arXiv subjects

J. Dudouet

Publications and source records attributed to J. Dudouet.

At least 19 recordsLinked to original sources

arXiv2026

Lifetime measurements in neutron-rich odd-A yttrium isotopes ($^{93-99}$Y): Investigation of shape coexistence and the intertwined quantum phase transition

Lifetimes of 16 excited states in the neutron-rich odd-$A$ nuclei $^{93-99}$Y were measured using fast-timing $\gamma$-$\gamma$ coincidence spectroscopy with fast scintillation detectors at the LOHENGRIN recoil separator. Particular attention is given to the region around $N \approx 59$, where rapid changes in nuclear deformation and shape coexistence occur. The lifetimes, determined using the generalized centroid difference method, are compared with interacting boson-fermion model calculations with configuration mixing, in which the odd-$A$ yttrium isotopes are described as a proton coupled to a bosonic core containing normal and intruder configurations. The results provide new constraints on theoretical descriptions of shape coexistence and structural evolution in neutron-rich nuclei near $A \approx 100$, particularly for odd-$A$ systems where experimental information remains limited.

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arXiv2026

First observation of multi-phonon $\gamma$-vibrations in an odd-odd nuclear system

The identification of the first multi-phonon $\gamma$-vibrational bands in an odd-odd neutron-rich nucleus of the nuclear chart is presented. These high spin structures of hard to access $^{104}_{41}$Nb$_{63}$, produced in fission, were studied by combining a spectrometer with isotopic resolution coupled to a $\gamma$-ray tracking array and independently high-fold $\gamma$ coincidence measurements. Triaxial Projected Shell Model calculations for the high-spin states are in good agreement with the measured observables for the yrast, one-phonon and two-phonon $\gamma$ bands. The possibility of an oblate shape of an isomeric state and coexistence of triaxial and oblate configurations are investigated from the decay of the 141 keV isomer. The present work illustrates the robustness of vibration excitations in the presence of odd valence proton and neutron as well as the possibly coexisting shapes beyond the $N=60$ transitional region.

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arXiv2026

Direct transfer to $^{46,48}$K as a survey of the $\pi(s_{1/2})$$-\nu(sdpf)$ interaction

The collapse of the canonical $N=28$ magic number in nuclei with $Z<20$ has drawn significant interest as it relates to the emergence of an island of inversion centered on $^{42}$Si and $^{44}$S. In particular, interactions between the $\pi s_{1/2}$ orbital -- empty in $^{42}$Si and full in $^{44}$S -- and the neutron orbitals just above and below the $N=28$ gap are expected to be critical in this region, but remain relatively unexplored. In this paper, we expand upon the results of our previous study of the direct transfer reaction $^{47}$K(d,p$\gamma$)$^{48}$K [C.\,J.~Paxman \textit{et al.}, Phys. Rev. Lett. 134, 162504 (2025)] with the results of the complementary $^{47}$K(d,t$\gamma$)$^{46}$K reaction. Through this study, we present a comprehensive scan of the interaction between the critical $\pi s_{1/2}$ orbital and a broad range of neutron orbitals spanning nearly two full shells. We identify several discrepancies between the experimental results and state-of-the-art shell model calculations, which suggest a deficiency of the shell model to fully capture the complex proton configuration mixing in this region, highlighting a significant challenge for single-particle descriptions of the island of inversion.

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arXiv2025

Fusion of 12C+28Si at deep sub-barrier energies

The existence of fusion hindrance is not well established in light heavy-ion systems. Studying slightly heavier cases allows extrapolating the trend to light systems of astrophysical interest. Fusion of 12C + 28Si has been measured down to deep sub-barrier energies, using 28Si beams from the XTU Tandem accelerator of LNL on thin 12C targets. The fusion-evaporation residues were detected by a detector telescope following an electrostatic beam separator, and coincidences between the gamma-ray array AGATA and segmented silicon detectors DSSD were performed, where the evaporated light charged particles were identified by pulse shape analysis. Fusion cross sections have been obtained in the wide range 150 mb-42 nb. Coupled-channel (CC) calculations using a Woods-Saxon potential reproduce the data above 0.1 mb. Below that, hindrance shows up and the CC results overestimate the cross sections which get close to the one-dimensional potential tunnelling limit. This suggests that the coupling strengths gradually vanish, as predicted by the adiabatic model. The hindrance threshold follows a recently updated phenomenological systematics.

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arXiv2025

Shape evolution in neutron-rich odd-even $^{105-109}$Nb isotopes

Neutron-rich nuclei around $Z\sim40$ exhibit multiple shape transitions. This region shows one of the sharpest transitions in the nuclear chart, from a spherical vibrator at $N=58$ to a strongly deformed prolate shape at $N=60$, with largest deformations seen for $_{38}$Sr and $_{40}$Zr. Below $Z=36$, a spherical-to-oblate transition is predicted, while above $Z=42$ and $N\ge60$, the shape evolves from axial to triaxial. Even-$Z$ nuclei have been well studied, but odd-$Z$ isotopes such as Nb offer additional insights into these mechanisms. The Nb isotopes lie at the boundary between axially deformed Zr and triaxially deformed Mo nuclei. This work explores the structure of neutron-rich Nb nuclei up to $N=68$, aiming to understand shape evolution with isospin and the onset of triaxiality. Two complementary fission experiments were used: (i) $^{238}$U+$^9$Be at GANIL in inverse kinematics with AGATA, EXOGAM, and VAMOS++, allowing prompt and delayed $\gamma$-ray spectroscopy with isotopic identification; (ii) spontaneous fission of $^{252}$Cf with the Gammasphere array providing high-fold $\gamma$-coincidence data. The level scheme of $^{105}$Nb was significantly extended with two new negative-parity bands. A revised scheme is proposed for $^{107}$Nb, differing from previous results, and new structures are reported in $^{109}$Nb. The signature splitting analysis indicates triaxial deformation for positive-parity bands, while negative-parity bands show axial symmetry, similar to Zr. This reveals a shape coexistence in neutron-rich Nb nuclei.

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arXiv2024

Shape evolution in even-mass $^{98-104}$Zr isotopes via lifetime measurements using the $\gamma\gamma$-coincidence technique

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $\gamma\gamma$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $\gamma\gamma$-coincidence and $\gamma$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

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arXiv2024

Probing exotic cross-shell interactions at N=28 with single-neutron transfer on 47K

We present the first measurement of the $^{47}$K($d,p\gamma$)$^{48}$K transfer reaction, performed in inverse kinematics using a reaccelerated beam of $^{47}$K. The level scheme of $^{48}$K has been greatly extended with nine new bound excited states identified and spectroscopic factors deduced. Detailed comparisons with SDPF-U and SDPF-MU shell-model calculations reveal a number of discrepancies with these results, and a preference for SDPF-MU is found. Intriguingly, an apparent systematic overestimation of spectroscopic factors and a poor reproduction of the energies for 1$^-$ states suggests that the mixing between the $\pi s^{\,\,\,1}_{1/2} d^{\,\,\,4}_{3/2}$ and $\pi s^{\,\,\,2}_{1/2} d^{\,\,\,3}_{3/2}$ proton configurations in $^{48}$K is not correctly described using current interactions, challenging our descriptions of light $N=28$ nuclei.

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arXiv2024

High-resolution spectroscopy of neutron-rich Br isotopes and signatures for a prolate-to-oblate shape transition at N=56

The first systematic experimental study of the neutron-rich Br isotopes with two complementary state-of-the-art techniques is presented. These isotopes have been populated in the fission process at two different facilities, GANIL and ILL. New spectroscopic information has been obtained for odd-even $^{87-93}$Br isotopes and the experimental results have been compared with state-of-the-art Large-Scale Shell-Model and DNO Shell-Model calculations. As a result of such theoretical approaches, a transition from prolate ($^{87,89}$Br) to oblate ($^{91,93}$Br) shapes is obtained from the subtle balance between proton and neutron quadrupole deformations, as a clear signature of pseudo-SU3 quadrupole regime.

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arXiv2024

High-precision spectroscopy of $^{20}$O benchmarking ab-initio calculations in light nuclei

The excited states of unstable $^{20}$O were investigated via $\gamma$-ray spectroscopy following the $^{19}$O$(d,p)^{20}$O reaction at 8 $A$MeV. By exploiting the Doppler Shift Attenuation Method, the lifetime of the 2$^+_2$ and 3$^+_1$ states were firmly established. From the $\gamma$-ray branching and E2/M1 mixing ratios for transitions deexciting the 2$^+_2$ and 3$^+_1$ states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of $\gamma$-ray transition probabilities with the valence space in medium similarity renormalization group ab-initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab-initio approaches using chiral EFT forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab-initio models.

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arXiv2024

Bayesian uncertainty quantification on nuclear level density data and their impact on $(p,\gamma)$ reactions of astrophysical interest

The $p$ process nucleosynthesis is responsible for the synthesis of 35 neutron-deficient nuclei from $^{35}$Se to $^{196}$Hg. An important input that can affect the modeling of this process is the nuclear level density at the relevant excitation energies of the nuclei involved in the reaction network. The OSLO method has been extensively used for the measurement of level densities in excitation energies of several MeV. In this work, Bayesian optimization has been used in order to estimate the 95% high density intervals for the parameters of two level density models optimized on the OSLO data. These uncertainties are then propagated on the cross sections of $(p,\gamma)$ reactions leading to the compound nuclei $^{105,106}$Pd and $^{105,106}$Cd inside the astrophysically relevant energy range. Imposing constraints in this region of the isotopic chart is important for network calculations involving the nearby $p$ nuclei $^{102}$Pd and $^{106}$Cd. We discuss the reduction of the range of cross sections due to the uncertainties arising from the level density data compared to the range of the six default level density models available in TALYS and we highlight the need for level density data inside the astrophysically relevant energy ranges.

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arXiv2023

Particle Identification at VAMOS++ with Machine Learning Techniques

Multi-nucleon transfer reaction between 136Xe beam and 198Pt target was performed using the VAMOS++ spectrometer at GANIL to study the structure of n-rich nuclei around N=126. Unambiguous charge state identification was obtained by combining two supervised machine learning methods, deep neural network (DNN) and positional correction using a gradient-boosting decision tree (GBDT). The new method reduced the complexity of the kinetic energy calibration and outperformed the conventional method, improving the charge state resolution by 8%

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arXiv2023

Advancements of $\gamma$-ray spectroscopy of isotopically identified fission fragments with AGATA and VAMOS++

$\gamma$-ray spectroscopy of fission fragments is a powerful method for studies of nuclear structure properties. Recent results on the spectroscopy of fission fragments, using the combination of the AGATA $\gamma$-ray tracking array and the VAMOS++ large acceptance magnetic spectrometer at GANIL, are reported. A comparison of the performance of the large germanium detector arrays EXOGAM and AGATA illustrates the advances in $\gamma$-ray spectroscopy of fission fragments. Selected results are highlighted for prompt $\gamma$-ray spectroscopy studies, measurements of short lifetimes of excited states with the Recoil Distance Doppler-Shift method, using both AGATA and VAMOS++ and prompt-delayed $\gamma$-ray spectroscopy studies using AGATA, VAMOS++ and EXOGAM.

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arXiv2023

AGATA: Advancements in Software Developments

Presently, gamma-ray tracking in germanium segmented detectors is realised by applying two advanced, complex algorithms. While they have already triggered an intensive R&D, they are still subject to further improvements. Making such algorithms effective, online in real time conditions and/or offline for deeper analysis, in data pipelines do require many additional software developments. This review paper gives an overview of the various bricks of software produced so far by the AGATA collaboration. It provides hints of what is foreseen for the next phases of the project up to its full configuration namely with 180 capsules in the array.

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arXiv2022

Search for $^{22}$Na in novae supported by a novel method for measuring femtosecond nuclear lifetimes

Classical novae are thermonuclear explosions in stellar binary systems, and important sources of $^{26}$Al and $^{22}$Na. While gamma rays from the decay of the former radioisotope have been observed throughout the Galaxy, $^{22}$Na remains untraceable. The half-life of $^{22}$Na (2.6 yr) would allow the observation of its 1.275 MeV gamma-ray line from a cosmic source. However, the prediction of such an observation requires good knowledge of the nuclear reactions involved in the production and destruction of this nucleus. The $^{22}$Na($p,\gamma$)$^{23}$Mg reaction remains the only source of large uncertainty about the amount of $^{22}$Na ejected. Its rate is dominated by a single resonance on the short-lived state at 7785.0(7) keV in $^{23}$Mg. In the present work, a combined analysis of particle-particle correlations and velocity-difference profiles is proposed to measure femtosecond nuclear lifetimes. The application of this novel method to the study of the $^{23}$Mg states, combining magnetic and highly-segmented tracking gamma-ray spectrometers, places strong limits on the amount of $^{22}$Na produced in novae, explains its non-observation to date in gamma rays (flux < 2.5x$10^{-4}$ ph/(cm$^2$s)), and constrains its detectability with future space-borne observatories.

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arXiv2022

$^{178}$Hg and asymmetric fission of neutron-deficient pre-actinides

Fission at low excitation energy is an ideal playground to probe the impact of nuclear structure on nuclear dynamics. While the importance of structural effects in the nascent fragments is well-established in the (trans-)actinide region, the observation of asymmetric fission in several neutron-deficient pre-actinides can be explained by various mechanisms. To deepen our insight into that puzzle, an innovative approach based on inverse kinematics and an enhanced version of the VAMOS++ heavy-ion spectrometer was implemented at the GANIL facility, Caen. Fission of $^{178}$Hg was induced by fusion of $^{124}$Xe and $^{54}$Fe. The two fragments were detected in coincidence using VAMOS++ supplemented with a new SEcond Detection arm. For the first time in the pre-actinide region, access to the pre-neutron mass and total kinetic energy distributions, and the simultaneous isotopic identification of one the fission fragment, was achieved. The present work describes the experimental approach, and discusses the pre-neutron observables in the context of an extended asymmetric-fission island located south-west of $^{208}Pb. A comparison with different models is performed, demonstrating the importance of this "new" asymmetric-fission island for elaborating on driving effects in fission.

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arXiv2022

Structure of $^{83}$As, $^{85}$As and $^{87}$As: from semi-magicity to $γ$-softness

The structure of $^{83}$As, $^{85}$As and $^{87}$As have been studied in fusion-fission reaction $^{238}$U+$^9$Be. Fission fragments were identified in mass and atomic number using the VAMOS++ spectrometer and the coincident $γ$-rays were detected in the $γ$-ray tracking array AGATA. New transitions in $^{83}$As and $^{85}$As are reported and placed in the level schemes. A level scheme of the excited states in $^{87}$As is proposed for the first time. The data are interpreted in frame of Large-Scale Shell-Model calculations, SU3 symmetries and Beyond Mean-Field frameworks. A spherical regime at magic number $N$=50 is predicted and the location of the proton $g_{9/2}$ orbital is proposed for the first time. Development of collectivity in a prolate deformed, $γ$-soft regime in the open shell cases $^{85}$As and $^{87}$As, most neutron-rich isotopes beyond $N$=50, is concluded. Data and theoretical calculations give confidence to a relatively high extrapolated excitation energy about 4 MeV of the $9/2^+$ state in $^{79}$Cu, one proton above $^{78}$Ni.

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arXiv2021

Narrow resonances in the continuum of the unbound nucleus $^{15}$F

The structure of the unbound $^{15}$F nucleus is investigated using the inverse kinematics resonant scattering of a radioactive $^{14}$O beam impinging on a CH$_2$ target. The analysis of $^{1}$H($^{14}$O,p)$^{14}$O and $^{1}$H($^{14}$O,2p)$^{13}$N reactions allowed the confirmation of the previously observed narrow $1/2^{-}$ resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2$^{-}$ and 3/2$^{-}$ resonances. The newly observed levels decay by 1p emission to the ground of $^{14}$O, and by sequential 2p emission to the ground state (g.s.) of $^{13}$N via the $1^-$ resonance of $^{14}$O. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2$^{-}$ and 3/2$^{-}$ resonances may be collectivized by the continuum coupling to nearby 2p- and 1p- decay channels. The observed excitation function $^{1}$H($^{14}$O,p)$^{14}$O and resonance spectrum in $^{15}$F are well reproduced in the unified framework of the GSM.

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arXiv2021

Evidence for enhanced neutron-proton correlations from the level structure of the $N=Z+1$ nucleus $^{87}_{43}$Tc$^{\ }_{44}$

The low-lying excited states in the neutron-deficient $N=Z+1$ nucleus $^{87}_{43}$Tc$^{\ }_{44}$ have been studied via the fusion-evaporation reaction $^{54}$Fe($^{36}$Ar, $2n1p$)$^{87}$Tc at the Grand Accélérateur National d'Ions Lourds (GANIL), France. The AGATA spectrometer was used in conjunction with the auxiliary NEDA, Neutron Wall, and DIAMANT detector arrays to measure coincident prompt $γ$-rays, neutrons, and charged particles emitted in the reaction. A level scheme of $^{87}$Tc from the (9/2$^{+}_{g.s.}$) state to the (33/2$^{+}_{1}$) state was established based on 6 mutually coincident $γ$-ray transitions. The constructed level structure exhibits a rotational behavior with a sharp backbending at $\hbarω\approx 0.50$ MeV. A decrease in alignment frequency and increase in alignment sharpness in the odd-mass isotonic chains around $N=44$ is proposed as an effect of the enhanced isoscalar neutron-proton interactions in odd-mass nuclei when approaching the $N=Z$ line.

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