arXiv subjects

J. L. Sarrao

Publications and source records attributed to J. L. Sarrao.

At least 37 records · Page 2Linked to original sources

arXiv2009

Hot electron relaxation in a heavy fermion system with tuned doping

Femtosecond time-resolved optical spectroscopy was used to systematically study photoexcited carrier relaxation dynamics in the intermediate-valence heavy fermion system Yb1-xLuxAl3 (0 < x < 1). Given the demonstrated sensitivity of this experimental technique to the presence of the low energy gaps in the charge excitation spectrum, the aim of this work was to study the effect of dilution of the Kondo lattice on its low energy electronic structure. The results imply that in Yb1-xLuxAl3 the hybridization gap, resulting from hybridization of local moments and conduction electrons, persists up to 30% doping. Interestingly, below some characteristic, doping dependent temperature T*(x) the relaxation time divergence, governed by the relaxation bottleneck due to the presence of the indirect hybridization gap, is truncated. This observation is attributed to the competing ballistic transport of hot electrons out of the probed volume at low temperatures. The derived theoretical model accounts for both the functional form of relaxation dynamics below T*(x), as well as the doping dependence of the low temperature relaxation rate in Yb1-xLuxAl3.

cond-mat.str-el↗

arXiv2009

Local structure and site occupancy of Cd and Hg substitutions in CeTIn5 (T=Co, Rh, Ir)

The CeTIn5 superconductors (T=Co, Rh, or Ir) have generated great interest due to their relatively Tc's, NFL behavior, and their proximity to AF order and quantum critical points. In contrast to small changes with the T-species, electron doping in CeT(In{1-x}Mx)5 with M=Sn and hole doping with Cd or Hg have a dramatic effect on the electronic properties at very low concentrations. The present work reports EXAFS measurements that address the substituent atom distribution as a function of T, M, and x, near the superconducting phase. Together with previous measurements for M=Sn, the proportion of the M atom residing on the In(1) site, f{In(1)}, increases in the order M=Cd, Sn, and Hg, ranging from about 40% to 70%, showing a strong preference for these substituents to occupy the In(1) site (random=20%). In addition, f{In(1)} ranges from 70% to 100% for M=Hg in the order T=Co, Rh, and Ir. These fractions track the changes in the atomic radii of the various species, and help explain the sharp dependence of Tc on substituting into the In site. However, it is difficult to reconcile the small concentrations of M with the dramatic changes in the ground state in the hole-doped materials with only an impurity scattering model. These results therefore indicate that while such substitutions have interesting local atomic structures with important electronic and magnetic consequences, other local changes in the electronic and magnetic structure are equally important in determining the bulk properties of these materials.

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arXiv2009

The electronic structure of CeCoIn5 from angle-resolved photoemission spectroscopy I: Comparison to LDA

We have investigated the low-energy electronic structure of the heavy fermion superconductor CeCoIn5 by angle-resolved photoemission and band structure calculations. We measured the Fermi surface and energy distribution maps along the high-symmetry directions at hn = 100 eV and T = 25 K. The compound has quasi two-dimensional Fermi surface sheets centered at the M-A line of the Brillouin zone. The band structure calculations have been carried out within the local density approximation where the 4f electrons have been treated either localized or itinerant. We discuss the comparison to the experimental data and the implications for the nature of the 4f electrons at the given temperature.

cond-mat.supr-con↗

arXiv2009

The electronic structure of CeCoIn5 from angle-resolved photoemission spectroscopy II: Hybridization effects

We have investigated the low-energy electronic structure of the heavy fermion superconductor CeCoIn5 by angle-resolved photoemission. We focus on the dispersion and the peak width of the prominent quasi-two-dimensional Fermi surface sheet at the corner of the Brillouin zone as a function of temperature along certain k-directions with a photon energy of hn = 100 eV. We find slight changes of the Fermi vector and an anomalous broadening of the peak width when the Fermi energy is approached. Additionally we performed resonant ARPES experiments with hn = 121 eV. A flat f-derived band is observed with a distinct temperature dependence and a k-dependent spectral weight. These results, including both off- and on-resonant measurements, fit qualitatively to a two level mixing model derived from the Periodic Anderson Model.

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arXiv2009

Isotropic Quantum Scattering and Unconventional Superconductivity

Superconductivity without phonons has been proposed for strongly correlated electron materials that are tuned close to a zero-temperature magnetic instability of itinerant charge carriers. Near this boundary, quantum fluctuations of magnetic degrees of freedom assume the role of phonons in conventional superconductors, creating an attractive interaction that glues electrons into superconducting pairs. Here we show that superconductivity can arise from a very different spectrum of fluctuations associated with a local or Kondo-breakdown quantum-critical point that is revealed in isotropic scattering of charge carriers and a sub-linear temperature-dependent electrical resistivity. At this critical point, accessed by applying pressure to the strongly correlated, local-moment antiferromagnet CeRhIn5, magnetic and charge fluctuations coexist and produce electronic scattering that is maximal at the optimal pressure for superconductivity. This previously unanticipated source of pairing glue opens possibilities for understanding and discovering new unconventional forms of superconductivity.

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arXiv2008

Analysis of the normal state magnetotransport in CeIrIn${_5}$

We present an analysis of the normal state magnetotransport in the heavy fermion superconductor CeIrIn${_5}$. The Hall effect and the transverse magnetoresistance in this material do not appear to be uniquely correlated, as inferred from the field dependence of the current ratio ($R_σ = σ_{xy} / σ_{xx}^2 H$). The Hall coefficient is seen to satisfy a scaling equation of the form $R_H = f [H / (a + b T^c)]$. These results are compared to those observed earlier in CeCoIn$_5$, and are discussed in terms of the contrasting phase diagram which the CeIrIn$_5$ system exhibits in relation to its Co counterpart.

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arXiv2008

Magnetotransport in the CeIrIn${_5}$ system: The influence of antiferromagnetic fluctuations

We present an overview of magnetotransport measurements on the heavy-fermion superconductor CeIrIn$_5$. Sensitive measurements of the Hall effect and magnetoresistance (MR) are used to elucidate the low temperature phase diagram of this system. The normal-state magnetotransport is highly anomalous, and experimental signatures of a pseudogap-like precursor state to superconductivity as well as evidence for two distinct scattering times governing the Hall effect and the MR are observed. Our observations point out the influence of antiferromagnetic fluctuations on the magnetotransport in this class of materials. The implications of these findings, both in the context of unconventional superconductivity in heavy-fermion systems as well as in relation to the high temperature superconducting cuprates are discussed.

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arXiv2008

The precursor state to superconductivity in CeIrIn${_5}$: Unusual scaling of magnetotransport

We present an analysis of the normal-state Hall effect and magnetoresistance in the heavy fermion superconductor CeIrIn${_5}$. It is demonstrated that the modified Kohler's scaling--which relates the magnetoresistance to the Hall angle--breaks down prior to the onset of superconductivity due to the presence of a precursor state to superconductivity in this system. A model-independent, single-parameter scaling of the Hall angle governed solely by this precursor state is observed. Neither the Hall coefficient nor the resistivity exhibit this scaling implying that this precursor state preferentially influences the Hall channel.

cond-mat.str-el↗

arXiv2008

High Field de Haas - van Alphen Studies of the Fermi Surfaces of LaMIn$_{5}$ (M = Co, Rh, Ir)

We report measurements of the de Haas - van Alphen effect on a series of compounds, LaMIn$_{5}$ (M = Co, Rh, Ir). The results show that each of the Co and Ir Fermi surfaces (FSs) exhibit some portions that are two dimensional and some portions that are three dimensional. The most two dimensional character is exhibited in LaCoIn$_{5}$, less two dimensional behavior is seen in LaIrIn$_{5}$, no part of Fermi surface of LaRhIn$_{5}$ is found to have a two dimensional character. Thus the two dimensionality of portions of the FSs is largely determined by the d character of the energy bands while all of the effective masses remain $\leq$ 1.2. This fact has implications for the causes of the heavy fermion nature of superconductivity and magnetism in the Ce-based compounds having the similar composition and structure. All of the measurements were performed at the National High Magnetic Field Laboratory using either cantilever magnetometry or field modulation methods.

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arXiv2008

Itinerant spin excitations near the hidden order transition in URu2Si2

By means of neutron scattering we show that the high-temperature precursor to the hidden order state of the heavy fermion superconductor URu$_{2}$Si$_{2}$ exhibits heavily damped incommensurate paramagnons whose strong energy dispersion is very similar to that of the long-lived longitudinal f-spin excitations that appear below T$_{0}$. Since the underlying local f-exchange is preserved we expect only the f-d interactions to change across the phase transition and to cause the paramagnetic damping. The damping exhibits single-ion behavior independent of wave vector and vanishes below the hidden order transition. We suggest that this arises from a transition from valence fluctuations to a hybridized f-d state below T$_{0}$. Here we present evidence that the itinerant excitations, like those in chromium, are due to Fermi surface nesting of hole and electron pockets so that the hidden order phase likely originates from a Fermi-surface instability. We identify wave vectors that span nested regions of a band calculation and that match the neutron spin crossover from incommensurate to commensurate on approach to the hidden order phase.

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arXiv2008

Electronic Duality in Strongly Correlated Matter

Superconductivity develops from an attractive interaction between itinerant electrons that creates electron pairs which condense into a macroscopic quantum state--the superconducting state. On the other hand, magnetic order in a metal arises from electrons localized close to the ionic core and whose interaction is mediated by itinerant electrons. The dichotomy between local moment magnetic order and superconductivity raises the question of whether these two states can coexist and involve the same electrons. Here we show that the single 4f-electron of cerium in CeRhIn5 simultaneously produces magnetism, characteristic of localization, and superconductivity that requires itinerancy. The dual nature of the 4f-electron allows microscopic coexistence of antiferromagnetic order and superconductivity whose competition is tuned by small changes in pressure and magnetic field. Electronic duality contrasts with conventional interpretations of coexisting spin-density magnetism and superconductivity and offers a new avenue for understanding complex states in classes of materials.

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arXiv2008

Andreev Reflection in Heavy-Fermion Superconductors and Order Parameter Symmetry in CeCoIn_5

Differential conductance spectra are obtained from nanoscale junctions on the heavy-fermion superconductor CeCoIn$_5$ along three major crystallographic orientations. Consistency and reproducibility of characteristic features among the junctions ensure their spectroscopic nature. All junctions show a similar conductance asymmetry and Andreev reflection-like conductance with reduced signal (~ 10%-13%), both commonly observed in heavy-fermion superconductor junctions. Analysis using the extended Blonder-Tinkham-Klapwijk model indicates that our data provide the first spectroscopic evidence for $d_{x^2-y^2}$ symmetry. To quantify our conductance spectra, we propose a model by considering the general phenomenology in heavy fermions, the two-fluid behavior, and an energy-dependent density of states. Our model fits to the experimental data remarkably well and should invigorate further investigations.

cond-mat.supr-con↗

arXiv2008

Dimensional crossover of quantum critical behavior in CeCoIn$_5$

The nature of quantum criticality in CeCoIn$_5$ is studied by low-temperature thermal expansion $α(T)$. At the field-induced quantum critical point at H=5 T a crossover scale $T^\star\approx 0.3$ K is observed, separating $α(T)/T\propto T^{-1}$ from a weaker $T^{-1/2}$ divergence. We ascribe this change to a crossover in the dimensionality of the critical fluctuations which may be coupled to a change from unconventional to conventional quantum criticality. Disorder, whose effect on quantum criticality is studied in CeCoIn$_{5-x}$Sn$_x$ ($0\leq x\leq 0.18$), shifts $T^\star$ towards higher temperatures.

cond-mat.str-el↗

arXiv2007

The Missing Link: Magnetism and Superconductivity

The effect of magnetic moments on superconductivity has long been a controversial subject in condensed matter physics. While Matthias and collaborators experimentally demonstrated the destruction of superconductivity in La by the addition of magnetic moments (Gd), it has since been suggested that magnetic fluctuations are in fact responsible for the development of superconducting order in other systems. Currently this debate is focused on several families of unconventional superconductors including high-Tc cuprates, borocarbides as well as heavy fermion systems where magnetism and superconductivity are known to coexist. Here we report a novel aspect of competition and coexistence of these two competing orders in an interesting class of heavy fermion compounds, namely the 1-1-5 series: CeTIn5 where T=Co, Ir, or Rh. Our optical experiments indicate the existence of regions in momentum space where local moments remain unscreened. The extent of these regions in momentum space appears to control both the normal and superconducting state properties in the 1-1-5 family of heavy fermion (HF) superconductors.

cond-mat.supr-con↗

arXiv2007

A precursor state to unconventional superconductivity in CeIrIn${_5}$

We present sensitive measurements of the Hall effect and magnetoresistance in CeIrIn${_5}$ down to temperatures of 50 mK and magnetic fields up to 15 T. The presence of a low temperature coherent Kondo state is established. Deviations from Kohler's rule and a quadratic temperature dependence of the cotangent of the Hall angle are reminiscent of properties observed in the high temperature superconducting cuprates. The most striking observation pertains to the presence of a \textit{precursor} state--characterized by a change in the Hall mobility--that appears to precede the superconductivity in this material, in similarity to the pseudogap in the cuprate high $T_c$ superconductors.

cond-mat.str-el↗

arXiv2007

Antiferromagnetic fluctuations and the Fulde-Ferrell-Larkin-Ovchinnikov state in CeCoIn5

The heavy-fermion superconductor CeCoIn5 is the first material, where different experimental probes show strong evidence pointing to the realization of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state. The inhomogeneous superconducting FFLO state with a periodically modulated order parameter was predicted to appear in Pauli-limited, sufficiently clean type-II superconductors already more than 40 years ago. On the other hand, CeCoIn5 is supposed to be close to a magnetic quantum critical point (QCP) showing strong antiferromagnetic (AFM) spin fluctuations (SF) at atmospheric pressure. We studied the evolution of the FFLO phase away from the influence of the strong AFM-SF by heat capacity experiments under pressure (0 GPa <= P <= 1.5 GPa, 0 T <= mu_0 H <= 14 T, and 100 mK <= T <= 4 K). Our results prove the stability of the the FFLO phase under pressure. It even expands, while the Pauli-limiting becomes weaker and the AFM-SF are suppressed. This shows the intriguing influence of the AFM-SF on the FFLO state.

cond-mat.str-el↗

arXiv2007

Quantifying structural damage from self-irradiation in a plutonium superconductor

The 18.5 K superconductor PuCoGa5 has many unusual properties, including those due to damage induced by self-irradiation. The superconducting transition temperature decreases sharply with time, suggesting a radiation-induced Frenkel defect concentration much larger than predicted by current radiation damage theories. Extended x-ray absorption fine-structure measurements demonstrate that while the local crystal structure in fresh material is well ordered, aged material is disordered much more strongly than expected from simple defects, consistent with strong disorder throughout the damage cascade region. These data highlight the potential impact of local lattice distortions relative to defects on the properties of irradiated materials and underscore the need for more atomic-resolution structural comparisons between radiation damage experiments and theory.

cond-mat.str-el↗

arXiv2007

Muon spin rotation measurements of the superfluid density in fresh and aged superconducting PuCoGa$_5$

We have measured the temperature dependence and magnitude of the superfluid density $ρ_{\rm s}(T)$ via the magnetic field penetration depth $λ(T)$ in PuCoGa$_5$ (nominal critical temperature $T_{c0} = 18.5$ K) using the muon spin rotation technique in order to investigate the symmetry of the order parameter, and to study the effects of aging on the superconducting properties of a radioactive material. The same single crystals were measured after 25 days ($T_c = 18.25$ K) and 400 days ($T_c = 15.0$ K) of aging at room temperature. The temperature dependence of the superfluid density is well described in both materials by a model using d-wave gap symmetry. The magnitude of the muon spin relaxation rate $σ$ in the aged sample, $σ\propto 1/λ^2\proptoρ_s/m^*$, where $m^*$ is the effective mass, is reduced by about 70% compared to fresh sample. This indicates that the scattering from self-irradiation induced defects is not in the limit of the conventional Abrikosov-Gor'kov pair-breaking theory, but rather in the limit of short coherence length (about 2 nm in PuCoGa$_5$) superconductivity.

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