arXiv subjects

Jeongmin Oh

Publications and source records attributed to Jeongmin Oh.

4 recordsLinked to original sources

arXiv2026

A miniature evaporator for in-operando deposition of isolated atoms in a low-temperature scanning tunneling microscope

Depositing dilute atomic ensembles onto cold samples is challenging in low-temperature scanning tunneling microscopes (STM) because radiation shields and restricted internal geometries often preclude a direct deposition path, particularly in instruments designed for millikelvin operation. We present a compact, milliwatt-range evaporation source fabricated from a commercial miniature incandescent lamp and integrated directly into a millikelvin STM head. The exposed tungsten filament is coated with a micrometre-thick Fe film and positioned about 1 cm from the sample. We deposit isolated Fe atoms onto MgO/Ag(100) while operating the microscope near 5 K. Evaporation increases the STM-body temperature by only about 2 K, and the same nanoscopic surface region can be readily scanned after deposition with a lateral displacement of less than 5 nm. Differential-conductance spectra displaying symmetric inelastic steps near $\pm$14 mV identify the deposited atoms on MgO as Fe. From STM images, we estimate a local deposition flux of $1.5\times10^{-5}~\mathrm{nm^{-2}\,s^{-1}}$, corresponding to a nominal evaporator lifetime of ~150 h. The fixed evaporator enables repeated low-flux deposition without a room-temperature line of sight, the need for movable radiation shields, or mechanical evaporator access after cooldown, while preserving access to the same atomic-scale surface region before and after deposition.

cond-mat.mes-hall↗

arXiv2026

All-electrical Coherent Control of a Single Rare-earth Spin Qubit

Electrical control of single spin qubits is a major frontier for nanoscale, high-speed, and scalable quantum devices. Yet, extending it to highly shielded rare-earth 4f electrons remains an experimental challenge across solid-state platforms. Here we demonstrate all-electrical coherent control of a single Er electron spin, which is exchange-coupled to a nearby Ti atom. Scanning tunneling microscopy-based electron spin resonance with three-dimensional magnetic-field control enables comprehensive mapping of the resonance and Rabi frequencies, revealing pronounced anisotropies in both the Er g-tensor and the Er-Ti exchange interaction. The electrical modulation of the anisotropic Er-Ti coupling results in an efficient drive of the Er spin, allowing us to achieve near-gigahertz Rabi frequencies - a ten-fold improvement over the present record for rare-earth spin qubits. By establishing anisotropic exchange as a general resource for electrically accessing shielded rare-earth spins, our results open a new route to ultrafast and local control of rare-earth spins in solid-state quantum devices.

cond-mat.mes-hall↗

arXiv2023

Electrically Driven Spin Resonance of 4f Electrons in a Single Atom on a Surface

A pivotal challenge in quantum technologies lies in reconciling long coherence times with efficient manipulation of the quantum states of a system. Lanthanide atoms, with their well-localized 4f electrons, emerge as a promising solution to this dilemma if provided with a rational design for manipulation and detection. Here we construct tailored spin structures to perform electron spin resonance on a single lanthanide atom using a scanning tunneling microscope. A magnetically coupled structure made of an erbium and a titanium atom enables us to both drive the erbium's 4f electron spins and indirectly probe them through the titanium's 3d electrons. In this coupled configuration, the erbium spin states exhibit a five-fold increase in the spin relaxation time and a two-fold increase in the driving efficiency compared to the 3d electron counterparts. Our work provides a new approach to accessing highly protected spin states, enabling their coherent control in an all-electric fashion.

cond-mat.mes-hall↗

arXiv2022

Development of a Scanning Tunneling Microscope for Variable Temperature Electron Spin Resonance

Recent advances in increasing the spectroscopic energy resolution in scanning tunneling microscopy (STM) have been achieved by integrating electron spin resonance (ESR) with STM. Here, we demonstrate the design and performance of a home-built STM capable of ESR at temperatures ranging from 1 K to 10 K. The STM is incorporated with a home-built Joule-Thomson refrigerator and a 2-axis vector magnet. Our STM design allows for the deposition of atoms and molecules directly into the cold STM, eliminating the need to extract the sample for deposition. In addition, we adopt two methods to apply radio-frequency (RF) voltages to the tunnel junction, the early design of wiring to the STM tip directly, and a more recent idea to use an RF antenna. Direct comparisons of ESR results measured using the two methods and simulations of electric field distribution around the tunnel junction show that, despite their different designs and capacitive couplings to the tunnel junction, there is no discernible difference in the driving and detection of ESR. Furthermore, at a magnetic field of 1.6 T, we observe ESR signals (near 40 GHz) sustained up to 10 K, which is the highest temperature for ESR-STM measurement reported to date, to the best of our knowledge. Although the ESR intensity exponentially decreases with increasing temperature, our ESR-STM system with low noise at the tunnel junction allows us to measure weak ESR signals with intensities in the sub-fA range. Our new design of ESR-STM, which is operational in a large frequency and temperature range, can broaden the use of ESR spectroscopy in STM and enable the simple modification of existing STM systems, which will hopefully accelerate a generalized use of ESR-STM.

cond-mat.mes-hall↗