arXiv subjects

J. Orenstein

Publications and source records attributed to J. Orenstein.

At least 37 records · Page 2Linked to original sources

arXiv2012

Coherent Propagation of Spin Helices in a Quantum-Well Confined Electron Gas

We use phase-resolved transient grating spectroscopy to measure the propagation of spin helices in a high mobility $n$-GaAs/AlGaAs quantum well with an applied in-plane electric field. At relatively low fields helical modes crossover from overdamped excitations where the spin-precession period exceeds the spin lifetime, to a regime of coherent propagation where several spin-precession periods can be observed. We demonstrate that the envelope of a spin polarization packet reaches a current-driven velocity of 10$^7$ cm s$^{-1}$ in an applied field of 70 V cm$^{-1}$.

cond-mat.mes-hall↗

arXiv2012

Berry phase mechanism for optical gyrotropy in stripe-ordered cuprates

Optical gyrotropy, the lifting of degeneracy between left and right circularly polarized light, can be generated by either time-reversal or chiral symmetry breaking. In the high-$T_c$ superconductor La$_{2-x}$Ba$_x$CuO$_4$ (LBCO), gyrotropy onsets at the same temperature as charge stripe order, suggesting that the rotation of the stripe direction from one plane to the next generates a helical pattern that breaks chiral symmetry. In order to further test this chiral stacking hypothesis it is necessary to develop an understanding of the physical mechanism by which chirality generates gyrotropy. In this paper we show that optical gyrotropy is a consequence of Berry curvature in the momentum space of chiral metals. We describe a physical picture showing that gyrotropy in chiral metals is closely related to the anomalous Hall effect in itinerant ferromagnets. We then calculate the magnitude of the gyrotropic response for a given Berry curvature using the semiclassical picture of anomalous velocity and Boltzmann transport theory. To connect this physical picture with experiment, we calculate the Berry curvature in two tight-binding models. The first model is motivated by the structure of LBCO and illustrates how the gyrotropy is created when the stripe perturbations are added to a simple cubic model. In the second model, we examine the dramatic enhancement of the gyrotropic coefficient when Rashba spin-orbit coupling is introduced. The magnitude of the rotation of polarization on reflection expected based these models is calculated and compared with experimental data.

cond-mat.str-el↗

arXiv2012

Kerr effect as evidence of gyrotropic order in the cuprates

The Kerr effect can arise in a time-reversal invariant dissipative medium that is "gyrotropic", i.e. one that breaks inversion ($\mathcal I$) and all mirror symmetries. Examples of such systems include electron analogs of cholesteric liquid crystals, and their descendants, such as systems with chiral charge ordering. We present arguments that the striking Kerr onset seen in the pseudogap phase of a large number of cuprate high temperature superconductors is evidence of chiral charge ordering. We discuss additional experimental consequences of a phase transition to a gyrotropic state, including the appearance of a zero field Nernst effect.

cond-mat.str-el↗

arXiv2012

Doppler velocimetry of spin propagation in a two-dimensional electron gas

Controlling the flow of electrons by manipulation of their spin is a key to the development of spin-based electronics. While recent demonstrations of electrical-gate control in spin-transistor configurations show great promise, operation at room temperature remains elusive. Further progress requires a deeper understanding of the propagation of spin polarization, particularly in the high mobility semiconductors used for devices. Here we report the application of Doppler velocimetry to resolve the motion of spin-polarized electrons in GaAs quantum wells driven by a drifting Fermi sea. We find that the spin mobility tracks the high electron mobility precisely as a function of T. However, we also observe that the coherent precession of spins driven by spin-orbit interaction, which is essential for the operation of a broad class of spin logic devices, breaks down at temperatures above 150 K for reasons that are not understood theoretically.

cond-mat.mes-hall↗

arXiv2012

Observation of Coherent Helimagnons and Gilbert damping in an Itinerant Magnet

We study the magnetic excitations of itinerant helimagnets by applying time-resolved optical spectroscopy to Fe0.8Co0.2Si. Optically excited oscillations of the magnetization in the helical state are found to disperse to lower frequency as the applied magnetic field is increased; the fingerprint of collective modes unique to helimagnets, known as helimagnons. The use of time-resolved spectroscopy allows us to address the fundamental magnetic relaxation processes by directly measuring the Gilbert damping, revealing the versatility of spin dynamics in chiral magnets. (*These authors contributed equally to this work)

cond-mat.str-el↗

arXiv2012

Dynamical Interplay between Coexisting Orders in the Electron-Doped Cuprate Superconductor Nd_{2-x}Ce_xCuO_4

We use coherent pump-probe spectroscopy to measure the photoinduced reflectivity \DeltaR, and complex dielectric function, δ\in, of the electron-doped cuprate superconductor Nd_{2-x}Ce_xCuO_{4+δ} at a value of x near optimal doping, as a function of time, temperature, and laser fluence. We observe the onset of a negative \DeltaR at T=85 K, above the superconducting transition temperature, T_c, of 23 K, that exhibits a form of scaling consistent with critical fluctuations in the time domain. A positive ΔR onsets at T_c that we associate with superconducting order. We find that the two signals are strongly coupled below T_c, in a manner that suggests a repulsive interaction between superconductivity and antiferromagnetic correlations.

cond-mat.supr-con↗

arXiv2011

Measurement of electron-hole friction in an n-doped GaAs/AlGaAs quantum well using optical transient grating spectroscopy

We use phase-resolved transient grating spectroscopy to measure the drift and diffusion of electron-hole density waves in a semiconductor quantum well. The unique aspects of this optical probe allow us to determine the frictional force between a two-dimensional Fermi liquid of electrons and a dilute gas of holes. Knowledge of electron-hole friction enables prediction of ambipolar dynamics in high-mobility electron systems.

cond-mat.mes-hall↗

arXiv2011

Random walk approach to spin dynamics in a two-dimensional electron gas with spin-orbit coupling

We introduce and solve a semi-classical random walk (RW) model that describes the dynamics of spin polarization waves in zinc-blende semiconductor quantum wells. We derive the dispersion relations for these waves, including the Rashba, linear and cubic Dresselhaus spin-orbit interactions, as well as the effects of an electric field applied parallel to the spin polarization wavevector. In agreement with fully quantum mechanical calculations [Kleinert and Bryksin, Phys. Rev. B \textbf{76}, 205326 (2007)], the RW approach predicts that spin waves acquire a phase velocity in the presence of the field that crosses zero at a nonzero wavevector, $q_0$. In addition, we show that the spin-wave decay rate is independent of field at $q_0$ but increases as $(q-q_0)^2$ for $q\neq q_0$. These predictions can be tested experimentally by suitable transient spin grating experiments.

cond-mat.mes-hall↗

arXiv2011

From a single-band metal to a high-temperature superconductor via two thermal phase transitions

The nature of the pseudogap phase of cuprate high-temperature superconductors is a major unsolved problem in condensed matter physics. We studied the commencement of the pseudogap state at temperature T* using three different techniques (angle-resolved photoemission spectroscopy, polar Kerr effect, and time-resolved reflectivity) on the same optimally-doped Bi2201 crystals. We observed the coincident, abrupt onset at T* of a particle-hole asymmetric antinodal gap in the electronic spectrum, a Kerr rotation in the reflected light polarization, and a change in the ultrafast relaxational dynamics, consistent with a phase transition. Upon further cooling, spectroscopic signatures of superconductivity begin to grow close to the superconducting transition temperature (Tc), entangled in an energy-momentum-dependent fashion with the pre-existing pseudogap features, ushering in a ground state with coexisting orders.

cond-mat.supr-con↗

arXiv2011

Optical non-reciprocity in magnetic structures related to high-Tc superconductors

Recent neutron scattering [1,2], and optical measurements [3,4] have detected evidence in underdoped cuprate superconductors for a phase transition near the pseudogap onset temperature T* to a time reversal-breaking state. The neutron scattering indicates antiferromagnetic ordering, while it is often assumed that optical polarization rotation requires at least a weak ferromagnetic component. In this note we identify several antiferromagnetic structures, compatible with neutron scattering data, that allow intrinsic polarization rotation through the magnetoelectic effect.

cond-mat.str-el↗

arXiv2010

Determination of the spin-flip time in ferromagnetic SrRuO3 from time-resolved Kerr measurements

We report time-resolved Kerr effect measurements of magnetization dynamics in ferromagnetic SrRuO3. We observe that the demagnetization time slows substantially at temperatures within 15K of the Curie temperature, which is ~ 150K. We analyze the data with a phenomenological model that relates the demagnetization time to the spin flip time. In agreement with our observations the model yields a demagnetization time that is inversely proportional to T-Tc. We also make a direct comparison of the spin flip rate and the Gilbert damping coefficient showing that their ratio very close to kBTc, indicating a common origin for these phenomena.

cond-mat.mtrl-sci↗

arXiv2010

Evidence for effective thermal boundary resistance from magnon/phonon disequilibrium

We use the time-resolved magneto-optical Kerr effect (TRMOKE) to measure the local temperature and heat flow dynamics in ferromagnetic SrRuO3 thin films. After heating by a pump pulse, the film temperature decays exponentially, indicating that the heat flow out of the film is limited by the film/substrate interface. We show that this behavior is consistent with an effective boundary resistance resulting from disequilibrium between the spin and phonon temperatures in the film.

cond-mat.mtrl-sci↗

arXiv2009

Confinement-induced Berry phase and helicity-dependent photocurrents

The photocurrent in an optically active metal is known to contain a component that switches sign with the helicity of the incident radiation. At low frequencies, this current depends on the orbital Berry phase of the Bloch electrons via the "anomalous velocity" of Karplus and Luttinger. We consider quantum wells in which the parent material, such as GaAs, is not optically active and the relevant Berry phase only arises as a result of quantum confinement. Using an envelope approximation that is supported by numerical tight-binding results, it is shown that the Berry phase contribution is determined for realistic wells by a cubic Berry phase intrinsic to the bulk material, the well width, and the well direction. These results for the magnitude of the Berry-phase effect suggest that it may already have been observed in quantum well experiments.

cond-mat.mes-hall↗

arXiv2009

Spin-Charge-Lattice Coupling through Resonant Multi-Magnon Excitations in Multiferroic BiFeO3

Spin-charge-lattice coupling mediated by multi-magnon processes is demonstrated in multiferroic BiFeO3. Experimental evidence of two and three magnons excitations as well as multimagnon coupling at electronic energy scales and high temperatures are reported. Temperature dependent Raman experiments show up to five resonant enhancements of the 2-magnon excitation below the Neel temperature. These are shown to be collective interactions between on-site Fe d-d electronic resonance, phonons and multimagnons

cond-mat.other↗

arXiv2008

Observation of ferromagnetic resonance in strontium ruthenate (SrRuO3)

We report the observation of ferromagnetic resonance (FMR) in SrRuO3 using the time-resolved magneto-optical Kerr effect. The FMR oscillations in the time-domain appear in response to a sudden, optically induced change in the direction of easy-axis anistropy. The high FMR frequency, 250 GHz, and large Gilbert damping parameter, alpha ~ 1, are consistent with strong spin-orbit coupling. We find that the parameters associated with the magnetization dynamics, including alpha, have a non-monotonic temperature dependence, suggestive of a link to the anomalous Hall effect.

cond-mat.mtrl-sci↗

arXiv2007

Two-phonon coupling to the antiferromagnetic phase transition in multiferroic BiFeO3

A prominent band centered at around 1000-1300 cm-1 and associated with resonant enhancement of two-phonon Raman scattering is reported in multiferroic BiFeO3 thin films and single crystals. A strong anomaly in this band occurs at the antiferromagnetic Neel temperature. This band is composed of three peaks, assigned to 2A4, 2E8, and 2E9 Raman modes. While all three peaks were found to be sensitive to the antiferromagnetic phase transition, the 2E8 mode, in particular, nearly disappears at TN on heating, indicating a strong spin-two phonon coupling in BiFeO3.

cond-mat.other↗

arXiv2006

Non-diffusive spin dynamics in a two-dimensional electron gas

We describe measurements of spin dynamics in the two-dimensional electron gas in GaAs/GaAlAs quantum wells. Optical techniques, including transient spin-grating spectroscopy, are used to probe the relaxation rates of spin polarization waves in the wavevector range from zero to $6\times 10^4$ cm$^{-1}$. We find that the spin polarization lifetime is maximal at nonzero wavevector, in contrast with expectation based on ordinary spin diffusion, but in quantitative agreement with recent theories that treat diffusion in the presence of spin-orbit coupling.

cond-mat.mes-hall↗

arXiv2006

An Exact SU(2) Symmetry and Persistent Spin Helix in a Spin-Orbit Coupled System

Spin-orbit coupled systems generally break the spin rotation symmetry. However, for a model with equal Rashba and Dresselhauss coupling constant (the ReD model), and for the $[110]$ Dresselhauss model, a new type of SU(2) spin rotation symmetry is discovered. This symmetry is robust against spin-independent disorder and interactions, and is generated by operators whose wavevector depends on the coupling strength. It renders the spin lifetime infinite at this wavevector, giving rise to a Persistent Spin Helix (PSH). We obtain the spin fluctuation dynamics at, and away, from the symmetry point, and suggest experiments to observe the PSH.

cond-mat.other↗