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J. C. Campuzano

Publications and source records attributed to J. C. Campuzano.

At least 37 records · Page 2Linked to original sources

From Fermi Arcs to the Nodal Metal: Scaling of the Pseudogap with Doping and Temperature

The pseudogap phase in the cuprates is a most unusual state of matter: it is a metal, but its Fermi surface is broken up into disconnected segments known as Fermi arcs. Using angle resolved photoemission spectroscopy, we show that the anisotropy of the pseudogap in momentum space and the resulting arcs depend only on the ratio T/T*(x), where T*(x) is the temperature below which the pseudogap first develops at a given hole doping x. In particular, the arcs collapse linearly with T/T* and extrapolate to zero extent as T goes to 0. This suggests that the T = 0 pseudogap state is a nodal liquid, a strange metallic state whose gapless excitations are located only at points in momentum space, just as in a d-wave superconductor.

cond-mat.supr-con↗

The change of Fermi surface topology in Bi2Sr2CaCu2O8 with doping

We report the observation of a change in Fermi surface topology of Bi2Sr2CaCu2O8 with doping. By collecting high statistics ARPES data from moderately and highly overdoped samples and dividing the data by the Fermi function, we answer a long standing question about the Fermi surface shape of Bi2Sr2CaCu2O8 close to the (pi,0) point. For moderately overdoped samples (Tc=80K) we find that both the bonding and antibonding sheets of the Fermi surface are hole-like. However for a doping level corresponding to Tc=55K we find that the antibonding sheet becomes electron-like. This change does not directly affect the critical temperature and therefore the superconductivity. However, since similar observations of the change of the topology of the Fermi surface were observed in LSCO and Bi2Sr2Cu2O6, it appears to be a generic feature of hole-doped superconductors. Because of bilayer splitting, though, this doping value is considerably lower than that for the single layer materials, which again argues that it is unrelated to Tc.

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Non-dispersive Fermi arcs and absence of charge ordering in the pseudogap phase of Bi2Sr2CaCu2O8+d

The autocorrelation of angle resolved photoemission data from the high temperature superconductor Bi2Sr2CaCu2O8+d shows distinct peaks in momentum space which disperse with binding energy in the superconducting state, but not in the pseudogap phase. Although it is tempting to attribute a non-dispersive behavior in momentum space to some ordering phenomenon, a de-construction of the autocorrelation reveals that the non-dispersive peaks arise not from ordering, but rather from the tips of the Fermi arcs, which themselves do not change with binding energy.

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Momentum anisotropy of the scattering rate in cuprate superconductors

We examine the momentum and energy dependence of the scattering rate of the high temperature cuprate superconductors using angle resolved photoemission spectroscopy. The scattering rate is of the form a + bw around the Fermi surface for under and optimal doping. The inelastic coefficient "b" is found to be isotropic. The elastic term, "a", however, is found to be highly anisotropic for under and optimally doped samples, with an anisotropy which correlates with that of the pseudogap. This is contrasted with heavily overdoped samples, which show an isotropic scattering rate and an absence of the pseudogap above T_c. We find this to be a generic property for both single and double layer compounds.

cond-mat.str-el↗

Momentum anisotropy of the scattering rate in cuprate superconductors

We examine the momentum and energy dependence of the scattering rate of the high temperature cuprate superconductors using angle resolved photoemission spectroscopy. The scattering rate is of the form a + b*w. The inelastic coefficient b is found to be isotropic. The elastic term, a, however, is found to be highly anisotropic in the pseudogap phase of optimal doped samples, with an anisotropy which correlates with that of the pseudogap. This can be contrasted with heavily overdoped samples, which show an isotropic scattering rate in the normal state.

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Identifying the Background Signal in ARPES of High Temperature Superconductors

One of the interesting features of the photoemission spectra of the high temperature cuprate superconductors is the presence of a large signal (referred to as the "background'') in the unoccupied region of the Brillouin zone. Here we present data indicating that the origin of this signal is extrinsic and is most likely due to strong scattering of the photoelectrons. We also present an analytical method that can be used to subtract the background signal.

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ARPES on Na$_{0.6}$CoO$_{2}$: Fermi surface, extended flat dispersion, and unusual band splitting

The electronic structure of single crystals Na$_{0.6}$CoO$_2$, which are closely related to the superconducting Na$_{0.3}$CoO$_2$.$y$H$_2$O ($T_c \sim 5K$), is studied by angle-resolved photoelectron spectroscopy. While the measured Fermi surface is found to be consistent with the prediction of a local density band theory, the energy dispersion is highly renormalized, with an anisotropy along the two principle axes ($Γ$-$K$, $Γ$-$M$). Our ARPES result also indicates that an extended flat band is formed slightly above $E_F$ along $Γ$-$K$. In addition, an unusual band splitting is observed in the vicinity of the Fermi surface along the $Γ$-$M$ direction, which differs from the predicted bilayer splitting.

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Angle Resolved Photemission Experiments to look for Time-reversal Violation in Cuprates

The recent experiments reported by Borisenko et al. (cond-mat/0305179 v2), are examined in light of the conditions to be satisfied in the search for time-reversal violation by circularly polarized ARPES. Two principal problems are found: (1) A lack of any evidence for the magnitude of the pseudogap or the temperature of its onset in the samples studied. (2) A difference in the dichroic signal at low and high temperatures. The difference is greater than the stated error bars and is contrary to the conclusions reached in the paper.

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Reply to Comment on: "Spontaneous breaking of time-reversal symmetry in the pseudogap state of a high-Tc superconductor"

In a recent comment [1], Armitage and Hu have suggested that our experiment observing dichroism in angle resolved photoemission (ARPES) [2] could not be conclusively interpreted as arising from time reversal symmetry breaking, arguing that our observations are likely due to structural effects. The concerns expressed by Armitage and Hu that our results could be due to a change in the mirror plane are as important as they are obvious. In fact the first part of their comment merely restates the results of Simon and Varma [3] about the relationship and contrast of effects due to time reversal symmetry breaking and those caused by crystallographic changes. In any test of time reversal symmetry one must ensure that parity alone is not inducing the observed changes. We have indeed considered this issue very carefully in the course of our study [2] and it is precisely the lack of temperature dependent structural changes significant enough to explain the magnitude of the observed dichroism that forced us to conclude that time reversal symmetry breaking is the only plausible explanation. Furthermore, recent experiments by Borisenko, et al. [4] confirm that changes in the mirror plane are unmeasurably small.

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Crossover from coherent to incoherent electronic excitations in the normal state of Bi2Sr2CaCu2O8

Angle resolved photoemission spectroscopy (ARPES) and resistivity measurements are used to explore the overdoped region of the high temperature superconductor Bi2Sr2CaCu2O8+delta. We find evidence for a new crossover line in the phase diagram between a coherent metal phase for lower temperatures and higher doping, and an incoherent metal phase for higher temperatures and lower doping. The former is characterized by two well-defined spectral peaks in ARPES due to coherent bilayer splitting and superlinear behavior in the resistivity, whereas the latter is characterized by a single broad spectral feature in ARPES and a linear temperature dependence of the resistivity.

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Photoemission in the High Tc Superconductors

We review angle resolved photoemission spectroscopy (ARPES) results on the high Tc superconductors, focusing primarily on results obtained on the quasi-two dimensional cuprate Bi2Sr2CaCu2O8 and its single layer counterpart Bi2Sr2CuO6. The topics treated include the basics of photoemission and methodologies for analyzing spectra, normal state electronic structure including the Fermi surface, the superconducting energy gap, the normal state pseudogap, and the electron self-energy as determined from photoemission lineshapes.

cond-mat.supr-con↗

Spontaneous time reversal symmetry breaking in the pseudogap state of high-Tc superconductors

When matter undergoes a phase transition from one state to another, usually a change in symmetry is observed, as some of the symmetries exhibited are said to be spontaneously broken. The superconducting phase transition in the underdoped high-Tc superconductors is rather unusual, in that it is not a mean-field transition as other superconducting transitions are. Instead, it is observed that a pseudo-gap in the electronic excitation spectrum appears at temperatures T* higher than Tc, while phase coherence, and superconductivity, are established at Tc (Refs. 1, 2). One would then wish to understand if T* is just a crossover, controlled by fluctuations in order which will set in at the lower Tc (Refs. 3, 4), or whether some symmetry is spontaneously broken at T* (Refs. 5-10). Here, using angle-resolved photoemission with circularly polarized light, we find that, in the pseudogap state, left-circularly polarized photons give a different photocurrent than right-circularly polarized photons, and therefore the state below T* is rather unusual, in that it breaks time reversal symmetry11. This observation of a phase transition at T* provides the answer to a major mystery of the phase diagram of the cuprates. The appearance of the anomalies below T* must be related to the order parameter that sets in at this characteristic temperature .

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Momentum Distribution Curves in the Superconducting State

We demonstrate that the E vs. k dispersion in the superconducting state extracted from momentum distribution curves differs qualitatively from the traditional dispersion extracted from energy distribution curves. This occurs because of a combination of many-body effects and the presence of an energy gap, along with the associated coherence factors. Analysis of such MDC dispersions can give important information on the microscopics of high temperature superconductors.

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On the determination of the Fermi surface in high-Tc superconductors by angle-resolved photoemission spectroscopy

We study the normal state electronic excitations probed by angle resolved photoemission spectroscopy (ARPES) in Bi2201 and Bi2212. Our main goal is to establish explicit criteria for determining the Fermi surface from ARPES data on strongly interacting systems where sharply defined quasiparticles do not exist and the dispersion is very weak in parts of the Brillouin zone. Additional complications arise from strong matrix element variations within the zone. We present detailed results as a function of incident photon energy, and show simple experimental tests to distinguish between an intensity drop due to matrix element effects and spectral weight loss due to a Fermi crossing. We reiterate the use of polarization selection rules in disentangling the effect of umklapps due to the BiO superlattice in Bi2212. We conclude that, despite all the complications, the Fermi surface can be determined unambiguously: it is a single large hole barrel centered about (pi,pi) in both materials.

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Magnetic Resonance, Electronic spectra and Bilayer Splitting in Underdoped Bi2212

We report the first inelastic neutron scattering (INS) experiments of the resonance in the underdoped regime of Bi2Sr2CaCu2O8+d. The energy of the resonance is found to be 34 meV and the temperature dependence shows a smooth evolution through Tc with a remnant persisting in the pseudogap state. Besides the INS data, we present also angle resolved photoemission (ARPES) spectra taken on the same crystals. As a function of temperature, the neutron intensity scales with the square of the ARPES gap estimated by the leading-edge midpoint at (pi,0). We also show that the energy of the collective mode inferred from the peak-dip-hump structure compares well with the energy of the resonance. Based on kinematics, we argue that the correlation of these two energies is consistent with the absence of bilayer splitting in the electronic dispersion.

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The Temperature Evolution of the Spectral Peak in High Temperature Superconductors

Recent photoemission data in the high temperature cuprate superconductor Bi2212 have been interpreted in terms of a sharp spectral peak with a temperature independent lifetime, whose weight strongly decreases upon heating. By a detailed analysis of the data, we are able to extract the temperature dependence of the electron self-energy, and demonstrate that this intepretation is misleading. Rather, the spectral peak loses its integrity above Tc due to a large reduction in the electron lifetime.

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Renormalization of spectral lineshape and dispersion below Tc in Bi2Sr2CaCu2O8+d

Angle-resolved photoemission (ARPES) data in the superconducting state of Bi2Sr2CaCu2O8+d show a kink in the dispersion along the zone diagonal, which is related via a Kramers-Kronig analysis to a drop in the low-energy scattering rate. As one moves towards (pi,0), this kink evolves into a spectral dip. The occurrence of these anomalies in the dispersion and lineshape throughout the zone indicate the presence of a new energy scale in the superconducting state.

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Coherent quasiparticle weight and its connection to high-T_c superconductivity from angle-resolved photoemission

In conventional superconductors, the pairing energy gap (Δ) and superconducting phase coherence go hand-in-hand. As the temperature is lowered, both the energy gap and phase coherence appear at the transition temperature T_c. In contrast, in underdoped high-T_c superconductors (HTSCs), a pseudogap appears at a much higher temperature T^*, smoothly evolving into the superconducting gap at T_c. Phase coherence on the other hand is only established at T_c, signaled by the appearance of a sharp quasiparticle (QP) peak in the excitation spectrum. Another important difference between the two types of superconductors is in the ratio of 2Δ/ T_c=R. In BCS theory, R~3.5, is constant. In the HTSCs this ratio varies widely, continuing to increase in the underdoped region, where the gap increases while T_c decreases. Here we report that in HTSCs it is the ratio z_AΔ_m/T_c which is approximately constant, where Δ_m is the maximum value of the d-wave gap, and z_A is the weight of the coherent excitations in the spectral function. This is highly unusual, since in nearly all phase transitions, T_c is determined by an energy scale alone. We further show that in the low-temperature limit, z_{\it A} increases monotonically with increasing doping x. The growth is linear, i.e. z_A(x)\propto x, in the underdoped to optimally doped regimes, and slows down in overdoped samples. The reduction of z_A with increasing temperature resembles that of the c-axis superfluid density.

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