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J. Dilling

Publications and source records attributed to J. Dilling.

At least 73 records · Page 4Linked to original sources

Unexpected distribution of $\nu1f_{7/2}$ strength in the calcium isotopes at $N$=30

The calcium isotopes have emerged as an important testing ground for new microscopically derived shell-model interactions, and a great deal of focus has been directed toward this region. We investigate the relative spectroscopic strengths associated with $1f_{7/2}$ neutron hole states in $^{47, 49}$Ca following one-neutron knockout reactions from $^{48,50}$Ca. The observed reduction of strength populating the lowest 7/2$^{-}_{1}$ state in $^{49}$Ca, as compared to $^{47}$Ca, is consistent with the description given by shell-model calculations based on two- and three-nucleon forces in the neutron $pf$ model space, implying a fragmentation of the $l$=3 strength to higher-lying states. The experimental result is inconsistent with both the GXPF1 interaction routinely used in this region of the nuclear chart and with microscopic calculations in an extended model space including the $\nu1g_{9/2}$ orbital.

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Cosmogenic Backgrounds to 0νββ in EXO-200

As neutrinoless double-beta decay experiments become more sensitive and intrinsic radioactivity in detector materials is reduced, previously minor contributions to the background must be understood and eliminated. With this in mind, cosmogenic backgrounds have been studied with the EXO-200 experiment. Using the EXO-200 TPC, the muon flux (through a flat horizontal surface) underground at the Waste Isolation Pilot Plant (WIPP) has been measured to be Φ = 4.07 $\pm$ 0.14 (sys) $\pm$ 0.03 (stat) $\times$ $10^{-7}$cm$^{-2}$ s$^{-1}$, with a vertical intensity of $I_{v}$ = 2.97$^{+0.14}_{-0.13}$ (sys) $\pm$ 0.02 (stat) $\times$ $10^{-7}$cm$^{-2}$ s$^{-1}$ sr$^{-1}$. Simulations of muon-induced backgrounds identified several potential cosmogenic radionuclides, though only 137Xe is a significant background for the 136Xe 0νββ search with EXO-200. Muon-induced neutron backgrounds were measured using γ-rays from neutron capture on the detector materials. This provided a measurement of 137Xe yield, and a test of the accuracy of the neutron production and transport simulations. The independently measured rates of 136Xe neutron capture and of 137Xe decay agree within uncertainties. Geant4 and FLUKA simulations were performed to estimate neutron capture rates, and these estimates agreed to within ~40% or better with measurements. The ability to identify 136Xe(n,γ) events will allow for rejection of 137Xe backgrounds in future 0νββ analyses.

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First Search for Lorentz and CPT Violation in Double Beta Decay with EXO-200

A search for Lorentz- and CPT-violating signals in the double beta decay spectrum of $^{136}$Xe has been performed using an exposure of 100 kg$\cdot$yr with the EXO-200 detector. No significant evidence of the spectral modification due to isotropic Lorentz-violation was found, and a two-sided limit of $-2.65 \times 10^{-5 } \; \textrm{GeV} < \mathring{a}^{(3)}_{\text{of}} < 7.60 \times 10^{-6} \; \textrm{GeV}$ (90% C.L.) is placed on the relevant coefficient within the Standard-Model Extension (SME). This is the first experimental study of the effect of the SME-defined oscillation-free and momentum-independent neutrino coupling operator on the double beta decay process.

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Mass measurements of neutron-rich Rb and Sr isotopes

We report on the mass measurements of several neutron-rich $\mathrm{Rb}$ and $\mathrm{Sr}$ isotopes in the $A \approx 100$ region with the TITAN Penning-trap mass spectrometer. Using highly charged ions in the charge state $q=10+$, the masses of $^{98,99}\mathrm{Rb}$ and $^{98-100}\mathrm{Sr}$ have been determined with a precision of $6 - 12\ \mathrm{keV}$, making their uncertainty negligible for r-process nucleosynthesis network calculations. The mass of $^{101}\mathrm{Sr}$ has been determined directly for the first time with a precision eight times higher than the previous indirect measurement and a deviation of $3σ$ when compared to the Atomic Mass Evaluation. We also confirm the mass of $^{100}\mathrm{Rb}$ from a previous measurement. Furthermore, our data indicates the existance of a low-lying isomer with $80\ \mathrm{keV}$ excitation energy in $^{98}\mathrm{Rb}$. We show that our updated mass values lead to minor changes in the r-process by calculating fractional abundances in the $A\approx 100$ region of the nuclear chart.

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Low-Background In-Trap Decay Spectroscopy with TITAN at TRIUMF

An in-trap decay spectroscopy setup has been developed and constructed for use with the TITAN facility at TRIUMF. The goal of this device is to observe weak electron-capture (EC) branching ratios for the odd-odd intermediate nuclei in the $ββ$ decay process. This apparatus consists of an up-to 6 Tesla, open-access spectroscopy ion-trap, surrounded radially by up to 7 planar Si(Li) detectors which are separated from the trap by thin Be windows. This configuration provides a significant increase in sensitivity for the detection of low-energy photons by providing backing-free ion storage and eliminating charged-particle-induced backgrounds. An intense electron beam is also employed to increase the charge-states of the trapped ions, thus providing storage times on the order of minutes, allowing for decay-spectroscopy measurements. The technique of multiple ion-bunch stacking was also recently demonstrated, which further extends the measurement possibilities of this apparatus. The current status of the facility and initial results from a $^{116}$In measurement are presented.

physics.ins-det↗

The TITAN in-trap decay spectroscopy facility at TRIUMF

This article presents an upgraded in-trap decay spectroscopy apparatus which has been developed and constructed for use with TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This device consists of an open-access electron-beam ion-trap (EBIT), which is surrounded radially by seven low-energy planar Si(Li) detectors. The environment of the EBIT allows for the detection of low-energy photons by providing backing-free storage of the radioactive ions, while guiding charged decay particles away from the trap centre via the strong (up to 6 T) magnetic field. In addition to excellent ion confinement and storage, the EBIT also provides a venue for performing decay spectroscopy on highly-charged radioactive ions. Recent technical advancements have been able to provide a significant increase in sensitivity for low-energy photon detection, towards the goal of measuring weak electron-capture branching ratios of the intermediate nuclei in the two-neutrino double beta ($2νββ$) decay process. The design, development, and commissioning of this apparatus are presented together with the main physics objectives. The future of the device and experimental technique are discussed.

physics.ins-det↗

Sensitivity Increases for the TITAN Decay Spectroscopy Program

The TITAN facility at TRIUMF has recently initiated a program of performing decay spectroscopy measurements in an electron-beam ion-trap (EBIT). The unique environment of the EBIT provides backing-free storage of the radioactive ions, while guiding charged decay particles from the trap centre via the strong magnetic field. This measurement technique is able to provide a significant increase in detection sensitivity for photons which result from radioactive decay. A brief overview of this device is presented, along with methods of improving the signal-to-background ratio for photon detection by reducing Compton scattered events, and eliminating vibrational noise.

physics.ins-det↗

Spectroscopy of Ba and Ba$^+$ deposits in solid xenon for barium tagging in nEXO

Progress on a method of barium tagging for the nEXO double beta decay experiment is reported. Absorption and emission spectra for deposits of barium atoms and ions in solid xenon matrices are presented. Excitation spectra for prominent emission lines, temperature dependence and bleaching of the fluorescence reveal the existence of different matrix sites. A regular series of sharp lines observed in Ba$^+$ deposits is identified with some type of barium hydride molecule. Lower limits for the fluorescence quantum efficiency of the principal Ba emission transition are reported. Under current conditions, an image of $\le10^4$ Ba atoms can be obtained. Prospects for imaging single Ba atoms in solid xenon are discussed.

physics.atom-ph↗

Breakdown of the Isobaric Multiplet Mass Equation for the A = 20 and 21 Multiplets

Using the Penning trap mass spectrometer TITAN, we performed the first direct mass measurements of 20,21Mg, isotopes that are the most proton-rich members of the A = 20 and A = 21 isospin multiplets. These measurements were possible through the use of a unique ion-guide laser ion source, a development that suppressed isobaric contamination by six orders of magnitude. Compared to the latest atomic mass evaluation, we find that the mass of 21Mg is in good agreement but that the mass of 20Mg deviates by 3σ. These measurements reduce the uncertainties in the masses of 20,21Mg by 15 and 22 times, respectively, resulting in a significant departure from the expected behavior of the isobaric multiplet mass equation in both the A = 20 and A = 21 multiplets. This presents a challenge to shell model calculations using either the isospin non-conserving USDA/B Hamiltonians or isospin non-conserving interactions based on chiral two- and three-nucleon forces.

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Trapped-ion decay spectroscopy towards the determination of ground-state components of double-beta decay matrix elements

A new technique has been developed at TRIUMF's TITAN facility to perform in-trap decay spectroscopy. The aim of this technique is to eventually measure weak electron capture branching ratios (ECBRs) and by this to consequently determine GT matrix elements of $ββ$ decaying nuclei. These branching ratios provide important input to the theoretical description of these decays. The feasibility and power of the technique is demonstrated by measuring the ECBR of $^{124}$Cs.

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Extinction of the N=20 neutron-shell closure for 32Mg examined by direct mass measurements

The 'island of inversion' around $^{32}$Mg is one of the most important paradigm for studying the disappearance of the stabilizing 'magic' of a shell closure. We present the first Penning-trap mass measurements of the exotic nuclides $^{29-31}$Na and $^{30-34}$Mg, which allow a precise determination of the empirical shell gap for $^{32}$Mg. The new value of 1.10(3) MeV is the lowest observed shell gap for any nuclide with a canonical magic number.

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New determination of double-beta-decay properties in 48Ca: high-precision Q-value measurement and improved nuclear matrix element calculations

We report a direct measurement of the Q-value of the neutrinoless double-beta-decay candidate 48Ca at the TITAN Penning-trap mass spectrometer, with the result that Q = 4267.98(32) keV. We measured the masses of both the mother and daughter nuclides, and in the latter case found a 1 keV deviation from the literature value. In addition to the Q-value, we also present results of a new calculation of the neutrinoless double-beta-decay nuclear matrix element of 48Ca. Using diagrammatic many-body perturbation theory to second order to account for physics outside the valence space, we constructed an effective shell-model double-beta-decay operator, which increased the nuclear matrix element by about 75% compared with that produced by the bare operator. The new Q-value and matrix element strengthen the case for a 48Ca double-beta-decay experiment.

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Penning-trap mass spectrometry of highly charged, neutron-rich Rb and Sr isotopes in the vicinity of $A\approx100$

The neutron-rich mass region around $A\approx100$ presents challenges for modeling the astrophysical $r$-process because of rapid shape transitions. We report on mass measurements using the TITAN Penning trap at TRIUMF-ISAC to attain more reliable theoretical predictions of $r$-process nucleosynthesis paths in this region. A new approach using highly charged ($q=15+$) ions has been applied which considerably saves measurement time and preserves accuracy. New mass measurements of neutron-rich $^{94,97,98}$Rb and $^{94,97-99}$Sr have uncertainties of less than 4 keV and show deviations of up to 11$σ$ to previous measurements. An analysis using a parameterized $r$-process model is performed and shows that mass uncertainties for the A=90 abundance region are eliminated.

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Elucidation of the anomalous A = 9 isospin quartet behaviour

Recent high-precision mass measurements of $^{9}$Li and $^{9}$Be, performed with the TITAN Penning trap at the TRIUMF ISAC facility, are analyzed in light of state-of-the-art shell model calculations. We find an explanation for the anomalous Isobaric Mass Multiplet Equation (IMME) behaviour for the two $A$ = 9 quartets. The presence of a cubic $d$ = 6.3(17) keV term for the $J^π$ = 3/2$^{-}$ quartet and the vanishing cubic term for the excited $J^π$ = 1/2$^{-}$ multiplet depend upon the presence of a nearby $T$ = 1/2 state in $^{9}$B and $^{9}$Be that induces isospin mixing. This is contrary to previous hypotheses involving purely Coulomb and charge-dependent effects. $T$ = 1/2 states have been observed near the calculated energy, above the $T$ = 3/2 state. However an experimental confirmation of their $J^π$ is needed.

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New precision mass measurements of neutron-rich calcium and potassium isotopes and three-nucleon forces

We present precision Penning-trap mass measurements of neutron-rich calcium and potassium isotopes in the vicinity of neutron number N=32. Using the TITAN system the mass of $^{51}$K was measured for the first time, and the precision of the $^{51,52}$Ca mass values were improved significantly. The new mass values show a dramatic increase of the binding energy compared to those reported in the atomic mass evaluation. In particular, $^{52}$Ca is more bound by 1.74 MeV, and the behavior with neutron number deviates substantially from the tabulated values. An increased binding was predicted recently based on calculations that include three-nucleon (3N) forces. We present a comparison to improved calculations, which agree remarkably with the evolution of masses with neutron number, making neutron-rich calcium isotopes an exciting region to probe 3N forces at neutron-rich extremes.

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TITAN's Digital RFQ Ion Beam Cooler and Buncher, Operation and Performance

We present a description of the Radio Frequency Quadrupole (RFQ) ion trap built as part of the TITAN facility. It consists of a gas-filled, segmented, linear Paul trap and is the first stage of the TITAN setup with the purpose of cooling and bunching radioactive ion beams delivered from ISAC-TRIUMF. This is the first such device to be driven digitally, i.e., using a high voltage ($V_{pp} = \rm{400 \, V}$), wide bandwidth ($0.2 < f < 1.2 \, \rm{MHz}$) square-wave as compared to the typical sinusoidal wave form. Results from the commissioning of the device as well as systematic studies with stable and radioactive ions are presented including efficiency measurements with stable $^{133}$Cs and radioactive $^{124, 126}$Cs. A novel and unique mode of operation of this device is also demonstrated where the cooled ion bunches are extracted in reverse mode, i.e., in the same direction as previously injected.

physics.acc-ph↗

Highly charged ions in Penning traps, a new tool for resolving low lying isomeric states

The use of highly charged ions increases the precision and resolving power, in particular for short-lived species produced at on-line radio-isotope beam facilities, achievable with Penning trap mass spectrometers. This increase in resolving power provides a new and unique access to resolving low-lying long-lived ($T_{1/2} > 50$ ms) nuclear isomers. Recently, the $111.19(22)$ keV (determined from $γ$-ray spectroscopy) isomeric state in $^{78}$Rb has been resolved from the ground state, in a charge state of $q=8+$ with the TITAN Penning trap at the TRIUMF-ISAC facility. The excitation energy of the isomer was measured to be $108.7(6.4)$ keV above the ground state. The extracted masses for both the ground and isomeric states, and their difference, agree with the AME2003 and Nuclear Data Sheet values. This proof of principle measurement demonstrates the feasibility of using Penning trap mass spectrometers coupled to charge breeders to study nuclear isomers and opens a new route for isomer searches.

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Penning-Trap Mass Measurements of the Neutron-Rich K and Ca Isotopes: Resurgence of the N = 28 Shell Strength

We present Penning-trap mass measurements of neutron-rich 44,47-50K and 49,50Ca isotopes carried out at the TITAN facility at TRIUMF-ISAC. The 44K mass measurement was performed with a charge-bred 4+ ion utilizing the TITAN EBIT, and agrees with the literature. The mass excesses obtained for 47K and 49,50Ca are more precise and agree with the values published in the 2003 Atomic Mass Evaluation (AME'03). The 48,49,50K mass excesses are more precise than the AME'03 values by more than one order of magnitude. For 48,49K, we find deviations by 7 sigma and 10 sigma, respectively. The new 49K mass excess lowers significantly the two-neutron separation energy at the neutron number N=30 compared with the separation energy calculated from the AME'03 mass-excess values, and thus, increases the N=28 neutron-shell gap energy at Z=19 by approximately 1 MeV.

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