arXiv subjects

J. M. Yeomans

Publications and source records attributed to J. M. Yeomans.

At least 37 records · Page 2Linked to original sources

arXiv2008

Shearing active gels close to the isotropic-nematic transition

We study numerically the rheological properties of a slab of active gel close o the isotropic-nematic transition. The flow behavior shows strong dependence on sample size, boundary conditions, and on the bulk constitutive curve, which, on entering the nematic phase, acquires an activity-induced discontinuity at the origin. The precursor of this within the metastable isotropic phase for contractile systems ({\em e.g.,} actomyosin gels) gives a viscosity divergence; its counterpart for extensile ({\em e.g.,} {\em B. subtilis}) suspensions admits instead a shear-banded flow with zero apparent viscosity.

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arXiv2008

Dumb-bell swimmers

We investigate the way in which oscillating dumb-bells, a simple microscopic model of apolar swimmers, move at low Reynold's number. In accordance with Purcell's Scallop Theorem a single dumb-bell cannot swim because its stroke is reciprocal in time. However the motion of two or more dumb-bells, with mutual phase differences, is not time reversal invariant, and hence swimming is possible. We use analytical and numerical solutions of the Stokes equations to calculate the hydrodynamic interaction between two dumb-bell swimmers and to discuss their relative motion. The cooperative effect of interactions between swimmers is explored by considering first regular, and then random arrays of dumb-bells. We find that a square array acts as a micropump. The long time behaviour of suspensions of dumb-bells is investigated and compared to that of model polar swimmers.

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arXiv2008

Anisotropic drop morphologies on corrugated surfaces

The spreading of liquid drops on surfaces corrugated with micron-scale parallel grooves is studied both experimentally and numerically. Because of the surface patterning, the typical final drop shape is no longer spherical. The elongation direction can be either parallel or perpendicular to the direction of the grooves, depending on the initial drop conditions. We interpret this result as a consequence of both the anisotropy of the contact line movement over the surface and the difference in the motion of the advancing and receding contact lines. Parallel to the grooves, we find little hysteresis due to the surface patterning and that the average contact angle approximately conforms to Wenzel's law as long as the drop radius is much larger than the typical length scale of the grooves. Perpendicular to the grooves, the contact line can be pinned at the edges of the ridges leading to large contact angle hysteresis.

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arXiv2008

The collapse transition on superhydrophobic surfaces

We investigate the transition between the Cassie-Baxter and Wenzel states of a slowly evaporating, micron-scale drop on a superhydrophobic surface. In two dimensions analytical results show that there are two collapse mechanisms. For long posts the drop collapses when it is able to overcome the free energy barrier presented by the hydrophobic posts. For short posts, as the drop loses volume, its curvature increases allowing it to touch the surface below the posts. We emphasise the importance of the contact line retreating across the surface as the drop becomes smaller: this often preempts the collapse. In a quasi-three dimensional simulation we find similar behaviour, with the additional feature that the drop can de-pin from all but the peripheral posts, so that its base resembles an inverted bowl.

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arXiv2007

Steady-state hydrodynamic instabilities of active liquid crystals: Hybrid lattice Boltzmann simulations

We report hybrid lattice Boltzmann (HLB) simulations of the hydrodynamics of an active nematic liquid crystal sandwiched between confining walls with various anchoring conditions. We confirm the existence of a transition between a passive phase and an active phase, in which there is spontaneous flow in the steady state. This transition is attained for sufficiently ``extensile'' rods, in the case of flow-aligning liquid crystals, and for sufficiently ``contractile'' ones for flow-tumbling materials. In a quasi-1D geometry, deep in the active phase of flow-aligning materials, our simulations give evidence of hysteresis and history-dependent steady states, as well as of spontaneous banded flow. Flow-tumbling materials, in contrast, re-arrange themselves so that only the two boundary layers flow in steady state. Two-dimensional simulations, with periodic boundary conditions, show additional instabilities, with the spontaneous flow appearing as patterns made up of ``convection rolls''. These results demonstrate a remarkable richness (including dependence on anchoring conditions) in the steady-state phase behaviour of active materials, even in the absence of external forcing; they have no counterpart for passive nematics. Our HLB methodology, which combines lattice Boltzmann for momentum transport with a finite difference scheme for the order parameter dynamics, offers a robust and efficient method for probing the complex hydrodynamic behaviour of active nematics.

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arXiv2007

Lattice Boltzmann simulations of spontaneous flow in active liquid crystals: the role of boundary conditions

Active liquid crystals or active gels are soft materials which can be physically realised e.g. by preparing a solution of cytoskeletal filaments interacting with molecular motors. We study the hydrodynamics of an active liquid crystal in a slab-like geometry with various boundary conditions, by solving numerically its equations of motion via lattice Boltzmann simulations. In all cases we find that active liquid crystals can sustain spontaneous flow in steady state contrarily to their passive counterparts, and in agreement with recent theoretical predictions. We further find that conflicting anchoring conditions at the boundaries lead to spontaneous flow for any value of the 'activity' parameter, while with unfrustrated anchoring at all boundaries spontaneous flow only occurs when the activity exceeds a critical threshold. We finally discuss the dynamic pathway leading to steady state in a few selected cases.

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arXiv2007

Swimming with a friend at low Reynolds number

We investigate the hydrodynamic interactions between microorganisms swimming at low Reynolds number. By considering simple model swimmers, and combining analytic and numerical approaches, we investigate the time-averaged flow field around a swimmer. At short distances the swimmer behaves like a pump. At large distances the velocity field depends on whether the swimming stroke is invariant under a combined time-reversal and parity transformation. We then consider two swimmers and find that the interaction between them consists of two parts; a dead term, independent of the motion of the second swimmer, which takes the expected dipolar form and a live term resulting from the simultaneous swimming action of both swimmers which does not. We argue that, in general, the latter dominates. The swimmer--swimmer interaction is a complicated function of their relative displacement, orientation and phase, leading to motion that can be attractive, repulsive or oscillatory.

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arXiv2007

Modeling microscopic swimmers at low Reynolds number

We employ three numerical methods to explore the motion of low Reynolds number swimmers, modeling the hydrodynamic interactions by means of the Oseen tensor approximation, lattice Boltzmann simulations and multiparticle collision dynamics. By applying the methods to a three bead linear swimmer, for which exact results are known, we are able to compare and assess the effectiveness of the different approaches. We then propose a new class of low Reynolds number swimmers, generalized three bead swimmers that can change both the length of their arms and the angle between them. Hence we suggest a design for a microstructure capable of moving in three dimensions. We discuss multiple bead, linear microstructures and show that they are highly efficient swimmers. We then turn to consider the swimming motion of elastic filaments. Using multiparticle collision dynamics we show that a driven filament behaves in a qualitatively similar way to the micron-scale swimming device recently demonstrated by Dreyfus et al.

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arXiv2006

Modelling contact angle hysteresis on chemically patterned and superhydrophobic surfaces

We investigate contact angle hysteresis on chemically patterned and superhydrophobic surfaces, as the drop volume is quasi-statically increased and decreased. We consider both two, and three, dimensions using analytical and numerical approaches to minimise the free energy of the drop. In two dimensions we find, in agreement with other authors, a slip, jump, stick motion of the contact line. In three dimensions this behaviour persists, but the position and magnitude of the contact line jumps are sensitive to the details of the surface patterning. In two dimensions we identify analytically the advancing and receding contact angles on the different surfaces and we use numerical insights to argue that these provide bounds for the three dimensional cases. We present explicit simulations to show that a simple average over the disorder is not sufficient to predict the details of the contact angle hysteresis, and to support an explanation for the low contact angle hysteresis of suspended drops on superhydrophobic surfaces.

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arXiv2006

Controlling drop size and polydispersity using chemically patterned surfaces

We explore numerically the feasibility of using chemical patterning to control the size and polydispersity of micron-scale drops. The simulations suggest that it is possible to sort drops by size or wetting properties by using an array of hydrophilic stripes of different widths. We also demonstrate that monodisperse drops can be generated by exploiting the pinning of a drop on a hydrophilic stripe. Our results follow from using a lattice Boltzmann algorithm to solve the hydrodynamic equations of motion of the drops and demonstrate the applicability of this approach as a design tool for micofluidic devices with chemically patterned surfaces.

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arXiv2006

Stabilising the Blue Phases

We present an investigation of the phase diagram of cholesteric liquid crystals within the framework of Landau - de Gennes theory. The free energy is modified to incorporate all three Frank elastic constants and to allow for a temperature dependent pitch in the cholesteric phase. It is found that the region of stability of the cubic blue phases depends significantly on the value of the elastic constants, being reduced when the bend elastic constant is larger than splay and when twist is smaller than the other two. Most dramatically we find a large increase in the region of stability of blue phase I, and a qualitative change in the phase diagram, in a system where the cholesteric phase displays helix inversion.

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arXiv2006

Polymer packaging and ejection in viral capsids: shape matters

We use a mesoscale simulation approach to explore the impact of different capsid geometries on the packaging and ejection dynamics of polymers of different flexibility. We find that both packing and ejection times are faster for flexible polymers. For such polymers a sphere packs more quickly and ejects more slowly than an ellipsoid. For semiflexible polymers, however, the case relevant to DNA, a sphere both packs and ejects more easily. We interpret our results by considering both the thermodynamics and the relaxational dynamics of the polymers. The predictions could be tested with bio-mimetic experiments with synthetic polymers inside artificial vesicles. Our results suggest that phages may have evolved to be roughly spherical in shape to optimise the speed of genome ejection, which is the first stage in infection.

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arXiv2006

Lattice Boltzmann simulations of phase separation in chemically reactive binary fluids

We use a lattice Boltzmann method to study pattern formation in chemically reactive binary fluids in the regime where hydrodynamic effects are important. The coupled equations solved by the method are a Cahn-Hilliard equation, modified by the inclusion of a reactive source term, and the Navier-Stokes equations for conservation of mass and momentum. The coupling is two-fold, resulting from the advection of the order-parameter by the velocity field and the effect of fluid composition on pressure. We study the the evolution of the system following a critical quench for a linear and for a quadratic reaction source term. Comparison is made between the high and low viscosity regimes to identify the influence of hydrodynamic flows. In both cases hydrodynamics is found to influence the pathways available for domain growth and the eventual steady-states.

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arXiv2006

Rheology of cholesteric blue phases

Blue phases of cholesteric liquid crystals offer a spectacular example of naturally occurring disclination line networks. Here we numerically solve the hydrodynamic equations of motion to investigate the response of three types of blue phases to an imposed Poiseuille flow. We show that shear forces bend and twist and can unzip the disclination lines. Under gentle forcing the network opposes the flow and the apparent viscosity is significantly higher than that of an isotropic liquid. With increased forcing we find strong shear thinning corresponding to the disruption of the defect network. As the viscosity starts to drop, the imposed flow sets the network into motion. Disclinations break-up and re-form with their neighbours in the flow direction. This gives rise to oscillations in the time-dependent measurement of the average stress.

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arXiv2006

Dynamics of sliding drops on superhydrophobic surfaces

We use a free energy lattice Boltzmann approach to investigate numerically the dynamics of drops moving across superhydrophobic surfaces. The surfaces comprise a regular array of posts small compared to the drop size. For drops suspended on the posts the velocity increases as the number of posts decreases. We show that this is because the velocity is primarily determined by the contact angle which, in turn, depends on the area covered by posts. Collapsed drops, which fill the interstices between the posts, behave in a very different way. The posts now impede the drop behaviour and the velocity falls as their density increases.

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arXiv2006

Drop dynamics on chemically patterned surfaces

We compare numerical and experimental results exploring the behaviour of liquid drops moving across a surface patterned with hydrophobic and hydrophilic stripes. A lattice Boltzmann algorithm is used to solve the hydrodynamic equations of motion of the drops allowing us to investigate their behaviour as the stripe widths and the wettability contrast are altered. We explain how the motion of the drop is determined by the interplay between the driving force and the variation in surface force as the drop moves between regions of different contact angle and we find that the shape of the drops can undergo large periodic deviations from spherical. When compared, the numerical results agree well with experiments on micron--scale drops moving across substrates patterned by microcontact printing.

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arXiv2005

Control of drop positioning using chemical patterning

We explore how chemical patterning on surfaces can be used to control drop wetting. Both numerical and experimental results are presented to show how the dynamic pathway and equilibrium shape of the drops are altered by a hydrophobic grid. The grid proves a successful way of confining drops and we show that it can be used to alleviate {\it mottle}, a degradation in image quality which results from uneven drop coalescence due to randomness in the positions of the drops within the jetted array.

cond-mat.soft↗

arXiv2005

Switching hydrodynamics in multi-domain, twisted nematic, liquid crystal devices

We study the switching dynamics in two-domain and four-domain twisted nematic liquid crystal devices. The equilibrium configuration of these devices involves the coexistence of regions characterised by different handedness of the inherent director twist. At the boundaries between these regions there are typically disclinations lines. The dynamics of the disclination lines controls the properties, and in particular the switching speed, of the devices. We describe their motion using a numerical solution of the Beris-Edwards equations of liquid crystal hydrodynamics. Hence we are able to explain why a conventional two-domain device switches off slowly and to propose a device design which circumvents this problem. We also explain the patterns of disclination creation and annihilation that lead to switching in the four-domain twisted nematic device.

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