive, obeying Ohm's law. However, the recent discovery and growth of high-purity materials with extremely long electronic mean free paths has sparked interest in non-ohmic alternatives, including viscous and ballistic flow. Although non-ohmic transport regimes have been discovered across a range of materials, including two-dimensional electron gases, graphene, topological semimetals, and the delafossite metals, determining their nature has proved to be challenging. Here, we report on a new approach to the problem, employing broadband microwave spectroscopy of the delafossite metal PdCoO$_{2}$ in three distinct sample geometries that would be identical for diffusive transport. The observed differences, which go as far as differing power laws, take advantage of the hexagonal symmetry of PdCoO$_{2}$. This permits a particularly elegant symmetry-based diagnostic for non-local electrodynamics, with the result favouring ballistic over strictly hydrodynamic flow. Furthermore, it uncovers a new effect for ballistic electron flow, owing to the highly facetted shape of the hexagonal Fermi surface. We combine our extensive dataset with an analysis of the Boltzmann equation to characterize the non-local regime in PdCoO$_{2}$. More broadly, our results highlight the potential of broadband microwave spectroscopy to play a central role in investigating exotic transport regimes in the new generation of ultra-high conductivity materials.

cond-mat.mes-hall↗

arXiv2023

Cascade of vestigial orders in two-component superconductors: nematic, ferromagnetic, s-wave charge-4e, and d-wave charge-4e states

Electronically ordered states that break multiple symmetries can melt in multiple stages, similarly to liquid crystals. In the partially-melted phases, known as vestigial phases, a bilinear made out of combinations of the multiple components of the primary order parameter condenses. Multi-component superconductors are thus natural candidates for vestigial order, since they break both the U(1)-gauge and also time-reversal or lattice symmetries. Here, we use group theory to classify all possible real-valued and complex-valued bilinears of a generic two-component superconductor on a tetragonal or hexagonal lattice. While the more widely investigated real-valued bilinears correspond to vestigial nematic or ferromagnetic order, the little explored complex-valued bilinears correspond to a vestigial charge-$4e$ condensate, which itself can have an underlying $s$-wave, $d_{x^2-y^2}$-wave, or $d_{xy}$-wave symmetry. To properly describe the fluctuating regime of the superconducting Ginzburg-Landau action and thus access these competing vestigial phases, we employ both a large-N and a variational method. We show that while vestigial order can be understood as a weak-coupling effect in the large-N approach, it is akin to a moderate-coupling effect in the variational method. Despite these distinctions, both methods yield similar results in wide regions of the parameter space spanned by the quartic Landau coefficients. Specifically, we find that the nematic and ferromagnetic phases are the leading vestigial instabilities, whereas the various types of charge-$4e$ order are attractive albeit subleading vestigial channels. The only exception is for the hexagonal case, in which the nematic and $s$-wave charge-4e vestigial states are degenerate. We discuss the limitations of our approach, as well as the implications of our results for the realization of exotic charge-4e states in material candidates.

cond-mat.supr-con↗

arXiv2023

Identification of multiple-flux-quanta vortices by core states in the two-band superconductor Pb

Superconductors are of type I or II depending on whether they form an Abrikosov vortex lattice. Although bulk lead (Pb) is classified as a prototypical type-I superconductor, we observe single-flux-quantum and multiple-flux-quanta vortices in the intermediate state using mK scanning tunneling microscopy. We show that the winding number of individual vortices can be determined from the real space wave function of its Caroli-de Gennes-Matricon bound states. This generalizes the index theorem put forward by Volovik for isotropic electronic states to realistic electronic structures. In addition, the bound states due to the two superconducting bands of Pb can be separately detected. This yields strong evidence for low inter-band coupling and an independent closure of the gaps inside vortices.

cond-mat.supr-con↗

arXiv2023

Kinetic theory of the non-local electrodynamic response in anisotropic metals: skin effect in 2D systems

The electrodynamic response of ultra-pure materials at low temperatures becomes spatially non-local. This non-locality gives rise to phenomena such as hydrodynamic flow in transport and the anomalous skin effect in optics. In systems characterized by an anisotropic electronic dispersion, the non-local dynamics becomes dependent on the relative orientation of the sample with respect to the applied field, in ways that go beyond the usual, homogeneous response. Such orientational dependence should manifest itself not only in transport experiments, as recently observed, but also in optical spectroscopy. In this paper we develop a kinetic theory for the distribution function and the transverse conductivity of two- and three-dimensional Fermi systems with anisotropic electronic dispersion. By expanding the collision integral into the eigenbasis of a collision operator, we include momentum-relaxing scattering as well as momentum-conserving collisions. We examine the isotropic 2D case as a reference, as well as anisotropic hexagonal and square Fermi-surface shapes. We apply our theory to the quantitative calculation of the skin depth and the surface impedance, in all regimes of skin effect. We find qualitative differences between the frequency dependence of the impedance in isotropic and anisotropic systems. Such differences are shown to persist even for more complex 2D Fermi surfaces, including the ''supercircle'' geometry and an experimental parametrization for PdCoO$_2$, which deviate from an ideal polygonal shape. We study the orientational dependence of skin effect due to Fermi-surface anisotropy, thus providing guidance for the experimental study of non-local optical effects.

cond-mat.str-el↗

arXiv2022

Chiral surface superconductivity in half-Heusler semimetals

We propose the metallic and weakly dispersive surface states of half-Heusler semimetals as a possible domain for the onset of unconventional surface superconductivity ahead of the bulk transition. Using density functional theory (DFT) calculations and the random phase approximation (RPA), we analyse the surface band structure of LuPtBi and its propensity towards Cooper pair formation induced by screened electron-electron interactions in the presence of strong spin-orbit coupling. Over a wide range of model parameters, we find an energetically favoured chiral superconducting condensate featuring Majorana edge modes, while low-dimensional order parameter fluctuations trigger time-reversal symmetry breaking to precede the superconducting transition.

cond-mat.supr-con↗

arXiv2022

3DSC - A New Dataset of Superconductors Including Crystal Structures

Data-driven methods, in particular machine learning, can help to speed up the discovery of new materials by finding hidden patterns in existing data and using them to identify promising candidate materials. In the case of superconductors, which are a highly interesting but also a complex class of materials with many relevant applications, the use of data science tools is to date slowed down by a lack of accessible data. In this work, we present a new and publicly available superconductivity dataset ('3DSC'), featuring the critical temperature $T_\mathrm{c}$ of superconducting materials additionally to tested non-superconductors. In contrast to existing databases such as the SuperCon database which contains information on the chemical composition, the 3DSC is augmented by the approximate three-dimensional crystal structure of each material. We perform a statistical analysis and machine learning experiments to show that access to this structural information improves the prediction of the critical temperature $T_\mathrm{c}$ of materials. Furthermore, we see the 3DSC not as a finished dataset, but we provide ideas and directions for further research to improve the 3DSC in multiple ways. We are confident that this database will be useful in applying state-of-the-art machine learning methods to eventually find new superconductors.

cond-mat.supr-con↗

arXiv2022

Direct evidence of a charge depletion region at the interface of Van der Waals monolayers and dielectric oxides: The case of superconducting FeSe/STO

The discovery of two dimensional Van der Waals materials has opened up several possibilities for designing novel devices. Yet a more promising way of designing exotic heterostutures with improved physical properties is to grow a monolayer of these materials on a substrate. For example, in the field of superconductivity it has been demonstrated that the superconducting transition temperature of a monolayer of FeSe grown on some oxide substrates e.g., strontium titanate (STO) is by far higher than its bulk counterpart. Although the system has been considered as a model system for understanding the phenomenon of high-temperature superconductivity, the physical mechanism responsible for this high transition temperature is still highly under debate. Here using momentum and energy resolved high-resolution electron energy-loss spectroscopy we probe the dynamic charge response of the FeSe/STO(001) system and demonstrate that the frequency- and momentum-dependent dynamic charge response is not compatible with a simple film/substrate model. Our analysis reveals the existence of a depletion region at the interface between this Van der Waals monolayer and the substrate. The presence of the depletion layer, accompanied with a considerably large charge transfer from STO into the FeSe monolayer, leads to a strong renormalization of the STO energy bands and a substantial band bending at the interface. Our results shed light on the electronic complexities of the FeSe/oxide interfaces and pave the way of designing novel low-dimensional high-temperature superconductors through interface engineering. We anticipate that the observed phenomenon is rather general and can take place in many two dimensional Van der Waals monolayers brought in contact with dielectric oxides or semiconducting substrates.

cond-mat.supr-con↗

arXiv2022

Elastocaloric determination of the phase diagram of Sr$_2$RuO$_4$

One of the main developments in unconventional superconductivity in the past two decades has been the discovery that most unconventional superconductors form phase diagrams that also contain other strongly correlated states. Many systems of interest are therefore close to more than one instability, and tuning between the resultant ordered phases is the subject of intense research1. In recent years, uniaxial pressure applied using piezoelectric-based devices has been shown to be a particularly versatile new method of tuning, leading to experiments that have advanced our understanding of the fascinating unconventional superconductor Sr$_2$RuO$_4$. Here we map out its phase diagram using high-precision measurements of the elastocaloric effect in what we believe to be the first such study including both the normal and the superconducting states. We observe a strong entropy quench on entering the superconducting state, in excellent agreement with a model calculation for pairing at the Van Hove point, and obtain a quantitative estimate of the entropy change associated with entry to a magnetic state that is observed in proximity to the superconductivity. The phase diagram is intriguing both for its similarity to those seen in other families of unconventional superconductors and for extra features unique, so far, to Sr$_2$RuO$_4$.

cond-mat.supr-con↗

arXiv2022

Topologically enabled superconductivity

Majorana zero modes are a much sought-after consequence of one-dimensional topological superconductivity. Here, we show that, in turn, zero modes accompanying dynamical instanton events strongly enhance -- in some cases even enable -- superconductivity. We find that the dynamics of a one-dimensional topological triplet superconductor is governed by a $θ$ term in the action. For isotropic triplets, this term enables algebraic charge-$2e$ superconductivity, which is destroyed by fluctuations in nontopological superconductors. For anisotropic triplets, zero modes suppress quantum phase slips and stabilize superconductivity over a large region of the phase diagram. We present predictions of correlation functions and thermodynamics for states of topologically enhanced superconductivity.

cond-mat.supr-con↗

arXiv2022

An Electronic Nematic Liquid in BaNi$_2$As$_2$

Understanding the organizing principles of interacting electrons and the emergence of novel electronic phases is a central endeavor of condensed matter physics. Electronic nematicity, in which the discrete rotational symmetry in the electron fluid is broken while the translational one remains unaffected, is a prominent example of such a phase. It has proven ubiquitous in correlated electron systems, and is of prime importance to understand Fe-based superconductors. Here, we find that fluctuations of such broken symmetry are exceptionally strong over an extended temperature range above phase transitions in \bnap, the nickel homologue to the Fe-based systems. This provides evidence for a type of electronic nematicity, dynamical in nature, which exhibits an unprecedented coupling to the underlying crystal lattice. Fluctuations between degenerate nematic configurations cause a splitting of phonon lines, without lifting degeneracies nor breaking symmetries, akin to spin liquids in magnetic systems.

cond-mat.str-el↗

arXiv2022

Integer and fractionalized vortex lattices and off-diagonal long-range order

We analyze the implication of off-diagonal long-range order (ODLRO) for inhomogeneous periodic field configurations and multi-component order parameters. For single component order parameters we show that the only static, periodic field configuration consistent with ODLRO is a vortex lattice with integer flux in units of the flux quantum in each unit cell. For a superconductor with $g$ degenerate components, fractional vortices are allowed. Depending on the precise order-parameter manifold, they tend to occur in units of $1/g$ of the flux quantum. These results are well known to emerge from the Ginzburg-Landau or BCS theories of superconductivity. Our results imply that they are valid even if these theories no-longer apply. Integer and fractional vortex lattices are transparently seen to emerge as a consequence of the macroscopic coherence and single valuedness of the condensate.

cond-mat.supr-con↗

arXiv2022

Nodal and nematic superconducting phases in NbSe2 monolayers from competing superconducting channels

Transition metal dichalcogenides like 2H-NbSe2 in their two-dimensional (2D) form exhibit Ising superconductivity with the quasiparticle spins are firmly pinned in the direction perpendicular to the basal plane. This enables them to withstand exceptionally high magnetic fields beyond the Pauli limit for superconductivity. Using field-angle-resolved magnetoresistance experiments for fields rotated in the basal plane we investigate the field-angle dependence of the upper critical field (Hc2), which directly reflects the symmetry of the superconducting order parameter. We observe a six-fold nodal symmetry superposed on a two-fold symmetry. This agrees with theoretical predictions of a nodal topological superconducting phase near Hc2, together with a nematic superconducting state. We demonstrate that in NbSe2 such unconventional superconducting states can arise from the presence of several competing superconducting channels.

cond-mat.supr-con↗

arXiv2021

Quantum critical Eliashberg theory, the SYK superconductor and their holographic duals

Superconductivity is abundant near quantum-critical points, where fluctuations suppress the formation of Fermi liquid quasiparticles and the BCS theory no longer applies. Two very distinct approaches have been developed to address this issue: quantum-critical Eliashberg theory and holographic superconductivity. The former includes a strongly retarded pairing interaction of ill-defined fermions, the latter is rooted in the duality of quantum field theory and gravity theory. We demonstrate that both are different perspectives of the same theory. We derive holographic superconductivity in form of a gravity theory with emergent space-time from a quantum many-body Hamiltonian - the Yukawa SYK model - where the Eliashberg formalism is exact. Exploiting the power of holography, we then determine the dynamic pairing susceptibility of the model. Our holographic map comes with the potential to use quantum gravity corrections to go beyond the Eliashberg regime.

cond-mat.str-el↗

arXiv2021

Fracton-elasticity duality in twisted moiré superlattices

We formulate a fracton-elasticity duality for twisted moiré superlattices, taking into account that they are incommensurate crystals with dissipative phason dynamics. From a dual tensor-gauge formulation, as compared to standard crystals, we identify twice the number of conserved charges that describe topological lattice defects, namely, disclinations and a new type of defect that we dub discompressions. The key implication of these conservation laws is that both glide and climb motions of lattice dislocations are suppressed, indicating that dislocation networks may become exceptionally stable. Our results also apply to other planar incommensurate crystals and quasicrystals.

cond-mat.str-el↗

arXiv2021

Breakdown of the Wiedemann-Franz law at the Lifshitz point of strained Sr$_2$RuO$_4$

Strain tuning Sr$_{2}$RuO$_{4}$ through the Lifshitz point, where the Van Hove singularity of the electronic spectrum crosses the Fermi energy, is expected to cause a change in the temperature dependence of the electrical resistivity from its Fermi liquid behavior $ρ\sim T^{2}$ to $ρ\sim T^{2}{\rm log}\left(1/T\right)$, a behavior consistent with experiments by Barber et al. [Phys. Rev. Lett. 120, 076601 (2018)]. This expectation originates from the same multi-band scattering processes with large momentum transfer that were recently shown to account for the linear in $T$ resistivity of the strange metal Sr$_{3}$Ru$_{2}$O$_{7}$. In contrast, the thermal resistivity $ρ_{Q}\equiv T/κ$, where $κ$ is the thermal conductivity, is governed by qualitatively distinct processes that involve a broad continuum of compressive modes, i.e. long wavelength density excitations in Van Hove systems. While these compressive modes do not affect the charge current, they couple to thermal transport and yield $ρ_{Q}\propto T^{3/2}$. As a result, we predict that the Wiedemann-Franz law in strained Sr$_{2}$RuO$_{4}$ should be violated with a Lorenz ratio $L\propto T^{1/2}{\rm log}\left(1/T\right)$. We expect this effect to be observable in the temperature and strain regime where the anomalous charge transport was established.

cond-mat.str-el↗

arXiv2021

Edwards-Anderson parameter and local Ising-nematicity in FeSe revealed via NMR spectral broadening

The NMR spectrum of FeSe shows a dramatic broadening on cooling towards the bulk nematic phase at $T_s=90$ K, due to the formation of a quasi-static, short-range-ordered nematic domain structure. However, a quantitative understanding of the NMR broadening and its relationship to the nematic susceptibility is still lacking. Here, we show that the temperature and pressure dependence of the broadening is in quantitative agreement with the mean-field Edwards-Anderson parameter of an Ising-nematic model in the presence of random-field disorder introduced by non-magnetic impurities. Furthermore, these results reconcile the interpretation of NMR and Raman spectroscopy data in FeSe under pressure.

cond-mat.str-el↗

arXiv2021

High sensitivity heat capacity measurements on Sr2RuO4 under uniaxial pressure

A key question regarding the unconventional superconductivity of Sr$_2$RuO$_4$ remains whether the order parameter is single- or two-component. Under a hypothesis of two-component superconductivity, uniaxial pressure is expected to lift their degeneracy, resulting in a split transition. The most direct and fundamental probe of a split transition is heat capacity. Here, we report measurement of heat capacity of samples subject to large and highly homogeneous uniaxial pressure. We place an upper limit on the heat-capacity signature of any second transition of a few per cent of that of the primary superconducting transition. The normalized jump in heat capacity, $ΔC/C$, grows smoothly as a function of uniaxial pressure, favouring order parameters which are allowed to maximize in the same part of the Brillouin zone as the well-studied van Hove singularity. Thanks to the high precision of our measurements, these findings place stringent constraints on theories of the superconductivity of Sr$_2$RuO$_4$.

cond-mat.supr-con↗