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J. Li

Publications and source records attributed to J. Li.

At least 325 records · Page 18Linked to original sources

Optomechanical measurement of a millimeter-sized mechanical oscillator near the quantum limit

Cavity optomechanics is a tool to study the interaction between light and micromechanical motion. Here we observe near-quantum limited optomechanical physics in a truly macroscopic oscillator. As the mechanical system, we use a mm-sized piezoelectric quartz disk oscillator. Its motion is coupled to a charge qubit which translates the piezo-induced charge into an effective radiation-pressure interaction between the disk and a microwave cavity. We measure the thermal motion of the lowest mechanical shear mode at 7MHz down to 35 mK, corresponding to roughly 100 quanta in a 20mg oscillator. The work opens up opportunities for macroscopic quantum experiments.

cond-mat.mes-hall↗

Characterization and Performance of Germanium Detectors with sub-keV Sensitivities for Neutrino and Dark Matter Experiments

Germanium ionization detectors with sensitivities as low as 100 eVee (electron-equivalent energy) open new windows for studies on neutrino and dark matter physics. The relevant physics subjects are summarized. The detectors have to measure physics signals whose amplitude is comparable to that of pedestal electronic noise. To fully exploit this new detector technique, various experimental issues including quenching factors, energy reconstruction and calibration, signal triggering and selection as well as evaluation of their associated efficiencies have to be attended. The efforts and results of a research program to address these challenges are presented.

physics.ins-det↗

Chemistry in confined spaces: Reactivity of the Zn-MOF-74 channels

Using infrared spectroscopy combined with ab initio methods we study reactions of H$_2$O and CO inside the confined spaces of Zn-MOF-74 channels. Our results show that, once the water dissociation reaction H$_2$O$\;\rightarrow\;$OH+H takes place at the metal centers, the addition of 40 Torr of CO at 200 $^{\circ}$C starts the production of formic acid via OH+H+CO$\;\rightarrow\;$HCO$_2$H. Our detailed analysis shows that the overall reaction H$_2$O+CO$\;\rightarrow\;$HCO$_2$H takes place in the confinement of MOF-74 without an external catalyst, unlike the same reaction on flat surfaces. This discovery has several important consequences: It opens the door to a new set of catalytic reactions inside the channels of the MOF-74 system, it suggests that a recovery of the MOF's adsorption capacity is possible after it has been exposed to water (which in turn stabilizes its crystal structure), and it produces the important industrial feedstock formic acid.

physics.chem-ph↗

X-ray and gamma-ray variability of Mrk 421

We present an ordinary case in the momentum diffusion equation for the electron spectrum evolution and investigate the energy spectra and time dependent properties of flare in Mrk 421 in the frame of a time-dependent one-zone synchrotron self-Compton model. In this model, electrons are accelerated to extra-relativistic energy through the strong magnetic turbulence and evolve with time, and non-thermal photons are produced by both synchrotron and inverse Comtpon scattering off synchrotron photons. Moreover, non-thermal photons during a pre-flare are produced by the relativistic electrons in the steady state and those during a flare are produced by the electrons whose injection rate is changed during some time interval. We apply the model to the energy spectra and time-dependent properties of flares in Mrk 421 by reproducing the pre-burst spectrum of the source and varying the injection rate in the Bohm diffusion (q=1) and the hard sphere approximation (q=2) case, respectively. Our results show that Bohm diffusion case leads to hard photon spectra, and hard sphere case approximation seems to reproduce the energy spectra and the time dependent properties of flare still better.

astro-ph.HE↗

Cluster Assisted Water Dissociation Mechanism in MOF-74 and Controlling it Using Helium

We show that the water dissociation reaction H$_2$O$\rightarrow$OH+H in the confined environment of MOF-74 channels can be precisely controlled by the addition of the noble gas He. Elucidating the entire reaction process with ab initio methods and infrared (IR) spectroscopy, we prove that the interaction between water molecules is critical to the formation of water clusters, which reduce the dissociation barrier by up to 37% and thus influence the reaction significantly. Our time-resolved IR measurements confirm that the formation of these clusters can be suppressed by introducing He gas, providing unprecedented control over water dissociation rates. Since the water dissociation reaction is the cause of the structural instability of MOF-74 in the presence of water, our finding of the reaction mechanism lays the groundwork for designing water stable versions of MOF-74 as well as understanding water related phenomena in MOFs in general.

cond-mat.mtrl-sci↗

Direct detection of pure spin-current by x-ray pump-probe measurements

By synchronizing a microwave waveform with the synchrotron x-ray pulses, we use the ferromagnetic resonance (FMR) of the Py (Ni81Fe19) layer in a Py/Cu/Cu75Mn25/Cu/Co multilayer to pump a pure spin current into the Cu75Mn25 spacer layer, and then directly probe the spin current in the Cu75Mn25 layer by a time-resolved x-ray magnetic circular dichroism (XMCD). This element-specific pump-probe measurement unambiguously identifies the AC spin current in the Cu75Mn25 layer. In addition, phase resolved x-ray measurements reveal a characteristic bipolar phase behavior of the Co spins that is a fingerprint of spin-current driven spin precession.

cond-mat.mtrl-sci↗

Cluster Decay of the High-lying excited states in $^{14}$C

A cluster-transfer experiment of $^9\rm{Be}(^9\rm{Be},^{14}\rm{C}\rightarrowα+^{10}\rm{Be})α$ at an incident energy of 45 MeV was carried out in order to investigate the molecular structure in high-lying resonant states in $^{14}$C. This reaction is of extremely large $Q$-value, making it an excellent case to select the reaction mechanism and the final states in outgoing nuclei. The high-lying resonances in $^{14}$C are reconstructed for three sets of well discriminated final states in $^{10}$Be. The results confirm the previous decay measurements with clearly improved decay-channel selections and show also a new state at 23.5(1) MeV. The resonant states at 22.4(3) and 24.0(3) MeV decay primarily into the typical molecular states at about 6 MeV in $^{10}$Be, indicating a well developed cluster structure in these high-lying states in $^{14}$C. Further measurements of more states of this kind are suggested.

nucl-ex↗

Cavity Mode Frequencies and Strong Optomechanical Coupling in Two-Membrane Cavity Optomechanics

We study the cavity mode frequencies of a Fabry-Pérot cavity containing two vibrating dielectric membranes. We derive the equations for the mode resonances and provide approximate analytical solutions for them as a function of the membrane positions, which act as an excellent approximation when the relative and center-of-mass position of the two membranes are much smaller than the cavity length. With these analytical solutions, one finds that extremely large optomechanical coupling of the membrane relative motion can be achieved in the limit of highly reflective membranes when the two membranes are placed very close to a resonance of the inner cavity formed by them. We also study the cavity finesse of the system and verify that, under the conditions of large coupling, it is not appreciably affected by the presence of the two membranes. The achievable large values of the ratio between the optomechanical coupling and the cavity decay rate, $g/κ$, make this two-membrane system the simplest promising platform for implementing cavity optomechanics in the strong coupling regime.

quant-ph↗

Searching the Gamma-ray Sky for Counterparts to Gravitational Wave Sources: Fermi GBM and LAT Observations of LVT151012 and GW151226

We present the Fermi Gamma-ray Burst Monitor (GBM) and Large Area Telescope (LAT) observations of the LIGO binary black hole merger event GW151226 and candi- date LVT151012. No candidate electromagnetic counterparts were detected by either the GBM or LAT. We present a detailed analysis of the GBM and LAT data over a range of timescales from seconds to years, using automated pipelines and new techniques for char- acterizing the upper limits across a large area of the sky. Due to the partial GBM and LAT coverage of the large LIGO localization regions at the trigger times for both events, dif- ferences in source distances and masses, as well as the uncertain degree to which emission from these sources could be beamed, these non-detections cannot be used to constrain the variety of theoretical models recently applied to explain the candidate GBM counterpart to GW150914.

astro-ph.HE↗

Search for solar axions with CsI(Tl) crystal detectors

The results of a search for solar axions from the Korea Invisible Mass Search (KIMS) experiment at the Yangyang Underground Laboratory are presented. Low-energy electron-recoil events would be produced by conversion of solar axions into electrons via the axio-electric effect in CsI(Tl) crystals. Using data from an exposure of 34,596 $\rm kg \cdot days$, we set a 90 \% confidence level upper limit on the axion-electron coupling, $g_{ae}$, of $1.39 \times 10^{-11}$ for an axion mass less than 1 keV/$\rm c^2$. This limit is lower than the indirect solar neutrino bound, and fully excludes QCD axions heavier than 0.48 eV/$\rm c^2$ and 140.9 eV/$\rm c^2$ for the DFSZ and KSVZ models respectively.

hep-ex↗

Measurement of the high-energy gamma-ray emission from the Moon with the Fermi Large Area Telescope

We have measured the gamma-ray emission spectrum of the Moon using the data collected by the Large Area Telescope onboard the Fermi satellite during its first 7 years of operation, in the energy range from 30 MeV up to a few GeV. We have also studied the time evolution of the flux, finding a correlation with the solar activity. We have developed a full Monte Carlo simulation describing the interactions of cosmic rays with the lunar surface. The results of the present analysis can be explained in the framework of this model, where the production of gamma rays is due to the interactions of cosmic-ray proton and helium nuclei with the surface of the Moon. Finally, we have used our simulation to derive the cosmic-ray proton and helium spectra near Earth from the Moon gamma-ray data.

astro-ph.HE↗

Understanding and Controlling Water Stability of MOF-74

Metal organic framework (MOF) materials in general, and MOF-74 in particular, have promising properties for many technologically important processes. However, their instability under humid conditions severely restricts practical use. We show that this instability and the accompanying reduction of the CO$_2$ uptake capacity of MOF-74 under humid conditions originate in the water dissociation reaction H$_2$O$\rightarrow$OH+H at the metal centers. After this dissociation, the OH groups coordinate to the metal centers, explaining the reduction in the MOF's CO$_2$ uptake capacity. This reduction thus strongly depends on the catalytic activity of MOF-74 towards the water dissociation reaction. We further show that-while the water molecules themselves only have a negligible effect on the crystal structure of MOF-74-the OH and H products of the dissociation reaction significantly weaken the MOF framework and lead to the observed crystal structure breakdown. With this knowledge, we propose a way to suppress this particular reaction by modifying the MOF-74 structure to increase the water dissociation energy barrier and thus control the stability of the system under humid conditions.

cond-mat.mtrl-sci↗

Computational Topology: Isotopic Convergence to a Stick Knot

Computational topology is a vibrant contemporary subfield and this article integrates knot theory and mathematical visualization. Previous work on computer graphics developed a sequence of smooth knots that were shown to converge point wise to a piecewise linear (PL) approximant. This is extended to isotopic convergence, with that discovery aided by computational experiments. Sufficient conditions to attain isotopic equivalence can be determined a priori. These sufficient conditions need not be tight bounds, providing opportunities for further optimizations. The results presented will facilitate further computational experiments on the theory of PL knots (also known as stick knots), where this theory is less mature than for smooth knots.

math.GT↗

Simulation of Stimulated Brillouin Scattering and Stimulated Raman Scattering In Shock Ignition

We study stimulated Brillouin scattering (SBS) and stimulated Raman scattering (SRS) in shock ignition by comparing fluid and PIC simulations. Under typical parameters for the OMEGA experiments [Theobald \emph{et al}., Phys. Plasmas \textbf{19}, 102706 (2012)], a series of 1D fluid simulations with laser intensities ranging between 2$\times$10$^{15}$ and 2$\times$10$^{16}$ W/cm$^2$ finds that SBS is the dominant instability, which increases significantly with the incident intensity. Strong pump depletion caused by SBS and SRS limits the transmitted intensity at the 0.17n$_c$ to be less than 3.5$\times$10$^{15}$ W/cm$^2$. The PIC simulations show similar physics but with higher saturation levels for SBS and SRS convective modes and stronger pump depletion due to higher seed levels for the electromagnetic fields in PIC codes. Plasma flow profiles are found to be important in proper modeling of SBS and limiting its reflectivity in both the fluid and PIC simulations.

physics.plasm-ph↗

Understanding internal backgrounds of NaI(Tl) crystals toward a 200~kg array for the KIMS-NaI experiment

The Korea Invisible Mass Search (KIMS) collaboration has developed low-background NaI(Tl) crystals that are suitable for the direct detection of WIMP dark matter. With experience built on the KIMS-CsI programs, the KIMS-NaI experiment will consist of a 200~kg NaI(Tl) crystal array surrounded by layers of shielding structures and will be operated at the Yangyang underground laboratory. The goal is to provide an unambiguous test of the DAMA/LIBRA's annual modulation signature. Measurements of six prototype crystals show progress in the reduction of internal contaminations of radioisotopes. Based on our understanding of these measurements, we expect to achieve a background level in the final detector configuration that is less than 1~count/day/keV/kg for recoil energies around 2~keV. The annual modulation sensitivity for the KIMS-NaI experiment shows that an unambiguous 7$σ$ test of the DAMA/LIBRA signature would be possible with a 600~kg$\cdot$year exposure with this system.

physics.ins-det↗

Density modulation-induced absolute laser-plasma-instabilities: simulations and theory

Fluid simulations show that when a sinusoidal density modulation is superimposed on a linear density profile, convective instabilities can become absolutely unstable. This conversion can occur for two-plasmon-decay and stimulated Raman Scattering instabilities under realistic direct-drive inertial confinement fusion conditions and can affect hot electron generation and laser energy deposition. Analysis of the three-wave model shows that a sufficiently large change of the density gradient in a linear density profile can turn convective instabilities into absolute ones. An analytical expression is given for the threshold of the gradient change, which depends on the convective gain only.

physics.plasm-ph↗

Development of the Model of Galactic Interstellar Emission for Standard Point-Source Analysis of Fermi Large Area Telescope Data

Most of the celestial gamma rays detected by the Large Area Telescope (LAT) aboard the Fermi Gamma-ray Space Telescope originate from the interstellar medium when energetic cosmic rays interact with interstellar nucleons and photons. Conventional point and extended source studies rely on the modeling of this diffuse emission for accurate characterization. We describe here the development of the Galactic Interstellar Emission Model (GIEM) that is the standard adopted by the LAT Collaboration and is publicly available. The model is based on a linear combination of maps for interstellar gas column density in Galactocentric annuli and for the inverse Compton emission produced in the Galaxy. We also include in the GIEM large-scale structures like Loop I and the Fermi bubbles. The measured gas emissivity spectra confirm that the cosmic-ray proton density decreases with Galactocentric distance beyond 5 kpc from the Galactic Center. The measurements also suggest a softening of the proton spectrum with Galactocentric distance. We observe that the Fermi bubbles have boundaries with a shape similar to a catenary at latitudes below 20 degrees and we observe an enhanced emission toward their base extending in the North and South Galactic direction and located within 4 degrees of the Galactic Center.

astro-ph.HE↗

A Search of Low-Mass WIMPs with p-type Point Contact Germanium Detector in the CDEX-1 Experiment

The CDEX-1 experiment conducted a search of low-mass (< 10 GeV/c2) Weakly Interacting Massive Particles (WIMPs) dark matter at the China Jinping Underground Laboratory using a p-type point-contact germanium detector with a fiducial mass of 915 g at a physics analysis threshold of 475 eVee. We report the hardware set-up, detector characterization, data acquisition and analysis procedures of this experiment. No excess of unidentified events are observed after subtraction of known background. Using 335.6 kg-days of data, exclusion constraints on the WIMP-nucleon spin-independent and spin-dependent couplings are derived.

hep-ex↗