arXiv subjects

Jason W. Christopher

Publications and source records attributed to Jason W. Christopher.

4 recordsLinked to original sources

arXiv2018

Modeling and Thermal Metrology of Thermally Isolated MEMS Electrothermal Actuators for Strain Engineering of 2D Materials

We present electrothermal microelectromechanical (MEMS) actuators as a practical platform for straining 2D materials. The advantages of the electrothermal actuator is its high output force and displacement for low input voltage, but its drawback is that it is actuated by generating high amounts of heat. It is crucial to mitigate the high temperatures generated during actuation for reliable 2D material strain device implementation. Here, we implement a chevron actuator design that incorporates a thermal isolation stage in order to avoid heating the 2D material from the high temperatures generated during the actuation. By comparing experiment and simulation, we ensure our design does not compromise output displacement, while keeping the 2D material strain device stage cool. We also provide a simple analytical model useful for quickly evaluating different thermal isolation stage designs.

physics.app-ph↗

arXiv2018

Monolayer MoS$_2$ Strained to 1.3\% with a Microelectromechanical System

We report on a modified transfer technique for atomically thin materials integrated onto microelectromechanical systems (MEMS) for studying strain physics and creating strain-based devices. Our method tolerates the non-planar structures and fragility of MEMS, while still providing precise positioning and crack free transfer of flakes. Further, our method used the transfer polymer to anchor the 2D crystal to the MEMS, which reduces the fabrication time, increases the yield, and allowed us to exploit the strong mechanical coupling between 2D crystal and polymer to strain the atomically thin system. We successfully strained single atomic layers of molybdenum disulfide (MoS$_2$) with MEMS devices for the first time and achieved greater than 1.3\% strain, marking a major milestone for incorporating 2D materials with MEMS We used the established strain response of MoS$_2$ Raman and Photoluminescence spectra to deduce the strain in our crystals and provide a consistency check. We found good comparison between our experiment and literature.

cond-mat.mtrl-sci↗

arXiv2016

Band Gap Engineering with Ultralarge Biaxial Strains in Suspended Monolayer MoS2

We demonstrate the continuous and reversible tuning of the optical band gap of suspended monolayer MoS2 membranes by as much as 500 meV by applying very large biaxial strains. By using chemical vapor deposition (CVD) to grow crystals that are highly impermeable to gas, we are able to apply a pressure difference across suspended membranes to induce biaxial strains. We observe the effect of strain on the energy and intensity of the peaks in the photoluminescence (PL) spectrum, and find a linear tuning rate of the optical band gap of 99 meV/%. This method is then used to study the PL spectra of bilayer and trilayer devices under strain, and to find the shift rates and Grüneisen parameters of two Raman modes in monolayer MoS2. Finally, we use this result to show that we can apply biaxial strains as large as 5.6% across micron sized areas, and report evidence for the strain tuning of higher level optical transitions.

cond-mat.mes-hall↗

arXiv2016

Long tailed trions in monolayer MoS$_2$: Temperature dependent asymmetry and red-shift of trion photoluminescence spectra

Monolayer molybdenum disulfide (MoS$_2$) has emerged as an excellent 2D model system because of its two inequivalent, direct-gap valleys that lead to exotic bound and excited states. Here we focus on one such bound state, the negatively charged trion. Unlike excitons, trions can radiatively decay with non-zero momentum by kicking out an electron, resulting in an asymmetric trion photoluminescence (PL) peak with a long low-energy tail. As a consequence, the peak position does not correspond to the zero momentum trion energy. By including the trion's long tail in our analysis we are able to accurately separate the exciton from the trion contributions to the PL spectra. According to theory, the asymmetric energy tail has both a size-dependent and a temperature-dependent contribution. Analysis of the temperature-dependent data reveals the effective trion size, consistent with literature, and the temperature dependence of the band gap and spin-orbit splitting of the valence band. Finally, we observe signatures of Pauli-blocking of the trion decay.

cond-mat.mtrl-sci↗