arXiv subjects

Jie Shan

Publications and source records attributed to Jie Shan.

At least 19 recordsLinked to original sources

arXiv2026

Competing Chern states revealed by quasiparticle charging in moir\'e rhombohedral graphene

Moir\'e materials realize a versatile platform for exploring the physics of fractional Chern insulators (FCIs). The recently observed evolution from FCIs to an extended quantum anomalous Hall background upon lowering the electronic temperature in moir\'e rhombohedral graphene (mRG)8 raises a fundamental question: Is it caused by a failure to equilibrate the edge states of an FCI or by a genuine phase transition in the bulk from an FCI to a generalized anomalous Hall crystal? Here we address this question by probing quasiparticle charging in a mesoscopic mRG antidot device and by bulk resistance measurements, both of which are bulk-sensitive and free from complications from edge states. Tunneling to the mRG antidot reveals quasiparticles carrying one electron charge for both Chern states at filling factors {\nu}=1 and 2/3 at low temperatures. Temperature dependence measurements of the bulk resistance near {\nu}=2/3 further suggest a thermodynamic phase transition from an FCI to a generalized anomalous Hall crystal at temperatures below about 150mK. The results clearly exclude the edge state equilibration scenario and favor the phase transition scenario. Our work establishes mesoscopic probes as a powerful approach to uncover competing ground states in moir\'e materials and provides a basis for probing fractionalized excitations in FCIs.

cond-mat.mes-hall↗

arXiv2026

Trion Hall effect in electron-hole double layers

The realization of Coulomb coupled electron-hole double layers in 2D semiconductor heterostructures has enabled the thermodynamic and transport studies of equilibrium exciton fluids without a magnetic field. By doping the exciton fluid with additional electrons/holes, an equilibrium fluid of trions - three particle bound states of electrons and holes - further emerge, providing the platform to explore new transport phenomena associated with such composite particles. Here we report the observation of a Hall effect for trions in MoSe2/WSe2 heterobilayers, which support Coulomb-coupled electron and hole fluids with tunable densities. The Hall effect arises from a Lorentz force on trions under a perpendicular magnetic field. It is manifested in both Hall drag measurements and standard Hall effect measurements on just one of the semiconductor layers. For negatively charged trions, an electron Hall effect is observed even in a hole doped WSe2 monolayer due to the presence of trion drags. The trion Hall effect also disappears when the trions are ionized at elevated temperatures and/or high trion densities. Our work opens the door for realizing quantum oscillations and the quantum Hall effect for trions.

cond-mat.mes-hall↗

arXiv2026

Stacking-order-dependent electronic properties of MoTe2/WSe2 moiré bilayers

Transition metal dichalcogenide (TMD) moiré bilayers have realized a wide range of strongly correlated and topological phenomena. The physics in these materials is often sensitive to the interlayer stacking order. Polarization-resolved optical second harmonic generation (SHG) is the most used technique for stacking order characterization but unverified for most heterobilayers. Here we calibrate the optical SHG for angle-aligned MoTe2/WSe2 bilayers by the scanning transmission electron microscopy (STEM). We directly compare the transport and magnetic properties and the electronic phase diagram for two distinct stacking orders. With the calibrated stacking order assignment, we clarify the interpretation of earlier results, including the nature of the Chern insulator, mechanism of an electric-field-tuned metal-insulator transition at half band filling, and the Kondo lattice physics. Our work provides a consistent picture of the relation between the stacking order and the electronic properties of MoTe2/WSe2 moiré bilayers.

cond-mat.mes-hall↗

arXiv2026

Engineering topological flat bands in $Γ$-valley moiré systems with Ising-type SOC: twisted 1T-ZrS$_2$ and 1T-SnSe$_2$

Twisted moiré superlattices hosting topological flat bands provide a platform to explore the interplay between topology and correlations. Here we investigate topological band structures in $Γ$-valley moiré systems based on 1T-ZrS$_2$ and 1T-SnSe$_2$. Using large-scale ab initio calculations and continuum modelling, we demonstrate that both materials exhibit an approximate spin-$U(1)$ symmetry and host isolated topological moiré valence bands, including quantum spin Hall and high spin Chern states. By constructing a hierarchy of $Γ$-valley moiré continuum models, we show that isolated moiré bands carry a trivial $C_3$ symmetry indicator when the low-energy physics is described by a single effective orbital and a single layer-hybridized branch, either bonding or antibonding. Topological bands therefore arise from inter-branch and/or inter-orbital coupling. Moreover, we determine interaction-driven phase diagrams using Hartree--Fock and exact diagonalization, finding various phases tunable by twist angle, interaction strength, and displacement field. We identify specific conditions under which fractional Chern insulators are favored. Together with previous work showing that the moiré conduction bands of 1T-ZrS$_2$ and 1T-SnSe$_2$ realize $M$-valley twisting and host quasi-one-dimensional physics, our results establish these systems as ideal platforms for strongly correlated moiré physics and provide a systematic framework for understanding topological band structures in $Γ$-valley moiré materials.

cond-mat.mtrl-sci↗

arXiv2026

Magnetic-field-induced superconductivity in hexalayer rhombohedral graphene

In conventional superconductors, superconductivity is generally suppressed by external magnetic fields due to spin-singlet pairing. Here, we report signatures of in-plane-magnetic-field-induced superconductivity in hexalayer rhombohedral graphene and reveal electric-field control of its depairing behavior. With the application of a small in-plane magnetic field $B_{\parallel}$, a superconducting state emerges within a narrow band along a phase boundary. Its properties evolve continuously with increasing $B_{\parallel}$: the superconducting region progressively shifts toward higher electric field as the $B_{\parallel}$ increases and the transition temperature rises with increasing $B_{\parallel}$. Remarkably, the superconducting state remains robust under $B_{\parallel}$ up to 14 T, far exceeding the conventional Pauli limit. Quantum oscillation measurements further reveal that the superconductivity emerges from nematic Fermi surface reconstruction. These results suggest a spin-polarized superconducting states with unconventional origins.

cond-mat.mes-hall↗

arXiv2026

Superconductivity and Ferroelectric Orbital Magnetism in Semimetallic Rhombohedral Hexalayer Graphene

Rhombohedral multilayer graphene has emerged as a promising platform for exploring correlated and topological quantum phases, enabled by its Berry-curvature-bearing flat bands. While prior work has focused on separated conduction and valence bands, we probe the extensive semimetallic regime of rhombohedral hexalayer graphene. We survey a rich phase diagram dominated by flavor-symmetry breaking and reveal an electric-field-driven band inversion by fermiology. Near this inversion, we observe two superconducting-like states confined to regions with coexisting electron and hole Fermi surfaces, suggesting a possible dual-carrier origin. In addition, we identify a ferroelectric orbital magnet that undergoes sharp switching under unipolar electric fields, signaling spontaneous electric polarization. Unlike previously reported multiferroicity near zero electric field, this new state exhibits magnetic hysteresis reversible by electric field, consistent with a phenomenological model of coupled electric and magnetic polarization. Our work elucidates the correlated semimetal regime in rhombohedral graphene and underscores its potential to host diverse quantum phases.

cond-mat.str-el↗

arXiv2026

Emergence of a symmetry-broken Chern insulator near a moiré Kondo breakdown

Moiré semiconductors built on angle-aligned transition metal dichalcogenide (TMD) heterobilayers provide a physical realization of the Kondo lattice model, in which one TMD layer is prepared in a Mott insulating state supporting a lattice of local magnetic moments and the other layer in a metallic state supporting itinerant carriers. The artificial Kondo lattice enables the exploration of exotic states of matter near a continuously tunable Kondo breakdown. Here we report the emergence of a symmetry-broken Chern insulator at a moiré hole filling factor 4/3 in angle-aligned MoTe2/WSe2 moiré bilayers, which realize a chiral Kondo lattice. The symmetry-broken Chern insulator, which exhibits integer quantized Hall conductance at a fractional moiré filling, breaks the translational symmetry of the lattice spontaneously; it also appears only near a magnetic field-induced Kondo breakdown in the mixed-valence regime of the material. We further demonstrate that the magnetic field required to induce the Kondo breakdown and to stabilize the symmetry-broken Chern insulator is twist angle dependent. The results present new opportunities for exploring the subtle interplay between topology and Kondo interactions in moiré semiconductors.

cond-mat.mes-hall↗

arXiv2026

Electric-field-tuned consecutive topological phase transitions between distinct correlated insulators in moire MoTe2/WSe2 heterobilayer

Consecutive topological phase transitions (TPTs) between strongly correlated electronic phases that differ simultaneously in symmetry breaking and topological order are of fundamental interest in condensed matter physics, yet are rarely realized experimentally. We report two consecutive electric-field-driven TPTs at half filling (nu = 1) in angle-aligned MoTe2/WSe2 moire heterobilayers. With increasing out-of-plane displacement field, a geometrically frustrated Mott insulator evolves into a ferromagnetic quantum anomalous Hall (QAH) Mott insulator, i.e., a spin-polarized topological Mott insulator without an observable charge-gap closure, and subsequently into an antiferromagnetic, valley-coherent Mott insulator (VC-AFM) accompanied by a continuous charge-gap collapse and the emergence of a critical metallic state. Layer-resolved magnetic circular dichroism (MCD), magneto-transport, and compressibility measurements jointly determine the phase diagram. The high-field evolution of the antiferromagnetic state reveals a metamagnetic-like transition at a critical field B*, above which a Chern insulating transport response reappears. Our results establish the MoTe2/WSe2 moire platform as a tunable realization of an extended Kane-Mele-Hubbard model hosting sequential correlation-topology-intertwined transitions.

cond-mat.str-el↗

arXiv2026

Mechanical sensing of metamagnetic tricriticality in two-dimensional CrI3

Layered Ising metamagnets are antiferromagnetic (AF) materials consisting of monolayer Ising ferromagnets coupled to each other via interlayer AF interactions. They exhibit rich magnetic phase diagrams, featuring tricritical and critical end points, due to the competing magnetic interactions and the Ising anisotropy. While conventional thermodynamic probes can identify these critical points in bulk Ising metamagnets, achieving this in the two-dimensional (2D) limit, where enhanced fluctuation effects can substantially modify critical phenomena, remains to be realized. Here, we combine specific heat capacity (C_V) and magnetic circular dichroism measurements to identify these critical points, extract a tricritical exponent, and map out the complete magnetic phase diagram of 2D Ising metamagnetic CrI3. This is achieved in a nanomechanical device of 6-layer CrI3, in which a direct measurement of the temperature derivative of its mechanical resonance frequency gives C_V. The tricritical point is identified by the onset of an abrupt spin-flip transition on one side and, on the other side, by a vanishing specific heat λ-anomaly for a continuous AF phase transition. In contrast, only the spin-flip transition remains near the critical end point. Our results establish nanomechanical calorimetry as a general route to classify metamagnetic phase transitions and to study multicritical phenomena in 2D magnets.

cond-mat.mes-hall↗

arXiv2025

Imaging propagating terahertz collective modes in two-dimensional semiconductor double layers

Two-dimensional transition metal dichalcogenide (TMD) semiconductors exhibit a wide range of novel phenomena at millielectronvolt (terahertz-frequency) energy scales, including superconducting and correlation-induced insulating gaps that are frequently accompanied by symmetry breaking. However, due to the subwavelength dimensions and the often low conductivities of these systems, their intrinsic THz plasmons and meV-scale excitation gaps are difficult to access experimentally. Here we report an optical readout method that can image propagating THz-frequency collective modes in real time. The method relies on a strong coupling between the optical polarons of monolayer TMD semiconductors and the local THz fields in a waveguide, which enables us to image THz plasmons with micron scale spatial resolution and determine their propagation group velocities. Moreover, at finite magnetic fields, we observe coherent cyclotron oscillations resulting from Landau level repopulation induced by the THz field. Our findings provide a new near-field platform for probing collective excitations in strongly correlated two-dimensional semiconductors and enable "all-photonic" TMD-based architectures for time-domain THz plasmonics and optoelectronics.

cond-mat.mes-hall↗

arXiv2025

Thermoelectricity of moiré heavy fermions in MoTe2/WSe2 bilayers

Tunable Kondo lattice and heavy fermion physics have been recently reported in moiré materials, but most of the studies have focused on the electrical and magnetic properties. Quantitative thermoelectric measurements, which can reveal entropic information of the heavy fermions, have yet to be achieved. Here, we report a comprehensive thermoelectric study on the moiré heavy fermion phase realized in hole-doped angle-aligned MoTe2/WSe2 bilayers. By electrically gating the material to the Kondo lattice region of the phase diagram, we observe a sign change in the Seebeck coefficient near the Kondo coherence temperature, where the heavy fermion phase with an electron-like Fermi surface evolves into an itinerant Fermi liquid with a hole-like Fermi surface. We compare the results with the semiclassical Mott relation and discuss the observed discrepancies. In addition to the thermal dissociation of Kondo singlets in the heavy Fermi liquid, a sign change accompanied by a strong peak in the Seebeck coefficient is also observed near a Zeeman breakdown of the Kondo singlets, signaling an entropy accumulation. Our results provide entropic information on both the formation and breakdown of heavy fermions in moiré semiconductors.

cond-mat.str-el↗

arXiv2025

Quantum oscillations between excitonic and quantum spin Hall insulators in moiré WSe2

Quantum spin Hall insulators (QSHIs) and excitonic insulators (EIs) are prototypical topological and correlated states of matter, respectively. The topological phase transition between the two has attracted much theoretical interest but experimental studies have been hindered by the availability of tunable materials that can access such a transition. Here, by utilizing the interaction-enhanced g-factor and the flat moiré bands in twisted bilayer WSe2 (tWSe2), we realize tunable electron-like and hole-like Landau levels (LLs) in the opposite valleys of tWSe2 under a perpendicular magnetic field. At half-band-filling, which corresponds to electron-hole charge neutrality, periodic oscillations between QSHIs (for fully filled LLs) and EIs (for half-filled LLs) are observed due to the interplay between the cyclotron energy and the intervalley correlation; QSHIs with up to four pairs of helical edge states can be resolved. We further analyze the effect of Fermi surface nesting on the stability of EIs via electric field-tuning of the moiré band structure. Our results demonstrate a novel QSHI-to-EI topological phase transition and provide a comprehensive understanding of the fermiology of tWSe2.

cond-mat.mes-hall↗

arXiv2025

Simulating high-temperature superconductivity in moiré WSe2

The emergence of high transition temperature (Tc) superconductivity in strongly correlated materials remains a major unsolved problem in physics. High-Tc materials, such as cuprates, are generally complex and not easily tunable, making theoretical modelling difficult. Although the Hubbard model--a simple theoretical model of interacting electrons on a lattice--is believed to capture the essential physics of high-Tc materials, obtaining accurate solutions of the model, especially in the relevant regime of moderate correlation, is challenging. The recent demonstration of robust superconductivity in moiré WSe2, whose low-energy electronic bands can be described by the Hubbard model and are highly tunable, presents a new platform for tackling the high-Tc problem. Here, we tune moiré WSe2 bilayers to the moderate correlation regime through the twist angle and map the phase diagram around one hole per moiré unit cell (v = 1) by electrostatic gating and electrical transport and magneto-optical measurements. We observe a range of high-Tc phenomenology, including an antiferromagnetic insulator at v = 1, superconducting domes upon electron and hole doping, and unusual metallic states at elevated temperatures including strange metallicity. The highest Tc occurs adjacent to the Mott transition, reaching about 6% of the effective Fermi temperature. Our results establish a new material system based on transition metal dichalcogenide (TMD) moiré superlattices that can be used to study high-Tc superconductivity in a highly controllable manner and beyond.

cond-mat.supr-con↗

arXiv2025

Evidence of topological Kondo insulating state in MoTe2/WSe2 moiré bilayers

Topological Kondo insulators (TKIs) are topologically protected insulating states induced not by single-particle band inversions, but by the Kondo interaction between itinerant electrons and a lattice of local magnetic moments. Although experiments have suggested the emergence of three-dimensional (3D) TKIs in the rare earth compound SmB6, its two-dimensional (2D) counterpart has not been demonstrated to date. Here we report experimental evidence of a TKI in angle-aligned MoTe2/WSe2 moiré bilayers, which support a Kondo lattice with topologically nontrivial Kondo interactions. We prepare in a dual-gated device a triangular lattice Mott insulator in the MoTe2 layer Kondo-coupled to a half-filled itinerant band in the WSe2 layer. Combined transport and compressibility measurements show that the prepared state supports metallic transport at high temperatures and, at low temperatures, an insulating bulk with conducting helical edge states protected by spin-Sz conservation. The presence of Kondo singlets is further evidenced by their breakdown at high magnetic fields. Such behaviors are in stark contrast to the simple metallic state when the Mott insulator in the MoTe2 layer is depleted by gating. Our results open the door for exploring tunable topological Kondo physics in moiré materials.

cond-mat.mes-hall↗

arXiv2025

Emergence of Chern metal in a moiré Kondo lattice

A Chern metal is a two-dimensional metallic state of matter carrying chiral edge states. It can emerge as a doped Chern insulator, but theoretical studies have also predicted its emergence near a Kondo breakdown separating a metallic chiral spin liquid and a heavy Fermi liquid in a frustrated lattice. To date, the latter exotic scenario has not been realized. Here, we report the observation of a Chern metal at the onset of the magnetic Kondo breakdown in a frustrated moiré Kondo lattice--angle-aligned MoTe2/WSe2 bilayers. The state is compressible and is manifested by a nearly quantized Hall resistance but a finite longitudinal resistance that arises from a bad metallic bulk. The state also separates an itinerant and a heavy Fermi liquid and appears far away from the band inversion critical point of the material, thus ruling out its origin from simply doping a Chern insulator. We demonstrate the presence of a chiral edge state by nonlocal transport measurements and current-induced quantum anomalous Hall breakdown. Magnetic circular dichroism measurements further reveal a magnetization plateau for the Chern metal before a metamagnetic transition at the Kondo breakdown. Our results open an opportunity for moiré engineering of exotic quantum phases of matter through the close interplay between band topology and Kondo interactions.

cond-mat.str-el↗

arXiv2025

Quantum oscillations in a dipolar excitonic insulator

Quantum oscillations in magnetization or resistivity are a defining feature of metals subject to an external magnetic field. The phenomenon is generally not expected in insulators without a Fermi surface. The observations of quantum oscillations in Kondo insulating materials have provided a rare counterexample and attracted much theoretical interest. However, the magnetic oscillations in correlated insulators remain poorly understood. Here we report the observations of resistivity quantum oscillations in an excitonic insulator realized in Coulomb-coupled electron-hole double layers with gate-tunability that allows the phenomenon to be explored in a more controllable fashion than in bulk materials. When the cyclotron energy of the electrons or holes is tuned to be comparable to or larger than the exciton binding energy, recurring transitions between excitonic insulators and electron-hole decoupled quantum Hall states are observed. Compressibility measurements show an oscillatory exciton binding energy as a function of magnetic field and electron-hole pair density. Coulomb drag measurements further reveal the formation of excitons with finite angular momentum. Our results are qualitatively captured by mean-field theory calculations. The study demonstrates a new platform for studying quantum oscillations in correlated insulators.

cond-mat.mes-hall↗

arXiv2025

Time-reversal symmetry breaking fractional quantum spin Hall insulator in moiré MoTe2

Twisted bilayer transition metal dichalcogenide semiconductors, which support flat Chern bands with enhanced interaction effects, realize a platform for fractional Chern insulators and fractional quantum spin Hall (FQSH) insulators. A recent experiment has reported the emergence of a FQSH insulator protected by spin-Sz conservation at a moiré lattice filling factor ν=3 in 2.1-degree twisted bilayer MoTe2. Theoretical studies have proposed both time-reversal symmetric and asymmetric ground states as possible candidates for the observed FQSH insulator, but the nature of the state remains unexplored. Here we report the observation of spontaneous time-reversal symmetry breaking at generic fillings in 2.1-degree twisted bilayer MoTe2 from ν<1 all the way to ν>6 except at ν=2, 4, and 6. Although zero Hall response is observed at ν=3 for magnetic fields higher than 20 mT, a finite anomalous Hall response accompanied by a magnetic hysteresis is observed at lower magnetic fields, demonstrating spontaneous time-reversal symmetry breaking. Our work shows the tendency towards ferromagnetism by doping the first three pairs of conjugate Chern bands in the material; it also sheds light on the nature of the FQSH insulator at ν=3.

cond-mat.mes-hall↗

arXiv2024

T-GMSI: A transformer-based generative model for spatial interpolation under sparse measurements

Generating continuous environmental models from sparsely sampled data is a critical challenge in spatial modeling, particularly for topography. Traditional spatial interpolation methods often struggle with handling sparse measurements. To address this, we propose a Transformer-based Generative Model for Spatial Interpolation (T-GMSI) using a vision transformer (ViT) architecture for digital elevation model (DEM) generation under sparse conditions. T-GMSI replaces traditional convolution-based methods with ViT for feature extraction and DEM interpolation while incorporating a terrain feature-aware loss function for enhanced accuracy. T-GMSI excels in producing high-quality elevation surfaces from datasets with over 70% sparsity and demonstrates strong transferability across diverse landscapes without fine-tuning. Its performance is validated through extensive experiments, outperforming traditional methods such as ordinary Kriging (OK) and natural neighbor (NN) and a conditional generative adversarial network (CGAN)-based model (CEDGAN). Compared to OK and NN, T-GMSI reduces root mean square error (RMSE) by 40% and 25% on airborne lidar data and by 23% and 10% on spaceborne lidar data. Against CEDGAN, T-GMSI achieves a 20% RMSE improvement on provided DEM data, requiring no fine-tuning. The ability of model on generalizing to large, unseen terrains underscores its transferability and potential applicability beyond topographic modeling. This research establishes T-GMSI as a state-of-the-art solution for spatial interpolation on sparse datasets and highlights its broader utility for other sparse data interpolation challenges.

cs.CV↗