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Jennifer Cano

Publications and source records attributed to Jennifer Cano.

At least 19 recordsLinked to original sources

Non-uniform quantum geometry stabilizes generalized Wigner crystals

Moir\'e materials host fractional Chern insulators and electron crystals in close proximity, but the mechanism selecting between them remains an open question. We address this competition in Chern bands with ideal but momentum-dependent quantum geometry -- Aharonov-Casher bands. We present an ansatz wave function for generalized Wigner crystals and, by comparing its energy to that of the competing Laughlin-like state, map out the phase diagram at filling fraction $\nu=1/m$ as a function of the degree of geometric non-uniformity. Our work identifies quantum geometry-controlled zero point fluctuations of the charge density of the generalized Wigner crystal as the mechanism controlling its relative stability, implying a kind of quantum Lindemann criterion for the crystal-liquid phase boundary.

cond-mat.str-el

Collinear altermagnetism for 3D chiral higher-order topological insulators

Despite significant progress in the study of higher-order topological insulators (HOTIs), the chiral $C_4\mathcal{T}$-protected HOTI has remained elusive in electronic materials, where $C_4\mathcal{T}$ denotes the product of a four-fold rotation and time-reversal symmetry. We show that altermagnetism, a recently discovered form of collinear magnetism, provides a new route to realize this elusive phase. Specifically, we construct a microscopic model that combines a three-dimensional topological insulator with a collinear $d$-wave altermagnet on a Lieb lattice. Through analytical and numerical calculations, we show that the magnetism shifts and gaps the surface Dirac cones to produce the desired chiral hinge channels. Finally, we identify promising material classes to realise our proposal. Our results establish collinear altermagnetism as a route to intrinsic chiral higher-order topology and open a new path toward the discovery of $C_4\mathcal{T}$-protected HOTIs in real materials.

cond-mat.mes-hall

Topology and compact molecular orbitals in twisted bilayer WSe$_2$

Recent observations of superconductivity in twisted bilayer WSe$_2$ (tWSe$_2$) have motivated theoretical proposals for unconventional pairing mechanisms. A central question is whether band topology plays an essential role in the system's correlation physics. In this letter, we develop a first-principles-based description of the top moir\'e valence bands in tWSe$_2$. Using density functional theory (DFT) calculations, we identify the bands in the relevant range of twist angles to be topologically non-trivial, with the top valence bands carrying Chern numbers $C=(+1,+1)$ for the $K$ valley. In order to treat the strong correlation physics, we construct compact molecular orbitals directly from the DFT wave functions through a partial Wannierization procedure and with the guidance of spinful $C_{3z}$ symmetry representations. This yields a localized $f$ orbital together with a complementary topological $c$ orbital, allowing us to extract hopping and hybridization amplitudes from first principles. The resulting parameters provide an ab initio benchmark for the effective Hamiltonian. Our work establishes a foundation for understanding superconductivity in moir\'e TMDs and highlights tWSe$_2$ as a promising platform for exploring topological superconductivity.

cond-mat.str-el

Chiral, Electronically Decoupled Layers of 1T'-WS2 Topological Insulator via Neutral-Molecule Intercalation

Monolayer 1T'-WS2 is predicted to be a two-dimensional topological insulator, but its intrinsic electronic properties are masked by strong interlayer coupling in its metallic and superconducting bulk parent phase, 2M-WS2. Isolating monolayers by mechanical exfoliation is also hindered by this coupling, preventing experimental examination of monolayer properties. Here we show that 2M-WS2 undergoes amine intercalation through a simple wet-chemical reaction, yielding superlattices in which the 1T' layers are structurally preserved but electronically decoupled by neutral molecular spacers. Intercalation expands the interlayer spacing from 0.5 to 1-4 nm and reconstructs the stacking while preserving the intralayer 1T' framework. Controlled (de)intercalation reversibly switches the system between a superconducting metal and an insulator with an activation gap matching that of the isolated monolayer. Density functional theory indicates that the electronically decoupled layers retain the nontrivial Z2 topology of the monolayer. Chiral amine intercalation further induces chiroptical activity in WS2 electronic transitions. Overall, the successful intercalation challenges the long-held view that group VIB dichalcogenides are inert toward neutral-molecule intercalation and demonstrates molecular intercalation as a general chemical route for realizing monolayer-like topological-insulator physics and enabling chiral van der Waals superlattices in bulk single crystals.

cond-mat.mtrl-sci

Ideal Quantum Geometry for Fractional Chern Insulators

Quantum geometry plays a fundamental role in many aspects of condensed matter physics. Among its central objects are the Berry curvature and the quantum metric -- quantities that, while distinct, are intertwined through geometric constraints. In this article, we survey recent progress in understanding when and how this bound is saturated, with particular emphasis on the emergence of momentum-space holomorphicity of Bloch states. These developments highlight a profound connection between certain ideal Bloch bands and the Hilbert space structure of the lowest Landau level. We elucidate this relationship through a review of quantum Hall physics in both homogeneous and spatially varying magnetic fields, and conclude by exploring its implications for the search for fractionalized phases in emerging platforms, including moir\'e materials.

cond-mat.str-el

Band mixing and particle-hole asymmetry in moir\'e fractional Chern insulators

We investigate the effect of remote band mixing on the stability of fractional Chern insulators in a family of models that approximate continuum descriptions of moir\'e materials. Our results suggest that the experimentally observed asymmetry between filling fractions $\nu=1/3$ and $\nu=2/3$ in twisted MoTe$_2$ originates from a competition between a fractional Chern insulator, an electron Wigner crystal, and a hole Wigner crystal. In the absence of band mixing, the leading instability at $\nu = 1/3$ is the electron crystal, whereas at $\nu = 2/3$ the main competing phase is the hole crystal. Remote band mixing substantially lowers the energy of the electron crystal but has only a weak effect on the hole crystal. Consequently, it destabilizes the fractional Chern insulator at $\nu=1/3$ more strongly than at $\nu=2/3$. This mechanism also provides an explanation for the emergence of re-entrant integer quantum anomalous Hall states in moir\'e MoTe$_2$ for fillings $\nu>1/2$.

cond-mat.str-el

A unifying framework for sum rules and bounds on optical, thermoelectric and thermal transport from quantum geometry

We present a geometric formulation of optical, thermoelectric, and thermal linear response in clean, zero temperature band insulators based on a single object: a generalized time-dependent quantum geometric tensor (g-tQGT) built from correlations of projected particle and heat polarization operators. Within this framework, the AC transport tensors admit compact expressions that make their geometric content explicit. The response splits into a Berry curvature contribution that remains finite in the DC limit and a frequency correction governed by the quantum metric, implying geometry driven effects even in topologically trivial insulators. At equal times, the g-tQGT recovers the usual integrated QGT and yields energy-weighted thermal analogs whose antisymmetric parts are fixed by orbital and heat magnetization. Importantly, in the thermal channel, a thermal quantum geometric tensor is obtained. Casting the theory in a Hilbert-Schmidt inner product form yields a bound on the trace of the thermal QGT, an uncertainty relation on the projected polarization operators and a purely geometric upper bound on the finite-time accumulated response. The latter is used in the optical channel to derive a geometric upper bound on the electric current. Finally, time derivatives of the g-tQGT are used to generate a hierarchy of generalized thermoelectric and thermal sum rules, and bounds on these sum rules are obtained. These bounds are used to find inequalities between different physical objects such as the optical mass, susceptibility functions and magnetizations.

cond-mat.mes-hall

Chiral Weyl-Kondo semimetals and hexagonal heavy fermion systems

Strong correlation, in concert with symmetry and topology, engenders novel gapless phases of matter, though only a tip of the iceberg has been seen. An exemplary framework is provided by Weyl-Kondo semimetals, in which Weyl fermions develop through crystalline symmetry constraints on the emergent low-energy heavy-fermion excitations. This paradigm has opened up new opportunities to explore correlated topologies without a noninteracting counterpart, but fully realizing this potential requires a large base of candidate materials. Here we confront the challenge on both fronts by studying heavy fermion systems with hexagonal space groups. This family contains a large number of chiral nonsymmorphic crystal structures that promote Weyl degeneracies and, in addition, feature geometric frustration in the $f$-electron magnetism. Our calculations for the heavy fermion states identify Weyl-Kondo semimetals with chiral or achiral Weyl nodes in the respective structural classes. We also develop the first search strategy of any kind for the difficult case of strongly correlated materials, which is also suitable for automation, using a combination of materials database, symmetry classification and search for desired experimental properties, and propose as candidate topological heavy fermion systems the chiral CePt$_2$B and achiral Ce$_2$NiGe$_3$ and Ce$_6$Co$_{2-\delta}$Si$_3$. Our findings raise the prospect for strongly correlated metallic topology in the unusual setting of exotic quantum magnetism and, moreover, point a way to go beyond serendipity in the search for novel strongly correlated quantum materials.

cond-mat.str-el

High-throughput discovery of moir\'e homobilayers guided by topology and energetics

Van der Waals heterostructures promise on-demand designer quantum phases through control of monolayer composition, stacking, twist angle, and external fields. Yet, experimental efforts have been narrowly focused, leaving much of this vast moir\'e landscape unexplored and potential promises unrealized. Here, we present a scalable workflow for high-throughput characterization of twisted homobilayers and apply it to $K$-valley semiconductors. Combining small-scale density functional theory with perturbation theory, we efficiently extract moir\'e band gaps, valley Chern numbers, magic angles, and the threshold for lattice relaxation. Beyond this rapid high-throughput characterization, we parameterize a continuum model for each material, which provides a starting point for more detailed study. Our survey delivers an actionable map for systematic exploration of correlated and topological phases in moir\'e homobilayers, and identifies promising new platforms: chromium-based transition metal dichalcogenides for high-temperature quantum anomalous Hall effects, transition metal nitride halides for intertwined superconducting and moir\'e physics, and atomically thin $\rm{III-V}$ semiconductors for room-temperature-scale moir\'e effects.

cond-mat.mtrl-sci

Two-dimensional helical superconductivity and gapless superconducting edge modes in the 1T$^\prime$-WS$_2$/2H-WS$_2$ heterophase bilayer

We propose a material platform comprised of transition metal dichalcogenide (TMDC) heterostructures to realize the two-dimensional (2D) helical superconductivity with an intrinsic gap. By van der Waals stacking a 2D superconductor (1T$^\prime$-WS$_2$ with inversion symmetry) on top of a 2D topological insulator (2H-WS$_2$ with mirror symmetry), the resulting TMDC bilayer exhibits Rashba superconductivity. Under an external in-plane magnetic field, the system can host finite-momentum Cooper pairing, evidenced by the divergence in the particle-particle susceptibility of a $k\cdot p$ Hamiltonian fitted to the \textit{ab initio} theory band structure. The resulting 2D helical superconducting phase can induce superconductivity in the edge states with its spatially varying order parameter. By varying the strength of the in-plane magnetic field, we demonstrate that the helical edge state can undergo a phase transition to a one-dimensional gapless phase with narrow Fermi segments corresponding to zero-energy Bogoliubov quasi-particles. The controllable one-dimensional gapless phase serves as a clear experimental fingerprint of 2D helical superconductivity. The proposed 2D TMDC heterostructure is promising for intrinsic nonreciprocal superconducting transport and the development of Majorana-based quantum devices.

cond-mat.supr-con

Efficient prediction of topological superlattice bands with spin-orbit coupling

We develop a symmetry indicator framework to efficiently predict the topology of superlattice-induced minibands with spin-orbit coupling. Our algorithm requires input only from the parent material before the superlattice is applied. The simplification arises by assuming a perturbatively weak superlattice potential; however, our results extend beyond the perturbative regime as long as the superlattice-induced gaps remain open. We first consider a time-reversal- and inversion-symmetric system subject to a weak superlattice potential and derive a compact formula for the $\mathbb{Z}_2$ invariant of the lowest miniband. We then extend to time-reversal breaking systems and compute the Chern number. We apply our theory to selected transition metal dichalcogenides, HgTe/CdTe quantum wells, and thin films of three-dimensional topological insulators and Dirac semimetals. We find topological superlattice bands can arise even from non-topological materials, broadening the pool of candidates for realizing topological flat bands. Our theory predicts which geometry and periodicity of superlattice will yield topological bands for a given material, providing a clear guiding principle for designing topological superlattice heterostructures.

cond-mat.mes-hall

Altermagnetism induced surface Chern insulator

We propose a new pathway to the quantized anomalous Hall effect (QAHE) by coupling an altermagnet to a topological crystalline insulator (TCI). The former gaps the topological surface states of the TCI, thereby realizing the QAHE in a robust and switchable platform with near- vanishing magnetization. We demonstrate the feasibility of this approach by studying a slab of the TCI SnTe coupled to an altermagnetic RuO2 layer. Our first-principles calculations reveal that the d-wave altermagnetism in RuO2 induces a 7 meV gap to the Dirac surface states on the (110) surface of SnTe, producing a finite anomalous Hall effect. Our approach generalizes to broader classes of altermagnetic materials and TCIs, thereby providing a family of topological altermagnetic heterostructures with small or vanishing magnetization that support nontrivial Chern numbers. Our results highlight a promising new topological platform with great tunability and applications to spintronics.

cond-mat.mes-hall

Charge density wave induced gapped nodal line

We investigate the interplay between charge density wave (CDW) order and topological nodal-line states in square-net materials. Our Ginzburg-Landau theory predicts a CDW instability that generically opens a gap at the Fermi energy while preserving the nodal line crossing. However, as the Fermi level approaches the nodal line, the density of states at the nodal line decreases, eventually disappearing as the CDW vector $\mathbf{Q}$ goes to zero. Exactly at $\mathbf{Q} = 0$, the order parameter explicitly breaks the glide symmetry protecting the nodal line, which allows a gap to open. Yet, for small but finite $\mathbf{Q}$, the nodal line may vanish within experimental resolution even when the glide symmetry is preserved. Our results provide a consistent explanation for recent experimental observations.

cond-mat.str-el

Topological chiral superconductivity from antiferromagnetic correlations in moir\'{e} bands with extreme spin-orbit coupling

Motivated by the strong-correlation phenomenology observed near the superconducting phase in twisted bilayer WSe$_2$, we study multi-orbital $t$-$J$ models that are derived from different parameter regimes. The models contain effective antiferromagnetic interactions that are influenced by the strong underlying spin-orbit coupling. The possible superconducting pairing states are investigated in these models. We find that the preferred pairing order parameters are associated with the $^{1,2}E$ representations of the three-fold rotation symmetry operator $C_3$, with the $p\pm i p$ component intermixing with the $d\pm id$ component. The chiral superconducting states are shown to be topological, based on the Wilson loops of the corresponding Bogoliubov quasiparticles. We discuss the implications of our findings for experimental observations, as well as the new connections our results uncover between the moir\'{e} superconductivity and its counterpart in bulk quantum materials.

cond-mat.supr-con

Majoranas with a twist: Tunable Majorana zero modes in altermagnetic heterostructures

Altermagnetism provides new routes to realize Majorana zero modes with vanishing net magnetization. We consider a recently proposed heterostructure consisting of a semiconducting wire on top of an altermagnet and with proximity-induced superconductivity. We demonstrate that rotating the wire serves as a tuning knob to induce the topological phase. For $d$-, $g$- and $i$-wave altermagnetic pairing, we derive angle-dependent topological gap-closing conditions. We derive symmetry constraints on angles where the induced altermagnetism must vanish, which we verify by explicit models. Our results imply that a bent or curved wire realizes a spatially-dependent topological invariant with Majorana zero modes pinned to positions where the topological invariant changes. This provides a new experimental set-up whereby a single wire can host both topologically trivial and nontrivial regimes without $in$ $situ$ tuning.

cond-mat.mes-hall

Quantum-geometric dipole: a topological boost to flavor ferromagnetism in flat bands

Robust flavor-polarized phases are a striking hallmark of many flat-band moir\'e materials. In this work, we trace the origin of this spontaneous polarization to a lesser-known quantum-geometric quantity: the quantum-geometric dipole. Analogous to how the quantum metric governs the spatial spread of wavepackets, we show that the quantum-geometric dipole sets the characteristic size of particle-hole excitations, e.g. magnons in a ferromagnet, which in turn boosts their gap and stiffness. Indeed, the larger the particle-hole separation, the weaker the mutual attraction, and the stronger the excitation energy. In topological bands, this energy enhancement admits a lower bound within the local-mode approximation, highlighting the crucial role of topology in flat-band ferromagnetism. We illustrate these effects in microscopic models, emphasizing their generality and relevance to moir\'e materials. Our results establish the quantum-geometric dipole as a predictive geometric indicator for ferromagnetism in flat bands, a crucial prerequisite for topological order.

cond-mat.mes-hall

Optimizing superlattice bilayer graphene for a fractional Chern insulator

Bernal-stacked bilayer graphene modulated by a superlattice potential is a highly tunable system predicted to realize isolated topological flat bands. In this work we calculate the band structure and quantum geometry of bilayer graphene subject to both triangular and square superlattices, across a wide range of gate voltages. We identify the parameter regime that optimizes the "single-particle indicators" for the stability of a fractional Chern insulator (FCI) when a topological flat band is partially filled. Our results guide the experimental realization of an FCI in this platform.

cond-mat.mes-hall

Tunable Topological Phases in Multilayer Graphene Coupled to a Chiral Cavity

Coupling photonic cavity fields to electronic degrees of freedom in 2D materials introduces an additional control knob to the toolbox of solid-state engineering. Here we demonstrate a subtle competition between cavity frequency and interlayer tunneling in graphene stacks that is responsible for topological phase transitions in light-matter Hilbert space and that cannot be captured by mean-field theory in vacuum. A systematic exploration of multilayer graphene heterostructures and stacking configurations in a chiral tHz cavity reveals that linear dispersion enhances the low-energy cavity-induced topological gap. Furthermore, in bilayer graphene, a displacement field drives the low-energy vacuum band from valley-Chern to Chern insulator, comprising a gate-tunable topological phase transition. Our findings pave the way for future control and engineering of graphene heterostructures with chiral cavity fields.

cond-mat.mes-hall