arXiv subjects

Julius Hohlfeld

Publications and source records attributed to Julius Hohlfeld.

13 recordsLinked to original sources

arXiv2026

Type-II-like ultrafast demagnetization behavior in NiCo2O4 thin films

Rare-earth-ferrimagnetic oxides are emerging as attractive platforms for investigating ultrafast spin dynamics. Here, we study the photoinduced magnetization dynamics of epitaxial NiCo2O4 (NCO) thin films by time-resolved magneto-optical Faraday effect using two independent pump-probe configurations: 1030/515 nm and 800/400 nm. In both measurements, photoexcitation induces an immediate reduction of the magneto-optical signal within the experimental time resolution, followed by a reproducible slower demagnetization component with a characteristic timescale of approximately 5-6 ps and a subsequent recovery on the ~100 ps timescale. Importantly, this picosecond demagnetization component is observed consistently across the two experimental configurations and excitation wavelengths, demonstrating that it is an intrinsic feature of the ultrafast magnetic response of NCO thin films. Because the earliest-time dip may contain a transient optical contribution, we describe the overall response as type-II-like, rather than assigning a definitive textbook type-II classification solely on the basis of the sub-resolution signal. These results establish a robust two-step ultrafast demagnetization behavior in NCO and highlight rare-earth-free oxide ferrimagnets as promising systems for exploring Mult sublattice spin dynamics on ultrafast timescales.

cond-mat.mtrl-sci↗

arXiv2025

Single-shot laser-pulse-induced magnetization reversal in CoFeB/MgO-based magnetic tunnel junctions

We demonstrate single-shot laser-pulse-induced magnetization reversal in rare-earth-free CoFeB/MgO magnetic tunnel junctions (MTJs), a material system widely adopted in spin-transfer torque magnetic random-access memory (STT-MRAM). By tuning the Ru capping layer thickness, we modify the laser energy absorption profile and observe magnetization reversal from the parallel (P) to antiparallel (AP) state, with switching observed for $t_\text{Ru} \geq 2.0\,$ nm. Furthermore, we detect magnetization reversal in a micro-scale MTJ device via the tunnel magnetoresistance (TMR) effect. Our findings suggest that ultrafast spin transport, dipolar interactions, or a combination of both may contribute to the switching process, although the precise mechanism remains to be clarified. This work represents a significant step toward integrating ultrafast optical control with MTJ technology.

cond-mat.mes-hall↗

arXiv2025

Exploring Co, Fe, and Ni Reference Layers for Single-Pulse All-Optical Reversal in Ferromagnetic Spin Valves

We investigate the magnetization reversal process induced by a single femtosecond laser pulse in ferromagnetic spin valves by systematically comparing reference layers composed of pure Co, Ni, and Fe. To circumvent the loss of perpendicular magnetic anisotropy associated with changes in reference layer material and thickness, we design spin valves with in plane magnetizations. While antiparallel to parallel switching is observed for all three elements, parallel to antiparallel switching occurs only with a Co reference layer and is absent with Ni and Fe. This difference is attributed to the distinct ultrafast magnetization dynamics of the reference materials. Our results support the hypothesis that parallel to antiparallel switching requires a rapid remagnetization of the reference layer, which generates a substantial negative spin current polarized opposite to the free layer magnetization an essential condition for triggering its reversal.

cond-mat.mes-hall↗

arXiv2025

Single-Shot Magnetization Reversal in Ferromagnetic Spin Valves Enabled via Heat Control

We study laser induced ultrafast magnetization reversal in a ferromagnetic spin valve by comparing the effects of direct laser excitation and ultrashort hot electron pulses. A wedged Cu layer is deposited atop the spin valve to tune energy transmission to the magnetic stack for both optical and hot-electron excitation. We demonstrate single shot magnetization reversal of the free layer using hot electron pulses. Moreover, such reversal is achieved even with picosecond laser pulses. The influence of laser fluence, Cu thickness ($t_{\mathrm{Cu}}$), and pulse duration is investigated in detail. Our results indicate that the key factor enabling magnetization reversal is full demagnetization of the free layer, driven by a rapid rise in its electronic temperature achieved via either direct laser or hot electron excitation. This work advances the understanding of ultrafast magnetization reversal via nonlocal heat and spin transport under strongly out of equilibrium conditions.

cond-mat.mtrl-sci↗

arXiv2025

Large spin accumulation signals in ultrafast magneto-optical experiments

Magneto-optical techniques have become essential tools in spintronics, enabling the investigation of spin dynamics in the ultrafast regime. A key challenge in this field has been to accurately isolate the contributions to magneto-optical signals of spin transport phenomena from the local magnetization dynamics. The contribution of transported and accumulated spins was long believed to be orders of magnitude smaller than that of the magnetization and thus previous approaches to disentangle these signals have relied on specific experimental designs, usually including thick metal layers. Here, we present experimental evidence demonstrating that the magneto-optical signal from ultrafast spin accumulations can, under certain conditions, be comparable to or even exceed that of the magnetic layer in a standard ultrafast demagnetization experiment. Our findings provide a new framework for accessing and isolating these spin accumulations, allowing for time and depth dependent probing of transported spin and/or orbital angular momentum.

cond-mat.mes-hall↗

arXiv2024

All-optical helicity-dependent switching in NiCo$_2$O$_4$ thin films

All-optical switching (AOS) involves manipulating magnetization using only pulsed laser, presenting a promising approach for next-generation magnetic recording devices. NiCo2O4 (NCO) thin films, a rare-earth-free ferrimagnetic oxide, exhibit a high Curie temperature and strong perpendicular magnetic anisotropy. This study demonstrates AOS in NCO thin films at room temperature using long-duration laser pulses and high repetition rates. Unlike previous findings, the AOS phenomena we report here are helicity-dependent and observable with an ultrashort pulsed laser. Consequently, two distinct types of AOS can be observed in a single NCO thin film, contingent on the characteristics of the laser pulses and temperature.

cond-mat.mtrl-sci↗

arXiv2024

Picosecond all-optical switching of Co/Gd based synthetic ferrimagnets

Single pulse all-optical switching of magnetization (AOS) in Co/Gd based synthetic ferrimagnets carries promises for hybrid spintronic-photonic integration. A crucial next step progressing towards this vision is to gain insight into AOS and multi-domain state (MDS) behavior using longer pulses, which is compatible with state-of-the-art integrated photonics. In this work, we present our studies on the AOS and MDS of [Co/Gd]n (n = 1, 2) using ps optical pulses across a large composition range. We theoretically and experimentally show that a large Gd layer thickness can enhance the AOS energy efficiency and maximum pulse duration. We have identified two augmenting roles of Gd in extending the maximum pulse duration. On the inter-atomic level, we found that more Gd offers a prolonged angular momentum supply to Co. On the micromagnetic level, a higher Gd content brings the system to be closer to magnetic compensation in the equilibrized hot state, thereby reducing the driving force for thermally assisted nucleation of domain walls, combating the formation of a MDS. Our study presents a composition overview of AOS in [Co/Gd]n and offers useful physical insights regarding AOS fundamentals as well as the projected photonic integration.

cond-mat.mes-hall↗

arXiv2023

Criteria to observe single-shot all-optical switching in Gd-based ferrimagnetic alloys

Single-shot all-optical helicity-independent switching (AO-HIS) induced by a femto-second laser pulse has been mainly reported in Gadolinium based rare earth-transition metal (RE-TM) alloys such as GdFeCo or GdCo, but the mechanism leading to magnetization switching is a hotly debated topic. Here, we elaborate on a large number of GdyRE1-x-yCox (RE = Dy, Tb, Ho) alloys to tune various magnetic parameters in order to define what the criteria are for observing AO-HIS in such systems. The state diagrams show that two laser fluences thresholds must be considered:the fluence which induces the single laser pulse switching (FSwitch) and the fluence at which the material breaks into a multi-domain state (FMulti). Those two fluences are shown to behave very differently as a function of the material properties and the laser pulse duration. Taking into account the parameters defining the conditions for which multi-domain states are created and considering only the angular momentum transfer from the Gd sublattice to the rest of the system explains in large our experimental results. The importance of the compensation in the ferrimagnetic alloys is also discussed. We believe the defined criteria will be an important tool for designing new ultra-fast spintronic devices based on all optical switching.

cond-mat.mtrl-sci↗

arXiv2023

Influence of interlayer exchange coupling on ultrafast laser-induced magnetization reversal in ferromagnetic spin valves

In this study, we explore the influence of interlayer exchange coupling on magnetization reversal triggered by femtosecond laser pulses in ferromagnetic spin valves. Our experiments, focused on femtosecond laser-induced magnetization reversal, methodically vary the thickness of the copper (Cu) spacer layer. We identify a critical Cu thickness threshold at 2.32 nm. Above this threshold, a stable reversed magnetic domain is consistently generated upon exposure to a single laser pulse. Conversely, with a Cu spacer thinner than 2.32 nm, the observed magnetization reversal from parallel (P) to anti-parallel (AP) states occurs only under continuous laser irradiation. Once the laser is stopped, the magnetic configuration relaxes back to its initial P state, influenced by ferromagnetic exchange coupling. This research enhances our understanding of the mechanisms that drive optically induced ultrafast magnetization reversal in ferromagnetic spin valves.

cond-mat.mtrl-sci↗

arXiv2023

Extending the scope and understanding of all-optical magnetization switching in Gd-based alloys by controlling the underlying temperature transients

We use the thickness of Cu layers to control all-optical switching of magnetization in adjacent Gd$_{24}$(Fe$_9$0Co$_{10}$)$_{76}$ films. While increasing the Cu thickness from 5 to 900nm has no effect on the switching threshold, it significantly enlarges the fluence and pulse duration at which multiple domains emerge. Having shown that thermally activated multi-domain formation limits the maximum fluence and pulse duration for controlled switching, we demonstrate that continuous magnetization reversal precedes multi-domain formation in Gd$_{18}$Dy$_4$Co$_{78}$ films excited with fluences slightly larger than the multi-domain threshold.

cond-mat.mtrl-sci↗

arXiv2023

Single laser pulse induced magnetization switching in in-plane magnetized GdCo alloys

The discovery of all-optical ultra-fast deterministic magnetization switching has opened up new possibilities for manipulating magnetization in devices using femtosecond laser pulses. Previous studies on single pulse all-optical helicity-independent switching (AO-HIS) have mainly focused on perpendicularly magnetized thin films. This work presents a comprehensive study on AO-HIS for in-plane magnetized GdxCo100-x thin films. Deterministic single femtosecond laser pulse toggle magnetization switching is demonstrated in a wider concentration range (x=10% to 25%) compared to the perpendicularly magnetized counterparts with GdCo thicknesses up to 30 nm. The switching time strongly depends on the GdxCo100-x concentration, with lower Gd concentration exhibiting shorter switching times (less than 500 fs). Our findings in this geometry provide insights into the underlying mechanisms governing single pulse AO-HIS, which challenge existing theoretical predictions. Moreover, in-plane magnetized GdxCo100-x thin films offer extended potential for opto-spintronic applications compared to their perpendicular magnetized counterparts.

cond-mat.mes-hall↗

arXiv2023

Uncovering the role of the light-induced reduction of the inter-atomic exchange in the ultrafast demagnetization of Fe, Co, and Ni

Time resolved measurements of the linear magneto-optical Kerr rotation reveal that, in the {\it 3d} ferromagnets Fe, Co and Ni, the amplitude of the demagnetization increases linearly with the fluence of the light. We rationalize this phenomenon as being linearly driven by the increase in temperature, the electron-phonon and electron-magnon scattering, and a reduction of the inter-atomic exchange. The amplitude of the latter phenomenon, which until the present study has been widely overlooked, is obtained through \textit{ab initio} density functional theory calculations, and is argued to be the principal source of demagnetization in Ni and Co, while still contributing largely in Fe.

cond-mat.mtrl-sci↗

arXiv2020

Picosecond Spin Orbit Torque Switching

Reducing energy dissipation while increasing speed in computation and memory is a long-standing challenge for spintronics research. In the last 20 years, femtosecond lasers have emerged as a tool to control the magnetization in specific magnetic materials at the picosecond timescale. However, the use of ultrafast optics in integrated circuits and memories would require a major paradigm shift. An ultrafast electrical control of the magnetization is far preferable for integrated systems. Here we demonstrate reliable and deterministic control of the out-of-plane magnetization of a 1 nm-thick Co layer with single 6 ps-wide electrical pulses that induce spin-orbit torques on the magnetization. We can monitor the ultrafast magnetization dynamics due to the spin-orbit torques on sub-picosecond timescales, thus far accessible only by numerical simulations. Due to the short duration of our pulses, we enter a counter-intuitive regime of switching where heat dissipation assists the reversal. Moreover, we estimate a low energy cost to switch the magnetization, projecting to below 1fJ for a (20 nm)^3 cell. These experiments prove that spintronic phenomena can be exploited on picosecond time-scales for full magnetic control and should launch a new regime of ultrafast spin torque studies and applications.

physics.app-ph↗