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J. Miao

Publications and source records attributed to J. Miao.

At least 19 recordsLinked to original sources

3D Imaging of Complex Skyrmion and Hopf Topologies in an Extended Sample

Spin textures are key for emergent magnetic phenomena such as topological protection and underpin novel spintronic device paradigms based on racetrack memory, logic gates, and neuromorphic computing. Using a coherent diffractive imaging technique called vector ptycho-tomography, in combination with algorithms that are robust to noise, we image the 3D magnetic texture of skyrmion and Hopf topologies with no prior assumptions about the sample. This directly reveals experimentally for the first time an extended 3D skyrmion lattice, including the domain wall shape, topological charge, helicity, and Hopf index. Our findings demonstrate experimentally that dipole stabilized skyrmions in Fe/Gd multilayers exhibit barrel-shaped skyrmion tubes with a twisted helicity, transitioning from N$\'e$el-type winding at the surfaces to both clockwise and counterclockwise Bloch-type winding in the bulk, that can also be described as fractional hopfions. We image a lattice of 24 skyrmions with topological charge 1, average depth-dependent domain wall width of 23 to 40 nm, depth-dependent twisted helicity from $\pm$155$\deg$ to $\pm$30$\deg$, and fractional Hopf index of $\pm$0.3. Over 10 TB of data were analyzed to yield a fully-resolved 3D reconstruction over a >0.4 $\mu$m$^3$ volume, with high fidelity down to the Nyquist limit of 8 nm. This method fills a key gap in the current landscape of magnetic imaging by enabling high-resolution, element-specific 3D reconstructions of full-field extended spin textures - offering a new route for exploring the topological complexity of magnetic materials in three dimensions.

cond-mat.mtrl-sci

Large non-reciprocal charge transport in Pt2MnGe up to room temperature

Non-reciprocal charge transport that is strongly associated with the structural or magnetic chirality of the quantum materials system is one of the most exotic properties of condensed matter physics. Here, using magnetic alloys film Pt2MnGe, we have realized the large non-reciprocal charge transport up to room temperature, which roots in the organic combination of chirality dependent carrier scattering and special magnetic configurations. In this framework, the conduction electrons are scattered asymmetrically by the emerging non-zero vector spin chirality under in-plane magnetic field, resulting in robust non-reciprocal response. More astonishingly, the vector spin chirality in Pt2MnGe film can be reversed by a spin-polarized current through spin Hall effect in a junction with Pt layer. Our work resolves the general limitation of non-reciprocal charge transport to cryogenic temperatures, and paves the way for extending its applications in the emerging field of chiral spintronics.

cond-mat.mtrl-sci

Interface-driven electrical magnetochiral anisotropy in Pt/PtMnGa bilayers

Nonreciprocal charge transport, which is frequently termed as electrical magnetochiral anisotropy (EMCA) in chiral conductors, touches the most important elements of modern condensed matter physics. Here, we have investigated the EMCA in Pt/PtMnGa (PMG) bilayers with the assitance of nonequilibrium fluctuation theorems. Large EMCA in the Pt/PMG bilayers can be attributed to nonreciprocal response of an interface-driven chiral transport channel. Due to the presence of large charge fluctuations for small current region, higher order EMCA coefficients should be added and they are all functions of current. A combination of asymmetrical electron scattering and spin-dependent scattering furnish the PMG thickness dependent chiral transport behaviors in Pt/PMG bilayers. The dramatically enhanced anomalous Hall angle of PMG further demonstrates the modified surface state properties by strong spin-orbit coupling.

cond-mat.mtrl-sci

Decoupling bulk and surface recombination properties in silicon by depth-dependent carrier lifetime measurements

Muons, as a bulk probe of materials, have been used to study the depth profile of charge carrier kinetics in Si wafers by scanning the muon implantation depth. The photoexcited muon spin spectroscopy technique can optically generate excess carriers in semiconductor wafers, while muons can measure the excess carrier density. As a result, carrier recombination lifetime spectra can be obtained. The depth-dependent lifetime spectra enable us to accurately measure the bulk carrier lifetime and surface recombination velocity by fitting the spectra to a simple 1-dimensional diffusion model. Unlike other traditional lifetime spectroscopy techniques, the bulk and surface recombination properties can be readily de-convoluted in this method. Here, we have applied the technique to study silicon wafers both with and without passivation treatment, and have demonstrated that the model can correctly describe the carrier kinetics in these two cases.

cond-mat.mtrl-sci

Disorder dependent spin-orbit torques in L10 FePt single layer

We report spin-orbit torques (SOT) in L10-ordered perpendicularly magnetized FePt single layer, which is significantly influenced by disorder. Recently, self-induced SOT in L10-FePt single layer has been investigated, which is ascribed to the composition gradient along the film normal direction. However, the determined mechanisms for magnetization switching have not been fully studied. With varying growth temperatures, we have prepared FePt single layers with same thickness (3 nm) but with different disordering. We have found that nearly full magnetization switching only happens in more disordered films, and the magnetization switching ratio becomes smaller as increasing L10 ordering. The method for deriving effective spin torque fields in the previous studies cannot fully explain the spin current generation and self-induced SOT in L10-FePt single layer. Combined with Magneto-Optical Kerr Effect microscopy and anomalous Hall effect measurements, we concluded that the disorder should determine the formation of domain walls, as well as the spin current generation.

cond-mat.mtrl-sci

Intrinsic mechanism for anisotropic magnetoresistance and experimental confirmation in Co$_x$Fe$_{1-x}$ single-crystal films

Using first-principles transport calculations, we predict that the anisotropic magnetoresistance (AMR) of single-crystal Co$_x$Fe$_{1-x}$ alloys is strongly dependent on the current orientation and alloy concentration. An intrinsic mechanism for AMR is found to arise from the band crossing due to magnetization-dependent symmetry protection. These special $k$-points can be shifted towards or away from the Fermi energy by varying the alloy composition and hence the exchange splitting, thus allowing AMR tunability. The prediction is confirmed by delicate transport measurements, which further reveal a reciprocal relationship of the longitudinal and transverse resistivities along different crystal axes.

cond-mat.mtrl-sci

Spin-orbit torques driven by the interface-generated spin currents

The spin currents generated by spin-orbit coupling (SOC) in the nonmagnetic metal layer or at the interface with broken inversion symmetry are of particular interest and importance. Here, we have explored the spin current generation mechanisms through the spin-orbit torques (SOTs) measurements in the Ru/Fe heterostructures with weak perpendicular magnetic anisotropy (PMA). Although the spin Hall angle (SHA) of Ru is smaller than that in Pt, Ta or W, reversible SOT in Ru/Fe heterostructures can still be realized. Through non-adiabatic harmonic Hall voltage measurements and macrospin simulation, the effective SHA in Ru/Fe heterostructures is compared with Pt. Moreover, we also explore that the spin current driven by interface strongly depends on the electrical conductivities. Our results suggest a new method for efficiently generating finite spin currents in ferromagnet/nonmagnetic metal bilayers, which establishes new opportunities for fundamental study of spin dynamics and transport in ferromagnetic systems.

cond-mat.mtrl-sci

Spin Hall magnetoresistance in Pt/YIG bilayers via varying magnon excitation

Spin Hall magnetoresistance (SMR) and magnon excitation magnetoresistance (MMR) that all generate via the spin Hall effect and inverse spin Hall effect in a nonmagnetic material are always related to each other. However, the influence of magnon excitation for SMR is often overlooked due to the negligible MMR. Here, we investigate the SMR in Pt/Y3Fe5O12 (YIG) bilayers from 5 to 300K, in which the YIG are treated after Ar+-ion milling. The SMR in the treated device is smaller than in the non-treated. According to theoretical simulation, we attribute this phenomenon to the reduction of the interfacial spin-mixing conductance at the treated Pt/YIG interface induced by the magnon suppression. Our experimental results point out that the SMR and the MMR are inter-connected, and the former could be modulated via magnon excitation. Our findings provide a new approach for separating and clarifying the underlying mechanisms.

cond-mat.mtrl-sci

Nonvolatile ferroelectric field control of the anomalous Hall effect in BiFeO3/SrRuO3 bilayer

In this work, the BiFeO3 (BFO)/SrRuO3 (SRO) heterostructure was fabricated and the anomalous Hall effect (AHE) was investigated the in BFO/SRO. It is found the nonmonotonic anomalous Hall resistivity behavior in BFO/SRO is originated from the inhomogeneous SRO layer instead of the topological Hall effect. It is surprised that the AHE in BFO/SRO structure can be manipulated by ferroelectric polarization of BFO. Moreover, an inhomogeneous phenomenological model has been applied on those structure. Furthermore, the modification of band structure in SRO under ferroelectric polarization was discussed by first principle calculation. The ferroelectric-manipulated AHE suggests a new pathway to realize nonvolatile, reversible and low energy-consuming voltage-controlled spintronic devices.

cond-mat.str-el

Combination of informational storage and logical processing based on an all-oxide asymmetric multiferroic tunnel junction

Multiferroic tunnel junctions (MFTJs) have already been proved to be promising candidates for application in spintronics devices. The coupling between tunnel magnetoresistance (TMR) and tunnel electroresistance (TER) in MFTJs can provide four distinct resistive states in a single memory cell. Here we show that in an all-oxide asymmetric MFTJ of La0.7Sr0.3MnO3 /PbZr0.2Ti0.8O3 /La0.7Te0.3MnO3 (LSMO/PZT/LTMO) with p-type and n-type electrodes, the intrinsic rectification is observed and can be modified by the ferroelectric polarization of PZT. Owing to the combined TMR, TER and diode effects, two different groups of four resistive states under opposite reading biases are performed. With two parallel asymmetric junctions and the appropriate series resistance, the coexistence of logic units and quaternary memory cells can be realized in the same array devices. The asymmetric MFTJ structure enables more possibilities for designing next generation of multi-states memory and logical devices with higher storage density, lower energy consumption and significantly increased integration level.

cond-mat.mtrl-sci

Controlling spin-orbit torque by polarization field in multiferroic BiFeO3 based heterostructures

In the last few years, some ideas of electric manipulations in ferromagnetic heterostructures have been proposed for developing next generation spintronic devices. Among them, the magnetization switching driven by spin-orbit torque (SOT) is being intensely pursued. Especially, how to control the switching current density, which is expected to enrich device functionalities, has aroused much interest among researchers all over the world. In this paper, a novel method to adjust the switching current is proposed, and the BiFeO3 (BFO) based heterostructures with opposite spontaneous polarizations fields show huge changes in both perpendicular magnetic anisotropy and the SOT-induced magnetization switching. The damping-like torques were estimated by using harmonic Hall voltage measurement, and the variation of effective spin Hall angles for the heterostructures with opposite polarizations was calculated to be 272%. At the end of this paper, we have also demonstrated the possible applications of our structure in memory and reconfigurable logic devices.

cond-mat.mtrl-sci

Anomalous Hall effect induced spin Hall magnetoresistance in an antiferromagnetic Cr2O3/Ta bilayer

The spin Hall magnetoresistance (SMR) and anomalous Hall effect (AHE) are observed in a Cr2O3/Ta structure. The structural and surface morphology of Cr2O3/Ta bilayers have been investigated. Temperature dependence of longitudinal and transverse resistances measurements confirm the relationship between SMR and AHE signals in Cr2O3/Ta structure. By means of temperature dependent magnetoresistance measurements, the physical origin of SMR in the Cr2O3/Ta structure is revealed, and the contribution to the SMR from the spin current generated by AHE has been proved. The so-called boundary magnetization due to the bulk antiferromagnetic order in Cr2O3 film may be responsible for the relationship of SMR and AHE in the Cr2O3/Ta bilayer.

cond-mat.mtrl-sci

Negative spin Hall magnetoresistance in antiferromagnetic Cr2O3/Ta bilayer at low temperature region

We investigate the observation of negative spin Hall magnetoresistance (SMR) in antiferromagnetic Cr2O3/Ta bilayers at low temperature. The sign of the SMR signals is changed from positive to negative monotonously from 300 K to 50 K. The change of the signs for SMR is related with the competitions between the surface ferromagnetism and bulky antiferromagnetic of Cr2O3. The surface magnetizations of Cr2O3 (0001) is considered to be dominated at higher temperature, while the bulky antiferromagnetics gets to be robust with decreasing of temperature. The slopes of the abnormal Hall curves coincide with the signs of SMR, confirming variational interface magnetism of Cr2O3 at different temperature. From the observed SMR ratio under 3 T, the spin mixing conductance at Cr2O3/Ta interface is estimated to be 1.12*10^14 (ohm^-1*m^-2), which is comparable to that of YIG/Pt structures and our early results of Cr2O3/W. (Appl. Phys. Lett. 110, 262401 (2017))

cond-mat.mtrl-sci

A new method for measuring excess carrier lifetime in bulk silicon: Photoexcited muon spin spectroscopy

We have measured the optically injected excess carrier lifetime in silicon using photoexcited muon spin spectroscopy. Positive muons implanted deep in a wafer can interact with the excess carriers and directly probe the bulk carrier lifetime whilst minimizing the effect from surface recombination. The method is based on the relaxation rate of muon spin asymmetry, which depends on the excess carrier concentration. The underlying microscopic mechanism has been understood by simulating the four-state muonium model in Si under illumination. We apply the technique to different injection levels and temperatures, and demonstrate its ability for injection- and temperature-dependent lifetime spectroscopy.

cond-mat.mtrl-sci

Electronic structure of FeS

Here we report the electronic structure of FeS, a recently identified iron-based superconductor. Our high-resolution angle-resolved photoemission spectroscopy studies show two hole-like ($α$ and $β$) and two electron-like ($η$ and $δ$) Fermi pockets around the Brillouin zone center and corner, respectively, all of which exhibit moderate dispersion along $k_z$. However, a third hole-like band ($γ$) is not observed, which is expected around the zone center from band calculations and is common in iron-based superconductors. Since this band has the highest renormalization factor and is known to be the most vulnerable to defects, its absence in our data is likely due to defect scattering --- and yet superconductivity can exist without coherent quasiparticles in the $γ$ band. This may help resolve the current controversy on the superconducting gap structure of FeS. Moreover, by comparing the $β$ bandwidths of various iron chalcogenides, including FeS, FeSe$_{1-x}$S$_x$, FeSe, and FeSe$_{1-x}$ Te$_x$, we find that the $β$ bandwidth of FeS is the broadest. However, the band renormalization factor of FeS is still quite large, when compared with the band calculations, which indicates sizable electron correlations. This explains why the unconventional superconductivity can persist over such a broad range of isovalent substitution in FeSe$_{1-x}$Te$_{x}$ and FeSe$_{1-x}$S$_{x}$.

cond-mat.supr-con

Enhanced spin-orbit torques in MnAl/Ta films with improving chemical ordering

We report the enhancement of spin-orbit torques in MnAl/Ta films with improving chemical ordering through annealing. The switching current density is increased due to enhanced saturation magnetization MS and effective anisotropy field HK after annealing. Both damplinglike effective field HD and fieldlike effective field HF have been increased in the temperature range of 50 to 300 K. HD varies inversely with MS in both of the films, while the HF becomes liner dependent on 1/MS in the annealed film. We infer that the improved chemical ordering has enhanced the interfacial spin transparency and the transmitting of the spin current in MnAl layer.

cond-mat.mtrl-sci

Surface electronic structure and evidence of plain s-wave superconductivity in (Li0.8Fe0.2)OHFeSe

(Li0.8Fe0.2)OHFeSe is a newly-discovered intercalated iron-selenide superconductor with a Tc above 40 K, which is much higher than the Tc of bulk FeSe (8 K). Here we report a systematic study of (Li0.8Fe0.2)OHFeSe by low temperature scanning tunneling microscopy (STM). We observed two kinds of surface terminations, namely FeSe and (Li0.8Fe0.2)OH surfaces. On the FeSe surface, the superconducting state is fully gapped with double coherence peaks, and a vortex core state with split peaks near EF is observed. Through quasi-particle interference (QPI) measurements, we clearly observed intra- and inter-pocket scatterings in between the electron pockets at the M point, as well as some evidence of scattering that connects gamma and M points. Upon applying magnetic field, the QPI intensity of all the scattering channels are found to behave similarly. Furthermore, we studied impurity effects on the superconductivity by investigating intentionally introduced impurities and intrinsic defects. We observed that magnetic impurities such as Cr adatoms can induce in-gap states and suppress superconductivity. However, nonmagnetic impurities such as Zn adatoms do not induce visible in-gap states. Meanwhile, we show that Zn adatoms can induce in-gap states in thick FeSe films, which is believed to have an (s+-)wave pairing symmetry. Our experimental results suggest it is likely that (Li0.8Fe0.2)OHFeSe is a plain s-wave superconductor, whose order parameter has the same sign on all Fermi surface sections.

cond-mat.supr-con

Anomalous Hall effect and spin orbit torques in MnGa/IrMn films: Modification from strong spin Hall effect of antiferromagnet

We report systematic measurements of anomalous Hall effect(AHE) and spin orbit torques(SOT) in MnGa/IrMn films,, in which a single MnGa epitaxial layer reveals obvious orbital two-channel Kondo (2CK) effect. As increasing the thickness of the antiferromagnet IrMn, the strong spin Hall effect(SHE)has gradually suppressed the orbital 2CK effect and modified the AHE of MnGa.A scaling involving multiple competing scattering mechanisms has been used to distinguish different contributions to the modified AHE. Finally, the sizeable SOT in the MnGa/IrMn films induced by the strong SHE of IrMn have been investigated.The IrMn layer also supplies an in-plane exchange bias field and enables nearly field-free magnetization reversal.

cond-mat.mes-hall