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Jacob B Khurgin

Publications and source records attributed to Jacob B Khurgin.

At least 19 recordsLinked to original sources

Can Second-Order Nonlinearity in Metal-Dielectric Metamaterials Pave a Way Toward Elusive Photonic Time Crystals?

While a tremendous amount of theoretical work has been dedicated to time-varying photonics, practical implementation in the optical range has relied almost exclusively on transparent conductive oxides , which remain severely constrained by being slow and highly lossy. To bypass these limitations, I propose an alternative platform utilizing ultrafast second-order nonlinearities within an epsilon-near-zero semiconductor-silver metamaterial. Due to the relatively low loss in silver and polarization-selective pumping, ultra-low pump absorption prevents thermal degradation, while absorption of the probe is sufficiently low to simultaneously permit the multi-cycle interaction lengths necessary for signal detection. I find that with pump powers of 100s of GW/cm2 one can open a wide momentum bandgap of tens of percents and achieve net parametric gain in time, offering a robust pathway to realizing photonic time crystals in optical range.

physics.optics

Revealing Sharp Spectral Features with Complex Frequency Excitations: Challenges and Opportunities

Broadening of spectral and spatial responses due to intrinsic loss in real materials often hides sharp features. One recently recognized route to recover those features is to probe the system with complex-frequency (CF) signals that decay exponentially in time: a suitably tailored temporal decay can compensate for loss and reveal an intrinsic, narrow response. However, generating rapidly decaying optical waveforms in real time is often challenging (the required decay times may be in the range of tens of femtoseconds). A recently proposed alternative synthesizes the CF response numerically after detection of conventional, real-frequency signals using Fourier post-processing. Here we explore advantages and challenges of these approaches: we show that a physical CF excitation robustly sharpens spectral features in the presence of noise, while a post-detection synthesized CF response shows only limited improvement once realistic detection and readout noise is considered. At the same time, in low-noise conditions a much simpler post-detection filtering procedure attains equal or better recovery than the synthesized CF reconstruction, making the synthesis unnecessary in practice.

physics.optics

Photonic Time Crystals and Parametric Amplification: similarity and distinction

Photonic Time crystals (PTC) arise in time-modulated media when the frequency of modulation of permittivity is on the order of twice the frequency of light and are manifested by the generation and amplification of so-called time reversed waves propagating in the direction opposite to the incoming light. Superficially, the observed phenomenon bears resemblance to the widely known phenomena of optical parametric generation (OPG) and amplification (OPA) using second or third order optical nonlinearities. I show that while indeed the same physical mechanism underpins both PTC and OPA , the difference arises from the boundary conditions. Thus , while dispersion for both PTC and OPA exhibit the same bandgap in momentum space, only in the case of PTC can one have propagation in that bandgap with exponential amplification. I also show that PTC can be engineered with both second and third order nonlinearities, and that rather unexpectedly, modulating permittivity on the ultrafast (few fs) rate is not a necessity, and that one can emulate all the PTC features using materials with a few picoseconds response time commensurate with the propagation time through the medium.

physics.optics

Energy and Power requirements for alteration of the refractive index

The ability to manipulate the refractive index is a fundamental principle underlying numerous photonic devices. Various techniques exist to modify the refractive index across diverse materials, making performance comparison far from straightforward. In evaluating these methods, power consumption emerges as a key performance characteristic, alongside bandwidth and footprint. Here I undertake a comprehensive comparison of the energy and power requirements for the most well-known index change schemes. The findings reveal that while the energy per volume for index change remains within the same order of magnitude across different techniques and materials, the power consumption required to achieve switching, 100% modulation, or 100% frequency conversion can differ significantly, spanning many orders of magnitude. As it turns out, the material used has less influence on power reduction than the specific resonant or traveling wave scheme employed to enhance the interaction time between light and matter. Though this work is not intended to serve as a design guide, it does establish the limitations and trade-offs involved in index modulation, thus providing valuable insights for photonics practitioners.

physics.optics

Nonlinear Optics: a look from the interaction time viewpoint and what it portends

I present a simple view of nonlinear optcal phenomena as being determined mostly by the length of interaction time between photons and matter. This may explain why in the last decades the progress in developing better nonlinear materials has not been as rapid as wished. A few tentative routes towards possible improvements in the efficiency of nonlinear optical phenomena are suggested.

physics.optics

Optical isolation by temporal modulation: size, frequency, and power constraints

Optical isolators are indispensable components of optical networks. Magneto-optic isolators have excellent operating characteristics, including low-to-no power consumption, but are not well suited for on-chip integration. The technique of temporal modulation of dielectric constant offers an alternative way to achieve isolation without magnetic field but is not without its own drawbacks. In this work I examine diverse methods of optical isolation via temporal modulation and show that independent on whether modulation is achieved by carrier injection, Pockels and acousto-optic effects, or any other conceivable method, there is essentially the same set of constraints on footprint, modulation frequency, and, most important, on power consumption required to achieve full isolation without excessive insertion loss. This power is estimated to be on the order of at least a hundred of milliwatts and whether this requirement is acceptable will depend on ongoing progress of both magneto-optic and time modulated integrated technologies.

physics.optics

On-chip low-loss all-optical MoSe$_2$ modulator

Monolayer transition metal dichalcogenides (TMDCs), like MoS$_2$, MoSe$_2$, WS$_2$, and WSe$_2$, feature direct bandgaps, strong spin-orbit coupling, and exciton-polariton interactions at the atomic scale, which could be harnessed for efficient light emission, valleytronics, and polaritonic lasing, respectively. Nevertheless, to build next-generation photonic devices that make use of these features, it is first essential to model the all-optical control mechanisms in TMDCs. Herein, a simple model is proposed to quantify the performance of a 35$\,$\textmu m long Si$_3$N$_4$ waveguide-integrated all-optical MoSe$_2$ modulator. Using this model, a switching energy of 14.6$\,$pJ is obtained for a transverse-magnetic (TM) and transverse-electric (TE) polarised pump signals at $λ=\,$480$\,$nm. Moreover, maximal extinction ratios of 20.6$\,$dB and 20.1$\,$dB are achieved for a TM and TE polarised probe signal at $λ=\,$500$\,$nm, respectively, with an ultra-low insertion loss of $<0.3\,$dB. Moreover, the device operates with an ultrafast recovery time of 50$\,$ps, while maintaining a high extinction ratio for practical applications. These findings facilitate modeling and designing novel TMDC-based photonic devices.

physics.optics

A simple technique for evaluating dipole moments of Bloch states in tetrahedral semiconductors

Permanent dipole moments of electronics states in non-centro-symmetric materials play pivotal role in many phenomena. Correctly evaluating them presents an arduous task and usually requires full knowledge of the band structure as well as understanding the intricate concepts of Berry curvature. Here we show that in a few cases (e.g. zinc blende and wurtzite) a rather facile first-principle analytical derivation of the permanent dipole moments using L Hopital rule can be performed, and the values and dispersion of these dipoles near high symmetry points can be found using just a couple of widely available material parameters. The results will hopefully contribute to better understanding of shift currents, optical rectification and other electro-optical phenomena.

cond-mat.other

Charge and Field Driven Integrated Optical Modulators: Comparative Analysis

Electro optic modulators being key for many signal processing systems must adhere to requirements given by both electrical and optical constrains. Distinguishing between charge driven (CD) and field driven (FD) designs, we answer the question of whether fundamental performance benefits can be claimed of modulators based on emerging electro-optic materials. Following primary metrics, we compare the performance of emerging electro-optic and electro-absorption modulators such as graphene, transparent conductive oxides, and Si, based on charge injection with that of the legacy FD modulators, such as those based on lithium niobate and quantum confined Stark effect. We show that for rather fundamental reasons, FD modulators always outperform CD ones in the conventional wavelength scale waveguides. However, for waveguide featuring a sub-wavelength optical mode, such as those assisted by plasmonics, the emerging CD devices are indeed highly competitive.

physics.app-ph

Expanding photonic palette: exploring high index materials

While the photonic community is being occupied with exotic concepts portending a grand future and fame if not a fortune, I respectfully entertain the possibility that a humble concept of simply increasing refractive index by a modest factor may have a far greater payoff in many walks of life. With that in mind, I explore why higher index materials have not yet materialized, and point out a few tentative directions for the search of these elusive materials, be they natural or artificial.

physics.optics

Adiabatic frequency shifting in epsilon near zero materials: The role of group velocity

We investigate adiabatic frequency conversion using epsilon near zero (ENZ) materials and show that while the maximum frequency conversion for a given change of permittivity does not exhibit increase in the vicinity of ε=0 condition. However, that change can be achieved in a shorter length, and if the pump is also in the ENZ vicinity, at a lower pump intensity. This slow propagation effect makes the conversion efficiency in the ENZ material comparable to that in microresonators and other structured slow light schemes, but unlike the latter no nanofabrication is required for ENZ materials which constitutes their major advantage over alternative frequency conversion approaches.

physics.optics

Generating hot carriers in plasmonic nanoparticles: when quantization does and does not matter?

Plasmon-assisted hot carrier processes in metal nanoparticles can be described either classically or using the full strength of quantum mechanics. We reconfirm that from the practical applications point of view, when it comes to description of the decay of plasmons in nanoparticles, classical description is sufficiently adequate for all but the smallest of the nanoparticles. At the same time, the electron temperature rise in nanoparticles is discrete (quantized) and neglecting this fact can lead to significant underestimating of hot carrier assisted effects, such as photo-catalysis.

physics.optics

Fundamental limits of hot carrier injection from metal in nanoplasmonics

Evolution of the nonequilibrium carriers excited in the process of decay of surface plasmon polaritons in metal is described for each step, from the carrier generation to their extraction from the metal. The relative importance of various carrier generating mechanism is discussed. It is shown that both carrier generation and their decay are inherently quantum processes as for realistic illumination conditions no more than a single SPP per nanoparticle exists at a given time. As a result, the distribution of non-equilibrium carriers cannot be described by a single temperature. It is also shown that the originally excited carriers that have not undergone a single electron-electron scattering event, are practically the only ones that contribute to the injection. The role of the momentum conservation in the carrier extraction is discussed and it is shown that if all the momentum conservation rules are relaxed, it is the density of states in the semiconductor/dielectric that determines the ultimate injection efficiency. A set of recommendations aimed at improving the efficiency of plasmonic-assisted photodetection and (to a lesser degree) photocatalysis is made in the end.

physics.optics

Pliable Polaritons: Wannier Exciton Plasmon Coupling in Metal Semiconductor Structures

Plasmonic structures are known to support the modes with subwavelength volumes in which the field matter interactions are greatly enhanced. Coupling between the molecular excitations and plasmons leading to formation of plexcitons has been investigated for a number of organic molecules. However, plasmon-exciton coupling in metal semiconductor structures have not experienced the same degree of attention. In this work we show that the very strong coupling regime in which the Rabi energy exceeds the exciton binding energy is attainable in semiconductor cladded plasmonic nanoparticles and leads to formation of Wannier Exciton Plasmon Polariton (WEPP) that is bound to the metal nanoparticle and characterized by dramatically smaller (by factor of few) excitonic radius and correspondingly higher ionization energy. This higher ionization energy exceeding approaching 100meV for the CdS/Ag structures may make room temperature Bose Einstein condensation and polariton lasing in plasmonic/semiconductor structures possible

physics.optics

Hot carriers generated by plasmons: where are they are generated and where do they go from there?

A physically transparent unified theory of optically and plasmon induced hot carrier generation in metals is developed with all the relevant mechanisms included. Analytical expressions that estimate the carrier generation rates, their locations, energy and direction of motion are obtained. Among four mechanisms considered: interband absorption, phonon and defect assisted absorption, electron electron scattering assisted absorption, and surface collision assisted absorption (Landau damping), it is the last one that generates hot carriers which are most useful for practical applications in photo detection and photo catalysis.

physics.optics

Linewidth of the Laser Optical Frequency Comb with Arbitrary Temporal Profile

For many applications Optical Frequency Combs (OFCs) require a high degree of temporal coherence (narrow linewidth). Commonly OFCs are generated in nonlinear media from a monochromatic narrow linewidth laser sources or from a mode-locked laser pulses but in the all-important mid-infrared (MIR) and terahertz (THz) regions of spectrum OFCs can be generated intrinsically by the free-running quantum cascade lasers (QCLs) with high efficiency. These combs do not look like conventional OFCs as the phases of each mode are different and in temporal domain the OFC is a seemingly random combination of amplitude- and phase-modulated signals rather than a short pulse. Despite this pseudo-randomness, the experimental evidence suggests that the linewidth of the QCL OFC is just as narrow as that of a QCL operating in the single mode. While universally acknowledged, this seemingly observation is not fully understood. In this work we rigorously prove this fact by deriving the expression for the Schawlow-Townes linewidth of QCL OFC and offer a transparent physical interpretation based on orthogonality of laser modes, indicating that despite their very different temporal profiles MIR and THz QCL OFCs are just as good for most applications as any other OFC.

physics.optics

Relative merits of Phononics vs. Plasmonics: the energy balance approach

The common feature of various plasmonic schemes is their ability to confine optical fields of surface plasmon polaritons (SPPs) into sub-wavelength volumes and thus achieve a large enhancement of linear and nonlinear optical properties. This ability, however, is severely limited by the large ohmic loss inherent to even the best of metals. However, in the mid and far infrared ranges of the spectrum there exists a viable alternative to metals, polar dielectrics and semiconductors in which dielectric permittivity (the real part) turns negative in the Reststrahlen region. This feature engenders the so-called surface phonon polaritons (SPhPs) capable of confining the field in a way akin to their plasmonic analogues, the SPPs. Since the damping rate of polar phonons is substantially less than that of free electrons, it is not unreasonable to expect that phononic devices may outperform their plasmonic counterparts. Yet a more rigorous analysis of the comparative merits of phononics and plasmonics reveals a more nuanced answer, namely that while phononic schemes do exhibit narrower resonances and can achieve a very high degree of energy concentration, most of the energy is contained in the form of lattice vibrations so that enhancement of the electric field, and hence the Purcell factor, is rather small compared to what can be achieved with metal nanoantennas. Still, the sheer narrowness of phononic resonances is expected to make phononics viable in applications where frequency selectivity is important.

physics.optics