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Johannes Knolle

Publications and source records attributed to Johannes Knolle.

At least 19 recordsLinked to original sources

Vestigial altermagnetism

Interaction effects and fluctuations govern the phase diagram of systems with multiple competing phases. In particular, as individual phases are destroyed by increasing temperature, fluctuations can still produce a composite `vestigial' order given by a product of individual order parameters. Here, we describe vestigial Altermagnetism (AM) from the thermal melting of antiferromagnetic (AFM) and orbital orders (OO) on the square lattice. The coexistence of AFM and OO can give rise to conventional AM with ordering wave vector $\mathbf{Q}=(π,π)$. We show that a distinct `vestigial AM' phase with $\mathbf{Q}=0$ can arise from thermal melting of AFM and OO, and investigate its generic phase diagram. We find that the transition from the high-temperature disordered phase into the vestigial AM phase can be either first or second order, depending on the AFM and OO bare susceptibilities and their interactions. We then investigate the unique experimental signatures by calculating the electron spectral function for a minimal two-orbital model. Despite the fact that the vestigial AM order parameter does not couple to electrons directly, fluctuations dominate the self-energy corrections giving rise to a spin- and orbital-dependent quasi-particle lifetime with the AM symmetry.

cond-mat.str-el

Rhombohedral Multilayer Graphene as a $p$-Wave Magnet

We propose rhombohedral multilayer graphene in an applied in-plane magnetic field as a highly tunable platform for nonrelativistic collinear $p$-wave magnetism. The orbital coupling to the magnetic field breaks time-reversal symmetry and, together with interaction-driven layer antiferromagnetism, generates an odd-in-momentum spin splitting without relying on spin-orbit coupling. Using a minimal low-energy effective theory, we show that the resulting $p$-wave spin splitting is strongly enhanced with increasing layer number. This enhancement originates from the surface-localized nature of the low-energy states and their layer-dependent orbital coupling to the in-plane field. The Zeeman coupling only weakly perturbs this predominantly orbital-field-induced mechanism. We further estimate stability of the $p$-wave magnetism under hole-doping and distinct transport signature using a more realistic Hubbard model. Our results establish orbital coupling to an external magnetic field as a controllable route to odd-parity spin splitting in collinear magnets.

cond-mat.str-el

A continuous confinement-deconfinement transition in a triangular quantum magnet

A continuous transition between phases hosting distinct excitations---bosonic magnons versus fermionic spinons---is a long-sought phenomenon in quantum magnetism, analogous to the confinement--deconfinement transition in quantum chromodynamics. We report evidence for such a transition in the triangular-lattice antiferromagnet TlYbS$_2$. Antiferromagnetic order develops below $T_\mathrm{N} \approx 0.53\,\mathrm{K}$. A $c$-axis field suppresses this order, driving the system into a gapless quantum spin liquid with a spinon Fermi surface above $μ_0 H_\mathrm{c} \approx 3\,\mathrm{T}$, evidenced by a finite residual linear term in thermal conductivity, a Pauli-like susceptibility, and a temperature-independent NMR Knight shift. Approaching $H_\mathrm{c}$ from above, the scattering rate of itinerant excitations is strongly enhanced while their density of states shows no critical enhancement, atypical of conventional magnetic quantum criticality. These results point to a continuous confinement--deconfinement transition governed by fractionalized excitations beyond the Ginzburg--Landau paradigm.

cond-mat.str-el

Electric-current control of anomalous Hall effect

We demonstrate robust and reversible electric-current control of the anomalous Hall effect (AHE) in a two-dimensional WTe2/Fe3GeTe2 (FGT) stack. Applying a current through Td-WTe2 leads to a giant modulation of the AHE of the adjacent FGT layer, with the relative change of the AHE conductivity exceeding 180%. Control experiments show that i) the observed effect is absent in pure FGT, ii) the modulation weakens in thicker FGT films, confirming its interfacial origin, and iii) the modulation peaks for bilayer WTe2, indicating that the Berry-curvature dipole (BCD) plays the dominant role in the modulation. We propose that the charge current I generates an out-of-plane magnetization Mz via BCD in WTe2 and Mz modifies the exchange splitting of FGT via the inverse magnetic proximity effect, thereby altering its Berry curvature and nontrivially influencing the AHE. The demonstrated method of AHE control offers new possibilities for magnetism control, i.e., for the study of AHE-transistors as well as electric-current control of quantum magnets, especially magnetic insulators.

cond-mat.mes-hall

Microscopic Emergence of Ancilla Lattice Physics in the Emery Model

We derive a controlled low-energy effective theory for the three-band Emery model on the Lieb lattice near (n=2) filling. Starting from the positive charge-transfer regime, a sequence of Schrieffer--Wolff transformations rigorously establishes a direct microscopic mapping onto an ancillary lattice structure. For realistic cuprate-like parameters, this framework naturally reproduces the conventional Fermi-liquid (FL) phase at a filling shifted by one electron per site. Our analysis identifies the precise microscopic conditions required to access the exotic fractionalized Fermi-liquid (FL$^*$) phase. We show that realizing FL$^*$ requires nonstandard cuprate parameter regimes together with additional interactions that stabilize a quantum spin liquid in the background ancilla layer. These results establish a microscopic foundation for ancilla physics in multiorbital materials and clarify the conditions for realizing FL$^*$. We discuss the possibility to replicate ancilla model physics in Lieb lattice cold atom simulations.

cond-mat.str-el

Altermagnetism from a Cu-Fe Lieb Lattice in FeSe/Cuprate Heterostructures

Realizing altermagnetism in high-$T_c$ cuprate-based systems would provide a direct route for studying spin-split electronic bands in the absence of net magnetization and investigate their interplay with unconventional superconductivity. Here, we propose that FeSe/cuprate heterostructures offer such a platform, where a 45$^\circ$ twist of Cu and Fe layers creates an effective CuFe$_2$ Lieb lattice in which Fe magnetic order and Cu-Fe hybridization through the ligands induces altermagnetic $d$-wave spin splitting. A minimal tight-binding model shows that this mechanism is generic. Furthermore, a substrate-induced inequivalence of the two Se sites in FeSe provides a second route in which altermagnetism originates in the Fe layer and is transferred to the cuprate layer by proximity. Density functional theory calculations for FeSe/Bi$_2$Sr$_2$CuO$_6$ heterostructures confirm the viability of both mechanisms and reveal ways to enhance the spin splitting. These results establish superconducting cuprate/transition metal chalcogenide heterostructures as a promising setting for engineering altermagnetism and studying its coupling to unconventional superconductivity.

cond-mat.str-el

Signatures of Topological Magnon Edge States in THz Spectroscopy and Cavity Response

Topological magnon insulators (TMIs) have emerged as promising platforms for low-energy spin-based information processing, due to their non-trivial bulk magnon topology and robust, chiral edge modes that support dissipationless transport. Although theoretical models predict these edge states, direct experimental detection remains challenging due to their limited sensitivity to conventional probes. In this work, we propose an all-optical pathway to detect topological magnon edge modes in ferromagnetic TMIs. Our approach harnesses parametric amplification of edge magnons via resonant electromagnetic driving, enabled by magnetoelectric coupling mechanisms. We concentrate on two-dimensional van der Waals ferromagnetic materials on the honeycomb lattice with magnonic band gaps in the terahertz (THz) range. We show that a spin-dependent effective electric dipole moment, arising from dynamic charge fluctuations and consistent with the lattice symmetry up to next-nearest-neighbor interactions, gives rise to one-photon-two-magnon processes leading to parametric amplification. On this basis, we propose a THz pump-probe spectroscopy protocol in which edge modes are selectively amplified and subsequently detected in absorption. Furthermore, we discuss the possibility of using THz cavities, enabling selective coupling to edge modes while filtering out bulk contributions. These findings establish a route for probing topological magnets and open new avenues for experimental exploration of exotic topological phenomena in magnetic quantum materials.

cond-mat.mes-hall

GHz non-reciprocal optical conductivity in hematite ($α$-$\text{Fe}_2\text{O}_3$)

We study the non-reciprocal properties of the iron oxide $α$-Fe$_2$O$_3$ (hematite) in the canted easy-plane antiferromagnetic phase, specifically in the GHz to THz frequency range. First, using the the microscopic spin Hamiltonian, we obtain the correct classical ground state where the canting is induced by the Dzyaloshinskii-Moriya interactions (DMI). The magnon spectrum is simulated using linear spin wave theory. We then compute the polarizability and the sub-gap optical conductivities using linear response. We find that the conductivity tensor contains frequency peaks at the zero momentum magnon gaps of order $0.1~$meV which can be tuned by the DMI and on-site anisotropic spin interactions. Furthermore, we show that the canting-induced net magnetic moment $\mathbf{m}$ represents a measure for the effective time-reversal-symmetry breaking and non-reciprocity of the system: a finite $\mathbf{m}$ results in a non-zero Hall conductivity. Finally, we discuss the prospective application of hematite in non-reciprocal circulator design, by computing the non-reciprocal circulator transmission amplitude using the conductivities as input.

cond-mat.str-el

Emergence of a monopole phase in the $J_1{-}J_2$ Heisenberg model on the triangular lattice for small magnetic fields

We investigate the ground-state phase diagram of the $J_1{-}J_2$ Heisenberg model on the triangular lattice under an external Zeeman field $H$ by using the variational Monte Carlo approach. We span a region with $0 \le J_2/J_1 \le 0.2$ and $0 \le H/J_1 \le 2$, to assess the fate of the (putative) spin-liquid phase that has been detected for $J_2/J_1=1/8$ at zero magnetic field. Simple variational ansatze are proposed for a few candidate states, and their energetics are compared on large clusters to obtain the phase diagram. For $J_2/J_1 \lesssim 1/6$, a continuous transition from a gapless "Y'' phase to a gapped "up-up-down'' phase is obtained, as predicted by spin-wave theory. Most importantly, around $J_2/J_1=1/8$, a condensate of monopoles (which are gapless gauge excitations of the spin liquid at $H=0$) is stabilized in a significant region of the phase diagram, for small Zeeman fields. Here, a finite scalar chirality is present, while no transverse magnetic order is detected. The stability of the monopole phase is confirmed by a field-theory approach that includes a self-consistent random-phase approximation of the low-lying spin fluctuations. The boundary between the monopole and "Y'' phases is also obtained with no free parameters.

cond-mat.str-el

From stable periodic orbits to many-body chaos: doubly tunable prethermalization via engineering of an emergent band structure

We uncover a family of many-body periodic orbits in a periodically driven (Floquet) spin system away from the high-frequency limit. While linear stability analysis predicts that perturbed many-body trajectories remain close to stable periodic orbits, thermodynamic principles dictate that Floquet heating will ultimately set in. Our work aims to resolve the tension between these two expectations. In particular, we show that perturbations away from the stable periodic orbits feature a description akin to a quasiparticle band structure. A long-lived prethermal regime appears when modes around the gapless point are slowly populated. The dispersion determines the prethermal lifetime, and we show how band engineering leads to a "doubly tunable" parametric dependence of the prethermal lifetime $R^{-W}$, with $R$ the width in momentum space of the quasiparticle distribution and $W$ the exponent of the dispersion around the gapless point. Our results not only establish a powerful route toward stabilizing non-equilibrium phases of matter in driven many-body systems but also establish a conceptual bridge between periodic orbits in 'low-dimensional' nonlinear systems and many-body chaos.

cond-mat.stat-mech

Topological Triplons in the Pinwheel Valence Bond Solid on the Kagome Lattice

We investigate the triplon excitations of the pinwheel valence-bond-solid phase on the deformed kagome lattice compound Rb2Cu3SnF12. Using bond-operator mean-field theory, we compute the triplon band structure, dynamical structure factor, Berry curvatures and the associated thermal Hall response. We show that the presence of Dzyaloshinskii-Moriya interactions and an external magnetic field are key for endowing triplon bands with nontrivial Chern numbers. We find good qualitative agreement of the low-energy dynamical structure factor with neutron-scattering experiments. An applied magnetic field can isolate the lowest triplon Chern band leading to a tunable thermal Hall conductivity for accessible temperature and field regimes. Our results establish the deformed kagome pinwheel valence-bond solid as a promising platform for topological triplon physics and for observing the associated thermal Hall effect.

cond-mat.str-el

Magnetic Bloch Oscillations in Odd-Wave Magnets and the Nonlinear Edelstein Effect

Bloch oscillations (BOs) are a quantum phenomenon in which electrons subjected to an electric field in a periodic potential exhibit an oscillating current without a net drift. In real conductors, scattering reduces the coherence required for BOs driving the system toward a steady state with a DC current. While previous studies have focused on charge transport, charge carriers also possess spin, raising the question of whether BOs can emerge in magnetic observables. Here, we show that the magnetization of odd-wave magnets can undergo BOs before relaxing to the steady-state Edelstein value, a phenomenon we term $\textit{magnetic}$ BOs. Using analytical and numerical methods, we demonstrate this effect in a minimal one-dimensional model of a p-wave magnet and generalize it to two dimensions. Our analysis further reveals that the Edelstein magnetization is generically nonlinear in the applied electric field. Finally, we argue that magnetic BOs can be detected in materials through higher-harmonic generation in THz sub-cycle lightwave spectroscopy. Magnetic BOs provide a genuine non-equilibrium signature of spin-charge coupling in unconventional magnets.

cond-mat.str-el

Dynamical magnetic breakdown and quantum oscillations from hot spot scattering

Quantum oscillations (QO) are a well-established probe of Fermi-surface (FS) geometry and in the presence of long-range density wave order can display new QO frequencies from reconstructed FS pockets. We show that such reconstructed frequencies can arise even in the absence of long-range density order. Considering electrons coupled to a fluctuating bosonic mode that scatters quasiparticles between sharp hot spots on the FS, we develop a semiclassical theory in which the interaction generates time-dependent tunneling processes analogous to magnetic breakdown. This dynamical magnetic breakdown produces new semiclassical orbits corresponding to reconstructed FS areas despite the absence of static order. Because tunneling probabilities depend on the thermal population of bosonic excitations, the resulting oscillation amplitudes exhibit characteristic deviations from standard Lifshitz-Kosevich behavior. Our results provide a mechanism to probe bosonic fluctuations in quantum critical metals and provide a framework for dynamical magnetic breakdown.

cond-mat.str-el

Composite Quantum Geometry and Semiclassical Dynamics

We derive semiclassical equations of motion for general composite bound states in insulators and semiconductors, covering excitations such as excitons and trions. For neutral composites we find that a uniform external electric field does not couple to a Berry curvature term, contrary to the naive expectation from single-electron dynamics. Instead, a distinct quantum geometric quantity appears generically in the equations of motion. This quantity is the difference between inequivalent Berry connections that can be defined for the composite, generalising the concept of the quantum geometric dipole previously studied for excitons. In the case of charged composites such as trions, we find an additional Berry curvature contribution to the equations of motion. As we demonstrate, however, there is an infinite family of inequivalent composite Berry curvatures, and so care must be taken to make the correct choice that describes the physical dynamics. We explain how this choice should be made dependent on the definition of a spatial centre for the composite. We end by discussing composite dynamics that have no single-electron counterpart. We find that trions in magic-angle twisted bilayer graphene undergo a transverse drift under an applied electric field and that this is driven not only by the Berry curvature contribution but also by the quantum geometric dipole. The interplay of these two geometric contributions further imprints itself on the trion's internal dynamics, causing its dipole moment to oscillate in time.

cond-mat.mes-hall

Odd-parity magnons in the Haldane-Hubbard model from topological exciton condensation

Odd-wave magnets are the counterparts to even-wave altermagnets realizing odd-parity spin splitting. Normally discussed for noncollinear systems, they have recently been shown to appear in collinear magnetic states in the presence of loop currents. Here we study collective excitations of the paramagnetic and magnetic phase of the seminal Haldane-Hubbard model. We identify the existence topological excitons in the paramagnetic phase, and their condensation as the driving mechanism into the collinear Néel state. The latter realizes an odd-wave magnet with odd-parity magnons displaying a characteristic $f$-wave splitting. We further uncover that an electron bandgap closing ensures magnon bandgap closing causing a change in odd-parity magnon topology, as well as a drastically enlarged spin splitting. Our results establish the presence of topological excitons and odd-parity magnons in the Haldane-Hubbard, with potential realizations in Floquet-driven materials and cold atomic gases.

cond-mat.str-el

Tensor network study of deconfined quantum criticality in a one-dimensional spin-phonon model

Deconfined quantum critical points (DQCPs) describe continuous transitions between ordered phases beyond the Landau paradigm. A simple example is the Néel antiferromagnet (AFM) to valence bond solid (VBS) transition in a 1D antiferromagnetic $J_1-J_2$ model. In analogy to the spin-Peierls instability of critical spin chains, DQCPs are predicted to be unstable towards lattice distortions below a critical phonon frequency. In this work, we use tensor network simulations to investigate this instability in the antiferromagnetic $J_1-J_2$ model coupled to lattice vibrations. We confirm the stability of DQCP for large phonon frequencies and demonstrate that the transition turns strongly first-order below a critical frequency. The instability is caused by a reduction of the Luttinger parameter due to spin-phonon interactions and we identify the effective theory of the behavior as the double sine-Gordon model. The same effective theory is known to describe the classical Ashkin-Teller model, which enables us to show that the critical endpoint is in the four-state Potts universality class. Furthermore, we provide quantitative numerical scaling results for the phonon spectral function, offering an experimental signature to probe DQCP-phonon coupling in low-dimensional materials.

cond-mat.str-el

Raman Circular Dichroism and Quantum Geometry of Chiral Quantum Spin Liquids

We show that the quantum geometry of fractionalized spin excitations in Mott-insulating quantum spin liquids (QSL) gives rise to a finite Raman circular dichroism (RCD) signal. We demonstrate the equivalence between the Loudon-Fleury framework and the light-matter coupling approach for effective spinon bands. Using the latter, we derive an analytical decomposition of the RCD into different contributions of the quantum geometry. This reveals the sensitivity of the RCD to the underlying structure of the wave functions and the handedness of the excitations, rather than a nonzero Chern number of spinon excitations. To illustrate this, we apply our approach to two examples, the Kitaev honeycomb model in a magnetic field and a chiral $U(1)$ QSL on the triangular lattice, and discuss its experimental relevance for candidate materials.

cond-mat.str-el

Fate of Topological Dirac Magnons in van der Waals Ferromagnets at Finite Temperature

Dirac magnons, the bosonic counterparts of Dirac fermions in graphene, provide a unique platform to explore symmetry-protected band crossings and quantum geometry in magnetic insulators, while promising high-velocity, low-dissipation spin transport for next-generation magnonic technologies. However, their stability under realistic, finite-temperature conditions remains an open question. Here, we develop a comprehensive microscopic theory of thermal magnon-magnon interactions in van der Waals honeycomb ferromagnets, focusing on both gapless and gapped Dirac magnons. Using nonlinear spin-wave theory with magnon self-energy corrections and a T-matrix resummation that captures two-magnon bound states, we quantitatively reproduce temperature- and momentum-dependent energy shifts and linewidths observed experimentally in the gapless Dirac magnon material CrBr$_3$, even near the Curie temperature. Our approach resolves discrepancies between prior theoretical predictions and experiment and highlight the significant role of bound states in enhancing magnon damping at low temperatures. For gapped Dirac magnon materials such as CrI$_3$, CrSiTe$_3$, and CrGeTe$_3$, we find a thermally induced reduction of the topological magnon gap but no evidence of thermally driven topological transitions. Classical atomistic spin dynamics simulations corroborate the gap' s robustness up to the Curie temperature. Furthermore, we establish a practical criterion for observing topological gaps by determining the minimum ratio of Dzyaloshinskii-Moriya interaction to Heisenberg exchange required to overcome thermal broadening throughout the ordered phase, typically around 5%. Our results clarify the interplay of thermal many-body effects and topology in low-dimensional magnets and provide a reliable framework for interpreting spectroscopic experiments.

cond-mat.str-el