arXiv subjects

Jelena Vučković

Publications and source records attributed to Jelena Vučković.

At least 91 records · Page 5Linked to original sources

arXiv2017

Tuning the Photon Statistics of a Strongly Coupled Nanophotonic System

We investigate the dynamics of single- and multi-photon emission from detuned strongly coupled systems based on the quantum-dot-photonic-crystal resonator platform. Transmitting light through such systems can generate a range of non-classical states of light with tunable photon counting statistics due to the nonlinear ladder of hybridized light-matter states. By controlling the detuning between emitter and resonator, the transmission can be tuned to strongly enhance either single- or two-photon emission processes. Despite the strongly-dissipative nature of these systems, we find that by utilizing a self-homodyne interference technique combined with frequency-filtering we are able to find a strong two-photon component of the emission in the multi-photon regime. In order to explain our correlation measurements, we propose rate equation models that capture the dominant processes of emission both in the single- and multi-photon regimes. These models are then supported by quantum-optical simulations that fully capture the frequency filtering of emission from our solid-state system.

physics.optics↗

arXiv2017

Scalable Quantum Photonics with Single Color Centers in Silicon Carbide

Silicon carbide is a promising platform for single photon sources, quantum bits (qubits) and nanoscale sensors based on individual color centers. Towards this goal, we develop a scalable array of nanopillars incorporating single silicon vacancy centers in 4H-SiC, readily available for efficient interfacing with free-space objective and lensed-fibers. A commercially obtained substrate is irradiated with 2 MeV electron beams to create vacancies. Subsequent lithographic process forms 800 nm tall nanopillars with 400-1,400 nm diameters. We obtain high collection efficiency, up to 22 kcounts/s optical saturation rates from a single silicon vacancy center, while preserving the single photon emission and the optically induced electron-spin polarization properties. Our study demonstrates silicon carbide as a readily available platform for scalable quantum photonics architecture relying on single photon sources and qubits.

physics.optics↗

arXiv2017

Complete Coherent Control of Silicon-Vacancies in Diamond Nanopillars Containing Single Defect Centers

Arrays of identical and individually addressable qubits lay the foundation for the creation of scalable quantum hardware such as quantum processors and repeaters. Silicon vacancy centers in diamond (SiV) offer excellent physical properties such as low inhomogeneous broadening, fast photon emission, and a large Debye-Waller factor, while the possibility for all-optical ultrafast manipulation and techniques to extend the spin coherence times make them very promising candidates for qubits. Here, we have developed arrays of nanopillars containing single SiV centers with high yield, and we demonstrate ultrafast all-optical complete coherent control of the state of a single SiV center. The high quality of the chemical vapor deposition (CVD) grown SiV centers provides excellent spectral stability, which allows us to coherently manipulate and quasi-resonantly read out the state of individual SiV centers on picosecond timescales using ultrafast optical pulses. This work opens new opportunities towards the creation of a scalable on-chip diamond platform for quantum information processing and scalable nanophotonics applications.

cond-mat.mes-hall↗

arXiv2016

Self-homodyne enabled generation of indistinguishable photons

The rapid generation of non-classical light serves as the foundation for exploring quantum optics and developing applications such as secure communication or generation of NOON-states. While strongly coupled quantum dot-photonic crystal resonator systems have great potential as non-classical light sources due to their promise of tailored output statistics, the generation of indistinguishable photons has been obscured due to the strongly dissipative nature of such systems. Here, we demonstrate that the recently discovered self-homodyne suppression technique can be used to overcome this limitation and tune the quantum statistics of transmitted light, achieving indistinguishable photon emission competitive with state-of-the-art metrics. Furthermore, our nanocavity-based platform directly lends itself to scalable on-chip architectures for quantum information.

cond-mat.mes-hall↗

arXiv2016

Self-homodyne measurement of a dynamic Mollow triplet in the solid state

The study of light-matter interaction at the quantum scale has been enabled by the cavity quantum electrodynamics (CQED) architecture, in which a quantum two-level system strongly couples to a single cavity mode. Originally implemented with atoms in optical cavities, CQED effects are now also observed with artificial atoms in solid-state environments. Such realizations of these systems exhibit fast dynamics, which makes them attractive candidates for devices including modulators and sources in high-throughput communications. However, these systems possess large photon out-coupling rates that obscure any quantum behavior at large excitation powers. Here, we have utilised a self-homodyning interferometric technique that fully employs the complex mode structure of our nanofabricated cavity to observe a quantum phenomenon known as the dynamic Mollow triplet. We expect this interference to facilitate the development of arbitrary on-chip quantum state generators, thereby strongly influencing quantum lithography, metrology, and imaging.

cond-mat.mes-hall↗

arXiv2016

Initialization of a spin qubit in a site-controlled nanowire quantum dot

A fault-tolerant quantum repeater or quantum computer using solid-state spin-based quantum bits will likely require a physical implementation with many spins arranged in a grid. Self-assembled quantum dots (QDs) have been established as attractive candidates for building spin-based quantum information processing devices, but such QDs are randomly positioned, which makes them unsuitable for constructing large-scale processors. Recent efforts have shown that quantum dots embedded in nanowires can be deterministically positioned in regular arrays, can store single charges, and have excellent optical properties, but so far there have been no demonstrations of spin qubit operations using nanowire quantum dots. Here we demonstrate optical pumping of individual spins trapped in site-controlled nanowire quantum dots, resulting in high-fidelity spin-qubit initialization. This represents the next step towards establishing spins in nanowire quantum dots as quantum memories suitable for use in a large-scale, fault-tolerant quantum computer or repeater based on all-optical control of the spin qubits.

cond-mat.mes-hall↗

arXiv2015

Hybrid Group IV Nanophotonic Structures Incorporating Diamond Silicon-Vacancy Color Centers

We demonstrate a new approach for engineering group IV semiconductor-based quantum photonic structures containing negatively charged silicon-vacancy (SiV$^-$) color centers in diamond as quantum emitters. Hybrid SiC/diamond structures are realized by combining the growth of nanoand micro-diamonds on silicon carbide (3C or 4H polytype) substrates, with the subsequent use of these diamond crystals as a hard mask for pattern transfer. SiV$^-$ color centers are incorporated in diamond during its synthesis from molecular diamond seeds (diamondoids), with no need for ionimplantation or annealing. We show that the same growth technique can be used to grow a diamond layer controllably doped with SiV$^-$ on top of a high purity bulk diamond, in which we subsequently fabricate nanopillar arrays containing high quality SiV$^-$ centers. Scanning confocal photoluminescence measurements reveal optically active SiV$^-$ lines both at room temperature and low temperature (5 K) from all fabricated structures, and, in particular, very narrow linewidths and small inhomogeneous broadening of SiV$^-$ lines from all-diamond nano-pillar arrays, which is a critical requirement for quantum computation. At low temperatures (5 K) we observe in these structures the signature typical of SiV$^-$ centers in bulk diamond, consistent with a double lambda. These results indicate that high quality color centers can be incorporated into nanophotonic structures synthetically with properties equivalent to those in bulk diamond, thereby opening opportunities for applications in classical and quantum information processing.

cond-mat.mtrl-sci↗

arXiv2015

Direct Bandgap Light Emission from Strained Ge Nanowires Coupled with High-Q Optical Cavities

A silicon-compatible light source is the final missing piece for completing high-speed, low-power on-chip optical interconnects. In this paper, we present a germanium-based light emitter that encompasses all the aspects of potential low-threshold lasers: highly strained germanium gain medium, strain-induced pseudo-heterostructure, and high-Q optical cavity. Our light emitting structure presents greatly enhanced photoluminescence into cavity modes with measured quality factors of up to 2,000. The emission wavelength is tuned over more than 400 nm with a single lithography step. We find increased optical gain in optical cavities formed with germanium under high (>2.3%) tensile strain. Through quantitative analysis of gain/loss mechanisms, we find that free carrier absorption from the hole bands dominates the gain, resulting in no net gain even from highly strained, n-type doped germanium.

physics.optics↗

arXiv2015

Ultrafast polariton-phonon dynamics of strongly coupled quantum dot-nanocavity systems

We investigate the influence of exciton-phonon coupling on the dynamics of a strongly coupled quantum dot-photonic crystal cavity system and explore the effects of this interaction on different schemes for non-classical light generation. By performing time-resolved measurements, we map out the detuning-dependent polariton lifetime and extract the spectrum of the polariton-to-phonon coupling with unprecedented precision. Photon-blockade experiments for different pulse-length and detuning conditions (supported by quantum optical simulations) reveal that achieving high-fidelity photon blockade requires an intricate understanding of the phonons' influence on the system dynamics. Finally, we achieve direct coherent control of the polariton states of a strongly coupled system and demonstrate that their efficient coupling to phonons can be exploited for novel concepts in high-fidelity single photon generation.

cond-mat.mes-hall↗

arXiv2015

Coherent generation of nonclassical light on chip via detuned photon blockade

The on-chip generation of non-classical states of light is a key-requirement for future optical quantum hardware. In solid-state cavity quantum electrodynamics, such non-classical light can be generated from self-assembled quantum dots strongly coupled to photonic crystal cavities. Their anharmonic strong light-matter interaction results in large optical nonlinearities at the single photon level, where the admission of a single photon into the cavity may enhance (photon-tunnelling) or diminish (photon-blockade) the probability for a second photon to enter the cavity. Here, we demonstrate that detuning the cavity and QD resonances enables the generation of high-purity non-classical light from strongly coupled systems. For specific detunings we show that not only the purity but also the efficiency of single-photon generation increases significantly, making high-quality single-photon generation by photon-blockade possible with current state-of-the-art samples.

cond-mat.mes-hall↗

arXiv2015

Inverse design and demonstration of a compact and broadband on-chip wavelength demultiplexer

Integrated photonic devices are poised to play a key role in a wide variety of applications, ranging from optical interconnects and sensors to quantum computing. However, only a small library of semi-analytically designed devices are currently known. In this paper, we demonstrate the use of an inverse design method that explores the full design space of fabricable devices and allows us to design devices with previously unattainable functionality, higher performance and robustness, and smaller footprints compared to conventional devices. We designed a silicon wavelength demultiplexer that splits $1300~\mathrm{nm}$ and $1550~\mathrm{nm}$ light from an input waveguide into two output waveguides, and fabricated and characterized several devices. The devices display low insertion loss $\left(2 - 4~\mathrm{dB}\right)$, high contrast $\left(12 - 17~\mathrm{dB}\right)$, and wide bandwidths $\left(\sim 100~\mathrm{nm} \right)$. The device footprint is $2.8 \times 2.8 ~\mathrm{μm}$, making this the smallest dielectric wavelength splitter to date.

physics.optics↗

arXiv2014

Visible Photoluminescence from Cubic (3C) Silicon Carbide Microdisks Coupled to High Quality Whispering Gallery Modes

We present the design, fabrication and characterization of cubic (3C) silicon carbide microdisk resonators with high quality factor modes at visible and near infrared wavelengths (600 - 950 nm). Whispering gallery modes with quality factors as high as 2,300 and corresponding mode volumes V ~ 2 (λ/n)^3 are measured using laser scanning confocal microscopy at room temperature. We obtain excellent correspondence between transverse-magnetic (TM) and transverse-electric (TE) polarized resonances simulated using Finite Difference Time Domain (FDTD) method and those observed in experiment. These structures based on ensembles of optically active impurities in 3C-SiC resonators could play an important role in diverse applications of nonlinear and quantum photonics, including low power optical switching and quantum memories.

physics.optics↗

arXiv2014

Inverse design and implementation of a wavelength demultiplexing grating coupler

Nanophotonics has emerged as a powerful tool for manipulating light on chips. Almost all of today's devices, however, have been designed using slow and ineffective brute-force search methods, leading in many cases to limited device performance. In this article, we provide a complete demonstration of our recently proposed inverse design technique, wherein the user specifies design constraints in the form of target fields rather than a dielectric constant profile, and in particular we use this method to demonstrate a new demultiplexing grating. The novel grating, which has not been developed using conventional techniques, accepts a vertical-incident Gaussian beam from a free-space and separates O-band $(1300\mathrm{nm})$ and C-band $(1550\mathrm{nm})$ light into separate waveguides. This inverse design concept is simple and extendable to a broad class of highly compact devices including frequency splitters, mode converters, and spatial mode multiplexers.

physics.optics↗

arXiv2014

Hole Spin Pumping and Re-pumping in a p-type δ-doped InAs Quantum Dot

We have grown high quality p-type δ-doped InAs quantum dots and have demonstrated coherent spin pumping and repumping of a hole spin in a positively charged quantum dot by means of a single-laser driving scheme under a high magnetic field in the Voigt configuration. Modeling of our system shows excellent qualitative agreement with the experimental findings and further explores the performance of the single-laser scheme for spin pumping and re-pumping.

quant-ph↗

arXiv2014

Second Harmonic Generation in Photonic Crystal Cavities in (111)-Oriented GaAs

We demonstrate second harmonic generation at telecommunications wavelengths in L3 photonic crystal cavities in (111)-oriented GaAs. The second harmonic power from photonic crystal cavities fabricated in (111)-oriented GaAs is significantly increased compared to those fabricated in conventional (001)-oriented GaAs.

physics.optics↗

arXiv2014

Photo-oxidative tuning of individual and coupled GaAs photonic crystal cavities

We demonstrate a new photo-induced oxidation technique for tuning GaAs photonic crystal cavities using a $390~\mathrm{nm}$ pulsed laser with an average power of $10~\mathrm{μW}$. The laser oxidizes a small $\left(\sim 500~\mathrm{nm}\right)$ diameter spot, reducing the local index of refraction and blueshifting the cavity. The tuning progress can be actively monitored in real time. We also demonstrate tuning an individual cavity within a pair of proximity-coupled cavities, showing that this method can be used to correct undesired frequency shifts caused by fabrication imperfections in cavity arrays.

physics.optics↗

arXiv2013

Photonic Crystal Cavities in Cubic (3C) Polytype Silicon Carbide Films

We present the design, fabrication, and characterization of high quality factor and small mode volume planar photonic crystal cavities from cubic (3C) thin films (thickness ~ 200 nm) of silicon carbide (SiC) grown epitaxially on a silicon substrate. We demonstrate cavity resonances across the telecommunications band, with wavelengths from 1,250 - 1,600 nm. Finally, we discuss possible applications in nonlinear optics, optical interconnects, and quantum information science.

physics.optics↗

arXiv2013

Control of Two-Dimensional Excitonic Light Emission via Photonic Crystal

Monolayers of transition metal dichalcogenides (TMDCs) have emerged as new optoelectronic materials in the two dimensional (2D) limit, exhibiting rich spin-valley interplays, tunable excitonic effects, and strong light-matter interactions. An essential yet undeveloped ingredient for many photonic applications is the manipulation of its light emission. Here we demonstrate the control of excitonic light emission from monolayer tungsten diselenide (WSe2) in an integrated photonic structure, achieved by transferring one monolayer onto a photonic crystal (PhC) with a cavity. In addition to the observation of greatly enhanced (~60 times) photoluminescence of WSe2 and an effectively coupled cavity-mode emission, we are able to redistribute the emitted photons both polarly and azimuthally in the far field through designing PhC structures, as revealed by momentum-resolved microscopy. A 2D optical antenna is thus constructed. Our work suggests a new way of manipulating photons in hybrid 2D photonics, important for future energy efficient optoelectronics and 2D nano-lasers.

cond-mat.mes-hall↗