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Jian Zi

Publications and source records attributed to Jian Zi.

At least 37 records · Page 2Linked to original sources

Observation of optical states below light cone with compound lattices

For optical systems, states inside the light cone could be detected by far-field measurement, while those below the light cone are not detectable by far-field measurement. A new method for far-field detection has been developed for observing states below the light cone with compound lattices. The basic mechanism involved is that periodic weak scattering leads to band folding, making the states out of the light cone to occur inside. By using polarization-resolved momentum-space imaging spectroscopy the band structures and iso-frequency contours of plasmonic lattices with different dimensions and symmetries are experimentally mapped out, in good agreement with the simulation.

physics.optics↗

Scattering of electromagnetic waves from a cone with conformal mapping: application to scanning near-field optical microscope

We study the response of a conical metallic surface to an external electromagnetic (EM) field by representing the fields in basis functions containing integrable singularities at the tip of the cone. A fast analytical solution is obtained by the conformal mapping between the cone and a round disk. We apply our calculation to the scattering- based scanning near-field optical microscope (s-SNOM) and successfully quantify the elastic light scattering from a vibrating metallic tip over a uniform sample. We find that the field-induced charge distribution consists of localized terms at the tip and the base and an extended bulk term along the body of the cone far away from the tip. In recent s-SNOM experiments at the visible-IR range (600nm - 1$μm$) the fundamental is found to be much larger than the higher harmonics whereas at THz range ($100 μm-3mm$) the fundamental becomes comparable to the higher harmonics. We find that the localized tip charge dominates the contribution to the higher harmonics and becomes bigger for the THz experiments, thus providing an intuitive understanding of the origin of the near-field signals. We demonstrate the application of our method by extracting a two-dimensional effective dielectric constant map from the s-SNOM image of a finite metallic disk, where the variation comes from the charge density induced by the EM field.

cond-mat.mes-hall↗

Observing half and integer polarization vortices at band degeneracies

Far-field polarization vortices were recently found on singlet bands in the momentum-space of two-dimensional photonic lattices, also known as the dark states and bound states in continuum. Here, we theoretically proposed and experimentally verified the existence of the polarization vortices at the degenerate points of photonic dispersions, whose vortex cores can be radiative bright states. Half-charged vortices were generated from the Dirac points of π Berry phase and integer-charged vortices were generated from a quadratic degeneracy. Using a home-made polarization-resolved momentum-space imaging spectroscopy, we observed the complete evolution of the splitting from one quadratic point to a pair of Dirac cones by tracking the winding of the polarization vectors and the full spectrum of iso-frequency contours.

physics.optics↗

Gate tunable third-order nonlinear optical response of massless Dirac fermions in graphene

Materials with massless Dirac fermions can possess exceptionally strong and widely tunable optical nonlinearities. Experiments on graphene monolayer have indeed found very large third-order nonlinear responses, but the reported variation of the nonlinear optical coefficient by orders of magnitude is not yet understood. A large part of the difficulty is the lack of information on how doping or chemical potential affects the different nonlinear optical processes. Here we report the first experimental study, in corroboration with theory, on third harmonic generation (THG) and four-wave mixing (FWM) in graphene that has its chemical potential tuned by ion-gel gating. THG was seen to have enhanced by ~30 times when pristine graphene was heavily doped, while difference-frequency FWM appeared just the opposite. The latter was found to have a strong divergence toward degenerate FWM in undoped graphene, leading to a giant third-order nonlinearity. These truly amazing characteristics of graphene come from the possibility to gate-control the chemical potential, which selectively switches on and off one- and multi-photon resonant transitions that coherently contribute to the optical nonlinearity, and therefore can be utilized to develop graphene-based nonlinear optoelectronic devices.

cond-mat.mes-hall↗

Observation of optical vortices in momentum space

Vortex, the winding of a vector field in two dimensions, has its core the field singularity and its topological charge defined by the quantized winding angle of the vector field. Vortices are one of the most fundamental topological excitations in nature, widely known in hair whorls as the winding of hair strings, in fluid dynamics as the winding of velocities, in angular-momentum beams as the winding of phase angle and in superconductors and superfluids as the winding of order parameters. Nevertheless, vortices have hardly been observed other than those in the real space. Although band degeneracies, such as Dirac cones, can be viewed as momentum-space vortices in their mathematical structures, there lacks a well-defined physical observable whose winding number is an arbitrary signed integer. Here, we experimentally observed momentum-space vortices as the winding of far-field polarization vectors in the Brillouin zone (BZ) of periodic plasmonic structures. Using a home-made polarization-resolved momentum-space imaging spectroscopy, we completely map out the dispersion, lifetime and polarization of all radiative states at the visible wavelengths. The momentum space vortices were experimentally identified by their winding patterns in the polarization-resolved iso-frequency contours and their diverging radiative quality factors. Such polarization vortices can exist robustly on any periodic systems of vectorial fields, while they are not captured by the existing topological band theory developed for scaler fields. This work opens up a promising avenue for exploring topological photonics in the momentum space, studying bound states in continuum (BICs), as well as for rendering and steering vector beams and designing high-Q plasmonic resonances.

physics.optics↗

Electromagnetic Scattering Laws in Weyl Systems

Wavelength determines the length scale of the cross section when electromagnetic waves are scattered by an electrically small object. The cross section diverges for resonant scattering, and diminishes for non-resonant scattering, when wavelength approaches infinity. This scattering law explains the color of the sky as well as the strength of a mobile phone signal. We show that such wavelength scaling comes from free space's conical dispersion at zero frequency. Emerging Weyl systems, offering similar dispersion at non-zero frequencies, lead to new laws of electromagnetic scattering that allow cross sections to be decoupled from the wavelength limit. Diverging and diminishing cross sections can be realized at any target wavelength in a Weyl system, providing unprecedented ability to tailor the strength of wave-matter interactions for radio-frequency and optical applications.

physics.optics↗

Topological phase transition and interface states in hybrid plasmonic-photonic systems

The geometric phase and topological property for one-dimensional hybrid plasmonic-photonic crystals consisting of a simple lattice of graphene sheets are investigated systematically. For transverse magnetic waves, both plasmonic and photonic modes exist in the momentum space. The accidental degeneracy point of these two kinds of modes is identified to be a diabolic point accompanied with a topological phase transition. For a closed loop around this degeneracy point, the Berry phase is Pi as a consequence of the discontinuous jump of the geometric Zak phase. The wave impedance is calculated analytically for the semi-infinite system, and the corresponding topological interface states either start from or terminate at the degeneracy point. This type of localized interface states may find potential applications in photonics and plasmonics.

physics.optics↗

Enhanced absorption in heterostructures with graphene and truncated photonic crystals

We theoretically and experimentally investigate the optical absorption properties of heterostructures composed of graphene films and truncated photonic crystals (PCs) in the visible range. The experimental results show that the absorption of the heterostructure is enhanced greatly in the whole forbidden gap of PCs compared with that of graphene alone. The absorption is enhanced over a wide angle of incidence for both transverse electric (TE) and transverse magnetic (TM) polarizations. The enhanced absorption band broadens for TE polarization but narrows for TM polarization as the incident angle increases. In the forbidden gap of the PCs, the maximum absorptance of the heterostructures is nearly four times of that of bare graphene films for arbitrary incident angles and polarizations. The optical experiments are in excellent agreement with the theoretical results.

physics.optics↗

Electromagnetic Scattering by Spheres of Topological Insulators

The electromagnetic scattering properties of topological insulator (TI) spheres are systematically studied in this paper. Unconventional backward scattering caused by the topological magneto-electric (TME) effect of TIs are found in both Rayleigh and Mie scattering regimes. This enhanced backward scattering can be achieved by introducing an impedance-matched background which can suppress the bulk scattering. For the cross-polarized scattering coefficients, interesting antiresonances are found in the Mie scattering regime, wherein the cross-polarized electromagnetic fields induced by the TME effect are trapped inside TI spheres. In the Rayleigh limit, the quantized TME effect of TIs can be determined by measuring the electric-field components of scattered waves in the far field.

physics.optics↗

Electron Temperature Dependence of the Optical Properties of Small Sodium Nanoparticles

We report a novel behavior of the surface plasmon linewidth in sodium nanospheres Na$_{1760}$ changing with the electron temperature, which monotonically decreases and bears a discontinuous sudden drop at high electron temperatures. Our calculation is based on the model constructed by splitting the total Hamiltonian of all valence electrons of a metallic nanoparticle into two sub-Hamiltonians and their coupling, and obtained results can be verified by the pump-probe femtosecond spectroscopy experiments. In addition, we propose that it is the size uncertainty of small nanoparticles that yields the intrinsic linewidth of the surface plasmon resonance, which is supported by the available data of clusters Na$_{8}$ and Na$_{20}$.

cond-mat.mes-hall↗

Determination of the quantized topological magneto-electric effect in topological insulators from Rayleigh scattering

Topological insulators (TIs) exhibit many exotic properties. In particular, a topological magneto-electric (TME) effect, quantized in units of the fine structure constant, exists in TIs. In this Letter, we study theoretically the scattering properties of electromagnetic waves by TI circular cylinders particularly in the Rayleigh scattering limit. Compared with ordinary dielectric cylinders, the scattering by TI cylinders shows many unusual features due to the TME effect. Two proposals are suggested to determine the TME effect of TIs simply based on measuring the electric-field components of scattered waves in the far field at one or two scattering angles. Our results could also offer a way to measure the fine structure constant.

cond-mat.mtrl-sci↗

Plasmon-phonon coupling in large-area graphene dot and antidot arrays

Nanostructured graphene on SiO2 substrates pave the way for enhanced light-matter interactions and explorations of strong plasmon-phonon hybridization in the mid-infrared regime. Unprecedented large-area graphene nanodot and antidot optical arrays are fabricated by nanosphere lithography, with structural control down to the sub-100 nanometer regime. The interaction between graphene plasmon modes and the substrate phonons is experimentally demonstrated and structural control is used to map out the hybridization of plasmons and phonons, showing coupling energies of the order 20 meV. Our findings are further supported by theoretical calculations and numerical simulations.

cond-mat.mes-hall↗

Enhanced light-matter interaction in graphene-covered gold nanovoid arrays

The combination of graphene with noble-metal nanostructures is currently being explored for strong light-graphene interaction enhanced by plasmons. We introduce a novel hybrid graphene-metal system for studying light-matter interactions with gold-void nanostructures exhibiting resonances in the visible range. Strong coupling of graphene layers to the plasmon modes of the nanovoid arrays results in significant frequency shifts of the underlying plasmon resonances, enabling more than 30% absolute light absorption in a single layer of graphene and up to 700-fold enhancement of the Raman response of the graphene. These new perspectives enable us to verify the presence of graphene on gold-void arrays and the enhancement even allows us to accurately quantify the number of layers. Experimental observations are further supported by numerical simulations and perturbation-theory analysis. The graphene gold-void platform is beneficial for sensing of molecules and placing R6G dye molecules on top of the graphene, we observe a strong enhancement of the R6G Raman fingerprints. These results pave the way toward advanced substrates for surface-enhanced Raman scattering (SERS) with potential for unambiguous single-molecule detection on the atomically well-defined layer of graphene.

cond-mat.mes-hall↗

Wideband trapping of light by edge states in honeycomb photonic crystals

We study theoretically light propagations at the zigzag edge of a honeycomb photonic crystal consisting of dielectric rods in air, analogous to graphene. Within the photonic band gap of the honeycomb photonic crystal, a unimodal edge state may exist with a sharp confinement of optical fields. Its dispersion can be tuned simply by adjusting the radius of the edge rods. For the edge rods with a graded variation in radius along the edge direction, we show numerically that light beams of different frequencies can be trapped sharply in different spatial locations, rendering wideband trapping of light.

cond-mat.mes-hall↗

Transfer matrix method for optics in graphene layers

A transfer matrix method is developed for optical calculations of non-interacting graphene layers. Within the framework of this method, optical properties such as reflection, transmission and absorption for single-, double- and multi-layer graphene are studied. We also apply the method to structures consisting of periodically arranged graphene layers, revealing well-defined photonic band structures and even photonic bandgaps. Finally, we discuss graphene plasmons and introduce a simple way to tune the plasmon dispersion.

cond-mat.mes-hall↗

All-angle zero reflection at metamaterial surfaces

The authors study theoretically reflection on the surface of a metamaterial with a hyperbolic dispersion. It is found that reflection is strongly dependent on how the surface is terminated with respect to the asymptote of the hyperbolic dispersion. For a surface terminated normally to the asymptote, zero reflection occurs for all incident angles. It is exemplified by a metamaterial made of a periodic metal-dielectric layered structure with its surface properly cut through numerical simulations.

physics.optics↗

Dirac Spectra and Edge States in Honeycomb Plasmonic Lattices

We study theoretically the dispersion of plasmonic honeycomb lattices and find Dirac spectra for both dipole and quadrupole modes. Zigzag edge states derived from Dirac points are found in ribbons of these honeycomb plasmonic lattices. The zigzag edge states for out-of-plane dipole modes are closely analogous to the electronic ones in graphene nanoribbons. The edge states for in-plane dipole modes and quadrupole modes, however, have rather unique characters due to the vector nature of the plasmonic excitations. The conditions for the existence of plasmonic edge states are derived analytically.

cond-mat.mtrl-sci↗

Extrinsic photonic crystals

Doped semiconductors are intrinsically homogeneous media. However, by applying an external magnetic field that has a spatially periodic variation, doped semiconductors can behave extrinsically like conventional photonic crystals. We show this possibility theoretically by calculating the photonic band structures of a doped semiconductor under an external, spatially periodic magnetic field. Homogeneous media, behaving like conventional photonic crystals under some external, spatially periodic fields, define a new kind of photonic crystals: extrinsic photonic crystals. The proposed extrinsic photonic crystals could not only extend the concept of photonic crystals but also lead to the control of the dispersion and propagation of electromagnetic waves in a unique way: simply manipulating the externally applied fields.

cond-mat.mtrl-sci↗