arXiv subjects

Jing Tao

Publications and source records attributed to Jing Tao.

90 records · Page 5Linked to original sources

arXiv2016

Differences in chemical doping matter - Superconductivity in Ti1-xTaxSe2 but not in Ti1-xNbxSe2

We report that 1T-TiSe2, an archetypical layered transition metal dichalcogenide, becomes superconducting when Ta is substituted for Ti but not when Nb is substituted for Ti. This is unexpected because Nb and Ta should be chemically equivalent electron donors. Superconductivity emerges near x = 0.02 for Ti1-xTaxSe2, while for Ti1-xNbxSe2, no superconducting transitions are observed above 0.4 K. The equivalent chemical nature of the dopants is confirmed by X-ray photoelectron spectroscopy. ARPES and Raman scattering studies show similarities and differences between the two systems, but the fundamental reasons why the Nb and Ta dopants yield such different behavior are unknown. We present a comparison of the electronic phase diagrams of many electron-doped 1T-TiSe2 systems, showing that they behave quite differently, which may have broad implications in the search for new superconductors. We propose that superconducting Ti0.8Ta0.2Se2 will be suitable for devices and other studies based on exfoliated crystal flakes.

cond-mat.supr-con↗

arXiv2015

Moss: A Scalable Tool for Efficiently Sampling and Counting 4- and 5-Node Graphlets

Counting the frequencies of 3-, 4-, and 5-node undirected motifs (also know as graphlets) is widely used for understanding complex networks such as social and biology networks. However, it is a great challenge to compute these metrics for a large graph due to the intensive computation. Despite recent efforts to count triangles (i.e., 3-node undirected motif counting), little attention has been given to developing scalable tools that can be used to characterize 4- and 5-node motifs. In this paper, we develop computational efficient methods to sample and count 4- and 5- node undirected motifs. Our methods provide unbiased estimators of motif frequencies, and we derive simple and exact formulas for the variances of the estimators. Moreover, our methods are designed to fit vertex centric programming models, so they can be easily applied to current graph computing systems such as Pregel and GraphLab. We conduct experiments on a variety of real-word datasets, and experimental results show that our methods are several orders of magnitude faster than the state-of-the-art methods under the same estimation errors.

cs.SI↗

arXiv2015

Growth Tight Actions

We introduce and systematically study the concept of a growth tight action. This generalizes growth tightness for word metrics as initiated by Grigorchuk and de la Harpe. Given a finitely generated, non-elementary group $G$ acting on a $G$--space $\mathcal{X}$, we prove that if $G$ contains a strongly contracting element and if $G$ is not too badly distorted in $\mathcal{X}$, then the action of $G$ on $\mathcal{X}$ is a growth tight action. It follows that if $\mathcal{X}$ is a cocompact, relatively hyperbolic $G$--space, then the action of $G$ on $\mathcal{X}$ is a growth tight action. This generalizes all previously known results for growth tightness of cocompact actions: every already known example of a group that admits a growth tight action and has some infinite, infinite index normal subgroups is relatively hyperbolic, and, conversely, relatively hyperbolic groups admit growth tight actions. This also allows us to prove that many CAT(0) groups, including flip-graph-manifold groups and many Right Angled Artin Groups, and snowflake groups admit cocompact, growth tight actions. These provide first examples of non-relatively hyperbolic groups admitting interesting growth tight actions. Our main result applies as well to cusp uniform actions on hyperbolic spaces and to the action of the mapping class group on Teichmueller space with the Teichmueller metric. Towards the proof of our main result, we give equivalent characterizations of strongly contracting elements and produce new examples of group actions with strongly contracting elements.

math.GR↗

arXiv2015

Graphene-Silicon Layered Structures on Single-crystalline Ir(111) Thin Films

Single-crystalline transition metal films are ideal playing fields for the epitaxial growth of graphene and graphene-base materials. Graphene-silicon layered structures were successfully constructed on Ir(111) thin film on Si substrate with an yttria-stabilized zirconia buffer layer via intercalation approach. Such hetero-layered structures are compatible with current Si-based microelectronic technique, showing high promise for applications in future micro- and nano-electronic devices.

cond-mat.mtrl-sci↗

arXiv2015

Growth Tight Actions of Product Groups

A group action on a metric space is called growth tight if the exponential growth rate of the group with respect to the induced pseudo-metric is strictly greater than that of its quotients. A prototypical example is the action of a free group on its Cayley graph with respect to a free generating set. More generally, with Arzhantseva we have shown that group actions with strongly contracting elements are growth tight. Examples of non-growth tight actions are product groups acting on the $L^1$ products of Cayley graphs of the factors. In this paper we consider actions of product groups on product spaces, where each factor group acts with a strongly contracting element on its respective factor space. We show that this action is growth tight with respect to the $L^p$ metric on the product space, for all $1<p\leq \infty$. In particular, the $L^\infty$ metric on a product of Cayley graphs corresponds to a word metric on the product group. This gives the first examples of groups that are growth tight with respect to an action on one of their Cayley graphs and non-growth tight with respect to an action on another, answering a question of Grigorchuk and de la Harpe.

math.GR↗

arXiv2015

Polytypism, polymorphism and superconductivity in TaSe2-xTex

Polymorphism in materials often leads to significantly different physical properties - the rutile and anatase polymorphs of TiO2 are a prime example. Polytypism is a special type of polymorphism, occurring in layered materials when the geometry of a repeating structural layer is maintained but the layer stacking sequence of the overall crystal structure can be varied; SiC is an example of a material with many polytypes. Although polymorphs can have radically different physical properties, it is much rarer for polytypism to impact physical properties in a dramatic fashion. Here we study the effects of polytypism and polymorphism on the superconductivity of TaSe2, one of the archetypal members of the large family of layered dichalcogenides. We show that it is possible to access 2 stable polytypes and 2 stable polymorphs in the TaSe2-xTex solid solution, and find that the 3R polytype shows a superconducting transition temperature that is nearly 17 times higher than that of the much more commonly found 2H polytype. The reason for this dramatic change is not apparent, but we propose that it arises either from a remarkable dependence of Tc on subtle differences in the characteristics of the single layers present, or from a surprising effect of the layer stacking sequence on electronic properties that instead are expected to be dominated by the properties of a single layer in materials of this kind.

cond-mat.supr-con↗

arXiv2014

Experimental Verification of Van Vleck Nature of Long-Range Ferromagnetic Order in Vanadium-Doped Three-Dimensional Topological Insulator Sb$_{2}$Te$_{3}$

We demonstrate by high resolution low temperature electron energy loss spectroscopy (EELS) measurements that the long range ferromagnetic (FM) order in vanadium (V)-doped topological insulator Sb$_2$Te$_3$ has the nature of van Vleck-type ferromagnetism. The positions and the relative amplitudes of two core-level peaks (L$_3$ and L$_2$) of the V EELS spectrum show unambiguous change when the sample is cooled from room temperature to T=10K. Magnetotransport and comparison of the measured and simulated EELS spectra confirm that these changes originate from onset of FM order. Crystal field analysis indicates that in V-doped Sb$_2$Te$_3$, partially filled core states contribute to the FM order. Since van Vleck magnetism is a result of summing over all states, this magnetization of core level verifies the van Vleck-type ferromagnetism in a direct manner.

cond-mat.mes-hall↗

arXiv2014

Unveiling the microscopic origin of the electronic smectic-nematic phase transition in La1/3Ca2/3MnO3

Electronic-liquid-crystal phases, in which part of the spatial symmetries are broken spontaneously, are considered to play a vital role in interpreting the structure-property relation in strongly-correlated materials. Although electronic-liquid-crystal phases have been inferred in studies of a wide range of materials, the nature of the transition between such phases has received little experimental attention. Here we report the direct observation of an electronic smectic-nematic phase transition in a doped manganite utilizing transmission electron microscopic techniques. We show that, in this case, the transition from the smectic to the nematic phase is driven by two mechanisms: the proliferation of dislocations and the development of mesoscale charge inhomogeneity. We observe the development of dislocation pairs within the commensurate smectic phase on approaching the transition (at 210 +/- 10 K) from below. Above the transition, the incommensurate nematic phase is accompanied by mesoscopic electronic phase separation.

cond-mat.str-el↗

arXiv2014

Titanic Magnetoresistance in WTe2

Magnetoresistance is the change of a material's electrical resistance in response to an applied magnetic field. In addition to its intrinsic scientific interest, it is a technologically important property, placing it in "Pasteur's quadrant" of research value: materials with large magnetorsistance have found use as magnetic sensors 1, in magnetic memory 2, hard drives 3, transistors 4, and are the subject of frequent study in the field of spintronics 5, 6. Here we report the observation of an extremely large one-dimensional positive magnetoresistance (XMR) in the layered transition metal dichalcogenide (TMD) WTe2; 452,700 percent at 4.5 Kelvin in a magnetic field of 14.7 Tesla, and 2.5 million percent at 0.4 Kelvin in 45 Tesla, with no saturation. The XMR is highly anisotropic, maximized in the crystallographic direction where small pockets of holes and electrons are found in the electronic structure. The determination of the origin of this effect and the fabrication of nanostructures and devices based on the XMR of WTe2 will represent a significant new direction in the study and uses of magnetoresistivity. *The published version of the paper includes co-authors Tian Liang and Max Hirschberger. **This paper has been published with new MR data to 60T where the MR of WTe2 reaches 13 million percent (at 0.5K) and still shows no signs of saturation. We also have new electron diffraction patterns to lower temperature (10K). We discuss the possible origin of the MR as coming from an electron-hole 'resonance' condition established by a perfect n/p ratio of 1 (more details in a new "extended data" section). This makes WTe2, possibly, the first realization of a perfectly balanced semimetal. ***The paper is published as "Large non-saturating magnetoresistance in WTe2" in Nature (2014), DOI:10.1038/nature13763

cond-mat.mtrl-sci↗

arXiv2014

Polar State in Freestanding Strontium Titanate Nanoparticles

Monodispersed strontium titanate nanoparticles were prepared and studied in detail. It is found that ~10 nm as-prepared stoichiometric nanoparticles are in a polar structural state (with possibly ferroelectric properties) over a broad temperature range. A tetragonal structure, with possible reduction of the electronic hybridization is found as the particle size is reduced. In the 10 nm particles, no change in the local Ti-off centering is seen between 20 and 300 K. The results indicate that nanoscale motifs of SrTiO3 may be utilized in data storage as assembled nano-particle arrays in applications where chemical stability, temperature stability and low toxicity are critical issues.

cond-mat.mtrl-sci↗

arXiv2014

Paramagnetic to ferromagnetic phase transition in lightly Fe-doped Cr$_2$B

Cr$_2$B displays temperature independent paramagnetism. We induce ferromagnetism by replacing less than $3\,\%$ of the Cr atoms by Fe. By the lowest Fe doping level made, Curie-Weiss behavior is observed; $Θ_{CW}$ changes from $-20\,$K for $0.5\,\%$ Fe-doped Cr$_2$B to positive values of about 50 K by $5\,\%$ Fe doping. The ferromagnetic T$_C$ is 8 K for $2.5\,\%$ Fe doping and increases linearly to 46 K by $5\,\%$ doping; we infer that a quantum phase transition occurs near the $2.0\,\%$ Fe level. Magnetic fluctuations at the intermediate doping levels are reflected in the linear resistance and an anomalous heat capacity at low temperatures. Imaging and chemical analysis down to the atomic scale show that the Fe dopant is randomly distributed.

cond-mat.str-el↗

arXiv2014

Ferromagnetism and Spin-dependent Transport in n-type Mn-Bi2Te3 Thin Films

We describe a detailed study of the structural, magnetic, and magneto-transport properties of single-crystal, n-type, Mn-doped Bi2Te3 thin films grown by molecular beam epitaxy. With increasing Mn concentration, the crystal structure changes from the tetradymite structure of the Bi2Te3 parent crystal at low Mn concentrations towards a BiTe phase in the (Bi2Te3)m(Bi2)n homologous series. Magnetization measurements reveal the onset of ferromagnetism with a Curie temperature in the range 13.8 K - 17 K in films with 2 % - 10 % Mn concentration. Magnetization hysteresis loops reveal that the magnetic easy axis is along the c-axis of the crystal (perpendicular to the plane). Polarized neutron reflectivity measurements of a 68 nm-thick sample show that the magnetization is uniform through the film. The presence of ferromagnetism is also manifest in a strong anomalous Hall effect and a hysteretic magnetoresistance arising from domain wall scattering. Ordinary Hall effect measurements show that the carrier density is n-type, increases with Mn doping, and is high enough (> 2.8 x 10^{13} cm^{-2}) to place the chemical potential in the conduction band. Thus, the observed ferromagnetism is likely associated with both bulk and surface states. Surprisingly, the Curie temperature does not show any clear dependence on the carrier density but does increase with Mn concentration. Our results suggest that the ferromagnetism probed in these Mn-doped Bi2Te3 films is not mediated by carriers in the conduction band or in an impurity band.

cond-mat.mtrl-sci↗

arXiv2013

A Peep on the Interplays between Online Video Websites and Online Social Networks

Many online video websites provide the shortcut links to facilitate the video sharing to other websites especially to the online social networks (OSNs). Such video sharing behavior greatly changes the interplays between the two types of websites. For example, users in OSNs may watch and re-share videos shared by their friends from online video websites, and this can also boost the popularity of videos in online video websites and attract more people to watch and share them. Characterizing these interplays can provide great insights for understanding the relationships among online video websites, OSNs, ISPs and so on. In this paper we conduct empirical experiments to study the interplays between video sharing websites and OSNs using three totally different data sources: online video websites, OSNs, and campus network traffic. We find that, a) there are many factors that can affect the external sharing probability of videos in online video websites. b) The popularity of a video itself in online video websites can greatly impact on its popularity in OSNs. Videos in Renren, Qzone (the top two most popular Chinese OSNs) usually attract more viewers than in Sina and Tencent Weibo (the top two most popular Chinese microblogs), which indicates the different natures of the two kinds of OSNs. c) The analysis based on real traffic data illustrates that 10\% of video flows are related to OSNs, and they account for 25\% of traffic generated by all videos.

cs.SI↗

arXiv2013

Diameter of the thick part of moduli space and simultaneous Whitehead moves

Let S be a surface of genus g with p punctures with negative Euler characteristic. We study the diameter of the $ε$-thick part of moduli space of S equipped with the Teichmüller or Thurston's Lipschitz metric. We show that the asymptotic behaviors in both metrics are of order $\log \frac{g+p}ε$. The same result also holds for the $ε$-thick part of the moduli space of metric graphs of rank n equipped with the Lipschitz metric. The proof involves a sorting algorithm that sorts an arbitrary labeled tree with n labels with simultaneous Whitehead moves, where the number of steps is of order log(n).

math.GT↗

arXiv2012

Linearly Bounded Conjugator Property for Mapping Class Groups

Given two conjugate mapping classes f and g, we produce a conjugating element w such that |w| < K(|f|+|g|), where |.| denotes the word metric with respect to a fixed generating set, and K is a constant depending only on the generating set. As a consequence, the conjugacy problem for mapping class groups is exponentially bounded.

math.GT↗

arXiv2012

Mixed-Valence-Driven Heavy-Fermion Behavior and Superconductivity in KNi$_2$Se$_2$

Based on specific heat and magnetoresistance measurements, we report that a "heavy" electronic state exists below $T \approx$ 20 K in KNi$_2$Se$_2$, with an increased carrier mobility and enhanced effective electronic band mass, $m$* = 6$m_b$ to 18$m_b$. This "heavy" state evolves into superconductivity at $T_c$ = 0.80(1) K. These properties resemble that of a many-body heavy-fermion state, which derives from the hybridization between localized magnetic states and conduction electrons. Yet, no evidence for localized magnetism or magnetic order is found in KNi$_2$Se$_2$ from magnetization measurements or neutron diffraction. Instead, neutron pair-distribution-function analysis reveals the presence of local charge-density-wave distortions that disappear on cooling, an effect opposite to what is typically observed, suggesting that the low-temperature electronic state of KNi$_2$Se$_2$ arises from cooperative Coulomb interactions and proximity to, but avoidance of, charge order.

cond-mat.supr-con↗

arXiv2012

Bulk Intergrowth of a Topological Insulator with a Room Temperature Ferromagnet

We demonstrate that the layered room temperature ferromagnet Fe7Se8 and the topological insulator Bi2Se3 form crystallographically oriented bulk composite intergrowth crystals. The morphology of the intergrowth in real space and reciprocal space is described. Critically, the basal planes of Bi2Se3 and Fe7Se8 are parallel and hence the good cleavage inherent in the bulk phases is retained. The intergrowth is on the micron scale. Both phases in the intergrowth crystals display their intrinsic bulk properties: the ferromagnetism of the Fe7Se8 is anisotropic, with magnetization easy axis in the plane of the crystals, and ARPES characterization shows that the topological surface states remain present on the Bi2Se3. Analogous behavior is found for what has been called "Fe-doped Bi2Se3."

cond-mat.mtrl-sci↗

arXiv2011

Bounded combinatorics and the Lipschitz metric on Teichmüller space

Considering the Teichmüller space of a surface equipped with Thurston's Lipschitz metric, we study geodesic segments whose endpoints have bounded combinatorics. We show that these geodesics are cobounded, and that the closest-point projection to these geodesics is strongly contracting. Consequently, these geodesics are stable. Our main tool is to show that one can get a good estimate for the Lipschitz distance by considering the length ratio of finitely many curves.

math.GT↗