arXiv subjects

Joachim von Zanthier

Publications and source records attributed to Joachim von Zanthier.

At least 37 records · Page 2Linked to original sources

arXiv2021

Testing higher-order quantum interference with many-particle states

Quantum theory permits interference between indistinguishable paths but, at the same time, restricts its order. Single-particle interference, for instance, is limited to the second order, that is, to pairs of single-particle paths. To date, all experimental efforts to search for higher-order interferences beyond those compatible with quantum mechanics have been based on such single-particle schemes. However, quantum physics is not bounded to single-particle interference. We here experimentally study many-particle higher-order interference using a two-photon-five-slit setup. We observe nonzero two-particle interference up to fourth order, corresponding to the interference of two distinct two-particle paths. We further show that fifth-order interference is restricted to $10^{-3}$ in the intensity-correlation regime and to $10^{-2}$ in the photon-correlation regime, thus providing novel bounds on higher-order quantum interference.

quant-ph↗

arXiv2020

Imaging trapped ion structures via fluorescence cross-correlation detection

Cross-correlation signals are recorded from fluorescence photons scattered in free space off a trapped ion structure. The analysis of the signal allows for unambiguously revealing the spatial frequency, thus the distance, as well as the spatial alignment of the ions. For the case of two ions we obtain from the cross-correlations a spatial frequency $f_\text{spatial}=1490 \pm 2_{stat.}\pm 8_{syst.}\,\text{rad}^{-1}$, where the statistical uncertainty improves with the integrated number of correlation events as $N^{-0.51\pm0.06}$. We independently determine the spatial frequency to be $1494\pm 11\,\text{rad}^{-1}$, proving excellent agreement. Expanding our method to the case of three ions, we demonstrate its functionality for two-dimensional arrays of emitters of indistinguishable photons, serving as a model system to yield structural information where direct imaging techniques fail.

quant-ph↗

arXiv2019

Light from an ion crystal: bunching or antibunching?

Photon statistics divides light sources into three different categories, characterized by bunched, antibunched or uncorrelated photon arrival times. Single atoms, ions, molecules, or solid state emitters display antibunching of photons, while classical thermal sources exhibit photon bunching. Here we demonstrate a light source in free space, where the photon statistics depends on the direction of observation, undergoing a continuous crossover between photon bunching and antibunching. We employ two trapped ions, observe their fluorescence under continuous laser light excitation, and record the spatially resolved autocorrelation function $g^{(2)}(τ)$ with a movable Hanbury Brown and Twiss detector. Varying the detector position we find a minimum value for antibunching, $g^{(2)}(0) = 0.60(5)$ and a maximum of $g^{(2)}(0)=1.46(8)$ for bunching, demonstrating that this source radiates fundamentally different types of light alike. The observed variation of the autocorrelation function is understood in the Dicke model of heralded entangled states and the observed maximum and minimum values are modeled, taking independently measured experimental parameters into account.

quant-ph↗

arXiv2018

Ghost Imaging at an XUV Free-Electron Laser

Radiation damage is one of the most severe resolution limiting factors in x-ray imaging, especially relevant to biological samples. One way of circumventing this problem is to exploit correlation-based methods developed in quantum imaging. Among these, there is ghost imaging (GI) in which the image is formed by radiation that has never interacted with the sample. Here, we demonstrate GI at an XUV free-electron laser by utilizing correlation techniques. We discuss the experimental challenges, optimal setup, and crucial ingredients to maximize the achievable resolution.

physics.optics↗

arXiv2018

Many-particle interference to test Born's rule

Born's rule, one of the cornerstones of quantum mechanics, relates detection probabilities to the modulus square of the wave function. Single-particle interference is accordingly limited to pairs of quantum paths and higher-order interferences are prohibited. Deviations from Born's law have been quantified via the Sorkin parameter which is proportional to the third-order term. We here extend this formalism to many-particle interferences and find that they exhibit a much richer structure. We demonstrate, in particular, that all interference terms of order $(2M+1)$ and greater vanish for $M$ particles. We further introduce a family of many-particle Sorkin parameters and show that they are exponentially more sensitive to deviations from Born's rule than their single-particle counterpart.

quant-ph↗

arXiv2018

Analysis of superresolution via 3D structured illumination intensity correlation microscopy

Intensity correlation microscopy (ICM), which is prominently known through antibunching microscopy or super-resolution optical fluctuation imaging (SOFI), provides superresolution through a correlation analysis of antibunching of independent quantum emitters or temporal fluctuations of blinking fluorophores. For correlation order $m$ the PSF in the signal is effectively taken to the $m$th power, and is thus directly shrunk by the factor $\sqrt{m}$. Combined with deconvolution a close to linear resolution improvement of factor $m$ can be obtained. Yet, analysis of high correlation orders is challenging, what limits the achievable resolutions. Here we propose to use three dimensional structured illumination along with $m$th-order correlation analysis to obtain an enhanced scaling of up to $m+m=2m$. Including the stokes shift or plasmonic sub-wavelength illumination enhancements beyond $2m$ can be achieved. Hence, resolutions far below the diffraction limit in full 3D imaging can potentially be achieved already with low correlation orders. Since ICM operates in the linear regime our approach may be particularly promising for enhancing the resolution in biological imaging at low illumination levels.

physics.optics↗

arXiv2018

Generation of N00N-like interferences with two thermal light sources

Measuring the $M$th-order intensity correlation function of light emitted by two statistically independent thermal light sources may display N00N-like interferences of arbitrary order $N = M/2$. We show that via a particular choice of detector positions one can isolate $M$-photon quantum paths where either all $M$ photons are emitted from the same source or $M/2$ photons are collectively emitted by both sources. The latter superposition displays N00N-like oscillations with $N = M/2$ which may serve, e.g., in astronomy, for imaging two distant thermal sources with $M/2$-fold increased resolution. We also discuss slightly modified detection schemes improving the visibility of the N00N-like interference pattern and present measurements verifying the theoretical predictions.

quant-ph↗

arXiv2018

Prime Number Decomposition using the Talbot Effect

We report on prime number decomposition by use of the Talbot effect, a well-known phenomenon in classical near field optics whose description is closely related to Gauss sums. The latter are a mathematical tool from number theory used to analyze the properties of prime numbers as well as to decompose composite numbers into their prime factors. We employ the well-established connection between the Talbot effect and Gauss sums to implement prime number decompositions with a novel approach, making use of the longitudinal intensity profile of the Talbot carpet. The new algorithm is experimentally verified and the limits of the approach are discussed.

physics.optics↗

arXiv2017

Directional Dicke Subradiance with Nonclassical and Classical Light Sources

We investigate Dicke subradiance of distant quantum sources in free space, i.e., the spatial emission pattern of spontaneously radiating non-interacting multi-level atoms or multi-photon sources, prepared in totally antisymmetric states. We find that the radiated intensity is marked by a strong suppression of spontaneous emission in particular directions. In resemblance to the analogous, yet inverted, superradiant emission profiles of $N$ distant two-level atoms prepared in symmetric Dicke states, we call the corresponding emission pattern $\textit{directional Dicke subradiance}$. We also show that higher order intensity correlations of the light incoherently emitted by statistically independent thermal light sources display the same directional Dicke subradiant behavior. We present measurements of directional Dicke subradiance for $N = 2, \ldots, 5$ distant thermal light sources corroborating the theoretical findings.

quant-ph↗

arXiv2017

Quantum Imaging with Incoherently Scattered Light from a Free-Electron Laser

The advent of accelerator-driven free-electron lasers (FEL) has opened new avenues for high-resolution structure determination via diffraction methods that go far beyond conventional x-ray crystallography methods. These techniques rely on coherent scattering processes that require the maintenance of first-order coherence of the radiation field throughout the imaging procedure. Here we show that higher-order degrees of coherence, displayed in the intensity correlations of incoherently scattered x-rays from an FEL, can be used to image two-dimensional objects with a spatial resolution close to or even below the Abbe limit. This constitutes a new approach towards structure determination based on incoherent processes, including Compton scattering, fluorescence emission or wavefront distortions, generally considered detrimental for imaging applications. Our method is an extension of the landmark intensity correlation measurements of Hanbury Brown and Twiss to higher than second-order paving the way towards determination of structure and dynamics of matter in regimes where coherent imaging methods have intrinsic limitations.

physics.ins-det↗

arXiv2017

Incoherent Diffractive Imaging via Intensity Correlations of hard X-rays

Established x-ray diffraction methods allow for high-resolution structure determination of crystals, crystallized protein structures or even single molecules. While these techniques rely on coherent scattering, incoherent processes like Compton scattering or fluorescence emission -- often the predominant scattering mechanisms -- are generally considered detrimental for imaging applications. Here we show that intensity correlations of incoherently scattered x-ray radiation can be used to image the full 3D structure of the scattering atoms with significantly higher resolution compared to conventional coherent diffraction imaging and crystallography, including additional three-dimensional information in Fourier space for a single sample orientation. We present a number of properties of incoherent diffractive imaging that are conceptually superior to those of coherent methods.

physics.optics↗

arXiv2017

Superresolution via Structured Illumination Quantum Correlation Microscopy (SIQCM)

We propose to use intensity correlation microscopy in combination with structured illumination to image quantum emitters that exhibit antibunching with a spatial resolution reaching far beyond the Rayleigh limit. Combining intensity measurements and intensity auto correlations up to order $m$ creates an effective PSF with FWHM shrunk by the factor $\sqrt{m}$. Structured Illumination microscopy on the other hand introduces a resolution improvement of factor 2 by use of the principle of moiré fringes. Here, we show that for linear low-intensity excitation and linear optical detection the simultaneous use of both techniques leads to an in theory unlimited resolution power with the improvement scaling favorably as $m + \sqrt{m}$ in dependence of the correlation order $m$. Hence, yielding this technique to be of interest in microscopy for imaging a variety of samples including biological ones. We present the underlying theory and simulations demonstrating the highly increased spatial superresolution, and point out requirements for an experimental implementation.

physics.optics↗

arXiv2016

An optical multimode fiber as pseudothermal light source

We report on a novel pseudothermal light source based on laser light coupled into an optical multimode fiber. The setup is simple, of low cost, exhibits inherently high directional light emission and allows for a flexible arrangement. By measuring the photon statistics and spatial two point intensity correlations in the far field we show that the setup exhibits all characteristics of a gaussian random source.

quant-ph↗

arXiv2016

Superresolving Imaging of Irregular Arrays of Thermal Light Sources using Multiphoton Interferences

We propose to use multiphoton interferences of photons emitted from statistically independent thermal light sources in combination with linear optical detection techniques to reconstruct, i.e., image, arbitrary source geometries in one dimension with subclassical resolution. The scheme is an extension of earlier work [Phys. Rev. Lett. 109, 233603 (2012)] where N regularly spaced sources in one dimension were imaged by use of the Nth-order intensity correlation function. Here, we generalize the scheme to reconstruct any number of independent thermal light sources at arbitrary separations in one dimension exploiting intensity correlation functions of order $m \geq 3$. We present experimental results confirming the imaging protocol and provide a rigorous mathematical proof for the obtained subclassical resolution.

quant-ph↗

arXiv2016

Visibility of Young's interference fringes: Scattered light from small ion crystals

We observe interference in the light scattered from trapped $^{40}$Ca$^+$ ion crystals. By varying the intensity of the excitation laser, we study the influence of elastic and inelastic scattering on the visibility of the fringe pattern and discriminate its effect from that of the ion temperature and wave-packet localization. In this way we determine the complex degree of coherence and the mutual coherence of light fields produced by individual atoms. We obtain interference fringes from crystals consisting of two, three and four ions in a harmonic trap. Control of the trapping potential allows for the adjustment of the interatomic distances and thus the formation of linear arrays of atoms serving as a regular grating of microscopic scatterers.

quant-ph↗

arXiv2015

Superbunching and Nonclassicality as new Hallmarks of Superradiance

Superradiance, i.e., spontaneous emission of coherent radiation by an ensemble of identical two-level atoms in collective states introduced by Dicke in 1954, is one of the enigmatic problems of quantum optics. The startling gist is that even though the atoms have no dipole moment they radiate with increased intensity in particular directions. Following the advances in our understanding of superradiant emission by atoms in entangled $W$ states we examine the quantum statistical properties of superradiance. Such investigations require the system to have at least two excitations as one needs to explore the photon-photon correlations of the radiation emitted by such states. We present specifically results for the spatially resolved photon-photon correlations of systems prepared in doubly excited $W$ states and give conditions when the atomic system emits nonclassial light. Equally, we derive the conditions for the occurrence of bunching and even of superbunching, a rare phenomenon otherwise known only from nonclassical states of light like the squeezed vacuum. We finally investigate the photon-photon cross correlations of the spontaneously scattered light and highlight the nonclassicalty of such correlations.

quant-ph↗

arXiv2015

Entanglement of Polarization and Orbital Angular Momentum

We investigate two-photon entangled states using two important degrees of freedom of the electromagnetic field, namely orbital angular momentum (OAM) and spin angular momentum. For photons propagating in the same direction we apply the idea of $\textit{entanglement duality}$ and develop schemes to do $\textit{entanglement sorting}$ based either on OAM or polarization. In each case the entanglement is tested using appropriate witnesses. We finally present generalizations of these ideas to three- and four-photon entangled states.

quant-ph↗

arXiv2015

Nonlocal photon correlations and violation of Bell inequalities for spatially separated classical light fields

It is theoretically and experimentally shown that photons emitted by statistically independent incoherent classical light sources and measured in the far field in spatially separated modes may display spatial correlations akin to path-entanglement of photons produced by quantum sources. By measuring higher order photon-correlations at different locations, i.e., $m$ photons in one mode and one photon in another mode, we experimentally demonstrate for $m \geq 6$ a violation of Bell-type inequalities for spatial degrees of freedom. The spatial correlations among the photons can be understood from state projection where the detection of the first $m$ photons projects the sources onto a state which emits the subsequent photon in a strongly correlated manner. From this perspective the entanglement and violation of Bell's inequalities appears as a consequence of nonvanishing cross correlations between noncommuting quadrature phase components of the two spatially separated fields after $m$ photons have been recorded. In this way we show that classical systems may produce spatial field correlations violating local realistic theories.

quant-ph↗