SearcharxivSearch

arXiv · 2402.11535

Bayesian uncertainty quantification on nuclear level density data and their impact on $(p,\gamma)$ reactions of astrophysical interest

Abstract

The $p$ process nucleosynthesis is responsible for the synthesis of 35 neutron-deficient nuclei from $^{35}$Se to $^{196}$Hg. An important input that can affect the modeling of this process is the nuclear level density at the relevant excitation energies of the nuclei involved in the reaction network. The OSLO method has been extensively used for the measurement of level densities in excitation energies of several MeV. In this work, Bayesian optimization has been used in order to estimate the 95% high density intervals for the parameters of two level density models optimized on the OSLO data. These uncertainties are then propagated on the cross sections of $(p,\gamma)$ reactions leading to the compound nuclei $^{105,106}$Pd and $^{105,106}$Cd inside the astrophysically relevant energy range. Imposing constraints in this region of the isotopic chart is important for network calculations involving the nearby $p$ nuclei $^{102}$Pd and $^{106}$Cd. We discuss the reduction of the range of cross sections due to the uncertainties arising from the level density data compared to the range of the six default level density models available in TALYS and we highlight the need for level density data inside the astrophysically relevant energy ranges.

Explore related subjects

Keep this discovery

BibTeXRIS

A. Chalil, C. Ducoin, O. Stézowski, N. Millard-Pinard, J. Dudouet, Y. Demane, M. Chamseddine. 2024-02-18. Bayesian uncertainty quantification on nuclear level density data and their impact on $(p,\gamma)$ reactions of astrophysical interest. https://arxiv.org/abs/2402.11535

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Fission Modes and Fragment Shell Structures in $^{258}$Md$^*$ from Six-Dimensional Langevin Calculations

The fission of $^{258}$Md$^*$ is calculated in the excitation energy range of $E^*=6$--36 MeV using a six-dimensional Langevin equation. The calculated events are classified into two symmetric and two asymmetric fission modes based on the fragment mass and the quadrupole deformations of the two fragments at scission. The symmetric modes are separated by their total kinetic energies into the short (high TKE) and superlong (low TKE) modes, whereas the asymmetric modes differ in mass asymmetry. With increasing excitation energy, the yield of the short mode decreases, whereas the combined yield of the two asymmetric modes increases, as observed in the in-beam prompt-fission study of $^{258}$Md$^*$. From an analysis of the fragment shapes and associated single-particle levels, the short mode and the dominant asymmetric mode with the smaller mass asymmetry are found to involve a compact fragment characterized by deformed shell gaps at $Z=52$ and $N=84$, while the complementary fragments have different quadrupole deformations in the two modes.

nucl-th

Classification of fission modes in $^{236}$U using a six-dimensional Langevin approach

Thermal neutron-induced fission of $^{235}$U is studied using a six-dimensional Langevin approach based on the Cassini shape parametrization. Scission events are classified into Asymmetric 1 (AS1), Asymmetric 2 (AS2), and Superlong (SL) fission modes by applying the $k$-means algorithm to the fragment mass and the quadrupole deformations of both fragments. For each mode, proton and neutron single-particle levels are calculated for representative fragments to examine their shell structures. The AS1 heavy fragment exhibits proton gaps at $Z=50$ and 52 and neutron gaps at $N=82$ and 84, whereas well-developed gaps appear at $Z=56$ and $N=88$ in the AS2 heavy fragment. The mass splits of AS1 and AS2 are close to those of the conventional Standard I and Standard II modes, respectively. However, the average total kinetic energy is lower for AS1 than for AS2, opposite to the conventional ordering of Standard I and Standard II. This reversal reflects the more elongated shape of the AS1 light fragment. The SL mode is conventionally interpreted in terms of macroscopic liquid-drop effects, whereas the pronounced proton shell gap at $Z=46$ suggests that proton shell effects also contribute to the elongated symmetric configuration. The classification based on fragment mass and the quadrupole deformations of both fragments provides a basis for distinguishing fission modes and examining the corresponding fragment shell structures at scission.

nucl-th

Gogny interaction from beginnings to current challenges

The main goal of the present review article is to gather for the first time various facets of the phenomenological effective Gogny interaction which was originally proposed in the 70's. This involves both nuclear phenomena of interest that led to its creation and evolution as well as highly technical aspects that led the objectives to be achieved. With this in mind, we propose a discussion structured around four points. After a general introduction, the history and philosophy of the Gogny interaction is exposed. In particular, one highlights an intuitive way of guiding the determination of the parameters of the phenomenological interaction with the results obtained from a realistic interaction using Hartree-Fock calculations and second order corrections and a G-matrix. One also shows that physical phenomena such as pairing or fission were essential to improve the parameterization. The evolution of the original analytical form over the years is also discussed. The second point concern the emulator that was used for the generation of parameterizations. Its modifications, consistent with the evolution of the analytical form, are given. Other fitting procedures, more recent, are also evoked. The third key point is dedicated to the role of the nuclear matter in the fitting process and the acceptance of a parameterization. The objective of the last key point is to highlight some results obtained with the Gogny interaction in nuclear structure, fission and reactions that have allowed to interpret experimental data.

nucl-th