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J. C. Campuzano

Publications and source records attributed to J. C. Campuzano.

At least 55 records · Page 3Linked to original sources

Photoemission and the Origin of High Temperature Superconductivity

The condensation energy can be shown to be a moment of the change in the occupied part of the spectral function when going from the normal to the superconducting state. As a consequence, there is a one to one correspondence between the energy gain associated with forming the superconducting ground state, and the dramatic changes seen in angle resolved photoemission spectra. Some implications this observation has are offered.

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Condensation Energy and Spectral Functions in High Temperature Superconductors

If high temperature cuprate superconductivity is due to electronic correlations, then the energy difference between the normal and superconducting states can be expressed in terms of the occupied part of the single particle spectral function. The latter can, in principle, be determined from angle resolved photoemission (ARPES) data. As a consequence, the energy gain driving the development of the superconducting state is intimately related to the dramatic changes in the photoemission lineshape when going below Tc. These points are illustrated in the context of the "mode" model used to fit ARPES data in the normal and superconducting states, where the question of kinetic energy versus potential energy driven superconductivity is explored in detail. We use our findings to comment on the relation of ARPES data to the condensation energy, and to various other experimental data. In particular, our results suggest that the nature of the superconducting transition is strongly related to how anomalous (non Fermi liquid like) the normal state spectral function is, and as such, is dependent upon the doping level.

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The Fermi surface of Bi2Sr2CaCu2O8

We study the Fermi surface of Bi2Sr2CaCu2O8 (Bi2212) using angle resolved photoemission (ARPES) with a momentum resolution of ~ 0.01 of the Brillouin zone. We show that, contrary to recent suggestions, the Fermi surface is a large hole barrel centered at (pi,pi), independent of the incident photon energy.

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Quasiparticles in the superconducting state of Bi2Sr2CaCu2O8

Recent improvements in momentum resolution by a factor of 32 lead to qualitatively new ARPES results on the spectra of Bi2Sr2CaCu2O8 (Bi2212) along the (pi,pi) direction, where there is a node in the superconducting gap. With improved resolution, we now see the intrinsic lineshape, which indicates the presence of true quasiparticles at the Fermi momentum in the superconducting state, and lack thereof in the normal state. The region of momentum space probed here is relevant for charge transport, motivating a comparison of our results to conductivity measurements by infrared reflectivity.

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Electronic Spectra and Their Relation to the (pi,pi) Collective Mode in High-Tc Superconductors

Photoemission spectra of Bi2Sr2CaCu2O8 reveal that the high energy feature near (pi,0), the "hump", scales with the superconducting gap and persists above Tc in the pseudogap phase. As the doping decreases, the dispersion of the hump increasingly reflects the wavevector (pi,pi) characteristic of the undoped insulator, despite the presence of a large Fermi surface. This can be understood from the interaction of the electrons with a collective mode, supported by our observation that the doping dependence of the resonance observed by neutron scattering is the same as that inferred from our data.

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Extraction of the Electron Self-Energy from Angle Resolved Photoemission Data: Application to Bi2212

The self-energy $Σ({\bf k},ω)$, the fundamental function which describes the effects of many-body interactions on an electron in a solid, is usually difficult to obtain directly from experimental data. In this paper, we show that by making certain reasonable assumptions, the self-energy can be directly determined from angle resolved photoemission data. We demonstrate this method on data for the high temperature superconductor $Bi_2Sr_2CaCu_2O_{8+x}$ (Bi2212) in the normal, superconducting, and pseudogap phases.

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Superconducting Gap Anisotropy and Quasiparticle Interactions: a Doping Dependent ARPES Study

Comparing ARPES measurements on Bi2212 with penetration depth data, we show that a description of the nodal excitations of the d-wave superconducting state in terms of non-interacting quasiparticles is inadequate, and we estimate the magnitude and doping dependence of the Landau interaction parameter which renormalizes the linear T contribution to the superfluid density. Furthermore, although consistent with d-wave symmetry, the gap with underdoping cannot be fit by the simple coskx-cosky form, which suggests an increasing importance of long range interactions as the insulator is approached.

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Temperature-induced spectral weight transfer in Bi_2Sr_2CaCu_2O_{8+delta}: a conventional view

In contrast with the recent photoemission observations by Shen et al. of anomalous temperature-induced momentum-dependent spectral weight transfer in Bi_2Sr_2CaCu_2O_{8+delta}, we find that in the same material, in spite of the unusual spectral lineshape change between superconducting and normal states, the integrated spectral weight displays minimum variation as a function of temperature, which is in agreement with the sum rule of angle-resolved photoemission: the integrated spectral weight is proportional to the momentum density, n(k).

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Hot Spots on the Fermi Surface of Bi2212: Stripes versus Superstructure

In a recent paper Saini et al. have reported evidence for a pseudogap around (pi,0) at room temperature in the optimally doped superconductor Bi2212. This result is in contradiction with previous ARPES measurements. Furthermore they observed at certain points on the Fermi surface hot spots of high spectral intensity which they relate to the existence of stripes in the CuO planes. They also claim to have identified a new electronic band along Gamma-M1 whose one dimensional character provides further evidence for stripes. We demonstrate in this Comment that all the measured features can be simply understood by correctly considering the superstructure (umklapp) and shadow bands which occur in Bi2212.

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Photoelectron Escape Depth and Inelastic Secondaries in High Temperature Superconductors

We calculate the photoelectron escape depth in the high temperature superconductor Bi2212 by use of electron energy-loss spectroscopy data. We find that the escape depth is only 3 Ang. for photon energies typically used in angle resolved photoemission measurements. We then use this to estimate the number of inelastic secondaries, and find this to be quite small near the Fermi energy. This implies that the large background seen near the Fermi energy in photoemission measurements is of some other origin.

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Destruction of the Fermi Surface in Underdoped High Tc Superconductors

The Fermi surface is a central concept in the theory of metals. Even though the optimally doped high temperature superconductors exhibit an anomalous normal state, angle resolved photoemission spectroscopy (ARPES) has revealed a large Fermi surface despite the absence of well-defined quasiparticles and the necessity of working at finite temperatures. However, the even more unusual behavior in the underdoped high temperature superconductors, which show a pseudogap above Tc, requires us to carefully re-examine this concept. Here, we present the first results on how the Fermi surface is destroyed as a function of temperature in underdoped Bi2212 using ARPES. We find the remarkable effect that different k points become gapped at different temperatures. This leads to a break up of the Fermi surface at a temperature T* into disconnected Fermi arcs which shrink with decreasing T, eventually collapsing to the point nodes of the dx2-y2 superconducting ground state below Tc. This novel behavior, where the Fermi surface does not form a continuous contour in momentum space, is unprecedented in that it occurs in the absence of long range order. Moreover, although the d-wave superconducting gap below Tc smoothly evolves into the pseudogap above Tc, the gaps at different k points are not related to one another above Tc the same way as they are below, implying an intimate, but non-trivial relation, between the two.

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ARPES study of the superconducting gap and pseudogap in Bi2Sr2CaCu2O8+x

In this paper, we review some of our ARPES results on the superconducting and pseudo gaps in Bi2Sr2CaCu2O8+x. We find that optimally and overdoped samples exhibit a d-wave gap, which closes at the same temperature, Tc, for all k points. In underdoped samples, a leading edge gap is found up to a temperature T* > Tc. We find that T* scales with the maximum low temperature gap, increasing as the doping is reduced. The momentum dependence of the pseudogap is similar to that of the superconducting gap; however, the pseudogap closes at different temperatures for different k points.

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Phenomenology of Photoemission Lineshapes of High Tc Superconductors

We introduce a simple phenomenological form for the self-energy which allows us to extract important information from angle resolved photoemission data on the high Tc superconductor Bi2212. First, we find a rapid suppression of the single particle scattering rate below Tc for all doping levels. Second, we find that in the overdoped materials the gap Delta at all k-points on the Fermi surface has significant temperature dependence and vanishes near Tc. In contrast, in the underdoped samples such behavior is found only at k-points close to the diagonal. Near (pi,0), Delta is essentially T-independent in the underdoped samples. The filling-in of the pseudogap with increasing T is described by a broadening proportional to T-Tc, which is naturally explained by pairing correlations above Tc.

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Electron Self-Energy of High Temperature Superconductors as Revealed by Angle Resolved Photoemission

In this paper, we review some of the work our group has done in the past few years to obtain the electron self-energy of high temperature superconductors by analysis of angle-resolved photoemission data. We focus on three examples which have revealed: (1) a d-wave superconducting gap, (2) a collective mode in the superconducting state, and (3) pairing correlations in the pseudogap phase. In each case, although a novel result is obtained which captures the essense of the data, the conventional physics used leads to an incomplete picture. This indicates that new physics needs to be developed to obtain a proper understanding of these materials.

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Bosonic Mode Mixing in the Superconducting State Spectral Function of Bi_2Sr_2CaCu_2O_{8+delta}

Photoemission spectra of Bi_2Sr_2CaCu_2O_{8+delta} below T_c show two features near the (pi,0) point of the zone: a sharp peak at low energy and a higher binding energy hump. We find that the sharp peak persists at low energy even as one moves towards (0,0), while the broad hump shows significant dispersion which correlates well with the normal state dispersion. We argue that these features are naturally explained by the mixing of electrons with a bosonic mode which appears only below T_c, and speculate that the latter may be related to the resonance seen in recent neutron data.

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Evolution of the Fermi surface with carrier concentration in Bi_2Sr_2CaCu_2O_{8+δ}

We show, by use of angle-resolved photoemission spectroscopy, that underdoped Bi_2Sr_2CaCu_2O_{8+δ} appears to have a large Fermi surface centered at (π,π), even for samples with a T_c as low as 15 K. No clear evidence of a Fermi surface pocket around (π/2,π/2) has been found. These conclusions are based on a determination of the minimum gap locus in the pseudogap regime T_c < T < T^*, which is found to coincide with the locus of gapless excitations in momentum space (Fermi surface) determined above T^*. These results suggest that the pseudogap is more likely of precursor pairing rather than magnetic origin.

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ARPES Study of the Superconducting Gap Anisotropy in Bi_2Sr_2CaCu_2O_8+x

We report measurements of the momentum dependence of the superconducting gap in Bi_2Sr_2CaCu_2O_{8+x} (Bi2212) with angle-resolved photoemission spectroscopy using a dense sampling of the Brillouin zone in the vicinity of the Fermi surface. In the Y quadrant of the zone, where there are no complications from ghost bands caused by the superlattice, we find a gap function consistent within error bars to the form cos(k_x)-cos(k_y) expected for a d-wave order parameter. Similar results are found in the X quadrant with the photon polarization chosen to enhance main band emission over that due to ghost bands.

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Direct observation of particle-hole mixing in the superconducting state by angle-resolved photoemission

Particle-hole (p-h) mixing is a fundamental consequence of the existence of a pair condensate. We present direct experimental evidence for p-h mixing in the angle-resolved photoemission (ARPES) spectra in the superconducting state of Bi_2Sr_2CaCu_2O_{8+δ}. In addition to its pedagogical importance, this establishes unambiguously that the gap observed in ARPES is associated with superconductivity.

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