arXiv subjects

Jennifer Cano

Publications and source records attributed to Jennifer Cano.

At least 37 records · Page 2Linked to original sources

arXiv2025

Tunable Topological Phases in Multilayer Graphene Coupled to a Chiral Cavity

Coupling photonic cavity fields to electronic degrees of freedom in 2D materials introduces an additional control knob to the toolbox of solid-state engineering. Here we demonstrate a subtle competition between cavity frequency and interlayer tunneling in graphene stacks that is responsible for topological phase transitions in light-matter Hilbert space and that cannot be captured by mean-field theory in vacuum. A systematic exploration of multilayer graphene heterostructures and stacking configurations in a chiral tHz cavity reveals that linear dispersion enhances the low-energy cavity-induced topological gap. Furthermore, in bilayer graphene, a displacement field drives the low-energy vacuum band from valley-Chern to Chern insulator, comprising a gate-tunable topological phase transition. Our findings pave the way for future control and engineering of graphene heterostructures with chiral cavity fields.

cond-mat.mes-hall↗

arXiv2025

Optimizing superlattice bilayer graphene for a fractional Chern insulator

Bernal-stacked bilayer graphene modulated by a superlattice potential is a highly tunable system predicted to realize isolated topological flat bands. In this work we calculate the band structure and quantum geometry of bilayer graphene subject to both triangular and square superlattices, across a wide range of gate voltages. We identify the parameter regime that optimizes the "single-particle indicators" for the stability of a fractional Chern insulator (FCI) when a topological flat band is partially filled. Our results guide the experimental realization of an FCI in this platform.

cond-mat.mes-hall↗

arXiv2025

Kondo-lattice phenomenology of twisted bilayer WSe$_2$ from compact molecular orbitals of topological bands

The discovery of superconductivity and correlated electronic phases in twisted bilayer WSe$_2$ (Xia et al., Nature 2024; Guo et al., Nature 2025) has generated considerable excitement. Accompanying the superconductivity and a correlated insulator phase is the Kondo-lattice-like phenomenology in transport properties. Here we consider how such phenomenology can develop when the combination of the active bands are topological. We advance a unique construction of compact molecular orbitals through a partial Wannierization that is symmetry preserving. The resulting Anderson lattice model provides the basis for a microscopic understanding of the experimental observation, including the involved energy scales. Our approach may apply to a broad range of settings where topology and correlations interplay.

cond-mat.str-el↗

arXiv2025

A Recipe for Flat Bands in Pyrochlore Materials: A Chemist's Perspective

Materials in which atoms are arranged in a pyrochlore lattice have found renewed interest, as, at least theoretically, orbitals on those lattices can form flat bands. However, real materials often do not behave according to theoretical models, which is why there has been a dearth of pyrochlore materials exhibiting flat band physics. Here we examine the conditions under which ideal 'pyrochlore bands' can exist in real materials and how to have those close to the Fermi level. We find that the simple model used in the literature does not apply to the bands at the Fermi level in real pyrochlore materials. However, surprisingly, certain oxide compounds which have oxygen orbitals inside the pyrochlore tetrahedra do exhibit near-ideal pyrochlore bands near the Fermi level. We explain this observation by a generalized tight-binding model including the oxygen orbitals. We further classify all known pyrochlore materials based on their crystal structure, band structure, and chemical characteristics and propose materials to study in future experiments.

cond-mat.mtrl-sci↗

arXiv2025

Metallic quantum criticality enabled by flat bands in a kagome lattice

Strange metals arise in a variety of platforms for strongly correlated electrons, ranging from the cuprates, heavy fermions to flat band systems. Motivated by recent experiments in kagome metals, we study a Hubbard model on a kagome lattice whose noninteracting limit contains flat bands. A Kondo lattice description is constructed, in which the correlation effects are captured by symmetry preserving and exponentially localized molecular orbitals. These compact molecular orbitals represent the local degrees of freedom that emerge from topological flat bands. We identify a quantum critical point at which quasiparticles are lost and strange metallicity emerges. Our theoretical work opens up a new route for realizing beyond-Landau quantum criticality, as well as the associated strange metallicity and emergent quantum phases.

cond-mat.str-el↗

arXiv2025

Superconductivity in twisted WSe$_2$ from topology-induced quantum fluctuations

Recently, superconductivity has been observed in twisted WSe$_2$ moiré structures (Xia et al., Nature 2024; Guo et al., Nature 2025). Its transition temperature is high, reaching a few percent of the Fermi temperature scale. Here, we advance a mechanism for superconductivity based on the notion that electronic topology enables quantum fluctuations in a suitable regime of intermediate correlations. In this regime, the Coulomb interaction requires that an active topological flat band and nearby wider bands are considered together. Compact molecular orbitals arise, which give rise to quantum fluctuations through topology-dictated hybridization with the other molecular orbitals. The hybridization competes with the active flat band's natural tendency towards static electronic ordering, thereby weakening the latter; we link this effect with certain salient observations by experiments. Furthermore, the competition yields a quantum critical regime where quasiparticles are lost. The corresponding quantum critical fluctuations drive superconductivity. Broader implications and new connections among correlated materials platforms are discussed.

cond-mat.str-el↗

arXiv2024

Uncovering the Hidden Ferroaxial Density Wave as the Origin of the Axial Higgs Mode in RTe$_3$

The recent discovery of an axial amplitude (Higgs) mode in the long-studied charge density wave (CDW) systems GdTe$_3$ and LaTe$_3$ suggests a heretofore unidentified hidden order. A theoretical study proposed that the axial Higgs results from a hidden ferroaxial component of the CDW, which could arise from non-trivial orbital texture. Here, we report extensive experimental studies on ErTe$_3$ and HoTe$_3$ that possess a high-temperature CDW similar to other RTe$_3$ (R = rare earth), along with an additional low-temperature CDW with an orthogonal ordering vector. Combining Raman spectroscopy with large-angle convergent beam electron diffraction (LACBED), rotational anisotropy second-harmonic generation (RA-SHG), and muon-spin relaxation ($μ$SR), we provide unambiguous evidence that the high-temperature CDW breaks translation, rotation, and all vertical and diagonal mirror symmetries, but not time-reversal or inversion. In contrast, the low-temperature CDW only additionally breaks translation symmetry. Simultaneously, Raman scattering shows the high-temperature CDW produces an axial Higgs mode while the low-temperature mode is scalar. The weak monoclinic structural distortion and clear axial response in Raman and SHG are consistent with a ferroaxial phase in RTe$_3$ driven by coupled orbital and charge orders. Thus, our study provides a new standard for uncovering unconventional orders and confirms the power of Higgs modes to reveal them.

cond-mat.str-el↗

arXiv2024

Efficient prediction of superlattice and anomalous miniband topology from quantum geometry

Two dimensional materials subject to long-wavelength modulations have emerged as novel platforms to study topological and correlated quantum phases. In this article, we develop a versatile and computationally inexpensive method to predict the topological properties of materials subjected to a superlattice potential by combining degenerate perturbation theory with the method of symmetry indicators. In the absence of electronic interactions, our analysis provides a systematic rule to find the Chern number of the superlattice-induced miniband starting from the harmonics of the applied potential and a few material-specific coefficients. Our method also applies to anomalous (interaction-generated) bands, for which we derive an efficient algorithm to determine all Chern numbers compatible with a self-consistent solution to the Hartree-Fock equations. Our approach gives a microscopic understanding of the quantum anomalous Hall insulators recently observed in rhombohedral graphene multilayers.

cond-mat.mes-hall↗

arXiv2024

Magnetic Weyl-Kondo semimetals induced by quantum fluctuations

Weyl-Kondo semimetals are strongly correlated topological semimetals that develop through the cooperation of the Kondo effect with space group symmetries. The Kondo effect, capturing quantum fluctuations associated with strong correlations, is usually suppressed by magnetic order. Here we develop the theory of magnetic Weyl-Kondo semimetal. The key of the proposed mechanism is that the magnetic order comes from conduction $d$ electrons, such that the local $f$ moments can still fluctuate. We illustrate the extreme case where the magnetic space group symmetries prevent any spontaneous magnetization on the sites with the $f$-orbitals. In this case, topological degeneracies, including hourglass Weyl-Kondo nodal lines, appear when the magnetic space group symmetry constrains the Kondo-driven low-energy excitations; they lead to a third-order nonlinear anomalous Hall response. Based on the proposed mechanism, we explore the interplay between strong correlations and symmetries with database search leading to several candidate materials. The most prominent candidates are antiferromagnetic $\rm UNiGa$ and $\rm UNiAl$, with a third-order anomalous Hall response, as well as ferromagnetic $\rm USbTe$ and $\rm CeCoPO$, with a first-order one. Our findings pave the way for future experimental and theoretical investigations that promise to further advance the overarching theme of strongly correlated topology.

cond-mat.str-el↗

arXiv2024

Inducing topological flat bands in bilayer graphene with electric and magnetic superlattices

It was recently argued that Bernal stacked bilayer graphene (BLG) exposed to a 2D superlattice (SL) potential exhibits a variety of intriguing behaviors [Ghorashi et al., Phys. Rev. Lett. 130, 196201 (2023)]. Chief among them is the appearance of flat Chern bands that are favorable to the appearance of fractional Chern insulator states. Here, we explore the application of spatially periodic out-of-plane orbital magnetic fields to the model of Ghorashi et al. to find additional means of inducing flat Chern bands. We focus on fields that vary on length scales much larger than the atomic spacing in BLG, generating what we refer to as magnetic SLs. The magnetic SLs we investigate either introduce no net magnetic flux to the SL unit cell, or a single quantum of flux. We find that magnetic SLs acting on their own can induce topological flat bands, but richer behavior, such as the appearance of flat and generic bands with high Chern numbers, can be observed when the magnetic SLs act in conjunction with commensurate electric SLs. Finally, we propose a method of generating unit-flux-quantum magnetic SLs along with concomitant electric SLs. The magnetic SL is generated by periodic arrays of flux vortices originating from type II superconductors, while the electric SL arises due to a magnetic SL-induced charge density on the surface of a magnetoelectric material. Tuning the vortex lattice and the magnetoelectric coupling permits control of both SLs, and we study their effects on the band structure of BLG.

cond-mat.mes-hall↗

arXiv2024

Topological Kondo semimetal and insulator in AB-stacked heterobilayer transition metal dichalcogenides

Recent experiments reported the realization of a heavy Fermi liquid in AB-stacked MoTe$_2$/WSe$_2$ heterobilayers. In this paper we show that the AB-stacked heterobilayer configuration is particularly suited to realize topological Kondo semimetal and topological Kondo insulator ground states at a doping of two holes per moiré unit cell. The small lattice mismatch between the MoTe$_2$ and WSe$_2$ monolayers and the different bandwidths of their highest lying moiré valence bands means that, in the experimentally relevant range of hole dopings, the MoTe$_2$ layer is effectively a Mott insulator with only low-lying magnetic excitations Kondo-coupled to more itinerant electrons in the WSe$_2$. The crucial consequence of the AB-stacking configuration is that the interlayer tunnelling connects orbitals of opposite parity in the two layers, leading to a chiral Kondo coupling. We show that the chiral Kondo coupling favors a topological Kondo semimetal at filling $ν=1+1$, with a non-quantized spin Hall conductance arising from edge modes, whose spectrum and overlap with bulk states we determine. We further show that a spatially random strain field that locally breaks the rotation symmetry can convert the Kondo semimetal to a narrow gap topological Kondo insulator featuring a quantized spin Hall conductance.

cond-mat.str-el↗

arXiv2024

Chern Bands' Optimally Localized Wannier Functions and Fractional Chern Insulators

Recent development on fractional Chern insulators and proximate phases call for a real space representation of isolated Chern bands. Here we propose a new method for a general construction of optimally localized Wannier functions from such Chern bands. We do so through an optimal gauge choice of the Bloch states of a Chern band with the singularity placed at any desired position in momentum space. We apply this method to construct the optimally localized Wannier functions for kagome lattice, and use it to identify channels of interactions that are favorable to the development of fractional Chern insulators. Implications of the approach for the interplay between correlations and topology in broader contexts are discussed.

cond-mat.mes-hall↗

arXiv2024

Symmetry constraints and spectral crossing in a Mott insulator with Green's function zeros

Lattice symmetries are central to the characterization of electronic topology. Recently, it was shown that Green's function eigenvectors form a representation of the space group. This formulation has allowed the identification of gapless topological states even when quasiparticles are absent. Here we demonstrate the profundity of the framework in the extreme case, when interactions lead to a Mott insulator, through a solvable model with long-range interactions. We find that both Mott poles and zeros are subject to the symmetry constraints, and relate the symmetry-enforced spectral crossings to degeneracies of the original non-interacting eigenstates. Our results lead to new understandings of topological quantum materials and highlight the utility of interacting Green's functions toward their symmetry-based design.

cond-mat.str-el↗

arXiv2024

Emergent flat band and topological Kondo semimetal driven by orbital-selective correlations

Flat electronic bands are expected to show proportionally enhanced electron correlations, which may generate a plethora of novel quantum phases and unusual low-energy excitations. They are increasingly being pursued in $d$-electron-based systems with crystalline lattices that feature destructive electronic interference, where they are often topological. Such flat bands, though, are generically located far away from the Fermi energy, which limits their capacity to partake in the low-energy physics. Here we show that electron correlations produce emergent flat bands that are pinned to the Fermi energy. We demonstrate this effect within a Hubbard model, in the regime described by Wannier orbitals where an effective Kondo description arises through orbital-selective Mott correlations. Moreover, the correlation effect cooperates with symmetry constraints to produce a topological Kondo semimetal. Our results motivate a novel design principle for Weyl Kondo semimetals in a new setting, viz. $d$-electron-based materials on suitable crystal lattices, and uncover interconnections among seemingly disparate systems that may inspire fresh understandings and realizations of correlated topological effects in quantum materials and beyond.

cond-mat.str-el↗

arXiv2024

Charge density-waves with non-trivial orbital textures in rare earth tritellurides

Motivated by recent experiments reporting unconventional collective modes in the charge density-wave (CDW) state of rare-earth tritellurides $R$Te$_3$, we derive from a multi-orbital microscopic model on the square net a CDW Ginzburg-Landau theory that allows for non-trivial orbital order. Our analysis reveals unconventional CDWs where order parameters with distinct orbital character coexist due to an approximate symmetry of the low-energy model, which becomes exact in the limit of nearest-neighbor-only hopping and decoupled $p_x$, $p_y$ orbitals. Because of this coexistence, the resulting CDW pattern displays an orbital texture that generally breaks additional symmetries of the lattice besides those explicitly broken by the CDW wave-vector. In particular, we find two competing phases that differ in whether they break or preserve inversion and vertical mirror symmetries. We explain the mechanisms that favor each outcome, and discuss experimental probes that can distinguish the different phases.

cond-mat.str-el↗

arXiv2024

Multifold topological semimetals

The discovery of topological semimetals with multifold band crossings has opened up a new and exciting frontier in the field of topological physics. These materials exhibit large Chern numbers, leading to long double Fermi arcs on their surfaces, which are protected by either crystal symmetries or topological order. The impact of these multifold crossings extends beyond surface science, as they are not constrained by the Poincaré classification of quasiparticles and only need to respect the crystal symmetry of one of the 1651 magnetic space groups. Consequently, we observe the emergence of free fermionic excitations in solid-state systems that have no high-energy counterparts, protected by non-symmorphic symmetries. In this work, we review the recent theoretical and experimental progress made in the field of multifold topological semimetals. We begin with the theoretical prediction of the so-called multifold fermions and discuss the subsequent discoveries of chiral and magnetic topological semimetals. Several experiments that have realized chiral semimetals in spectroscopic measurements are described, and we discuss the future prospects of this field. These exciting developments have the potential to deepen our understanding of the fundamental properties of quantum matter and inspire new technological applications in the future.

cond-mat.mtrl-sci↗

arXiv2024

Sublattice structure and topology in spontaneously crystallized electronic states

The prediction and realization of the quantum anomalous Hall effect are often intimately connected to honeycomb lattices in which the sublattice degree of freedom plays a central role in the nontrivial topology. Two-dimensional Wigner crystals, on the other hand, form triangular lattices without sublattice degrees of freedom, resulting in a topologically trivial state. In this Letter, we discuss the possibility of spontaneously formed honeycomb-lattice crystals that exhibit the quantum anomalous Hall effect. Starting from a single-band system with nontrivial quantum geometry, we derive the mean-field energy functional of a class of crystal states and express it as a model of sublattice pseudospins in momentum space. We find that nontrivial quantum geometry leads to extra terms in the pseudospin model that break an effective `time-reversal symmetry' and favor a topologically nontrivial pseudospin texture. When the effects of these extra terms dominate over the ferromagnetic exchange coupling between pseudospins, the anomalous Hall crystal state becomes energetically favorable over the trivial Wigner crystal state.

cond-mat.str-el↗

arXiv2024

Dirac zeros in an orbital selective Mott phase: Green's function Berry curvature and flux quantization

How electronic topology develops in strongly correlated systems represents a fundamental challenge in the field of quantum materials. Recent studies have advanced the characterization and diagnosis of topology in Mott insulators whose underlying electronic structure is topologically nontrivial, through ``Green's function zeros". However, their counterparts in metallic systems have yet to be explored. Here, we address this problem in an orbital-selective Mott phase (OSMP), which is of extensive interest to a variety of strongly correlated systems with a short-range Coulomb repulsion. We demonstrate symmetry protected crossing of the zeros in an OSMP. Utilizing the concept of Green's function Berry curvature, we show that the zero crossing has a quantized Berry flux. The resulting notion of Dirac zeros provides a window into the largely hidden landscape of topological zeros in strongly correlated metallic systems and, moreover, opens up a means to diagnose strongly correlated topology in new materials classes.

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