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J. Fabian

Publications and source records attributed to J. Fabian.

At least 19 recordsLinked to original sources
arXiv2026

Electron spin resonance driven photogalvanic effect in graphene-based structures

We report an electron-spin-resonance-driven linear photogalvanic effect (LPGE) in unbiased monolayer graphene and WSe_2/graphene heterostructures. Under linearly polarized 45--75 GHz radiation, the photovoltage exhibits pronounced resonant features in both Faraday and Voigt geometries. Multiple resonances associated with the electron spin resonance in graphene are observed for both out-of-plane and in-plane magnetic-field orientations. Their magnetic-field positions vary linearly with frequency, their amplitudes reverse sign across the charge-neutrality point, and the resonant contribution has the opposite sign to the nonresonant Drude photogalvanic background. We develop a microscopic theory in which radiation-induced momentum alignment followed by skew scattering generates both contributions. Their opposite signs originate from the orthogonal momentum alignments produced by indirect Drude absorption and direct spin-resonant transitions. The theory describes well the main features of the observed resonant photocurrent and provides a microscopic description of ESR-induced LPGE in two-dimensional systems. These results establish the photogalvanic response as a probe of ESR in unbiased micron-scale graphene-based devices.

cond-mat.mtrl-sci↗
arXiv2023

Charge transfer and asymmetric coupling of MoSe$_2$ valleys to the magnetic order of CrSBr

Van der Waals (vdW) heterostructures composed of two-dimensional (2D) transition metal dichalcogenides (TMD) and vdW magnetic materials offer an intriguing platform to functionalize valley and excitonic properties in non-magnetic TMDs. Here, we report magneto-photoluminescence (PL) investigations of monolayer (ML) MoSe$_2$ on the layered A-type antiferromagnetic (AFM) semiconductor CrSBr under different magnetic field orientations. Our results reveal a clear influence of the CrSBr magnetic order on the optical properties of MoSe$_2$, such as an anomalous linear-polarization dependence, changes of the exciton/trion energies, a magnetic-field dependence of the PL intensities, and a valley $g$-factor with signatures of an asymmetric magnetic proximity interaction. Furthermore, first principles calculations suggest that MoSe$_2$/CrSBr forms a broken-gap (type-III) band alignment, facilitating charge transfer processes. The work establishes that antiferromagnetic-nonmagnetic interfaces can be used to control the valley and excitonic properties of TMDs, relevant for the development of opto-spintronics devices.

cond-mat.mes-hall↗
arXiv2023

Ultralong 100 ns Spin Relaxation Time in Graphite at Room Temperature

Graphite has been intensively studied, yet its electron spins dynamics remains an unresolved problem even 70 years after the first experiments. The central quantities, the longitudinal ($T_1$) and transverse ($T_2$) relaxation times were postulated to be equal, mirroring standard metals, but $T_1$ has never been measured for graphite. Here, based on a detailed band structure calculation including spin-orbit coupling, we predict an unexpected behavior of the relaxation times. We find, based on saturation ESR measurements, that $T_1$ is markedly different from $T_2$. Spins injected with perpendicular polarization with respect to the graphene plane have an extraordinarily long lifetime of $100$ ns at room temperature. This is ten times more than in the best graphene samples. The spin diffusion length across graphite planes is thus expected to be ultralong, on the scale of $\sim 70~μ$m, suggesting that thin films of graphite -- or multilayer AB graphene stacks -- can be excellent platforms for spintronics applications compatible with 2D van der Waals technologies. Finally, we provide a qualitative account of the observed spin relaxation based on the anisotropic spin admixture of the Bloch states in graphite obtained from density functional theory calculations.

cond-mat.mes-hall↗
arXiv2018

Unusual spin properties of InP wurtzite nanowires revealed by Zeeman splitting spectroscopy

In this study, we present a complete experimental and theoretical investigation of the fundamental exciton Zeeman splitting in wurtzite InP nanowires. We determined the exciton gyromagnetic factor, $g_{exc}$, by magneto-photoluminescence spectroscopy using magnetic fields up to 29 T. We found that $g_{exc}$ is strongly anisotropic with values differing in excess of 50\% between the magnetic field oriented parallel and perpendicular to the nanowire long axis. Furthermore, for magnetic fields oriented along the nanowire axis, $g_{exc}$ is nearly three times larger than in bulk zincblende InP and it shows a marked sublinear dependence on the magnetic field, a common feature to other non-nitride III-V wurtzite nanowires but not properly understood. Remarkably, this nonlinearity originates from only one Zeeman branch characterized by a specific type of light polarization. All the experimental findings are modeled theoretically by a robust approach combining the $k \cdot p$ method with the envelope function approximation and including the electron-hole interaction. We revealed that the nonlinear features arise due to the coupling between Landau levels pertaining to the A (heavy-hole like) and B (light-hole like) valence bands of the wurtzite crystal structure. This general behavior is particularly relevant for the understanding of the spin properties of several wurtzite nanowires that host the set for the observation of topological phases potentially at the base of quantum computing platforms.

cond-mat.mes-hall↗
arXiv2018

Electric-field modification of interfacial spin-orbit field-vector

Current induced spin-orbit magnetic fields (iSOFs), arising either in single-crystalline ferromagnets with broken inversion symmetry1,2 or in non-magnetic metal/ferromagnetic metal bilayers3,4, can produce spin-orbit torques which act on a ferromagnet's magnetization,thus offering an efficient way for its manipulation.To further reduce power consumption in spin-orbit torque devices, it is highly desirable to control iSOFs by the field-effect, where power consumption is determined by charging/discharging a capacitor5,6. In particular, efficient electric-field control of iSOFs acting on ferromagnetic metals is of vital importance for practical applications. It is known that in single crystalline Fe/GaAs (001) heterostructures with C2v symmetry, interfacial SOFs emerge at the Fe/GaAs (001) interface due to the lack of inversion symmetry7,8. Here, we show that by applying a gate-voltage across the Fe/GaAs interface, interfacial SOFs acting on Fe can be robustly modulated via the change of the magnitude of the interfacial spin-orbit interaction. Our results show that, for the first time, the electric-field in a Schottky barrier is capable of modifying SOFs, which can be exploited for the development of low-power-consumption spin-orbit torque devices.

cond-mat.mes-hall↗
arXiv2017

An intuitive approach to the unified theory of spin-relaxation

Spin-relaxation is conventionally discussed using two different approaches for materials with and without inversion symmetry. The former is known as the Elliott-Yafet (EY) theory and for the latter the D'yakonov-Perel' (DP) theory applies, respectively. We discuss herein a simple and intuitive approach to demonstrate that the two seemingly disparate mechanisms are closely related. A compelling analogy between the respective Hamiltonian is presented and that the usual derivation of spin-relaxation times, in the respective frameworks of the two theories, can be performed. The result also allows to obtain the less canonical spin-relaxation regimes; the generalization of the EY when the material has a large quasiparticle broadening and the DP mechanism in ultrapure semiconductors. The method also allows a practical and intuitive numerical implementation of the spin-relaxation calculation, which is demonstrated for MgB$_2$ that has anomalous spin-relaxation properties.

cond-mat.mes-hall↗
arXiv2015

Electric field control of spin lifetimes in Nb-SrTiO$_3$ by spin-orbit fields

We show electric field control of the spin accumulation at the interface of the oxide semiconductor Nb-SrTiO$_{3}$ with Co/AlO$_{x}$ spin injection contacts at room temperature. The in-plane spin lifetime $τ_\parallel$ as well as the ratio of the out-of-plane to in-plane spin lifetime $τ_\perp/τ_\parallel$ is manipulated by the built-in electric field at the semiconductor surface, without any additional gate contact. The origin of this manipulation is attributed to Rashba Spin-Orbit Fields (SOFs) at the Nb-SrTiO$_3$ surface and shown to be consistent with theoretical model calculations based on SOF spin flip scattering. Additionally, the junction can be set in a high or low resistance state, leading to a non-volatile control of $τ_\perp/τ_\parallel$, consistent with the manipulation of the Rashba SOF strength. Such room temperature electric field control over the spin state is essential for developing energy-efficient spintronic devices and shows promise for complex oxide based (spin)electronics

cond-mat.mtrl-sci↗
arXiv2013

Spin-orbit interaction induced singularity of the charge density relaxation propagator

The charge density relaxation propagator of a two dimensional electron system, which is the slope of the imaginary part of the polarization function, exhibits singularities for bosonic momenta having the order of the spin-orbit momentum and depending on the momentum orientation. We have provided an intuitive understanding for this non-analytic behavior in terms of the inter chirality subband electronic transitions, induced by the combined action of Bychkov-Rashba (BR) and Dresselhaus (D) spin-orbit coupling. It is shown that the regular behavior of the relaxation propagator is recovered in the presence of only one BR or D spin-orbit field or for spin-orbit interaction with equal BR and D coupling strengths. This creates a new possibility to influence carrier relaxation properties by means of an applied electric field.

cond-mat.mes-hall↗
arXiv2012

Theory of thermal spin-charge coupling in electronic systems

The interplay between spin transport and thermoelectricity offers several novel ways of generating, manipulating, and detecting nonequilibrium spin in a wide range of materials. Here we formulate a phenomenological model in the spirit of the standard model of electrical spin injection to describe the electronic mechanism coupling charge, spin, and heat transport and employ the model to analyze several different geometries containing ferromagnetic (F) and nonmagnetic (N) regions: F, F/N, and F/N/F junctions which are subject to thermal gradients. We present analytical formulas for the spin accumulation and spin current profiles in those junctions that are valid for both tunnel and transparent (as well as intermediate) contacts. For F/N junctions we calculate the thermal spin injection efficiency and the spin accumulation induced nonequilibrium thermopower. We find conditions for countering thermal spin effects in the N region with electrical spin injection. This compensating effect should be particularly useful for distinguishing electronic from other mechanisms of spin injection by thermal gradients. For F/N/F junctions we analyze the differences in the nonequilibrium thermopower (and chemical potentials) for parallel and antiparallel orientations of the F magnetizations, as evidence and a quantitative measure of the spin accumulation in N. Furthermore, we study the Peltier and spin Peltier effects in F/N and F/N/F junctions and present analytical formulas for the heat evolution at the interfaces of isothermal junctions.

cond-mat.mes-hall↗
arXiv2011

Theory of optical spin orientation in silicon

We theoretically investigate the indirect optical injection of carriers and spins in bulk silicon, using an empirical pseudopotential description of electron states and an adiabatic bond charge model for phonon states. We identify the selection rules, the contribution to the carrier and spin injection in each conduction band valley from each phonon branch and each valence band, and the temperature dependence of these processes. The transition from the heavy hole band to the lowest conduction band dominates the injection due to the large joint density of states. For incident light propagating along the $[00\bar{1}]$ direction, the injection rates and the degree of spin polarization of injected electrons show strong valley anisotropy. The maximum degree of spin polarization is at the injection edge with values 25% at low temperature and 15% at high temperature.

cond-mat.mtrl-sci↗
arXiv2010

Spin relaxation and spin dynamics in semiconductors

A chapter contribution to book: "Handbook of Spin Transport and Magnetism", ed. by Evegeny Y. Tsymbal and Igor Zutic (Chapman & Hall/CRC, 2011) http://www.crcpress.com/product/isbn/9781439803776 .

cond-mat.mes-hall↗
arXiv2010

Spin edge helices in a perpendicular magnetic field

We present an exact solution to the problem of the spin edge states in the presence of equal Bychkov-Rashba and Dresselhaus spin-orbit fields in a two-dimensional electron system, restricted by a hard-wall confining potential and exposed to a perpendicular magnetic field. We find that the spectrum of the spin edge states depends critically on the orientation of the sample edges with respect to the crystallographic axes. Such a strikingly different spectral behavior generates new modes of the persistent spin helix-spin edge helices with novel properties, which can be tuned by the applied electric and magnetic fields.

cond-mat.mes-hall↗
arXiv2010

Pseudospin excitations in coaxial nanotubes

In a 2DEG confined to two coaxial tubes the `tube degree of freedom' can be described in terms of pseudospin-1/2 dynamics. The presence of tunneling between the two tubes leads to a collective oscillation known as pseudospin resonance. We employ perturbation theory to examine the dependence of the frequency of this mode with respect to a coaxial magnetic field for the case of small intertube distances. Coulomb interaction leads to a shift of the resonance frequency and to a finite lifetime of the pseudospin excitations. The presence of the coaxial magnetic field gives rise to pronounced peaks in the shift of the resonance frequency. For large magnetic fields this shift vanishes due to the effects of Zeeman splitting. Finally, an expression for the linewidth of the resonance is derived. Numerical analysis of this expression suggests that the linewidth strongly depends on the coaxial magnetic field, which leads to several peaks of the linewidth as well as regions where damping is almost completely suppressed.

cond-mat.other↗
arXiv2009

Beating of Friedel oscillations induced by spin-orbit interaction

By exploiting our recently derived exact formula for the Lindhard polarization function in the presence of Bychkov-Rashba (BR) and Dresselhaus (D) spin-orbit interaction (SOI), we show that the interplay of different SOI mechanisms induces highly anisotropic modifications of the static dielectric function. We find that under certain circumstances the polarization function exhibits doubly-singular behavior, which leads to an intriguing novel phenomenon, beating of Friedel oscillations. This effect is a general feature of systems with BR+D SOI and should be observed in structures with a sufficiently strong SOI.

cond-mat.mes-hall↗
arXiv2009

Theory of the spin relaxation of conduction electrons in silicon

A realistic pseudopotential model is introduced to investigate the phonon-induced spin relaxation of conduction electrons in bulk silicon. We find a surprisingly subtle interference of the Elliott and Yafet processes affecting the spin relaxation over a wide temperature range, suppressing the significance of the intravalley spin-flip scattering, previously considered dominant, above roughly 120 K. The calculated spin relaxation times $T_1$ agree with the spin resonance and spin injection data, following a $T^{-3}$ temperature dependence. The valley anisotropy of $T_1$ and the spin relaxation rates for hot electrons are predicted.

cond-mat.mtrl-sci↗
arXiv2009

Magnetic circular dichroism in GaMnAs: (no) evidence for an impurity band

Magneto-optical properties of the ferromagnetic semiconductor GaMnAs are studied in a material specific multi-band tight-binding approach. Two realistic models are compared: one has no impurity band while the other shows an impurity band for low Mn concentrations. The calculated magnetic circular dichroism (MCD) is positive for both models proving that, unlike previously asserted, the observed positive MCD signal is inconclusive as to the presence or absence of an impurity band in GaMnAs. The positive MCD is due to the antiferromagnetic p-d coupling and the transitions into the conduction band.

cond-mat.mtrl-sci↗
arXiv2009

Band-structure topologies of graphene: spin-orbit coupling effects from first principles

The electronic band structure of graphene in the presence of spin-orbit coupling and transverse electric field is investigated from first principles using the linearized augmented plane-wave method. The spin-orbit coupling opens a gap at the $K(K')$-point of the magnitude of 24 $μ$eV (0.28 K). This intrinsic splitting comes 96% from the usually neglected $d$ and higher orbitals. The electric field induces an additional (extrinsic) Bychkov-Rashba-type splitting of 10 $μ$eV (0.11 K) per V/nm, coming from the $σ$-$π$ mixing. A 'mini-ripple' configuration with every other atom is shifted out of the sheet by less than 1% differs little from the intrinsic case.

cond-mat.mtrl-sci↗