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J. D. Holt

Publications and source records attributed to J. D. Holt.

At least 109 records · Page 6Linked to original sources

Precision mass measurements of magnesium isotopes and implications on the validity of the Isobaric Mass Multiplet Equation

If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the Isobaric Mass Multiplet Equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of $^{29}$Cl and $^{30}$Ar. The atomic mass of $^{27}$Mg was found to be within 1.6$σ$ of the value stated in the Atomic Mass Evaluation. The atomic masses of $^{28,29}$Mg were measured to be both within 1$σ$, while being 8 and 34 times more precise, respectively. Using the $^{29}$Mg mass excess and previous measurements of $^{29}$Cl we uncovered a cubic coefficient of $d$ = 28(7) keV, which is the largest known cubic coefficient of the IMME. This departure, however, could also be caused by experimental data with unknown systematic errors. Hence there is a need to confirm the mass excess of $^{28}$S and the one-neutron separation energy of $^{29}$Cl, which have both come from a single measurement. Finally, our results were compared to ab initio calculations from the valence-space in-medium similarity renormalization group, resulting in a good agreement.

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Neutrinoless double-beta decay matrix elements in large shell-model spaces with the generator-coordinate method

We use the generator-coordinate method with realistic shell-model interactions to closely approximate full shell-model calculations of the matrix elements for the neutrinoless double-beta decay of $^{48}$Ca, $^{76}$Ge, and $^{82}$Se. We work in one major shell for the first isotope, in the $f_{5/2}pg_{9/2}$ space for the second and third, and finally in two major shells for all three. Our coordinates include not only the usual axial deformation parameter $β$, but also the triaxiality angle $γ$ and neutron-proton pairing amplitudes. In the smaller model spaces our matrix elements agree well with those of full shell-model diagonalization, suggesting that our Hamiltonian-based GCM captures most of the important valence-space correlations. In two major shells, where exact diagonalization is not currently possible, our matrix elements are only slightly different from those in a single shell.

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Saturation with chiral interactions and consequences for finite nuclei

We explore the impact of nuclear matter saturation on the properties and systematics of finite nuclei across the nuclear chart. Using the ab initio in-medium similarity renormalization group (IM-SRG), we study ground-state energies and charge radii of closed-shell nuclei from $^4$He to $^{78}$Ni, based on a set of low-resolution two- and three-nucleon interactions that predict realistic saturation properties. We first investigate in detail the convergence properties of these Hamiltonians with respect to model-space truncations for both two- and three-body interactions. We find one particular interaction that reproduces well the ground-state energies of all closed-shell nuclei studied. As expected from their saturation points relative to this interaction, the other Hamiltonians underbind nuclei, but lead to a remarkably similar systematics of ground-state energies. Extending our calculations to complete isotopic chains in the $sd$ and $pf$ shells with the valence-space IM-SRG, the same interaction reproduces not only experimental ground states but two-neutron-separation energies and first excited $2^+$ states. We also calculate radii with the valence-space IM-SRG for the first time. Since this particular interaction saturates at too high density, charge radii are still too small compared with experiment. Except for this underprediction, the radii systematics is, however, well reproduced. Our results highlight the importance of nuclear matter as a theoretical benchmark for the development of next-generation chiral interactions.

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Unexpected distribution of $\nu1f_{7/2}$ strength in the calcium isotopes at $N$=30

The calcium isotopes have emerged as an important testing ground for new microscopically derived shell-model interactions, and a great deal of focus has been directed toward this region. We investigate the relative spectroscopic strengths associated with $1f_{7/2}$ neutron hole states in $^{47, 49}$Ca following one-neutron knockout reactions from $^{48,50}$Ca. The observed reduction of strength populating the lowest 7/2$^{-}_{1}$ state in $^{49}$Ca, as compared to $^{47}$Ca, is consistent with the description given by shell-model calculations based on two- and three-nucleon forces in the neutron $pf$ model space, implying a fragmentation of the $l$=3 strength to higher-lying states. The experimental result is inconsistent with both the GXPF1 interaction routinely used in this region of the nuclear chart and with microscopic calculations in an extended model space including the $\nu1g_{9/2}$ orbital.

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Radii and binding energies in oxygen isotopes: a puzzle for nuclear forces

We present a systematic study of both nuclear radii and binding energies in (even) oxygen isotopes from the valley of stability to the neutron drip line. Both charge and matter radii are compared to state-of-the-art {\it ab initio} calculations along with binding energy systematics. Experimental matter radii are obtained through a complete evaluation of the available elastic proton scattering data of oxygen isotopes. We show that, in spite of a good reproduction of binding energies, {\it ab initio} calculations with conventional nuclear interactions derived within chiral effective field theory fail to provide a realistic description of charge and matter radii. A novel version of two- and three-nucleon forces leads to considerable improvement of the simultaneous description of the three observables for stable isotopes, but shows deficiencies for the most neutron-rich systems. Thus, crucial challenges related to the development of nuclear interactions remain.

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A nucleus-dependent valence-space approach to nuclear structure

We present a nucleus-dependent valence-space approach for calculating ground and excited states of nuclei, which generalizes the shell-model in-medium similarity renormalization group to an ensemble reference with fractionally filled orbitals. Because the ensemble is used only as a reference, and not to represent physical states, no symmetry restoration is required. This allows us to capture 3N forces among valence nucleons with a valence-space Hamiltonian specifically targeted to each nucleus of interest. Predicted ground-state energies from carbon through nickel agree with results of other large-space ab initio methods, generally to the 1\% level. In addition, we show that this new approach is required in order to obtain convergence for nuclei in the upper $p$ and $sd$ shells. Finally, we address the $1^+$/$3^+$ ground-state inversion problem in $^{22}\text{Na}$ and $^{46}\text{V}$. This approach extends the reach of ab initio nuclear structure calculations to essentially all light- and medium-mass nuclei.

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A Search for $0^+$ States in $^{50}$Cr: Implications for the Superallowed $β$-decay of $^{50}$Mn

A $^{52}$Cr$(p,t)$$^{50}$Cr two-neutron pickup reaction was performed using the Q3D magnetic spectrograph at the Maier-Leibnitz-Laboratorium in Garching, Germany. Excited states in $^{50}$Cr were observed up to an excitation energy of 5.3 MeV. Despite significantly increased sensitivity and resolution over previous work, no evidence of the previously assigned first excited $0^+$ state was found. As a result, the $0^+_2$ state is reassigned at an excitation energy of $E_x=3895.0(5)$ keV in $^{50}$Cr. This reassignment directly impacts direct searches for a non-analogue Fermi $β^+$ decay branch in $^{50}$Mn. These results also show better systematic agreement with the theoretical predictions for the $0^+$ state spectrum in $^{50}$Cr using the same formalism as the isospin-symmetry-breaking correction calculations for superallowed nuclei. The experimental data are also compared to $ab$-$initio$ shell-model predictions using the IM-SRG formalism based on $NN$ and $3N$ forces from chiral-EFT in the $pf$-shell for the first time.

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Ground and excited states of doubly open-shell nuclei from ab initio valence-space Hamiltonians

We present ab initio predictions for ground and excited states of doubly open-shell fluorine and neon isotopes based on chiral two- and three-nucleon interactions. We use the in-medium similarity renormalization group, in both flow-equation and Magnus formulations, to derive mass-dependent sd valence-space Hamiltonians. The experimental ground-state energies are reproduced through neutron number N=14, beyond which a new targeted normal-ordering procedure improves agreement with data and large-scale multi-reference calculations. For spectroscopy, we focus on neutron-rich 23-26F and 24-26Ne isotopes near N=14,16 magic numbers. In all cases we find an agreement with experiment competitive with established phenomenology. Moreover, yrast states are well described in 20Ne and 24Mg, providing an ab initio description of deformation in the medium-mass region.

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Unexpectedly large charge radii of neutron-rich calcium isotopes

Despite being a complex many-body system, the atomic nucleus exhibits simple structures for certain "magic" numbers of protons and neutrons. The calcium chain in particular is both unique and puzzling: evidence of doubly-magic features are known in 40,48Ca, and recently suggested in two radioactive isotopes, 52,54Ca. Although many properties of experimentally known Ca isotopes have been successfully described by nuclear theory, it is still a challenge to predict their charge radii evolution. Here we present the first measurements of the charge radii of 49,51,52Ca, obtained from laser spectroscopy experiments at ISOLDE, CERN. The experimental results are complemented by state-of-the-art theoretical calculations. The large and unexpected increase of the size of the neutron-rich calcium isotopes beyond N = 28 challenges the doubly-magic nature of 52Ca and opens new intriguing questions on the evolution of nuclear sizes away from stability, which are of importance for our understanding of neutron-rich atomic nuclei.

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Non-observable nature of the nuclear shell structure. Meaning, illustrations and consequences

The concept of single-nucleon shells constitutes a basic pillar of our understanding of nuclear structure. Effective single-particle energies (ESPEs) introduced by French and Baranger represent the most appropriate tool to relate many-body observables to a single-nucleon shell structure. As briefly discussed in [T. Duguet, G. Hagen, Phys. Rev. C {\bf 85}, 034330 (2012)], the dependence of ESPEs on one-nucleon transfer probability matrices makes them purely theoretical quantities that "run" with the non-observable resolution scale $λ$ employed in the calculation. Given that ESPEs provide a way to interpret the many-body problem in terms of simpler theoretical ingredients, the goal is to specify the terms, i.e. the exact sense and conditions, in which this interpretation can be conducted meaningfully. State-of-the-art multi-reference in-medium similarity renormalization group and self-consistent Gorkov Green's function many-body calculations are employed to corroborate the formal analysis. This is done by comparing the behavior of several observables and of non-observable ESPEs (and spectroscopic factors) under (quasi) unitary similarity renormalization group transformations of the Hamiltonian parameterized by the resolution scale $λ$. The non-observable nature of the nuclear shell structure, i.e. the fact that it constitutes an intrinsically theoretical object with no counterpart in the empirical world, must be recognized and assimilated. Eventually, practitioners can refer to nuclear shells and spectroscopic factors in their analyses of nuclear phenomena if, and only if, they use consistent structure and reaction theoretical schemes based on a fixed resolution scale they have agreed on prior to performing their analysis and comparisons.

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Nuclear forces and their impact on neutron-rich nuclei and neutron-rich matter

We review the impact of nuclear forces on matter at neutron-rich extremes. Recent results have shown that neutron-rich nuclei become increasingly sensitive to three-nucleon forces, which are at the forefront of theoretical developments based on effective field theories of quantum chromodynamics. This includes the formation of shell structure, the spectroscopy of exotic nuclei, and the location of the neutron dripline. Nuclear forces also constrain the properties of neutron-rich matter, including the neutron skin, the symmetry energy, and the structure of neutron stars. We first review our understanding of three-nucleon forces and show how chiral effective field theory makes unique predictions for many-body forces. Then, we survey results with three-nucleon forces in neutron-rich oxygen and calcium isotopes and neutron-rich matter, which have been explored with a range of many-body methods. Three-nucleon forces therefore provide an exciting link between theoretical, experimental and observational nuclear physics frontiers.

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Exploring sd-shell nuclei from two- and three-nucleon interactions with realistic saturation properties

We study ground- and excited-state properties of all sd-shell nuclei with neutron and proton numbers 8 <= N,Z <= 20, based on a set of low-resolution two- and three-nucleon interactions that predict realistic saturation properties of nuclear matter. We focus on estimating the theoretical uncertainties due to variation of the resolution scale, the low-energy couplings, as well as from the many-body method. The experimental two-neutron and two-proton separation energies are reasonably well reproduced, with an uncertainty range of about 5 MeV. The first excited 2+ energies also show overall agreement, with a more narrow uncertainty range of about 500 keV. In most cases, this range is dominated by the uncertainties in the Hamiltonian.

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Ground-State Electromagnetic Moments of Calcium Isotopes

High-resolution bunched-beam collinear laser spectroscopy was used to measure the optical hyperfine spectra of the $^{43-51}$Ca isotopes. The ground state magnetic moments of $^{49,51}$Ca and quadrupole moments of $^{47,49,51}$Ca were measured for the first time, and the $^{51}$Ca ground state spin $I=3/2$ was determined in a model-independent way. Our results provide a critical test of modern nuclear theories based on shell-model calculations using phenomenological as well as microscopic interactions. The results for the neutron-rich isotopes are in excellent agreement with predictions using interactions derived from chiral effective field theory including three-nucleon forces, while lighter isotopes illustrate the presence of particle-hole excitations of the $^{40}$Ca core in their ground state.

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Nuclear structure studies of $^{24}$F

The structure of the $^{24}$F nucleus has been studied at GANIL using the $β$ decay of $^{24}$O and the in-beam $γ$-ray spectroscopy from the fragmentation of projectile nuclei. Combining these complementary experimental techniques, the level scheme of $^{24}$F has been constructed up to 3.6 Mev by means of particle-$γ$ and particle-$γγ$ coincidence relations. Experimental results are compared to shell-model calculations using the standard USDA and USDB interactions as well as ab-initio valence-space Hamiltonians calculated from the in-medium similarity renormalization group based on chiral two- and three-nucleon forces. Both methods reproduce the measured level spacings well, and this close agreement allows unidentified spins and parities to be consistently assigned.

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Nonperturbative shell-model interactions from the in-medium similarity renormalization group

We present the first ab initio construction of valence-space Hamiltonians for medium-mass nuclei based on chiral two- and three-nucleon interactions using the in-medium similarity renormalization group. When applied to the oxygen isotopes, we find experimental ground-state energies are well reproduced, including the flat trend beyond the drip line at 24O. Similarly, natural-parity spectra in 21,22,23,24O are in agreement with experiment, and we present predictions for excited states in 25,26O. The results exhibit a weak dependence on the harmonic-oscillator basis parameter and reproduce spectroscopy within the standard sd valence space.

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Breakdown of the Isobaric Multiplet Mass Equation for the A = 20 and 21 Multiplets

Using the Penning trap mass spectrometer TITAN, we performed the first direct mass measurements of 20,21Mg, isotopes that are the most proton-rich members of the A = 20 and A = 21 isospin multiplets. These measurements were possible through the use of a unique ion-guide laser ion source, a development that suppressed isobaric contamination by six orders of magnitude. Compared to the latest atomic mass evaluation, we find that the mass of 21Mg is in good agreement but that the mass of 20Mg deviates by 3σ. These measurements reduce the uncertainties in the masses of 20,21Mg by 15 and 22 times, respectively, resulting in a significant departure from the expected behavior of the isobaric multiplet mass equation in both the A = 20 and A = 21 multiplets. This presents a challenge to shell model calculations using either the isospin non-conserving USDA/B Hamiltonians or isospin non-conserving interactions based on chiral two- and three-nucleon forces.

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Three-nucleon forces and spectroscopy of neutron-rich calcium isotopes

We study excited-state properties of neutron-rich calcium isotopes based on chiral two- and three-nucleon interactions. We first discuss the details of our many-body framework, investigate convergence properties, and for two-nucleon interactions benchmark against coupled-cluster calculations. We then focus on the spectroscopy of 47-56Ca, finding that with both 3N forces and an extended pfg9/2 valence space, we obtain a good level of agreement with experiment. We also study electromagnetic transitions and find that experimental data are well described by our calculations. In addition, we provide predictions for unexplored properties of neutron-rich calcium isotopes.

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Beyond the Neutron Drip-Line: The Unbound Oxygen Isotopes 25O and 26O

The very neutron-rich oxygen isotopes 25O and 26O are investigated experimentally and theoret- ically. In this first R3B-LAND experiment, the unbound states are populated at GSI via proton- knockout reactions from 26F and 27F at relativistic energies around 450 MeV/nucleon. From the kinematically complete measurement of the decay into 24O plus one or two neutrons, the 25O ground- state energy and lifetime are determined, and upper limits for the 26O ground state are extracted. In addition, the results provide evidence for an excited state in 26O at around 4 MeV. The ex- perimental findings are compared to theoretical shell-model calculations based on chiral two- and three-nucleon (3N) forces, including for the first time residual 3N forces, which are shown to be amplified as valence neutrons are added.

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