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J. Gou

Publications and source records attributed to J. Gou.

3 recordsLinked to original sources

Direct Determination of Spin-Splitting Energy in Magnetic Graphene by Landau Fan Shifts

Spin-polarized two-dimensional materials with large and tunable spin-splitting energy promise the field of 2D spintronics. While graphene has been a canonical 2D material, its spin properties and tunability are limited. Here, we demonstrate the emergence of robust spin-polarization in graphene with large and tunable spin-splitting energy of up to 132 meV at zero applied magnetic fields. The spin polarization is induced through a magnetic exchange interaction between graphene and the underlying ferrimagnetic oxide insulating layer, Tm3Fe5O12, as confirmed by its X-ray magnetic circular dichroism. The spin-splitting energies are directly measured and visualized by the shift in their landau fan diagram mapped by analyzing the measured subnikov-de-Haas oscillations as a function of applied electric fields, showing consistent fit with our first-principles and machine learning calculations. Further, the observed spin-splitting energies can be tuned over a broad range between 98 and 166 meV by cooling fields. Our methods and results are applicable to other two-dimensional (magnetic) materials and heterostructures, and offer great potential for developing next-generation spin logic and memory devices.

cond-mat.mtrl-sci

Room-temperature colossal magnetoresistance in terraced single-layer graphene

Disorder-induced magnetoresistance (MR) effect is quadratic at low perpendicular magnetic fields and linear at high fields. This effect is technologically appealing, especially in the two-dimensional (2D) materials such as graphene, since it offers potential applications in magnetic sensors with nanoscale spatial resolution. However, it is a great challenge to realize a graphene magnetic sensor based on this effect because of the difficulty in controlling the spatial distribution of disorder and enhancing the MR sensitivity in the single-layer regime. Here, we report a room-temperature colossal MR of up to 5,000% at 9 T in terraced single-layer graphene. By laminating single-layer graphene on a terraced substrate, such as TiO2 terminated SrTiO3, we demonstrate a universal one order of magnitude enhancement in the MR compared to conventional single-layer graphene devices. Strikingly, a colossal MR of >1,000% was also achieved in the terraced graphene even at a high carrier density of ~1012 cm-2. Systematic studies of the MR of single-layer graphene on various oxide- and non-oxide-based terraced surfaces demonstrate that the terraced structure is the dominant factor driving the MR enhancement. Our results open a new route for tailoring the physical property of 2D materials by engineering the strain through a terraced substrate.

cond-mat.mes-hall

An Asymptotic Analysis of a 2-D Model of Dynamically Active Compartments Coupled by Bulk Diffusion

A class of coupled cell-bulk ODE-PDE models is formulated and analyzed in a two-dimensional domain, which is relevant to studying quorum sensing behavior on thin substrates. In this model, spatially segregated dynamically active signaling cells of a common small radius $ε\ll 1$ are coupled through a passive bulk diffusion field. The method of matched asymptotic expansions is used to construct steady-state solutions and to formulate a spectral problem that characterizes the linear stability properties of these solutions, with the aim of predicting whether temporal oscillations can be triggered by the cell-bulk coupling. Phase diagrams in parameter space where such collective oscillations can occur are illustrated for two specific choices of the intracellular kinetics. In the limit of very large bulk diffusion, it is shown that the ODE-PDE system can be approximated by a finite-dimensional dynamical system, which is studied both analytically and numerically. For one illustrative example of the theory it is shown that when the number of cells exceeds some critical number, the bulk diffusion field can trigger oscillations that would otherwise not occur without the coupling. Moreover, for two specific models for the intracellular dynamics, we show that there are rather wide regions in parameter space where these triggered oscillations are synchronous in nature. Unless the bulk diffusivity is asymptotically large, it is shown that a clustered spatial configuration of cells inside the domain leads to larger regions in parameter space where synchronous collective oscillations between the small cells can occur. Finally, the linear stability analysis for these cell-bulk models is shown to be qualitatively rather similar to that of localized spot patterns for activator-inhibitor reaction-diffusion systems in the limit of long-range inhibition and short-range activation.

nlin.PS