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Jun-ichiro Kishine

Publications and source records attributed to Jun-ichiro Kishine.

At least 19 recordsLinked to original sources

Chirality in Condensed Matter: Symmetry, Waves, and Quasiparticles

Chirality has become a recurring concept throughout condensed-matter physics, appearing in contexts ranging from optical activity and chiral phonons to magnetic excitations and hybrid quasiparticles. As its use has expanded, however, the concept has often become intertwined with related notions such as angular momentum, polarization, helicity, and nonreciprocity, obscuring its precise symmetry-based meaning. Although chirality is universally associated with broken spatial-inversion ($\mathcal{P}$) symmetry and preserved time-reversal ($\mathcal{T}$) symmetry, its physical manifestation and quantitative characterization strongly depend on the system and phenomenon under consideration. In this review, we examine chirality across photons, phonons, magnons, and hybrid excitations. We show that, while no universal measure of chirality exists, different physical systems admit different $\mathcal{P}$-odd and $\mathcal{T}$-even quantities that characterize specific chiral phenomena. We further argue that chirality is often best understood through chirality-selective interactions between waves, matter, and quasiparticles rather than as an intrinsic property of isolated excitations. From this perspective, hybridization provides a particularly promising setting for the emergence, transfer, and control of chirality in condensed-matter systems.

cond-mat.mes-hall

Effective electron coupling to phonon mechanical angular momentum in helical systems

In chiral crystals, two types of phonon angular momenta have been introduced. One is crystal angular momentum (CAM) arising from the rotational or screw-rotational symmetry and the other is mechanical angular momentum (MAM) associated with the circular motion of atomic displacements about equilibrium positions. Recently, the electron-phonon coupling that respects the screw-rotational symmetry is derived, whereby the CAM between electrons and phonons is interconverted. Here, we show that, in addition to CAM, MAM can also be converted to the electronic degrees of freedom by deriving a second-order perturbative Hamiltonian proportional to phonon MAM. This finding highlights that the electronic motion is directly affected by phonon MAM, and consequently, that phonon degrees of freedom can play a crucial role in phenomena related to electronic orbital polarization.

cond-mat.mtrl-sci

Microscopic Theory of Chiral-Phonon-Induced Orbital Selectivity in Helical Crystals

We present a microscopic theory of chirality-induced orbital selectivity (CIOS) in helical crystals, in which truly chiral phonons selectively transfer angular momentum to electronic orbital degrees of freedom. For a threefold helical crystal with line-group symmetry $L3_1$, we show that phonon-induced local rotations generate a rotational electron-phonon interaction proportional to $\hat{L}^{\pm}$, which drives the orbital transfer $m_{\ell}\to m_{\ell}-m_{s}$ in accordance with crystal angular momentum (CAM) conservation, where $m_{s}=\pm 1$ denotes the eigenvalue of the phonon rotational mode. Evaluating $\langle\hat{L}^{z}\rangle$ to leading order in perturbation theory, we find that the orbital response is suppressed near the $Γ$ point and the BZ boundary, and enhanced at intermediate wave vectors -- a feature intimately tied to the degeneracy structure of the phonon bands.

cond-mat.other

Chirality-dependent spin polarization in metals: linear and quadratic responses

We study spin polarization induced by locally injected electric currents in a metal whose spin--orbit coupling reflects its structural chirality. We reveal both spin polarization in the bulk in the linear response and antiparallel spin polarization near the interface in the quadratic response to external electric currents, and reproduce the experimentally observed correlation between the chirality of the metal and the direction of spin polarization. In particular, we elucidate that the sign of the spin polarization in the quadratic response is opposite to that expected from the bulk spin current. This sign discrepancy originates from spin polarization induced by dipole-like charge distribution appearing in the quadratic response.

cond-mat.mes-hall

Inverse Chiral Phonon Zeeman Effect in Noncentrosymmetric Crystals

We present a microscopic theory of the inverse chiral phonon Zeeman effect in noncentrosymmetric crystals. Within micropolar elasticity, coupled translational displacements and microrotations give rise to intrinsically chiral phonons, which generate an elliptically polarized internal magnetic field through dynamical piezoelectricity. In the high-frequency Floquet regime and under incomplete electronic screening, this field acts as an effective longitudinal Zeeman field on electronic spins, leading to spin polarization and band splitting. The results establish a purely lattice-driven mechanism for the inverse chiral phonon Zeeman effect in noncentrosymmetric crystals.

cond-mat.mtrl-sci

Electron-Chiral Phonon Coupling, Crystal Angular Momentum, and Phonon Chirality

We explicitly derive the wavefunctions of chiral phonons propagating along the helical axis in chiral crystals and clarify the characteristics of electron-phonon interactions in chiral helical crystals. In particular, we elucidate how the conservation of not only the crystal momentum (CM) but also the crystal angular momentum (CAM) manifests in the interaction vertex. This formulation provides a microscopic framework for describing physical processes involving chiral phonons. Furthermore, we construct a phononic analogue of Zilch, a known measure of chirality carried by light, and discuss its relationship with phonon angular momentum.

cond-mat.mtrl-sci

Emergence of chirality by multipole interconversion

A clear understanding of chirality in spin-active electronic states is discussed in order to address confusions about chiral effects recently discovered in materials science. Electronic toroidal monopole $G_0$ can serve as a measure of chirality in this categorization, which can be clearly related to the chiral density operator in the Dirac equation. We extend the concepts of chirality not only to those of materials but also to those of physical fields, and to material-field composites. Additionally, we illustrate specific examples from physics and chemistry that demonstrate the process of acquiring chirality through the combination of seemingly achiral degrees of freedom, which we term the emergence of chirality. Interference among multiple chiralities exhibiting phenomena specific to handedness is also discussed.

cond-mat.mtrl-sci

Note on Angular Momentum of Phonons in Chiral Crystals

Phonon angular momentum in chiral materials has been widely studied in spintronics and condensed matter physics. In chiral crystals, this is not the conserved quantity in contrast to the pseudo-angular momentum. To highlight this point and to understand the behavior of the angular momentum, we reexamined phonon dispersion theory based on the irreducible representation of helix and found the distinction of these angular momentum is originated from chirality.

cond-mat.mtrl-sci

Chiral phonons: circularly polarized Raman spectroscopy and $\textit{ab initio}$ calculations in a chiral crystal tellurium

Recently, phonons with chirality (chiral phonons) have attracted significant attention. Chiral phonons exhibit angular and pseudo-angular momenta. In circularly polarized Raman spectroscopy, the peak split of the $Γ_3$ mode is detectable along the principal axis of the chiral crystal in the backscattering configuration. In addition, peak splitting occurs when the pseudo-angular momenta of the incident and scattered circularly polarized light are reversed. Until now, chiral phonons in binary crystals have been observed, whereas those in unary crystals have not been observed. Here, we observe chiral phonons in a chiral unary crystal Te. The pseudo-angular momentum of the phonon is obtained in Te by an $\textit{ab initio}$ calculation. From this calculation, we verified the conservation law of pseudo-angular momentum in Raman scattering. From this conservation law, we determined the handedness of the chiral crystals. We also evaluated the true chirality of the phonons using a measure with symmetry similar to that of an electric toroidal monopole.

cond-mat.mtrl-sci

Truly chiral phonons in α-HgS

Chirality is a manifestation of the asymmetry inherent in nature. It has been defined as the symmetry breaking of the parity of static objects, and the definition was extended to dynamic motion such that true and false chiralities were distinguished. Recently, rotating, yet not propagating, atomic motions were predicted and observed in two-dimensional materials, and they were referred to as "chiral phonons" . A natural development would be the discovery of truly chiral phonons that propagate while rotating in three-dimensional materials. Here, we used circularly polarised Raman scattering and first-principles calculations to identify truly chiral phonons in chiral bulk crystals. This approach enabled us to determine the chirality of a crystal in a non-contact and non-destructive manner. In addition, we demonstrated that the law of the conservation of pseudo-angular momentum holds between circularly polarised photons and chiral phonons. These findings are expected to help develop ways for transferring the pseudo-angular momentum from photons to electron spins via the propagating chiral phonons in opto-phononic-spintronic devices.

cond-mat.mtrl-sci

On the definition of chirality and enantioselective fields

In solid state physics, any symmetry breaking is known to be associated with emergence of an order parameter. However, the order parameter for molecular and crystal chirality, which is a consequence of parity and mirror symmetry breaking, has not been known since its discovery. In this article, the authors show that the order parameter for chirality can be defined by electric toroidal monopole G_0. By this definition, one becomes able to discuss external filed that can distinguish two different enantiomers only by physical fields. In addition, dynamics and fluctuations of the order parameter G_0 can be discussed, with which one can obtain fruitful insights on a spin filtering effect called CISS (Chirality Induced Spin Selectivity). Emergence of time-reversal-odd dipole M_z by time propagation of G_0 quantities is discussed to explain the enantioselective effect (chiral resolution) at a ferromagnetic surface.

cond-mat.mtrl-sci

Chirality-Induced Spin Filtering in Pseudo Jahn-Teller Molecules

Chirality-induced spin selectivity (CISS) refers to an ability to induce a spin polarization of an electron transmitted through chiral materials. An important experimental observation is that incredibly large spin polarization is realized at room temperature even for organic molecules that have weak spin-orbit coupling (SOC), although SOC is the only interaction that can manipulate the electrons' spins in the setups. Therefore, the mechanism of the CISS needs to be constructed in a way insensitive to or enhancing the magnitude of the SOC strength. In this paper, we describe a theoretical study of CISS with a model chiral molecule that belongs to the point group $\mathrm{C}_3$. In this molecule, electronic translational and rotational degrees of freedom for an injected electron are coupled to one another via the nuclear vibrational mode with a pseudo Jahn-Teller effect. By properly taking the molecular symmetry as well as the time-reversal symmetry into account and classifying the molecular ground states by their angular- and spin-momentum quantum numbers, we show that the chiral molecule can act as an efficient spin filter. The efficiency of this spin filtering can be nearly independent of the SOC strength in this model, while it well exceeds the spin polarization relying solely on the SOC. The nuclear vibrations turned out to have the role of not only mediating the translation-rotation coupling, but also enhancing the spin-filtering efficiency.

cond-mat.mtrl-sci

Modification of Selection Rules of Landau-Quantized Electron by Coupling with Obliquely Irradiated Optical Vortex Beams

We discuss selection rules and intensities of photocurrent of a two-dimensional electron gas in a strong magnetic field via absorptions of orbital angular momentum carried by obliquely irradiated optical vortex beams. By angular deflection, optical vortex beams on the two-dimensional electron gas interface can be seen as a superposition of the various orbital angular momentum states. As a result, it is demonstrated that it is yielded that the angular momentum selection rules and induced currents are modified from the case of vertical incidence.

cond-mat.mes-hall

Selection Rules for Optical Vortex Absorption by Landau-quantized Electrons

An optical vortex beam carries orbital angular momentum $\ell$ in addition to spin angular momentum $σ$. We demonstrate that a Landau-quantized two dimensional electron system absorbs the optical vortex beam through modified selection rules, reflecting two kinds of angular momenta. The lowest Landau level electron absorbs the optical vortex beams with $σ=1$ (positive helicity) and $\ell=0$ or $σ=-1$ (negative helicity) and $\ell=2$ in the electric dipole transition. The induced electric currents survive only along the edge of the sample, due to cancellation of the bulk currents. Thus, the magnetization can be induced by only the edge current. It is shown that the induced orbital magnetization disappears when the dark ring of the beam coincides with the disk edge. This scheme may provide a helicity-dependent absorption using the optical vortex beam.

cond-mat.mes-hall

Cavity Optomechanics of Topological Spin Textures in Magnetic Insulators

Collective dynamics of topological magnetic textures can be thought of as a massive particle moving in a magnetic pinning potential. We demonstrate that inside a cavity resonator this effective mechanical system can feel the electromagnetic radiation pressure from cavity photons through the magneto-optical inverse Faraday and Cotton-Mouton effects. We estimate values for the effective parameters of the optomechanical coupling for two spin textures -- a Bloch domain wall and a chiral magnetic soliton lattice. The soliton lattice has magnetic chirality, so that in circularly polarized light it behaves like a chiral particle with the sign of the optomechanical coupling determined by the helicity of the light and chirality of the lattice. Most interestingly, we find a level attraction regime for the soliton lattice, which is tunable through an applied magnetic field.

cond-mat.mes-hall

Tunable spin dynamics in chiral soliton lattice

We study dynamics of a chiral soliton lattice (CSL) in a classical one-dimensional spin chain coupled to the conduction electrons under an electric field. The CSL has attracted much interest because its period can be easily controlled by an external magnetic field. We clarify the dependence of the CSL dynamics on its period. A collective coordinate and an SU(2) gauge method are used for the analysis. It turns out that the velocity of the CSL becomes slower as the period becomes longer. We also mention a relation between the velocity and the magnetic resistance.

cond-mat.mes-hall

Excitation of magnon spin photocurrents in antiferromagnetic insulators

In the circular photogalvanic effect, circularly polarized light can produce a direct electron photocurrent in metals and the direction of the current depends on the polarization. We suggest that an analogous nonlinear effect exists for antiferromagnetic insulators wherein the total spin of light and spin waves is conserved. In consequence, a spin angular momentum is expected to be transfered from photons to magnons so that a circularly polarized electromagnetic field will generate a direct magnon spin current. The direction of the current is determined by the helicity of the light. We show that this resonant effect appears as a second order light-matter interaction. We find also a geometric contribution to the spin photocurrent, which appears for materials with complex lattice structures and Dzyaloshinskii-Moriya interactions.

cond-mat.mes-hall

Theory of magnetoelastic resonance in a mono-axial chiral helimagnet

We study magnetoelastic resonance phenomena in a mono-axial chiral helimagnet belonging to hexagonal crystal class. By computing the spectrum of coupled elastic wave and spin wave, it is demonstrated how hybridization occurs depending on their chirality. Specific features of the magnetoelastic resonance are discussed for the conical phase and the soliton lattice phase stabilized in the mono-axial chiral helimagnet. The former phase exhibits appreciable non-reciprocity of the spectrum, the latter is characterized by a multi-resonance behavior. We propose that the non-reciprocal spin wave around the forced-ferromagnetic state has potential capability to convert the linearly polarized elastic wave to circularly polarized one with the chirality opposite to the spin wave chirality.

cond-mat.mtrl-sci