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Jianan Fang

Publications and source records attributed to Jianan Fang.

At least 19 recordsLinked to original sources

Single-photon time-stretch computational ghost spectroscopy

Time-stretch spectroscopy is powerful for capturing transient spectral phenomena but remains fundamentally limited by detector bandwidth or timing jitter, especially under photon-starved conditions. Here, we devise and implement single-photon time-stretch computational ghost spectroscopy, which integrates dispersive wavelength-to-time mapping with programmable temporal encoding and correlation-based reconstruction to overcome these detection limitations. Specifically, temporally stretched ultrashort pulses are modulated by predefined encoding patterns and detected by a low-bandwidth detector, allowing reconstruction of near-infrared spectra with 450 resolvable channels across 1530-1590 nm without direct high-speed waveform acquisition. By further incorporating compressive sensing, accurate spectral recovery is achieved at sub-Nyquist sampling rates, substantially reducing acquisition requirements to facilitate high-speed operation at 210 kHz. In the single-photon regime, computational ghost reconstruction effectively suppresses the intrinsic detector timing jitter, yielding high-fidelity spectra at illumination fluxes down to 0.01 photons/pulse. By jointly enabling broadband coverage, high spectral resolution, high acquisition speed, and single-photon sensitivity, this approach establishes a computation-enhanced paradigm for time-stretch spectroscopy and provides a versatile platform for ultrafast and photon-efficient spectroscopic applications.

physics.optics

Mid-infrared snapshot spectral imaging via nonlinear radial dispersion

Mid-infrared (MIR) spectral imaging provides chemically specific contrast through molecular vibrational fingerprints, yet snapshot acquisition remains severely limited by the lack of high-sensitivity detectors and efficient spectral encoding mechanisms. Here we introduce snapshot MIR spectral imaging based on intrinsic nonlinear radial dispersion, in which wavelength-dependent phase matching simultaneously enables frequency upconversion and spectral multiplexing. Different spectral components are mapped to distinct output angles within a 4$f$ imaging architecture, enabling single-shot spectral encoding without external dispersive elements. In combination with speckle illumination encoding, spectral information is compressed and recovered without additional coding components. Leveraging nonlinear upconversion to the visible, the approach achieves room-temperature MIR spectral imaging with sensitivity approaching 1 photon/pixel/pulse across a broad spectral range from 2.5 to 4.0 $μ$m. This work transforms spectral encoding from an external optical function into an inherent property of the nonlinear imaging process, providing a general route to high-sensitivity snapshot MIR spectral imaging.

physics.optics

Highly efficient difference-frequency generation for mid-infrared pulses by passively synchronous seeding

We have proposed and experimentally demonstrated a novel scheme for efficient mid-infrared difference-frequency generation based on passively synchronized fiber lasers. The adoption of coincident seeding pulses in the nonlinear conversion process could substantially lower the pumping threshold for mid-infrared parametric emission. Consequently, a picosecond mid-infrared source at 3.1 $μ$m was prepared with watt-level average power, and a maximum power conversion efficiency of 77\% was realized from pump to down-converted light. Additionally, the long-term stability of generated power was manifested with a relative fluctuation as low as 0.17\% over one hour. Thanks to the all-optical passive synchronization and all-polarization-maintaining fiber architecture, the implemented laser system was also featured with simplicity, compactness and robustness, which would favor subsequent applications beyond laboratory operation.

physics.optics

Mid-infrared photon counting and resolving via efficient frequency upconversion

Optical detectors with single-photon sensitivity and large dynamic range would facilitate a variety of applications. Especially, the capability of extending operation wavelengths into the mid-infrared region is highly attractive. Here we implement a mid-infrared frequency upconversion detector for counting and resolving photons at 3 $μ$m. Thanks to the spectro-temporal engineering of the involved optical fields, the mid-infrared photons could be spectrally translated into the visible band with a conversion efficiency of 80\%. In combination with a silicon avalanche photodiode, we obtained unprecedented performances with a high overall detection efficiency of 37\% and a low noise equivalent power of 1.8$\times$10$^{-17}$ W/Hz$^{1/2}$. Furthermore, photon-number-resolving detection at mid-infrared wavelengths was demonstrated, for the first time to our knowledge, with a multi-pixel photon counter. The implemented upconversion detector exhibited a maximal resolving photon number up to 9 with a noise probability per pulse of 0.14\% at the peak detection efficiency. The achieved photon counting and resolving performance might open up new possibilities in trace molecule spectroscopy, sensitive biochemical sensing, and free-space communications, among others.

physics.optics

Wide-field mid-infrared single-photon upconversion imaging

Frequency upconversion technique, where the infrared signal is nonlinearly translated into the visible band to leverage the silicon sensors, offers a promising alternation for the mid-infrared (MIR) imaging. However, the intrinsic field of view (FOV) is typically limited by the phase-matching condition, thus imposing a remaining challenge to promote subsequent applications. Here, we demonstrate a wide-field upconversion imaging based on the aperiodic quasi-phase-matching configuration. The acceptance angle is significantly expanded to about 30$^\circ$, over tenfold larger than that with the periodical poling crystal. The extended FOV is realized in one shot without the need of parameter scanning or post-processing. Consequently, a fast snapshot allows to facilitate high-speed imaging at a frame rate up to 216 kHz. Alternatively, single-photon imaging at room temperature is permitted due to the substantially suppressed background noise by the spectro-temporal filtering. Furthermore, we have implemented high-resolution time-of-flight 3D imaging based on the picosecond optical gating. These presented MIR imaging features with wide field, fast speed, and high sensitivity might stimulate immediate applications, such as non-destructive defect inspection, in-vivo biomedical examination, and high-speed volumetric tomography.

physics.optics

Highly sensitive detection for infrared photons by non-degenerate two-photon absorption under mid-infrared pumping

We have demonstrated highly-sensitive photon counting in the infrared based on the two-photon absorption (2PA) in a silicon avalanche photodiode, where the required photon energy for inducing effective conductivity was provided by an intense mid-infrared (MIR) field at 3 $μ$m. The used MIR pumping scheme could not only benefit from the enhanced 2PA coefficient in the non-degenerate regime, but also eliminate the detrimental background noises due to the pump harmonic excitation of the pump. Consequently, the enhancement factor for the signal counting rate unprecedented reached to about $10^{5}$ with input infrared pulses at the femtojoule level. Additionally, the noise equivalent power was substantially improved by two orders of magnitude comparing to conventional schemes with near-infrared pumping. Therefore, the presented configuration might provide an alternative to realize sensitive infrared detection and imaging with desirable features of room-temperature operation, no phase-matching requirement, and broadband responding window, which would find a variety of applications including remote ranging, sensitive sensing, biochemical imaging, and trace spectroscopy.

physics.optics

Passive repetition-rate stabilization for a mode-locked fiber laser by electro-optic modulation

We report a passive stabilization of the repetition rate for a mode-locked fiber laser by using an electro-optic modulator in a phase-biased nonlinear amplifying loop mirror. The underlying mechanism, in contrast to active feedback operations, lies in the cross-phase modulation between electrical and optical pulses within an electro-optic crystal. The resulting spectral shift can automatically compensate the cavity-length drift via the group velocity dispersion. Consequently, the artificial actuator enables to obtain a capture range up to 2.3 mm, much longer than that achieved by index changes of the modulator. A robust and tight locking for the repetition rate is then realized with a standard deviation as low as 9 $μ$Hz with a 1-s sample time over 11 hours, corresponding to a fractional instability of 4.3$\times$10$^{-13}$. Furthermore, a dynamic optical sampling by repetition-rate tuning has been manifested with a fast refresh rate at 100 kHz and a broad scanning range over 305 ps. The demonstrated passive servo action may provide a simple yet effective way to stabilize the repetition rate with high precision, large bandwidth and wide tunability.

physics.optics

Mid-Infrared Single-Photon Edge Enhanced Imaging based on Nonlinear Vortex Filtering

Edge enhanced imaging via the spiral phase contrast enables to reveal the phase or amplitude gradients of a target, which has been proved useful in feature recognition, machine vision, and object identification. A long quest is to extend the operation wavelength into the mid-infrared (MIR) region, as highly demanded in various fields including infrared sensing, astronomic observation, and biomedical diagnosis. Here, we demonstrated ultra-sensitive MIR imaging at the single-photon level based on nonlinear frequency upconversion, where the spectrally converted replica of the MIR object image at 3070 nm was captured by a silicon electron multiplying charged coupled device. The imaging sensitivity was significantly improved by the coincidence pulsed pumping with a spectro-temporal optimization. Furthermore, the edge enhancement has been realized by imprinting the spiral phase pattern of the pump onto the upconverted field at the Fourier plane within the nonlinear crystal. Such a nonlinear spatial filter not only provided an effective way to implement the required high-fidelity vortex screening in the edge enhanced detection, but also rendered the MIR illumination into a visible image in an efficient and low-noise fashion. The presented system for MIR edge enhanced imaging might facilitate immediate applications in label-free histopathological diagnosis and non-destructive defect inspection.

physics.optics

Single-Photon Infrared Imaging with a Silicon Camera Based on Long-Wavelength-Pumping Two-Photon Absorption

We experimentally demonstrated an ultra-sensitive imaging system for telecom photons based on the non-degenerate two-photon absorption in a silicon-based electron multiplying charge-coupled device (EMCCD). The proposed long-wavelength-pumping scheme with mid-infrared pulsed excitation could not only effectively increase the two-photon absorption coefficient, but also significantly suppress the background noise caused by the harmonic absorption of the strong pumping field. In comparison to the photoelectric response via the degenerate two-photon absorption, the implemented configuration could offer over 30-folded enhancement of the photon-counting rate in the infrared imaging. The resulting detection sensitivity up to 1 photon/pixel/pulse was unprecedentedly approached, thus facilitating the single-photon operation. The elimination of the stringent phase matching as typically required in the optical parametric conversion has led to a high spatial resolution of 13 $μ$m. Moreover, the on-chip nonlinearity of the optical imager would enable a broadband spectral window and an enlarged field of view. In combination with the 5-ps temporal resolution due to the coincident optical gating, the presented imaging system would find various promising applications, such as low-light fluorescence lifetime microscopy and photon counting time-of-flight 3D imaging.

physics.optics

High-precision passive stabilization of repetition rate for a mode-locked fiber laser based on optical pulse injection

We have proposed and implemented a novel scheme to obtain high-precision repetition rate stabilization for a polarization-maintaining mode-locked fiber laser. The essential technique lies in the periodic injection of electronically modulated optical pulses into a nonlinear amplifying loop mirror within the laser resonator. Thanks to the nonlinear cross-phase modulation effect, the injected pulses referenced to an external clock serves as a stable and precise timing trigger for an effective intensity modulator. Consequently, synchronous mode-locking can be initiated to output ultrafast pulses with a passively stabilized repetition rate. The capture range of the locking system reaches to a record of 1 mm, which enables a long-term stable operation over 15 hours without the need of temperature stabilization and vibration isolation. Meanwhile, the achieved standard deviation is as low as 100 $μ$Hz with a 1-s sample time, corresponding to a fluctuation instability of 5.0$\times10^{-12}$. Additionally, the repetition rate stabilization performance based on the passive synchronization has been systematically investigated by varying the average power, central wavelength and pulse duration of the optical injection.

physics.optics

High-speed mid-infrared single-photon upconversion spectrometer

Sensitive and fast mid-infrared (MIR) spectroscopy is highly attractive in a variety of applications including astronomical observation, pharmaceutical synthesis, and environmental monitoring. However, the performance of conventional MIR spectrometers has long been hindered by the limited sensitivity of narrow-bandgap detectors and/or the deficient brightness of broadband light sources. Here, we devise and implement an ultra-sensitive and broadband MIR upconversion spectrometer, which integrates a supercontinuum source covering 1.5-4.2 $μ$m based on a silicon nitride nanophotonic waveguide. High-efficiency and low-noise nonlinear frequency upconversion is realized based on coincidence pulsed pumping with spectro-temporal optimization, which enables to leverage silicon detectors for facilitating MIR single-photon spectroscopy at 0.2 photons/nm/pulse. Furthermore, the upconversion-based array spectrometer is manifested with high-speed spectral acquisition rates beyond 200 kHz, which is about ten-fold faster than the state-of-the-art scan rates for FTIR-based spectrometers at a comparable spectral resolution. The achieved features of broadband spectral coverage, single-photon sensitivity, and sub-MHz refreshing rate might open up new possibilities in infrared transient spectral measurements in combustion analysis, high-throughput sorting and reaction tracking, among others.

physics.optics

Mid-infrared single-photon 3D imaging

Active mid-infrared (MIR) imagers capable of retrieving three-dimensional (3D) structure and reflectivity information are highly attractive in a wide range of biomedical and industrial applications. However, the infrared 3D imaging at low-light levels is still challenging due to the deficiency of sensitive and fast MIR sensors. Here we propose and implement a MIR time-of-flight imaging system that operates at single-photon sensitivity and femtosecond timing resolution. Specifically, back-scattered infrared photons from a scene are optically gated by delay-controlled ultrashort pump pulses through nonlinear frequency upconversion. The upconverted images with time stamps are then recorded by a silicon camera to facilitate the 3D reconstruction with high lateral and depth resolutions. Moreover, an effective numerical denoiser based on spatiotemporal correlation allows us to reveal the object profile and reflectivity under photon-starving conditions with a detected flux below 0.05 photons/pixel/second. The presented MIR 3D imager features with high detection sensitivity, precise timing resolution, and wide-field operation, which may open new possibilities in life and material sciences.

physics.optics

Mid-infrared single-pixel imaging at the single-photon level

Single-pixel cameras have recently emerged as promising alternatives to multi-pixel sensors due to reduced costs and superior durability, which are particularly attractive for mid-infrared (MIR) imaging pertinent to applications including industry inspection and biomedical diagnosis. To date, MIR single-pixel photon-sparse imaging has yet been realized, which urgently calls for high-sensitivity optical detectors and high-fidelity spatial modulators. Here, we demonstrate a MIR single-photon computational imaging with a single-element silicon detector. The underlying methodology relies on nonlinear structured detection, where the encoded time-varying pump patterns are optically imprinted onto the MIR object image through sum-frequency generation. Simultaneously, the MIR radiation is spectrally translated into the visible region, thus permitting infrared single-photon upconversion detection. Then, the use of advanced algorithms of compress sensing and deep learning allows us to reconstruct MIR images under sub-Nyquist sampling and photon-starving illumination. The presented paradigm of single-pixel upconversion imaging is featured with single-pixel simplicity, single-photon sensitivity, and room-temperature operation, which would establish a new path for sensitive imaging at longer infrared wavelengths or terahertz frequencies, where high-sensitivity photon counters and high-fidelity spatial modulators are typically hard to access.

physics.optics

Single-photon time-stretch infrared spectroscopy

Sensitive mid-infrared (MIR) spectroscopy is highly demanded in various fields ranging from industrial inspection, biomedical diagnosis to astronomical observation. However, the detection sensitivity of conventional MIR spectrometers has been severely limited by excessive noises for existing infrared sensors, which hinders widespread use in photon-scarce scenarios. Here, we devise and implement a broadband MIR single-photon time-stretch spectrometer based on high-fidelity spectral upconversion and time-correlated coincidence counting. Specifically, a nanophotonic supercontinuum illumination covering 2.4-4.2 $μ$m is nonlinearly converted to the near-infrared band, where low-loss single-mode fiber and high-performance silicon detector can be leveraged to facilitate dispersive operation and sensitive detection, respectively. The arrival time for the dispersed upconversion photons is precisely registered with a low-timing-jitter photon counter, which enables us to obtain a high spectral resolution about 0.5 cm$^{-1}$ under a low-light-level illumination down to 0.14 photons/nm/pulse. In comparison to previous MIR upconversion spectrometers, the presented time-stretch architecture favors single-pixel simplicity and high-throughput acquisition for the single-photon spectral measurement. The achieved MIR spectroscopic features of broadband spectral coverage, sub-wavenumber resolution, single-photon sensitivity, and room-temperature operation would stimulate immediate applications in material and life sciences.

physics.optics

Wide-field mid-infrared hyperspectral imaging beyond video rate

Mid-infrared hyperspectral imaging has become an indispensable tool to spatially resolve chemical information in a wide variety of samples. However, acquiring three-dimensional data cubes is typically time-consuming due to the limited speed of raster scanning or wavelength tuning, which impedes real-time visualization with high spatial definition across broad spectral bands. Here, we devise and implement a high-speed, wide-field mid-infrared hyperspectral imaging system relying on broadband parametric upconversion of high-brightness supercontinuum illumination at the Fourier plane. The upconverted replica is spectrally decomposed by a rapid acousto-optic tunable filter, which records high-definition monochromatic images at a frame rate of 10 kHz based on a megapixel silicon camera. Consequently, the hyperspectral imager allows us to acquire 100 spectral bands over 2600-4085 cm$^{-1}$ in 10 ms, corresponding to a refreshing rate of 100 Hz. Moreover, the angular dependence of phase matching in the image upconversion is leveraged to realize snapshot operation with spatial multiplexing for multiple spectral channels, which may further boost the spectral imaging rate. The high acquisition rate, wide-field operation, and broadband spectral coverage could open new possibilities for high-throughput characterization of transient processes in material and life sciences.

physics.optics

Highly-sensitive mid-infrared upconversion detection based on external-cavity pump enhancement

Sensitive mid-infrared (MIR) detection is highly demanded in various applications, ranging from remote sensing, infrared surveillance, environmental monitoring to industrial inspection. Among others, upconversion infrared detectors have recently attracted increasing attention due to the advantageous features of high sensitivity, fast response, and room-temperature operation. However, it remains challenging to realize high-performance passive MIR sensing due to the stringent requirement of high-power continuous-wave pumping. Here, we propose and implement a high-efficiency and low-noise MIR upconversion detection system based on pumping enhancement via a low-loss optical cavity. Specifically, a single-longitudinal-mode pump at 1064 nm is significantly enhanced by a factor of 36, thus allowing for a peak conversion efficiency of up to 22\% at an intra-cavity average power of 55 W. The corresponding noise equivalent power is achieved as low as 0.3 fW/Hz$^{1/2}$, which indicates at least a ten-fold improvement over previous results. Notably, the involved single-frequency pumping would facilitate high-fidelity spectral mapping, which is particularly attractive for high-precision MIR upconversion spectroscopy in photon-starved scenarios.

physics.optics

Mid-Infrared Single-Photon Compressive Spectroscopy

Sensitive mid-infrared (MIR) spectroscopy plays an indispensable role in various photon-starved conditions. However, the detection sensitivity of conventional MIR spectrometers is severely limited by excessive noises of the involved infrared sensors, especially for multi-pixel arrays in parallel spectral acquisition. Here, we devise and implement an ultra-sensitive MIR single-pixel spectrometer, which relies on high-fidelity spectral upconversion and wavelength-encoding compressive measurement. Specifically, a MIR nanophotonic supercontinuum from 3.1 to 3.9 $μ$m is nonlinearly converted to the near-infrared band via synchronous chirped-pulse pumping, which facilitates both the precise spectral mapping and sensitive upconversion detection. The upconverted signal is then spatially dispersed onto a programmable digital micromirror device, before being registered by a single-element silicon detector. Consequently, the spectral information can be deciphered from the correlation between encoded patterns and recorded measurements, which results in a spectral resolution of 0.5 cm$^{-1}$ under an illumination flux down to 0.01 photons/nm/pulse. Moreover, we demonstrate faithful reconstructions at sub-Nyquist sampling rates by using the compressive sensing algorithm, which leads to a 95\% reduction in data acquisition time. The presented single-pixel computational spectrometer features wavelength multiplexing, high throughput, and efficient sampling, which thus paves a new way for sensitive and fast spectroscopic analysis at the single-photon level.

physics.optics

High-speed mid-infrared imaging via nonlinear multiplexed detection

High-speed mid-infrared (MIR) videography constitutes an enabling tool to monitor and analyze various dynamics in scientific research and industrial applications, such as combustion diagnostics, explosion reactions, photosynthetic tracking, and thermal surveillance. However, the frame rate of conventional MIR imagers is typically limited by readout electronics and detection sensitivity, especially for large spatial formats with massive pixels. Here, we devise and implement a high-speed MIR upconversion imaging system based on time-multiplexed nonlinear structured pumping. Specifically, the dynamic infrared scene is optically gated by a sequence of spatially periodical pump patterns in a nonlinear crystal, which facilitates both rapid temporal encryption and sensitive upconversion detection. Then, the upconverted frames are superimposed onto a silicon camera within a single exposure, thus resulting in a multiplexed snapshot in the spatial-frequency domain. Finally, the sub-exposure images, corresponding to distinct transient events, can be computationally deciphered and reconstructed by the frequency recognition algorithm based on band-pass filtering and Fourier transform operations. The achieved frame rate is tenfold boosted to 10,000 frames per second without compromising the megapixel spatial format, which allows continuous real-time MIR videography at high speed and high definition. The presented approach could be readily extended to far-infrared or terahertz spectral regions, with an aim of performing high-throughput and high-sensitivity observation of transient phenomena with high temporal complexity.

physics.optics