arXiv subjects

Jianguo Wan

Publications and source records attributed to Jianguo Wan.

14 recordsLinked to original sources

arXiv2026

A Sc2C2@C88 cluster based ultra-compact multi-level probabilistic bit for matrix multiplication

Information units are progressively approaching the fundamental physical limits of the integration density, including in terms of extremely small sizes, multistates and probabilistic traversal. However, simultaneously encompassing all of these characteristics in a unit remains elusive. Here, via real-time in situ electrical monitoring, we clearly observed stochastic alterations of multiple conductance states in Sc2C2@C88. The true random bit sequence generated exhibited an autocorrelation function whose confidence interval fell within \pm 0.02, demonstrating high-quality randomness. The alterations of multiple conductance states are controllable, that is, whose probability distributions could traverse from 0 to 1, enabling us to factorize 551 into its prime factors. Furthermore, we proposed a matrix-chain multiplication scheme and experimentally verified the multiplication of two 4 \times 4 state-transition matrices with a small maximum error < 0.05. Combined with theoretical calculations, the stochastic but controllable multistates are probably attributed to the rich energy landscape, which could be stepwise changed by the electric field. Our findings reveal extremely small multi-level probabilistic bit for matrix multiplication, which pave the way for ultracompact intelligent electronic devices.

cond-mat.mtrl-sci↗

arXiv2024

Modular Study of a Force-Magnetic Coupling System

A magnetic-mechanical oscillating system consists of two identical leaf springs, a non-magnetic base, and some magnets. The leaf springs are fixed at the bottom to the non-magnetic base, while the magnet is attached to the top of the leaf springs. This paper investigates the overall motion characteristics of the magnetic-mechanical oscillating system. Adopting the modular modeling concept, we simplify the system into three inter-coupled modules: the leaf springs, magnetic interactions, and the system's dissipation process. We conduct physical modeling and theoretical analysis on these modules and derived the system's dynamic equations. The research indicates that the system is a normal mode system with two degrees of freedom. In addition, we alter parameters and conduct multiple innovative experiments, obtaining intuitive vibration images that characterize the vibration modes and the periodic energy transfer. Furthermore, we employ the simulation software COMSOL Multiphysics simulation to substitute the theory for auxiliary validation, achieving a comprehensive research loop of theory-experiment-simulation. The experimental results show good consistency with the theoretical calculations and simulation results. This research provides a good teaching case for magnetic-coupling complex systems. This modular analysis and rather practical experimental design could solve the previous difficulty that the solution to such problem is too complex, and is conducive to the implementation of education.

physics.ed-ph↗

arXiv2024

Electrically controlled nonvolatile switching of single-atom magnetism in a Dy@C84 single-molecule transistor

Single-atom magnetism switching is a key technique towards the ultimate data storage density of computer hard disks and has been conceptually realized by leveraging the spin bistability of a magnetic atom under a scanning tunnelling microscope. However, it has rarely been applied to solid-state transistors, an advancement that would be highly desirable for enabling various applications. Here, we demonstrate realization of the electrically controlled Zeeman effect in Dy@C84 single-molecule transistors, thus revealing a transition in the magnetic moment from 3.8 μB to 5.1 μB for the ground-state GN at an electric field strength of 3-10 MV/cm. The consequent magnetoresistance significantly increases from 600% to 1100% at the resonant tunneling point. Density functional theory calculations further corroborate our realization of nonvolatile switching of single-atom magnetism, and the switching stability emanates from an energy barrier of 92 meV for atomic relaxation. These results highlight the potential of using endohedral metallofullerenes for high-temperature, high-stability, high-speed, and compact single-atom magnetic data storage.

cond-mat.mtrl-sci↗

arXiv2022

Fano Interference in a Single-Molecule Junction

Trends of miniaturized devices and quantum interference electronics lead to the long desire of Fano interference in single-molecule junctions, here, which is successfully demonstrated using the 2,7-di(4-pyridyl)-9,9'-spirobifluorene molecule with a long backbone group and a short side group. Experimentally, the two electrically coupled groups are found to contribute to two blurred degenerate points in the differential conductance mapping. This forms a characteristic non-centrosymmetric double-crossing feature, with distinct temperature response for each crossing. Theoretically, we describe the practical in-junction electron transmission using a new two-tunnelling-channel coupling model and obtain a working formula with a Fano term and a Breit-Wigner term. The formula is shown to provide a good fit for all the mapping data and their temperature dependence in three dimensions, identifying the Fano component. Our work thus forms a complete set of evidence of the Fano interference in a single-molecule junction induced by two-tunnelling-channel coupling transport. Density functional theory calculations are used to corroborate this new physics.

cond-mat.mes-hall↗

arXiv2015

Lateral Heterojunction Sb2Te3/Bi2Te3 and its topological transport

A lateral heterojunction of topological insulator Sb2Te3/Bi2Te3 was successfully synthesized using a two-step solvothermal method. The two crystalline components were separated well by a sharp lattice-matched interface when the optimized procedure was used. Inspecting the heterojunction using high-resolution transmission electron microscopy showed that epitaxial growth occurred along the horizontal plane. A rectification curve was observed at low temperatures. Quantum correction from the weak antilocalization reveals the transport of the topological surface state. There was, therefore, a staggered-gap lateral heterojunction with a small junction voltage, which is appealing for a platform for spin filters and one-dimensional topological interface states.

cond-mat.mes-hall↗

arXiv2013

Shubnikov de Haas quantum oscillation of the surface states in the metallic Bismuth Telluride sheets

Metallic Bi2Te3 crystalline sheets with the room-temperature resistivity of above 10 mΩ cm were prepared and their magnetoresistive transport was measured in a field of up to 9 Tesla. The Shubnikov de Haas oscillations were identified from the secondly-derived magnetoresistance curves. While changing the angle between the field and normal axis of the sheets, we find that the oscillation periods present a cosine dependence on the angle. This indicates a two-dimensional transport due to the surface state. The work reveals a resolvable surface contribution to the overall conduction even in a metallic topological insulator.

cond-mat.mes-hall↗

arXiv2012

Two-dimensional universal conductance fluctuations and the electron-phonon interaction of topological surface states in Bi2Te2Se nanoribbons

The universal conductance fluctuations (UCFs), one of the most important manifestations of mesoscopic electronic interference, have not yet been demonstrated for the two-dimensional surface state of topological insulators (TIs). Even if one delicately suppresses the bulk conductance by improving the quality of TI crystals, the fluctuation of the bulk conductance still keeps competitive and difficult to be separated from the desired UCFs of surface carriers. Here we report on the experimental evidence of the UCFs of the two-dimensional surface state in the bulk insulating Bi2Te2Se nanoribbons. The solely-B\perp-dependent UCF is achieved and its temperature dependence is investigated. The surface transport is further revealed by weak antilocalizations. Such survived UCFs of the topological surface states result from the limited dephasing length of the bulk carriers in ternary crystals. The electron-phonon interaction is addressed as a secondary source of the surface state dephasing based on the temperature-dependent scaling behavior.

cond-mat.mes-hall↗

arXiv2012

Visualizing plasmon coupling in closely-spaced chains of Ag nanoparticles by electron energy loss spectroscopy

Anisotropic plasmon coupling in closely-spaced chains of Ag nanoparticles was visualized using the electron energy loss spectroscopy in a scanning transmission electron microscope. For dimers as the simplest chain, mapping the plasmon excitations with nanometers' spatial resolution and 0.27 eV energy resolution intuitively identified two coupling plasmons. The in-phase mode redshifted from the ultraviolet region as the inter-particle spacing was reduced, reaching the visible range at 2.7 eV. Calculations based on the discrete dipole approximation confirmed its optical activeness, where the longitudinal direction was constructed as the path for light transportation. Two coupling paths were then observed in an inflexed 4-particle chain.

cond-mat.mes-hall↗

arXiv2012

Experimental evidence on the Altshuler-Aronov-Spivak interference of the topological surface states in the exfoliated Bi2Te3 nanoflakes

Here we demonstrate the Altshuler-Aronov-Spivak (AAS) interference of the topological surface states on the exfoliated Bi2Te3 microflakes by a flux period of h/2e in their magnetoresistance oscillations and its weak field character. Both the osillations with the period of h/e and h/2e are observed. The h/2e-period AAS oscillation gradually dominates with increasing the sample widths and the temperatures. This reveals the transition of the Dirac Fermions' transport to the diffusive regime.

cond-mat.mes-hall↗

arXiv2010

Visualizing topological insulating Bi2Te3 quintuple layers on SiO2-capped Si substrates and its contrast optimization

Thin Bi2Te3 flakes, with as few as 3 quintuple layers, are optically visualized on the SiO2-capped Si substrates. Their optical contrasts vary with the illumination wavelength, flake thickness and capping layers. The maximum contrast appears at the optimized light with the 570nm wavelength. The contrast turns reversed when the flake is reduced to less than 20 quintuple layers. A calculation based on the Fresnel law describes the above observation with the constructions of the layer number-wave length-contrast three-dimensional (3D) diagram and the cap thickness-wavelength-contrast 3D diagram, applicative in the current studies of topological insulating flakes.

cond-mat.mes-hall↗

arXiv2010

Calibrating the atomic balance by carbon nanoclusters

Carbon atoms are counted at near atomic-level precision using a scanning transmission electron microscope calibrated by carbon nanocluster mass standards. A linear calibration curve governs the working zone from a few carbon atoms up to 34,000 atoms. This linearity enables adequate averaging of the scattering cross sections, imparting the experiment with near atomic-level precision despite the use of a coarse mass reference. An example of this approach is provided for thin layers of stacked graphene sheets. Suspended sheets with a thickness below 100 nm are visualized, providing quantitative measurement in a regime inaccessible to optical and scanning probe methods.

cond-mat.mes-hall↗

arXiv2010

Two-step splitting the expandable graphite for few-layer graphene

Few-layer graphene sheets are prepared by splitting the expanded graphites using a high-power sonication. Atomic-level quantitative scanning transmission electron microscopy (Q-STEM) is employed to carry out the efficient layer statisticsm, enabling global optimization of the experimental conditions. A two-step splitting mechanism is thus revealed, in which the mean layer number was firstly reduced to less than 20 by heating to 1100°C and then tuned to the few-layer region by a 5-minute 104W/litre sonication. Raman spectroscopic analysis confirms the above mechanism and demonstrates that the sheets are largely free of defects and oxides.

cond-mat.mes-hall↗

arXiv2010

Experimental observation of nanojets formed by heating the PbO-coated Pb clusters

In this article, we will present the first experimental observation of nanojets formed by heating PbO-coated Pb clusters, which has been predicted theoretically by M. Moseler and U Landman. During the heating, the hot liquid ejects through the broken orifice into vacuum, and forms a condensed trail in the tadpole shape as shown in the TEM micrographs. The temperature-variable Raman spectra indicates that the nanojet formation is closely related to the heating temperature and thus essentially to the internal pressure in the coated clusters. The pressure inside the shell, which rises from the inner core's melting and its confined volume expansion and then drops after the final explosion, dominates the whole nanojetting process.

cond-mat.mes-hall↗

arXiv2010

Films with the discrete nano-DLC-particles as the field emission cascade

The films with the discrete diamond-like-carbon nanoparticles were prepared by the deposition of the carbon nanoparticle beam. Their morphologies were imaged by Scanning Electron Microscopy (SEM) and Atomic Force Microscopy (AFM). The nanoparticles were found distributed on the silicon (100) substrate discretely. The semisphere shapes of the nanoparticles were demonstrated by the AFM line profile. EELS was measured and the sp3 ratio as high as 86% was found. The field-induced electron emission of the as-prepared cascade (nanoDLC/ Si) was tested and the current density of 1mA/cm2 was achieved at 10.2V/μm.

cond-mat.mes-hall↗