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Jung Hoon Han

Publications and source records attributed to Jung Hoon Han.

At least 55 records · Page 3Linked to original sources

Phase Instability amid Dimensional Crossover in Artificial Oxide Crystal

Artificial crystals synthesized by atomic-scale epitaxy provides the ability to control the dimensions of the quantum phases and associated phase transitions via precise thickness modulation. In particular, reduction in dimensionality via quantized control of atomic layers is a powerful approach to revealing hidden electronic and magnetic phases. Here, we demonstrate a dimensionality-controlled and induced metal-insulator transition (MIT) in atomically designed superlattices by synthesizing a genuine two dimensional (2D) SrRuO3 crystal with highly suppressed charge transfer. The tendency to ferromagnetically align the spins in SrRuO3 layer diminishes in 2D as the interlayer exchange interaction vanishes, accompanying the 2D localization of electrons. Furthermore, electronic and magnetic instabilities in the two SrRuO3 unit cell layers induce a thermally-driven MIT along with a metamagnetic transition.

cond-mat.str-el↗

Hump-like structure in Hall signal from SrRuO$_3$ ultra-thin films without inhomogeneous anomalous Hall effect

A controversy arose over the interpretation of the recently observed hump features in Hall resistivity $ρ_{xy}$ from ultra-thin SrRuO$_3$ (SRO) film; it was initially interpreted to be due to topological Hall effect but was later proposed to be from existence of regions with different anomalous Hall effect (AHE). In order to settle down the issue, we performed Hall effect as well as magneto-optic Kerr-effect measurements on 4 unit cell SRO films grown on SrTiO$_3$ (001) substrates. Clear hump features are observed in the measured $ρ_{xy}$, whereas neither hump feature nor double hysteresis loop is seen in the Kerr rotation which should be proportional to the magnetization. In addition, magnetization measurement by superconducting quantum interference device shows no sign of multiple coercive fields. These results show that inhomogeneous AHE alone cannot explain the observed hump behavior in $ρ_{xy}$ data from our SRO ultra-thin films. We found that emergence of the hump structure in $ρ_{xy}$ is closely related to the growth condition, high quality films having clear sign of humps.

cond-mat.str-el↗

Competing Spin Liquid Phases in the S=$\frac{1}{2}$ Heisenberg Model on the Kagome Lattice

The properties of ground state of spin-$\frac{1}{2}$ kagome antiferromagnetic Heisenberg (KAFH) model have attracted considerable interest in the past few decades, and recent numerical simulations reported a spin liquid phase. The nature of the spin liquid phase remains unclear. For instance, the interplay between symmetries and $Z_2$ topological order leads to different types of $Z_2$ spin liquid phases. In this paper, we develop a numerical simulation method based on symmetric projected entangled-pair states (PEPS), which is generally applicable to strongly correlated model systems in two spatial dimensions. We then apply this method to study the nature of the ground state of the KAFH model. Our results are consistent with that the ground state is a $U(1)$ Dirac spin liquid rather than a $Z_2$ spin liquid.

cond-mat.str-el↗

Low-energy dynamics of the Affleck-Kennedy-Lieb-Tasaki model in the one- and two-triplon basis

The elementary excitation in the antiferromagnetic spin-1 model known as the Affleck-Kennedy-Lieb-Tasaki (AKLT) Hamiltonian has been described alternatively as magnons or kink-like solitons (triplons). The latter, which we call the triplon throughout this paper, has been proven equivalent descriptions of the same magnon excitation and not an independent branch of excited states. On the other hand, no careful examination of multi-magnon and multi-triplon equivalence was made in the past. In this paper we prove that two-magnon and two-triplon states are also identical descriptions of the same excited states, and furthermore that their energies break down as the sum of one-triplon energies exactly for the AKLT Hamiltonian. The statement holds despite the fact that the model is non-integrable. Such magnon/triplon dichotomy is conjectured to hold for arbitrary n-magnon and n-triplon states. The one- and two-triplon states form orthogonal sets that can be used to span the low-energy Hilbert space. We construct an effective version of the AKLT Hamiltonian within such subspace, and work out the correction to the one-triplon energy gap that finds excellent agreement with the known exact value.

cond-mat.str-el↗

Consideration of Thermal Hall Effect in Undoped Cuprates

A recent observation of thermal Hall effect of magnetic origin in underdoped cuprates calls for critical re-examination of low-energy magnetic dynamics in undoped antiferromagnetic compound on square lattice, where traditional, renormalized spin-wave theory was believed to work well. Using Holstein-Primakoff boson formalism, we find that magnon-based theories can lead to finite Berry curvature in the magnon band once the Dzyaloshinskii-Moriya spin interaction is taken into account explicitly, but fail to produce non-zero thermal Hall conductivity. Assuming accidental doping by impurities and magnon scattering off of such impurity sites fails to predict skew scattering at the level of Born approximation. Local formation of skyrmion defects is also found incapable of generating magnon thermal Hall effect. Turning to spinon-based scenario, we write down a simple model by adding spin-dependent diagonal hopping to the well-known π-flux model of spinons. The resulting two-band model has Chern number in the band structure, and generates thermal Hall conductivity whose magnetic field and temperature dependences mimic closely the observed thermal Hall signals. In disclaimer, there is no firm microscopic basis of this model and we do not claim to have found an explanation of the data, but given the unexpected nature of the experimental observation, it is hoped this work could serve as a first step towards reaching some level of understanding.

cond-mat.str-el↗

Machine Learning Application to Two-Dimensional Dzyaloshinskii-Moriya Ferromagnets

Principles of machine learning are applied to models that support skyrmion phases in two dimensions. Successful feature predictions on various phases of the skyrmion model were possible with several layers of convolutional neural network inserted together with several neural network layers. A new training scheme based on features of the input configuration such as magnetization and spin chirality is introduced. It proved possible to further train external parameters such as the magnetic field and temperature and make reliable predictions on them. Algorithms trained on only the z-component or the xy-components of the spin gave equally reliable predictions. The predictive capacity of the algorithm extended to configurations not generated by the original model, but related ones. A procedure for integrating the machine learning algorithm into the interpretation of experimental data is given.

cond-mat.dis-nn↗

Spin Thermal Hall Conductivity of a Kagomé Antiferromagnet

A clear thermal Hall signal ($κ_{xy}$) was observed in the spin liquid phase of the $S=1/2$ kagomé antiferromagnet Ca kapellasite (CaCu$_3$(OH)$_6$Cl$_2\cdot 0.6$H$_2$O). We found that $κ_{xy}$ is well reproduced, both qualitatively and quantitatively, using the Schwinger-boson mean-field theory with the Dzyaloshinskii--Moriya interaction of $D/J \sim 0.1$. In particular, $κ_{xy}$ values of Ca kapellasite and those of another kagomé antiferromagnet, volborthite, converge to one single curve in simulations modeled using Schwinger bosons, indicating a common temperature dependence of $κ_{xy}$ for the spins of a kagomé antiferromagnet.

cond-mat.str-el↗

Type-II Dirac line node in strained Na3N

Dirac line node (DLN) semimetals are a class of topological semimetals that feature band-crossing lines in momentum space. We study the type-I and type-II classification of DLN semimetals by developing a criterion that determines the type using band velocities. Using first-principles calculations, we also predict that Na3N under an epitaxial tensile strain realizes a type-II DLN semimetal with vanishing spin-orbit coupling (SOC), characterized by the Berry phase that is Z2-quantized in the presence of inversion and time-reversal symmetries. The surface energy spectrum is calculated to demonstrate the topological phase, and the type-II nature is demonstrated by calculating the band velocities. We also develop a tight-binding model and a low-energy effective Hamiltonian that describe the low-energy electronic structure of strained Na3N. The occurrence of a DLN in Na3N under strain is captured in the optical conductivity, which we propose as a means to experimentally confirm the type-II class of the DLN semimetal.

cond-mat.mtrl-sci↗

Statistical recovery of the classical spin Hamiltonian

We propose a simple procedure by which the interaction parameters of the classical spin Hamiltonian can be determined from the knowledge of four-point correlation functions and specific heat. The proposal is demonstrated by using the correlation and specific heat data generated by Monte Carlo method on one- and two-dimensional Ising-like models, and on the two-dimensional Heisenberg model with Dzyaloshinkii-Moriya interaction. A recipe for applying our scheme to experimental images of magnetization such as those made by magnetic force microscopy is outlined.

cond-mat.stat-mech↗

Applications of gradient descent method to magnetic Skyrmion problems

The conjugate gradient (CG) method, a standard and vital way of minimizing the energy of a variational state, is applied to solve several problems in Skyrmion physics. The single-Skyrmion profile optimizing the energy of a two-dimensional chiral magnet is found without relying on specific boundary conditions. The two-dimensional Skyrmion lattice and three-dimensional hedgehog crystal state is recovered with efficiency using the modified CG (p-GD) method. The p-GD method is proposed as a complement to the traditional Monte Carlo annealing method, which still gives better results for the ground state but at the far greater cost in computation time.

cond-mat.dis-nn↗

Experimental observation of hidden Berry curvature in inversion-symmetric bulk 2H-WSe2

We investigate the hidden Berry curvature in bulk 2H-WSe2 by utilizing the surface sensitivity of angle resolved photoemission (ARPES). The symmetry in the electronic structure of transition metal dichalcogenides is used to uniquely determine the local orbital angular momentum (OAM) contribution to the circular dichroism (CD) in ARPES. The extracted CD signals for the K and K' valleys are almost identical but their signs, which should be determined by the valley index, are opposite. In addition, the sign is found to be the same for the two spin-split bands, indicating that it is independent of spin state. These observed CD behaviors are what are expected from Berry curvature of a monolayer of WSe2. In order to see if CD-ARPES is indeed representative of hidden Berry curvature within a layer, we use tight binding analysis as well as density functional calculation to calculate the Berry curvature and local OAM of a monolayer WSe2. We find that measured CD-ARPES is approximately proportional to the calculated Berry curvature as well as local OAM, further supporting our interpretation.

cond-mat.mtrl-sci↗

Proposal of a spin-one chain model with competing dimer and trimer interactions

A new kind of spin-1 chain Hamiltonian consisting of competing dimer and trimer projection operators is proposed. As the relative strengths and signs of the interactions are varied, the model exhibits a number of different phases including the gapped dimer phase and the gapless trimer phase with critical correlations described by a conformal field theory with central charge $c=2$. A symmetry-protected topological phase also exists in this model, even though the microscopic interactions are not the simple adiabatic extensions of the well-known Heisenberg and the Affleck-Kennedy-Lieb-Tasaki model and contains both two- and three-particle permutations. A fourth phase is characterized by macroscopically degenerate ground states. While bearing almost a one-to-one resemblance to the phase diagram of the bilinear-biquadratic spin-1 chain Hamiltonian, our model is rooted on very different physical origin, namely the two competing tendencies of spin-1 particles to form singlets through either dimer or trimer formation.

cond-mat.str-el↗

Resonating Valence Bond States with Trimer Motifs

The trimer resonating valence bond (tRVB) state consisting of an equal-weight superposition of trimer coverings on a square lattice is proposed. A model Hamiltonian of the Rokhsar-Kivelson type for which the tRVB becomes the exact ground state is written. The state is shown to have $9^g$ topological degeneracy on genus g surface and support $Z_3$ vortex excitations. Correlation functions show exponential behavior with a very short correlation length consistent with the gapped spectrum. The classical problem of the degeneracy of trimer configurations is investigated by the transfer matrix method.

cond-mat.str-el↗

Entanglement and corner Hamiltonian spectra of integrable open spin chains

Entanglement spectra (ES) for the critical SU(N) (2 <= N <= 4) spin chains and other integrable models of finite length are studied with the density matrix renormalization group method. For all models under investigation, the level spacings and the degeneracy structure of the ES are in excellent agreement with the spectra of the corner Hamiltonian, defined as the generator of the associated corner transfer matrix. The correspondence holds between the ES (n) at the n-th cut position from the edge of the spin model, and the corner Hamiltonian of length n, for all small values of n. The cut position dependence of the ES shows a period-N oscillatory behavior for a given SU(N) chain, reminiscent of the oscillatory part of the entanglement entropy observed in the past for the same models. Oscillations of the ES do not die out in the bulk of the chain, in contrast to the asymptotically vanishing oscillation of the entanglement entropy. Heuristic argument based on Young tableaux consideration can explain the period-N structure of the ES qualitatively.

cond-mat.str-el↗

Type-II Weyl cone transitions in driven semimetals

Periodically driven systems provide tunable platforms to realize interesting Floquet topological phases and phase transitions. In electronic systems with Weyl dispersions, the band crossings are topologically protected even in the presence of time-periodic perturbations. This robustness permits various routes to shift and tilt the Weyl spectra in the momentum and energy space using circularly polarized light of sufficient intensity. We show that type-II Weyl fermions, in which the Weyl dispersions are tilted with the appearance of pocket-like Fermi surfaces, can be induced in driven Dirac semimetals and line node semimetals. Under a circularly polarized drive, both semimemtal systems immediately generate Weyl node pairs whose types can be further controlled by the driving amplitude and direction. The resultant phase diagrams demonstrate experimental feasibilities.

cond-mat.mes-hall↗

Adiabatic Green's function technique and the transient behavior in time-dependent fermion-boson coupled models

The Lang-Firsov Hamiltonian, a well-known solvable model of interacting fermion-boson system with sideband features in the fermion spectral weight, is generalized to have the time-dependent fermion-boson coupling constant. We show how to derive the two-time Green's function for the time-dependent problem in the adiabatic limit, defined as the slow temporal variation of the coupling over the characteristic oscillator period. The idea we use in deriving the Green's function is akin to the use of instantaneous basis states in solving the adiabatic evolution problem in quantum mechanics. With such "adiabatic Green's function" at hand we analyze the transient behavior of the spectral weight as the coupling is gradually tuned to zero. Time-dependent generalization of a related model, the spin-boson Hamiltonian, is analyzed in the same way. In both cases the sidebands arising from the fermion-boson coupling can be seen to gradually lose their spectral weights over time. Connections of our solution to the two-dimensional Dirac electrons coupled to quantized photons are discussed.

cond-mat.mes-hall↗

Classification of trivial spin-1 tensor network states on a square lattice

Classification of possible quantum spin liquid (QSL) states of interacting spin-1/2's in two dimensions has been a fascinating topic of condensed matter for decades, resulting in enormous progress in our understanding of low-dimensional quantum matter. By contrast, relatively little work exists on the identification, let alone classification, of QSL phases for spin-1 systems in dimensions higher than one. Employing the powerful ideas of tensor network theory and its classification, we develop general methods for writing QSL wave functions of spin-1 respecting all the lattice symmetries, spin rotation, and time reversal with trivial gauge structure on the square lattice. We find $2^5$ distinct classes characterized by five binary quantum numbers. Several explicit constructions of such wave functions are given for bond dimensions $D$ ranging from two to four, along with thorough numerical analyses to identify their physical characters. Both gapless and gapped states are found. The topological entanglement entropy of the gapped states are close to zero, indicative of topologically trivial states. In $D=4$, several different tensors can be linearly combined to produce a family of states within the same symmetry class. A rich "phase diagram" can be worked out among the phases of these tensors, as well as the phase transitions among them. Among the states we identified in this putative phase diagram is the plaquette-ordered phase, gapped resonating valence bond phase, and a critical phase. A continuous transition separates the plaquette-ordered phase from the resonating valence bond phase.

cond-mat.str-el↗

Chirality-driven Hall Transport Phenomena of Spins

Experimental and theoretical aspects of Hall-type transport of spins in magnetic insulators are reviewed, with emphasis on their spin chirality origin. A general formalism for linear response theory of thermal Hall transport in the spin model is developed, which can be applied to both the magnon and the paramagnetic, spin-liquid regimes. Recent experiments on magnon-mediated thermal Hall transport in the two-dimensional kagome, and three-dimensional pyrochlore ferromagnetic insulators are reviewed in light of the multi-band magnon theory of Hall transport, and compared to the more mysterious thermal Hall transport found in the putative quantum spin ice material. As realizations of spin-chirality driven magnon transport in the real space, we review the general theory of emergent gauge fields governing the magnon dynamics in the textured magnet, and discuss its application to the magnon-Skyrmion scattering problem. Topological magnon Hall effect driven by the Skyrmion texture is discussed.

cond-mat.str-el↗