arXiv subjects

Jae-Pil So

Publications and source records attributed to Jae-Pil So.

4 recordsLinked to original sources

arXiv2026

Magneto-Optical Detection of Anisotropic Spin Currents in Altermagnetic RuO2

Altermagnets are a recently identified class of collinear antiferromagnets that host large spin-split electronic bands, offering a promising platform for efficient spin-current generation. Among proposed candidates, the metallic oxide RuO2 is predicted to exhibit strong altermagnetic spin splitting; however, whether it sustains robust magnetic order beyond the ultrathin thickness limit remains unresolved. Here, we employ optical probes to investigate charge-to-spin conversion in a 12-nm-thick (101)-oriented RuO2 film grown on sapphire. Polarization-resolved second-harmonic generation reveals nonlinear optical responses consistent with the surface symmetry and N\'eel order of RuO2. Under an applied current, both second-harmonic generation and polar magneto-optical Kerr effect measurements detect a pronounced, directionally anisotropic spin polarization, exhibiting enhanced signals for current along [010] and strongly suppressed responses for current along [-101], in agreement with the symmetry of the altermagnetic spin-splitter effect. Non-magnetic or Rashba-type mechanisms cannot explain this symmetry-selective response. Scanning transmission electron microscopy further reveals that substantial strain persists even in relatively thick films, providing a possible explanation for the observed behavior. Therefore, these results establish RuO2 as an efficient spin source and demonstrate the potential of altermagnets for field-free spintronic devices.

cond-mat.mtrl-sci↗

arXiv2024

Purcell enhancement and spin spectroscopy of silicon vacancy centers in silicon carbide using an ultra-small mode-volume plasmonic cavity

Silicon vacancy (V$_{Si}$) centers in 4H-silicon carbide have emerged as a strong candidate for quantum networking applications due to their robust electronic and optical properties including a long spin coherence lifetime and bright, stable emission. Here, we report the integration of V$_{Si}$ centers with a plasmonic nanocavity to Purcell enhance the emission, which is critical for scalable quantum networking. Employing a simple fabrication process, we demonstrate plasmonic cavities that support a nanoscale mode volume and exhibit an increase in the spontaneous emission rate with a measured Purcell factor of up to 48. In addition to investigating the optical resonance modes, we demonstrate that an improvement in the optical stability of the spin-preserving resonant optical transitions relative to the radiation-limited value. The results highlight the potential of nanophotonic structures for advancing quantum networking technologies and emphasizes the importance of optimizing emitter-cavity interactions for efficient quantum photonic applications.

quant-ph↗

arXiv2024

Tuning exciton emission via ferroelectric polarization at a heterogeneous interface between a monolayer transition metal dichalcogenide and a perovskite oxide membrane

We demonstrate the integration of a thin BaTiO$_3$ (BTO) membrane with monolayer MoSe$_2$ in a dual gate device that enables in-situ manipulation of the BTO ferroelectric polarization with a voltage pulse. While two-dimensional (2D) transition metal dichalcogenides (TMDs) offer remarkable adaptability, their hybrid integration with other families of functional materials beyond the realm of 2D materials has been challenging. Released functional oxide membranes offer a solution for 2D/3D integration via stacking. 2D TMD excitons can serve as a local probe of the ferroelectric polarization in BTO at a heterogeneous interface. Using photoluminescence (PL) of MoSe$_2$ excitons to optically readout the doping level, we find that the relative population of charge carriers in MoSe$_2$ depends sensitively on the ferroelectric polarization. This finding points to a promising avenue for future-generations versatile sensing devices with high sensitivity, fast read-out, and diverse applicability for advanced signal processing.

cond-mat.mtrl-sci↗

arXiv2021

Electrically driven strain-induced deterministic single-photon emitters in a van der Waals heterostructure

Quantum confinement in atomically-thin TMDCs enables the realization of deterministic single-photon emitters. The position and polarization control of single photons have been achieved via local strain engineering using nanostructures. However, most existing TMDC-based emitters are operated by optical pumping, while the emission sites in electrically pumped emitters are uncontrolled. Here, we demonstrate electrically driven single-photon emitters located at the positions where strains are induced by atomic-force-microscope indentation on a van der Waals heterostructure consisting of graphene, hexagonal-boron nitride, and tungsten diselenide. The optical, electrical, and mechanical properties induced by the local strain gradient were systematically analyzed. In particular, single-photon emission was observed at the indentation sites at 4 K. The emission exhibits photon anti-bunching behavior with a g(2)(0) value of ~0.3, intensity saturation and a linearly cross-polarized doublet. This robust spatial control of electrically driven single-photon emitters will pave the way for the practical implementation of integrated quantum light sources.

cond-mat.mes-hall↗