arXiv subjects

Ji Ung Lee

Publications and source records attributed to Ji Ung Lee.

At least 19 recordsLinked to original sources

arXiv2026

Intrinsic magnetization of the superconducting condensate in Fe(Te,Se)

A spin-polarized superconducting condensate generates a net magnetization with measurable signatures. We present evidence for an intrinsic magnetic field in mesoscopic Fe(Te,Se) rings. The intrinsic field, encoded in the phase of superconducting quantum oscillations, scales linearly with the DC bias current, and its orientation exhibits an anomalous dependence on polarity and magnitude of the applied current. The magnetoresistance displays a dual flux-quantization effect with respect to the external magnetic field and the DC current. A minimal model incorporating Rashba coupling with an effective anisotropic out-of-plane interaction accounts for the experimental observations. These results provide evidence for spin-polarized superconductivity at the device scale and open new opportunities for superconducting spintronic and quantum information platforms.

cond-mat.supr-con↗

arXiv2026

Coupling of Klein-Andreev Resonant States in Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$-graphene-Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ Devices

Quantum devices require coherent coupling over macroscopic distances. Recently, resonances due to Klein tunneling and Andreev reflection states (KARS) have been observed in a naturally occurring p-n junction at the interface between Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ (BSCCO), a high-Tc superconductor (HTS), and graphene. The resonances appear as conductance oscillations with gating. Here, we show coupling between the KARS in BSCCO-graphene-BSCCO devices of varying separation (L). The coupling is evidenced by a power-law decay of resonance period as L increases from tens of nanometers to single microns. These results demonstrate the long-distance coupling of KARS cavities in graphene-HTS junctions. The length dependence seen in experiments is supported by single-particle spectral functions which show KARS are coupled by transport modes in graphene. The strong coupling between KARS in BSCCO-graphene-BSCCO junctions showcases the novelty of HTS-graphene junctions for quantum circuits and unconventional Josephson junctions.

cond-mat.supr-con↗

arXiv2025

Aharonov-Bohm interference from coherent spin-polarized edge transport in Fe(Te,Se) superconducting rings

We report the coexistence of Aharonov-Bohm and Little-Parks oscillations in mesoscopic Fe(Te,Se) rings. The magnetoresistance shows two distinct periodicities: an $h/e$ component from ballistic edge interference and an $h/2e$ component from fluxoid quantization of Cooper pairs. Aharonov-Bohm oscillations persist deep into the superconducting phase, exhibit current-field symmetry, and follow a temperature dependence captured by a helical Luttinger liquid model, consistent with edge states in a topological superconductor.

cond-mat.supr-con↗

arXiv2025

Observation of Half-Quantum Vorticity in an Iron-based Superconductor

Half-quantum vortices -- topological excitations carrying half the superconducting flux quantum -- are predicted to emerge in spin-triplet superconductors, where the spin component of order parameter enables fractional flux quantization. We present direct transport signatures of half-quantum vorticity in single-crystal Fe(Te,Se), an iron-based superconductor with helical Dirac surface states. Using mesoscopic superconducting ring devices, we observe half-integer quantum oscillations arising from the splitting of quantized fluxoid states, further supported by distinct signatures of trapped half-integer fluxoids. The quantum oscillations are modulated by a background symmetry, set by the relative orientation of the DC bias current and perpendicular magnetic field, consistent with strong spin-orbit coupling. These findings demonstrate the long-sought half-quantum vorticity in spin-polarized superconductors and open new directions toward non-Abelian excitations in quantum materials and scalable topological qubits.

cond-mat.supr-con↗

arXiv2023

Andreev Reflection and Klein Tunneling in High-Temperature Superconductor/Graphene Junctions

Scattering processes in quantum materials emerge as resonances in electronic transport, including confined modes, Andreev states, and Yu-Shiba-Rusinov states. However, in most instances, these resonances are driven by a single scattering mechanism. Here we show the appearance of resonances due to the combination of two simultaneous scattering mechanisms, one from superconductivity and the other from graphene p-n junctions. These resonances stem from Andreev reflection and Klein tunneling that occur at two different interfaces of a hole-doped region of graphene formed at the boundary with superconducting graphene due to proximity effects from Bi$_2$Sr$_2$Ca$_1$Cu$_2$O$_{8+δ}$. The resonances persist with gating the from p$^+$-p and p-n configurations. The suppression of the oscillation amplitude above the bias energy comparable to the induced superconducting gap indicates the contribution from Andreev reflection. Our experimental measurements are supported by quantum transport calculations in such interfaces, leading to analogous resonances. Our results put forward a hybrid scattering mechanism in graphene/high-temperature superconductor heterojunctions of potential impact for graphene-based Josephson junctions.

cond-mat.supr-con↗

arXiv2022

Measuring the Electronic Bandgap of Carbon Nanotube Networks in Non-ideal p-n Diodes

The measurement of the bandgap in quasi-one dimensional materials such as carbon nanotubes is challenging due to its dimensionality. In this work, we measure the electronic bandgap of networks of polymer-wrapped semiconducting single-walled carbon nanotubes (s-SWCNTs) using non-ideal p-n diodes. Using these diodes, we measure the electronic bandgap and excitonic levels of different polymer-wrapped s-SWCNTs with varying diameters: arc discharge (~1.55nm), (7,5) (0.83nm), and (6,5) (0.76nm). Our values are consistent with theoretical predictions, providing insight into the fundamental properties of networks of s-SWCNTs.

physics.app-ph↗

arXiv2022

All-carbon nanotube solar cell devices mimic photosynthesis

Photovoltaics has two main processes: Optical absorption and power conversion. In photosynthesis, the two equivalent processes are optical absorption and chemical conversion. Whereas in the latter, the two processes are carried out by distinct proteins, in conventional photovoltaic diodes, the two processes are convoluted because the optical and transport paths are the same, leading to inefficiencies. Here, we separate the site and direction of light absorption from those of power generation to show that semiconducting single-walled carbon nanotubes (s-SWCNTs) provide an artificial system that models photosynthesis in a tandem geometry. Using different s-SWCNT chiralities, we implement an energy funnel in dual-gated p-n diodes. This enables the capture of photons from multiple regions of the solar spectrum and the funneling of photogenerated excitons to the smallest bandgap s-SWCNT layer, where they become free carriers. As a result, we demonstrate an increase in the magnitude and spectral response of photocurrent by adding more s-SWCNT layers of different bandgaps without a corresponding deleterious increase in the dark leakage current.

cond-mat.mes-hall↗

arXiv2021

Geometric interference in a high-mobility graphene annulus p-n junction device

The emergence of interference is observed in the resistance of a graphene annulus pn junction device as a result of applying two separate gate voltages. The observed resistance patterns are carefully inspected, and it is determined that the position of the peaks resulting from those patterns are independent of temperature and magnetic field. Furthermore, these patterns are not attributable to Aharonov-Bohm oscillations, Fabry Perot interference at the junction, or moiré potentials. The device data are compared with those of another device fabricated with a traditional Hall bar geometry, as well as with quantum transport simulation data. Since the two devices are of different topological classes, the subtle differences observed in the corresponding measured data indicate that the most likely source of the observed geometric interference patterns is quantum scarring.

cond-mat.mes-hall↗

arXiv2020

Scalable Gate-Defined Majorana Fermions in 2D p-Wave Superconductors

We provide a conceptual framework for developing a scalable topological quantum computer. It relies on forming Majorana fermions using circular electronic gates in two-dimensional p-wave superconductors. The gates allow the precise control of the number, position, and dynamics of Majorana fermions. Using an array of such gates, one can implement the full features of topological quantum computation, including the braiding and fusion of Majoranas in space-time. The gates serve two purposes: They modulate the chemical potential locally to turn a topological superconductor into a normal conductor, and they are used to move the Majoranas in space-time. With a perpendicular magnetic field, the normal region localizes a quantum of magnetic flux. Under these conditions, the boundary between the normal region and the superconducting region supports a single zero-energy Majorana bound state. The localized zero mode is sufficiently separate from other states and can be dragged by sequentially applying voltages to the adjacent gates to implement quantum computation. We briefly describe the fabrication process to construct the device and determine key properties from experimentally determined parameters. The digital qualities of topological protection provide intrinsic immunity to the inevitable fabrication nonuniformities.

cond-mat.mes-hall↗

arXiv2019

Strong equilibration of Landau levels edge-states at the graphene edge

We present the results of an experimental study of the interaction of quantized Landau level (LL) edge-states at the physical edge of graphene by using a graphene pn junction device with a ring-shaped geometry for the channel. The unique device geometry allows the interactions between edge-states to be probed at both electrostatic edges defined by pn junctions and at the graphene physical edge. Measurements show that while the lowest LL edge-state is decoupled from the other LLs along the electrostatic junction, all the edge-states strongly equilibrate at the graphene physical edge despite the relatively short distance that they travel along the edge in our device. These findings are fundamental for the engineering of future high-performance graphene field-effect transistors based upon electron optics.

cond-mat.mes-hall↗

arXiv2019

Direct Measurement of the Electron Beam Intensity Profile via Carbon Nanotube Tomography

Electron microscopes have been improved to achieve ever smaller beam spots, a key parameter that determines the instrument's resolution. The techniques to measure the size of the beam, however, have not progressed to the same degree. There is an on-going need to develop detection technologies that can potentially characterize the smallest electron beam to further improve the capabilities of these instruments. We report on a new electron beam detector based on a single-walled carbon nanotube. Nanotubes are atomically smooth, have a well-defined diameter that is similar in size to the finest electron probes and can be used to directly measure the beam profile. By scanning the beam at different angles to the nanotube, we can accurately determine the spatial profile of an electron beam by applying tomographic reconstruction techniques.

physics.app-ph↗

arXiv2018

Super-ideal diodes at the Schottky-Mott limit in gated graphene-WSe$_2$ heterojunctions

Metal-semiconductor interfaces, known as Schottky junctions, have long been hindered by defects and impurities. Such imperfections dominate the electrical characteristics of the junction by pinning the metal Fermi energy. We report measurements on a boron nitride encapsulated graphene-tungsten diselenide (WSe$_2$) Schottky junction which exhibits ideal diode characteristics and a complete lack of Fermi-level pinning. The Schottky barrier height of the device is rigidly tuned by electrostatic gating of the WSe$_2$, enabling experimental verification of the Schottky-Mott limit in a single device. Utilizing this exceptional gate control, we realize a super-ideal gated-Schottky diode which surpasses the ideal diode limit. Our results provide a pathway for defect-free electrical contact to two-dimensional semiconductors and open up possibilities for circuits with efficient switching characteristics and higher efficiency optoelectronic devices.

cond-mat.mes-hall↗

arXiv2018

Atomic scale characterization of graphene p-n junctions for electron-optical applications

Graphene p-n junctions offer a potentially powerful approach towards controlling electron trajectories via collimation and focusing in ballistic solid-state devices. The ability of p-n junctions to control electron trajectories depends crucially on the doping profile and roughness of the junction. Here, we use four-probe scanning tunneling microscopy and spectroscopy (STM/STS) to characterize two state-of-the-art graphene p-n junction geometries at the atomic scale, one with CMOS polySi gates and another with naturally cleaved graphite gates. Using spectroscopic imaging, we characterize the local doping profile across and along the p-n junctions. We find that realistic junctions exhibit non-ideality both in their geometry as well as in the doping profile across the junction. We show that the geometry of the junction can be improved by using the cleaved edge of van der Waals metals such as graphite to define the junction. We quantify the geometric roughness and doping profiles of junctions experimentally and use these parameters in Nonequilibrium Green's Function based simulations of focusing and collimation in these realistic junctions. We find that for realizing Veselago focusing, it is crucial to minimize lateral interface roughness which only natural graphite gates achieve, and to reduce junction width, in which both devices under investigation underperform. We also find that carrier collimation is currently limited by the non-linearity of the doping profile across the junction. Our work provides benchmarks of the current graphene p-n junction quality and provides guidance for future improvements.

cond-mat.mes-hall↗

arXiv2018

Two-Parameter Quasi-Ballistic Transport Model for Nanoscale Transistors

We show that by adding only two fitting parameters to a purely ballistic transport model, we can accurately characterize the current-voltage characteristics of nanoscale MOSFETs. The model is an extension to a ballistic model (J. Appl. Phys. 76, 4879 (1994)) and includes transmission probability and the drain-channel coupling capacitor. The latter parameter gives rise to a theoretical RON that is significantly larger than those predicted previously. To validate our model, we fabricated n-channel MOSFETs with varying channel lengths. We show the length dependence of these parameters to support a quasi-ballistic description of our devices.

cond-mat.mes-hall↗

arXiv2017

Tunneling Spectroscopy of Quantum Hall States in Bilayer Graphene PN Networks

Two dimensional electronic systems under strong magnetic field form quantum Hall (QH) edge states, which propagate along the boundary of a sample with a dissipationless current. Engineering the pathway of these propagating one-dimensional chiral modes enables the investigation of quantum tunneling between adjacent QH states. Here, we report tunneling transport in spatially controlled networks of QH edge states in bilayer graphene. We observe resonant tunneling between co-propagating QH edges across barriers formed by electrically defining incompressible strips. Employing spectroscopic tunneling measurements enable the direct probing of the spatial profile, density of states, and compressibility of the QH edge states with an unprecedented energy resolution. The capability to engineer the QH edge network provides an opportunity to build future quantum electronic devices supported by rich underline physics.

cond-mat.mes-hall↗

arXiv2016

Understanding magnetic focusing in graphene $p$-$n$ junctions through quantum modeling

We present a quantum model which provides enhanced understanding of recent transverse magnetic focusing experiments on graphene $p$-$n$ junctions. Spatially resolved flow maps of local particle current density show quantum interference and $p$-$n$ junction filtering effects which are crucial to explaining the device operation. The Landauer-Büttiker formula is used alongside dephasing edge contacts to give exceptional agreement between simulated non-local resistance and the recent experiment by Chen $\textit{et al}$ ($\textit{Science}$, 2016). The origin of positive and negative focusing resonances and off resonance characteristics are explained in terms of quantum transmission functions. Our model also captures subtle features from experiment, such as the previously unexplained $p$-$p^-$ to $p$-$p^+$ transition and the second $p$-$n$ focusing resonance.

cond-mat.mes-hall↗

arXiv2016

Theory of Landau level mixing in heavily graded graphene p-n junctions

We demonstrate the use of a quantum transport model to study heavily graded graphene p-n junctions in the quantum Hall regime. A combination of p-n interface roughness and delta function disorder potential allows us to compare experimental results on different devices from the literature. We find that wide p-n junctions suppress mixing of $n \neq 0$ Landau levels. Our simulations spatially resolve carrier transport in the device, for the first time, revealing separation of higher order Landau levels in strongly graded junctions, which suppresses mixing.

cond-mat.mes-hall↗

arXiv2016

Reverse degradation of nickel graphene junction by hydrogen annealing

Metal contacts are fundamental building components for graphene based electronic devices and their properties are greatly influenced by interface quality during device fabrication, leading to resistance variation. Here we show that nickel graphene junction degrades after air exposure, due to interfacial oxidation, thus creating a tunneling barrier. Most importantly, we demonstrate that hydrogen annealing at moderate temperature (300 0C) is an effective technique to reverse the degradation.

physics.chem-ph↗