arXiv subjects

Jiangfeng Du

Publications and source records attributed to Jiangfeng Du.

At least 37 records · Page 2Linked to original sources

arXiv2025

Experimental observation of parity-symmetry-protected phenomena in the quantum Rabi model with a trapped ion

Symmetry is crucial for gaining insights into the fundamental properties of physical systems, bringing possibilities in studying exotic phenomena such as quantum phase transitions and ground state entanglement. Here, we experimentally simulate a highly controllable extended quantum Rabi model, capable of tuning into the ultra-strong or deep coupling regime, in a spin-motion-coupled trapped ion. We observe that the phonon driven by such a model with parity symmetry preserved (broken) would experience double (single) excitation in the ultra-strong coupling regime. Quantum phenomena such as strong ground state entanglement and quantum superposition in systems occur with parity symmetry, and these phenomena disappear following the symmetry breaking. We also find sensitive responses for the two-level system entropy and phonon Wigner function in the deep coupling regime, depending on the parameter across the symmetry transition point. This work offers the prospect of exploring symmetry-controlled quantum phenomena and their applications in high-precision quantum technologies.

quant-ph↗

arXiv2025

Single-molecule Scale Magnetic Resonance Spectroscopy using Nitrogen-Vacancy Centers in Diamond

Single-molecule technology stands as a powerful tool, enabling the characterization of intricate structural and dynamic information that would otherwise remain concealed within the averaged behaviors of numerous molecules. This technology finds extensive application across diverse fields including physics, chemistry, biology, and medicine. Quantum sensing, particularly leveraging nitrogen-vacancy (NV) centers within diamond structures, presents a promising avenue for single-molecule magnetic resonance, offering prospects for sensing and imaging technology at the single-molecule level. Notably, while significant strides have been made in single-molecule scale magnetic resonance using NV centers over the past two decades, current approaches still exhibit limitations in magnetic sensitivity, spectral resolution, and spatial resolution. Particularly, the full reconstruction of three-dimensional positions of nuclear spins within single molecules remains an unattained goal. This review provides a comprehensive overview of the current state-of-the-art in single-molecule scale magnetic resonance, encompassing an analysis of various relevant techniques involving NV centers. Additionally, it explores the optimization of technical parameters associated with these methods. This detailed analysis serves as a foundation for the development of new technologies and the exploration of potential applications.

quant-ph↗

arXiv2024

Discovery of an anomalous non-evaporating sub-nanometre water layer in open environment

Water exhibits complex behaviors as a result of hydrogen bonding, and low-dimensional confined water plays a key role in material science, geology, and biology science. Conventional techniques like STM, TEM, and AFM enable atomic-scale observations but face limitations under ambient conditions and surface topographies. NV center magnetic resonance technology provides an opportunity to overcome these limitations, offering non-contact atomic-scale measurements with chemical resolution capability. In this study, a nanoscale layer dissection method was developed utilizing NV center technology to analyze water layers with diverse physicochemical properties. It unveiled the presence of a non-evaporating sub-nanometer water layer on a diamond surface under ambient conditions. This layer demonstrated impervious to atmospheric water vapor and exhibited unique electronic transport mediated via hydrogen bonding. These findings provide new perspectives and a platform for studying the structure and behavior of low-dimensional water, as well as the surface properties influenced by adsorbed water under native conditions.

cond-mat.mtrl-sci↗

arXiv2024

Spin-wave frequency multiplication by magnetic vortex cores

Frequency multiplication involves generating harmonics from an input frequency, a technique particularly useful for integrating spin-wave devices operating at different frequencies. While topological magnetic textures offer distinct advantages in spin-wave applications, frequency multiplication has not yet been observed in these structures. Here, we study the magnetization dynamics of magnetic vortices formed in micron-sized disks and squares via wide-field magnetic imaging. We found the occurrence of coherent spin-wave harmonics arising from the gyration of vortex cores driven by microwave fields. This phenomenon reveals a universal mechanism where the periodical motion of delta function-like objects such as vortex cores gives rise to a frequency comb. Our results pave the way for creating nanoscale, tunable spin-based frequency multipliers and open new possibilities for frequency comb generation in a variety of systems.

cond-mat.mes-hall↗

arXiv2024

Programmable simulation of high-order exceptional point with a trapped ion

The nontrivial degeneracies in non-Hermitian systems, exceptional points (EPs), have attracted extensive attention due to intriguing phenomena. Compared with commonly observed second-order EPs, high-order EPs show rich physics due to their extended dimension and parameter space, ranging from the coalescence of EPs into higher order to potential applications in topological properties. However, these features also pose challenges in controlling multiple coherent and dissipative elements in a scaled system. Here we experimentally demonstrate a native programmable control to simulate a high-order non-Hermitian Hamiltonian in a multi-dimensional trapped ion system. We simulate a series of non-Hermitian systems with varied parameters and observe the coalescence of second-order EPs into a fourth-order EP. Our results pave the way for scalable quantum simulation of high-dimensional dissipative systems and can be beneficial for the application of high-order EPs in quantum sensing and quantum control.

quant-ph↗

arXiv2024

Searches for exotic spin-dependent interactions with spin sensors

Numerous theories have postulated the existence of exotic spin-dependent interactions beyond the Standard Model of particle physics. Spin-based quantum sensors, which utilize the quantum properties of spins to enhance measurement precision, emerge as powerful tools for probing these exotic interactions. These sensors encompass a wide range of technologies, such as optically pumped magnetometers, atomic comagnetometers, spin masers, nuclear magnetic resonance, spin amplifiers, and nitrogen-vacancy centers. These technologies stand out for their ultrahigh sensitivity, compact tabletop design, and cost-effectiveness, offering complementary approaches to the large-scale particle colliders and astrophysical observations. This article reviews the underlying physical principles of various spin sensors and highlights the recent theoretical and experimental progress in the searches for exotic spin-dependent interactions with these quantum sensors. Investigations covered include the exotic interactions of spins with ultralight dark matter, exotic spin-dependent forces, electric dipole moment, spin-gravity interactions, and among others. Ongoing and forthcoming experiments using advanced spin-based sensors to investigate exotic spin-dependent interactions are discussed.

quant-ph↗

arXiv2024

A Powder Diffraction-AI Solution for Crystalline Structure

Determining the atomic-level structure of crystalline solids is critically important across a wide array of scientific disciplines. The challenges associated with obtaining samples suitable for single-crystal diffraction, coupled with the limitations inherent in classical structure determination methods that primarily utilize powder diffraction for most polycrystalline materials, underscore an urgent need to develop alternative approaches for elucidating the structures of commonly encountered crystalline compounds. In this work, we present an artificial intelligence-directed leapfrog model capable of accurately determining the structures of both organic and inorganic-organic hybrid crystalline solids through direct analysis of powder X-ray diffraction data. This model not only offers a comprehensive solution that effectively circumvents issues related to insoluble challenges in conventional structure solution methodologies but also demonstrates applicability to crystal structures across all conceivable space groups. Furthermore, it exhibits notable compatibility with routine powder diffraction data typically generated by standard instruments, featuring rapid data collection and normal resolution levels.

cond-mat.mtrl-sci↗

arXiv2024

Hot electron lifetime exceeds 300 nanoseconds in quantum dots with high quantum efficiency

Hot electrons are theoretically predicted to be long-lived in strongly confined quantum dots, which could play vital roles in quantum dot-based optoelectronics; however, existing photoexcitation transient spectroscopy investigations reveal that their lifetime is less than 1 ps in well-passivated quantum dots because of the ultrafast electron-hole Auger-assisted cooling. Therefore, they are generally considered absent in quantum dot optoelectronic devices. Here, by using our newly developed electrically excited transient absorption spectroscopy, we surprisingly observed abundant hot electrons in both II-VI and III-VI compound quantum dot light-emitting diodes at elevated bias (>4 V), of which the lifetimes reach 59 to 371 ns, lengthened by more than 5 orders of magnitude compared with the photoexcited hot electrons. These results experimentally prove the presence of a strong phonon bottleneck effect, refreshing our understanding of the role of hot electrons in quantum dot optoelectronics.

cond-mat.mes-hall↗

arXiv2024

Electric imaging and dynamics of photo-charged graphene edge

The one-dimensional side gate based on graphene edges shows a significant capability of reducing the channel length of field-effect transistors, further increasing the integration density of semiconductor devices. The nano-scale electric field distribution near the edge provides the physical limit of the effective channel length, however, its imaging under ambient conditions still lacks, which is a critical aspect for the practical deployment of semiconductor devices. Here, we used scanning nitrogen-vacancy microscopy to investigate the electric field distribution near edges of a single-layer-graphene. Real-space scanning maps of photo-charged floating graphene flakes were acquired with a spatial resolution of $\sim$ 10 nm, and the electric edge effect was quantitatively studied by analyzing the NV spin energy level shifts due to the electric Stark effect. Since the graphene flakes are isolated from external electric sources, we brought out a theory based on photo-thermionic effect to explain the charge transfer from graphene to oxygen-terminated diamond probe with a disordered distribution of charge traps. Real-time tracing of electric fields detected the photo-thermionic emission process and the recombination process of the emitted electrons. This study provides a new perspective for graphene-based one-dimensional gates and opto-electronics with nanoscale real-space imaging, and moreover, offers a novel method to tune the chemical environment of diamond surfaces based on optical charge transfer.

cond-mat.mes-hall↗

arXiv2024

Experimental investigation of coherent ergotropy in a single spin system

Ergotropy is defined as the maximum amount of work that can be extracted through a unitary cyclic evolution. It plays a crucial role in assessing the work capacity of a quantum system. Recently, the significance of quantum coherence in work extraction has been theoretically identified, revealing that quantum states with more coherence possess more ergotropy compared to their dephased counterparts. However, an experimental study of the coherent ergotropy remains absent. Here, we report an experimental investigation of the coherent ergotropy in a single spin system. Based on the method of measuring ergotropy with an ancilla qubit, both the coherent and incoherent components of the ergotropy for the non-equilibrium state were successfully extracted. The increase in ergotropy induced by the increase in the coherence of the system was observed by varying the coherence of the state. Our work reveals the interplay between quantum thermodynamics and quantum information theory, future investigations could further explore the role other quantum attributes play in thermodynamic protocols.

quant-ph↗

arXiv2024

Four-order power reduction in nanoscale electron-nuclear double resonance with a nitrogen-vacancy center in diamond

Detecting nuclear spins using single Nitrogen-Vacancy (NV) centers is of particular importance in nano-scale science and engineering, but often suffers from the heating effect of microwave fields for spin manipulation, especially under high magnetic fields. Here, we realize an energy-efficient nano-scale nuclear-spin detection using a phase-modulation electron-nuclear double resonance scheme. The microwave field can be reduced to 1/250 of previous requirements and the corresponding power is over four orders lower. Meanwhile, the microwave-induced broadening to the line-width of the spectroscopy is significantly canceled and we achieve a nuclear-spin spectrum with a resolution down to 2.1 kHz under a magnetic field at 1840 Gs. The spectral resolution can be further improved by upgrading the experimental control precision. This scheme can also be used in sensing microwave fields and extended to a wide range of applications in the future.

quant-ph↗

arXiv2024

Long-baseline quantum sensor network as dark matter haloscope

Ultralight dark photons constitute a well-motivated candidate for dark matter. A coherent electromagnetic wave is expected to be induced by dark photons when coupled with Standard-Model photons through kinetic mixing mechanism, and should be spatially correlated within the de Broglie wavelength of dark photons. Here we report the first search for correlated dark-photon signals using a long-baseline network of 15 atomic magnetometers, which are situated in two separated meter-scale shield rooms with a distance of about 1700 km. Both the network's multiple sensors and the shields large size significantly enhance the expected dark-photon electromagnetic signals, and long-baseline measurements confidently reduce many local noise sources. Using this network, we constrain the kinetic mixing coefficient of dark photon dark matter over the mass range 4.1 feV-2.1 peV, which represents the most stringent constraints derived from any terrestrial experiments operating over the aforementioned mass range. Our prospect indicates that future data releases may go beyond the astrophysical constraints from the cosmic microwave background and the plasma heating.

quant-ph↗

arXiv2024

Critical fluctuation and noise spectra in two-dimensional Fe$_{3}$GeTe$_{2}$ magnets

Critical fluctuations play a fundamental role in determining the spin orders for low-dimensional quantum materials, especially for recently discovered two-dimensional (2D) magnets. Here we employ the quantum decoherence imaging technique utilizing nitrogen-vacancy centers in diamond to explore the critical magnetic fluctuations and the associated temporal spin noise in van der Waals magnet $\rm{Fe_{3}GeTe_{2}}$. We show that the critical fluctuation contributes to a random magnetic field characterized by the noise spectra, which can be changed dramatically near the critical temperature $T_c$. A theoretical model to describe this phenomenon is developed, showing that the spectral density is characterized by a $1/f$ noise near the $T_c$, while away from this point it behaves like a white noise. The crossover at a certain temperature between these two situations is determined by changing of the distance between the sample and the diamond. This work provides a new way to study critical fluctuation and to extract some of the critical exponents, which may greatly deepen our understanding of criticality in a wide range of physical systems.

cond-mat.mes-hall↗

arXiv2024

Emergent Universal Quench Dynamics in Randomly Interacting Spin Models

Universality often emerges in low-energy equilibrium physics of quantum many-body systems, despite their microscopic complexity and variety. Recently, there has been a growing interest in studying far-from-equilibrium dynamics of quantum many-body systems. Such dynamics usually involves highly excited states beyond the traditional low-energy theory description. Whether universal behaviors can also emerge in such non-equilibrium dynamics is a central issue at the frontier of quantum dynamics. Here we report the experimental observation of universal dynamics by monitoring the spin depolarization process in a solid-state NMR system described by an ensemble of randomly interacting spins. The spin depolarization can be related to temporal spin-spin correlation functions at high temperatures. We discover a remarkable phenomenon that these correlation functions obey a universal functional form. This experimental fact helps us identify the dominant interacting processes in the spin depolarization dynamics that lead to this universality. Our observation demonstrates the existence of universality even in non-equilibrium dynamics at high temperatures, thereby complementing the well-established universality in low-energy physics.

cond-mat.str-el↗

arXiv2024

Challenging theories of dark energy with levitated force sensor

The nature of dark energy is one of the most outstanding problems in physical science, and various theories have been proposed. It is therefore essential to directly verify or rule out these theories experimentally. However, despite substantial efforts in astrophysical observations and laboratory experiments, previous tests have not yet acquired enough accuracy to provide decisive conclusions as to the validity of these theories. Here, using a diamagnetically levitated force sensor, we carry out a test on one of the most compelling explanations for dark energy to date, namely the Chameleon theory, an ultra-light scalar field with screening mechanisms, which couples to normal-matter fields and leaves a detectable fifth force. Our results extend previous results by nearly two orders of magnitude to the entire physical plausible parameter space of cosmologically viable chameleon models. We find no evidence for such a fifth force. Our results decisively rule out the basic chameleon model as a candidate for dark energy. Our work, thus, demonstrates the robustness of laboratory experiments in unveiling the nature of dark energy in the future. The methodology developed here can be further applied to study a broad range of fundamental physics.

gr-qc↗

arXiv2024

An energy efficient quantum-enhanced machine

Quantum friction, a quantum analog of classical friction, reduces the performance of quantum machines, such as heat engines, and makes them less energy efficient. We here report the experimental realization of an energy efficient quantum engine coupled to a quantum battery that stores the produced work, using a single ion in a linear Paul trap. We first establish the quantum nature of the device by observing nonclassical work oscillations with the number of cycles as verified by energy measurements of the battery. We moreover successfully apply shortcut-to-adiabaticity techniques to suppress quantum friction and improve work production. While the average energy cost of the shortcut protocol is only about $3\%$, the work output is enhanced by up to approximately 33$\%$, making the machine significantly more energy efficient. In addition, we show that the quantum engine consistently outperforms its classical counterpart in this regime. Our results pave the way for energy efficient machines with quantum-enhanced performance.

quant-ph↗

arXiv2024

Near-Quantum-limited Haloscope Detection of Dark Photon Dark Matter Enhanced by a High-Q Superconducting Cavit

We report new experimental results on the search for dark photons based on a near-quantum-limited haloscope equipped with a superconducting cavity. The loaded quality factor of the superconducting cavity is $6\times10^{5}$, so that the expected signal from dark photon dark matter can be enhanced by more than one order compared to a copper cavity. A Josephson parametric amplifier with a near-quantum-limited noise temperature has been utilized to minimize the noise during the search. Furthermore, a digital acquisition card based on field programmable gate arrays has been utilized to maximize data collection efficiency with a duty cycle being 100$\%$. This work has established the most stringent constraints on dark photons at around 26.965 $μ$eV. In the future, our apparatus can be extended to search for other dark matter candidates, such as axions and axion-like particles, and scrutinize new physics beyond the Standard Model.

hep-ex↗

arXiv2024

New Constraints on Exotic Spin-Spin-Velocity-Dependent Interactions with Solid-State Quantum Sensors

We report new experimental results on exotic spin-spin-velocity-dependent interactions between electron spins. We designed an elaborate setup that is equipped with two nitrogen-vacancy (NV) ensembles in diamonds. One of the NV ensembles serves as the spin source, while the other functions as the spin sensor. By coherently manipulating the quantum states of two NV ensembles and their relative velocity at the micrometer scale, we are able to scrutinize exotic spin-spin-velocity-dependent interactions at short force ranges. For a T-violating interaction, $V_6$, new limits on the corresponding coupling coefficient, $f_6$, have been established for the force range shorter than 1 cm. For a P,T-violating interaction, $V_{14}$, new constraints on the corresponding coupling coefficient, $f_{14}$, have been obtained for the force range shorter than 1 km.

hep-ex↗